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Noninvasive optical measurements of the shockwave propagation velocity using multiple pulse illumination allow deducing the shockwave pressure amplitude through Hugoniot relations and an appropriate equation of state of the medium. This technique is particularly useful for spatially resolved measurements near the shockwave emission site. Due to diffraction, however, a shockwave front can significantly change its morphology, rendering precise velocity measurements non-trivial. As solution we propose a wave front evolution (WaFE) velocimetry technique, which applies Huygens principle. We take a shadowgraph of the wave front at subsequent times as initial condition for the acoustic Helmholtz equation and numerically propagate the fronts in time. From the instance of time, when two subsequently taken wave front shadows numerically interfere and form one sharp wave front, the local shock velocity is obtained and the local shock pressure amplitude measured. With artificial test images, it is shown that this technique has excellent sub-pixel accuracy, robustness to noise, and can work with low contrast images and even overlapping and interfering wave fronts. The software is made available freely and can be applied to general shock front velocity measurements. We apply WaFE to determine the anisotropic shockwave emission from an elongated laser-induced plasma in water from shadowgraphs of the shockwave front imaged four times onto the same camera frame using multiple pulse illumination at a repetition rate of 60 MHz. The direction dependence of attenuation of the shockwave pressure amplitude is measured at distances of 50–300 μm to the plasma. [ABSTRACT FROM AUTHOR]

Laser microstructuring has been studied extensively in the last decades due to its versatile, contactless processing and outstanding precision and structure quality on a wide range of materials. A limitation of the approach has been identified in the utilization of high average laser powers, with scanner movement fundamentally limited by laws of inertia. In this work, we apply a nanosecond UV laser working in an intrinsic pulse-on-demand mode, ensuring maximal utilization of the fastest commercially available galvanometric scanners at scanning speeds from 0 to 20 m/s. The effects of high-frequency pulse-on-demand operation were analyzed in terms of processing speeds, ablation efficiency, resulting surface quality, repeatability, and precision of the approach. Additionally, laser pulse duration was varied in single-digit nanosecond pulse durations and applied to high throughput microstructuring. We studied the effects of scanning speed on pulse-on-demand operation, single- and multipass laser percussion drilling performance, surface structuring of sensitive materials, and ablation efficiency for pulse durations in the range of 1–4 ns. We confirmed the pulse-on-demand operation suitability for microstructuring for a range of frequencies from below 1 kHz to 1.0 MHz with 5 ns timing precision and identified the scanners as the limiting factor even at full utilization. The ablation efficiency was improved with longer pulse durations, but structure quality degraded. [ABSTRACT FROM AUTHOR]

In a growing number of applications, fast and localized pressure measurement in aqueous media is desired. To perform such measurements, a custom-made single-mode fiber-optic probe hydrophone (FOPH) was designed and used to measure the pressure pulse generated by laser-induced breakdown (LIB) in water. The sensor enabled sub-nanosecond pressure rise time measurement. Both the rise time and the duration of the shockwave were found to be shorter in the direction perpendicular to the breakdown generating laser beam, compared to the shockwave observed in the parallel direction. Simultaneous high-frame-rate imaging was used to qualitatively validate the novel hydrophone data and to observe the shockwave evolution. The measurements were performed also on pressure pulses emitted during the generation of miniature ($150~\boldsymbol \mu \text{m}$ diameter) laser-induced bubbles at very small distances (down to $40~\boldsymbol \mu \text{m}$), further demonstrating the capabilities of the small-size sensor and the ability to measure locally. The results improve understanding of LIB shockwave characteristics dependence on laser pulse energy and duration. [ABSTRACT FROM AUTHOR]

In this manuscript we present a true pulse-on-demand laser design concept using two different approaches. First, we present a fiber master oscillator power amplifier (MOPA) based quasi-continuous wave (CW) laser, working at high modulation bandwidths, for generation of nanosecond pulses. Second, we present a hybrid chirped pulse amplification (CPA)-based laser, combining a chirped-pulse fiber amplifier and an additional solid-state amplifier, for generation of femtosecond pulses. The pulse-on-demand operation is achieved without an external optical modulator/shutter at high-average powers and flexible repetition rates up to 40 MHz, using two variants of the approach for near-constant gain in the amplifier chain. The idler and marker seed sources are combined in the amplifier stages and separated at the out using either wavelength-based separation or second harmonic generation (SHG)-generation-based separation. The nanosecond laser source is further applied to high throughput processing of thin film materials. The laser is combined with a resonant scanner, using the intrinsic pulse-on-demand operation to compensate the scanner's sinusoidal movement. We applied the setup to processing of indium tin oxide (ITO) and metallic films on flexible substrates. [ABSTRACT FROM AUTHOR]

