1. Signatures of a surface spin-orbital chiral metal
- Author
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Mazzola, Federico, Brzezicki, Wojciech, Mercaldo, Maria Teresa, Guarino, Anita, Bigi, Chiara, Miwa, Jill A., De Fazio, Domenico, Crepaldi, Alberto, Fujii, Jun, Rossi, Giorgio, Orgiani, Pasquale, Chaluvadi, Sandeep Kumar, Chalil, Shyni Punathum, Panaccione, Giancarlo, Jana, Anupam, Polewczyk, Vincent, Vobornik, Ivana, Kim, Changyoung, Granozio, Fabio Miletto, Fittipaldi, Rosalba, Ortix, Carmine, Cuoco, Mario, and Vecchione, Antonio
- Subjects
Condensed Matter - Strongly Correlated Electrons ,Condensed Matter - Mesoscale and Nanoscale Physics - Abstract
The relation between crystal symmetries, electron correlations, and electronic structure steers the formation of a large array of unconventional phases of matter, including magneto-electric loop currents and chiral magnetism. Detection of such hidden orders is a major goal in condensed matter physics. However, to date, nonstandard forms of magnetism with chiral electronic ordering have been experimentally elusive. Here, we develop a theory for symmetry-broken chiral ground states and propose a methodology based on circularly polarized spin-selective angular-resolved photoelectron spectroscopy to probe them. We exploit the archetypal quantum material Sr2RuO4 and reveal spectroscopic signatures which, even though subtle, may be reconciled with the formation of spin-orbital chiral currents at the material surface. As we shed light on these chiral regimes, our findings pave the way for a deeper understanding of ordering phenomena and unconventional magnetism.
- Published
- 2024
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