This paper presents an investigation of pulse-on-demand operation in fibre and hybrid lasers. Two methods for efficient gain control that enable the generation of laser pulses at arbitrary times with controlled pulse parameters are presented. The method of direct modulation of the pump power in the high-power laser oscillator is shown to generate pulses with a duration in the nanosecond range, with repetition rates varying during operation from a single shot to over 1 MHz. An advanced method using a combination of marker and idler seeding a fibre amplifier chain is investigated. Such a system can easily achieve repetition rates of several tens of MHz. The lasers' performances were successfully tested in a real environment on an industrial platform for laser transfer printing. Similar concepts were used for a laser source with ultrashort laser pulses (femtosecond range) on demand by using a mode-locked seed as a source and a solid-state amplifier to achieve high pulse energy and peak power. [ABSTRACT FROM AUTHOR]

In this manuscript, an implementation of a tunable nonlinear phase compensation method is demonstrated on a typical femtosecond hybrid laser consisting of a fiber pre-amplifier and an additional solid-state amplifier. This enables one to achieve constant laser pulse parameters over a wide range of pulse repetition rates in such a laser. As the gain in the solid-state amplifier is inversely proportional to the input power, the shortfall in the solid-state gain at higher repetition rates must be compensated for with fiber pre-amplifier to ensure constant pulse energy. This increases the accumulated nonlinear phase and consequently alters the laser pulse parameters such as pulse duration and Strehl ratio. To overcome this issue, the nonlinear phase must be compensated for, and what is more it should be compensated for to a different extent at different pulse repetition rates. This is achieved with a tunable CFBG, used also as a pulse stretcher. Using this concept, we demonstrate that constant laser pulse parameters such as pulse energy, pulse duration and Strehl ratio can be achieved in a hybrid laser regardless of the pulse repetition rate. [ABSTRACT FROM AUTHOR]

• Laser patterning of thin films on flexible substrates. • Observation and analysis of patterning-induced surface effects. • Insight into rapid nanosecond ablation properties in thin film materials. • Demonstration of ultra-fast scanning utilization on in-demand electronic materials. Modern electronics facilitate the need for fast, efficient, and reliable methods for direct laser-based surface engineering of conductive thin film materials on flexible substrates. Recent advances in pulsed laser source development only incrementally increased the processing speeds, as those are limited by the available scanning systems. Our goal was to combine a high pulse repetition frequency high-power pulse-on-demand fiber laser source with an ultra-fast resonant scanner to achieve high throughput surface engineering. The enabling factor to compensate a resonant scanner's sinusoidal movement were the laser's intrinsic pulse-on-demand capabilities beyond simple pulse picking solutions. The high temporal resolution at full laser power was exploited for spatially controlled surface texturing, allowing a minimally 3 μm positioning accuracy throughout the scanner's range at up to 60 m/s scan speed with a 10 μm laser spot size. We applied the setup to processing of ITO and metallic films on flexible substrates for touchscreens, position sensors, or EM shielding. Surface modification and patterning of the conductive layer was successfully demonstrated while keeping the underlying surface intact. We employed a simple laser ablation model in comparison to the experimental data to improve the understanding of the ablation process. The resulting surface topography was observed and analysed. [ABSTRACT FROM AUTHOR]

• Visualization of the growth of cavitation bubbles near the nucleation energy threshold. • Report on low and high conversion of excitation energy to the cavitation. • Visualization supported shockwave pressure measurement and modeling. • Laser induced cavitation bubbles of few μm diameter generated by 60 ps 515 nm laser. The nucleation and growth of cavitation bubbles few micrometers in size in water generated by a 60 ps 515 nm fiber laser is observed and visualized near nucleation threshold. The study is performed by monitoring the plasma size, the cavitation bubble size and the emitted shock waves. The latter two aspects are supported by the Gilmore model using a Noble-Abel-stiffened-gas (NASG) equations of state. For the first time, two types of cavitation events are identified and visualized that exhibit a difference of more than two orders of magnitude in the excitation energy converted to mechanical effects with minimal change in excitation laser pulse energy. The result is localized cavitation and reduced mechanical stress on water-based media with potentially positive implications for laser treatments of biological tissue. [ABSTRACT FROM AUTHOR]