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In this work we investigate the two-neutron decay of 13Li and of the excited states of 11Li populated via one-proton removal from 14Be and 12Be, respectively. A phenomenological model is used to describe the decay of 11Li and 13Li. While the first one displays important sequential components, the second one appears dominated by the direct two-neutron decay. A microscopic three-body model is used to extract information on the spatial configuration of the emitted neutrons before the decay and shows that the average distance between the neutrons increases going from 11Li to 13Li.

The calcium isotopes are an ideal system to investigate the evolution of shell structure and magic numbers. Although the properties of surface nucleons in calcium have been well studied, probing the structure of deeply bound nucleons remains a challenge. Here, we report on the first measurement of unbound states in 53Ca and 55Ca, populated from 54,56Ca(p,pn) reactions at a beam energy of around 216 MeV/nucleon at the RIKEN Radioactive Isotopes Beam Factory. The resonance properties, partial cross sections, and momentum distributions of these unbound states were analyzed. Orbital angular momentum l assignments were extracted from momentum distributions based on calculations using the distorted wave impulse approximation (DWIA) reaction model. The resonances at excitation energies of 5516(41)keV in 53Ca and 6000(250)keV in 55Ca indicate a significant l =3 component, providing the first experimental evidence for the ν0f7/2 single-particle strength of unbound hole states in the neutron-rich Ca isotopes. The observed excitation energies and cross-sections point towards extremely localized and well separated strength distributions, with some fragmentation for the ν0f7/2 orbital in 55Ca. These results are in good agreement with predictions from shell-model calculations using the effective GXPF1Bs interaction and ab initio calculations and diverge markedly from the experimental distributions in the nickel isotones at Z=28.

The low-lying structure of 15C has been investigated via the neutron-removal 16C(d,t) reaction. Along with the known bound neutron sd-shell states, unbound p-shell hole states have been observed. The excitation energies and the deduced spectroscopic factors of the cross-shell states are an important measure of the [(p)−1(sd)2] neutron configurations in 15C. Our results show a very good agreement with shell-model calculations using the SFO-tls interaction for 15C. However, this same interaction predicted energies that were too low for the corresponding hole states in the N=9 isotone 17O and adjustment of the p-sd and sd-sd monopole terms was required to match the 17O energies. In addition, the excitation energies and spectroscopic factors have been compared to the first calculations of 15C with the ab initio self-consistent Green's function method employing the NNLOsat interaction. The results show the sensitivity to the size of the N=8 shell gap and highlight the need to go beyond the current truncation scheme.

The nuclear structure of 66Se, nucleus beyond the N=Z line on the proton-rich side of the valley of stability, was investigated by the neutron knock-out reaction 67Se(12C,X)66Se using a 12C target. The analysis of the singles spectrum of the γ-rays emitted during the de-excitation of the populated low-lying excited states revealed two previously detected (927(4) keV, 1460(32) keV) and three new (744(6) keV, 1210(17) keV, 1661(23) keV) transitions. The 744-keV, the 1210-keV, and the 1460-keV transitions were found to be in coincidence with the one at 927 keV. The spectrum coincident with the 927-keV transition showed a further possible transition at 299(35) keV, which was obscured by significant atomic background in the singles spectrum. This transition might correspond to a peak previously reported at 273(5) keV that could not be assigned to 66Se unambiguously. Based on a comparison of the experimental data to theoretical calculations, four new excited states are proposed which suggest that 66Se exhibits shape coexistence.

Gamma decays were observed in 56Ca and 58Ca following quasi-free one-proton knockout reactions from 57,59Sc beams at ≈200 MeV/nucleon. For 56Ca, a γ ray transition was measured to be 1456(12) keV, while for 58Ca an indication for a transition was observed at 1115(34) keV. Both transitions were tentatively assigned as the 21+→0gs+ decays, and were compared to results from ab initio and conventional shell-model approaches. A shell-model calculation in a wide model space with a marginally modified effective nucleon-nucleon interaction depicts excellent agreement with experiment for 21+ level energies, two-neutron separation energies, and reaction cross sections, corroborating the formation of a new nuclear shell above the N = 34 shell. Its constituents, the 0f5/2 and 0g9/2 orbitals, are almost degenerate. This degeneracy precludes the possibility for a doubly magic 60Ca and potentially drives the dripline of Ca isotopes to 70Ca or even beyond.

Detailed γ-ray spectroscopy of the exotic neon isotope 28Ne has been performed for the first time using the one-neutron removal reaction from 29Ne on a liquid hydrogen target at 240 MeV/nucleon. Based on an analysis of parallel momentum distributions, a level scheme with spin-parity assignments has been constructed for 28Ne and the negative-parity states are identified for the first time. The measured partial cross sections and momentum distributions reveal a significant intruder p-wave strength providing evidence of the breakdown of the N=20 and N=28 shell gaps. Only a weak, possible f-wave strength was observed to bound final states. Large-scale shell-model calculations with different effective interactions do not reproduce the large p-wave and small f-wave strength observed experimentally, indicating an ongoing challenge for a complete theoretical description of the transition into the island of inversion along the Ne isotopic chain.

The dineutron correlation is systematically studied in three different Borromean nuclei near the neutron dripline, 11Li, 14Be and 17B, via the (p,pn) knockout reaction measured at the RIBF facility in RIKEN. For the three nuclei, the correlation angle between the valence neutrons is found to be largest in the same range of intrinsic momenta, which can be associated to the nuclear surface. This result reinforces the prediction that the formation of the dineutron is universal in environments with low neutron density, such as the surface of neutron-rich Borromean nuclei.

Unbound states in C17 were investigated via one-neutron removal from a C18 beam at an energy of 245 MeV/nucleon on a carbon target. The energy spectrum of C17, above the single-neutron decay threshold, was reconstructed using invariant mass spectroscopy from the measured momenta of the C16 fragment and neutron, and was found to exhibit resonances at Er=0.52(2), 0.77(2), 1.36(1), 1.91(1), 2.22(3) and 3.20(1) MeV. The resonance at Er=0.77(2) MeV [Ex=1.51(3) MeV] was provisionally assigned as the second 5/2+ state. The two resonances at Er=1.91(1) and 3.20(1) MeV [Ex=2.65(2) and 3.94(2) MeV] were identified, through comparison of the energies, cross sections and momentum distributions with shell-model and eikonal reaction calculations, as p-shell hole states with spin-parities 1/21− and 3/21−, respectively. A detailed comparison was made with the results obtained using a range of shell-model interactions. The YSOX shell-model Hamiltonian, the cross-shell part of which is based on the monopole-based universal interaction, was found to provide a very good description of the present results and those for the neighbouring odd-A carbon isotopes – in particular for the negative parity cross-shell states.

The isovector and isoscalar components of neutron-proton pairing are investigated in the N=Z unstable nuclei of the fp-shell through the two-nucleon transfer reaction (p,3He) in inverse kinematics. The combination of particle and gamma-ray detection with radioactive beams of 56Ni and 52Fe, produced by fragmentation at the GANIL/LISE facility, made it possible to carry out this study for the first time in a closed and an open-shell nucleus in the fp-shell. The transfer cross-sections for ground-state to ground-state (J=0+, T=1) and to the first (J=1+, T=0) state were extracted for both cases together with the transfer cross-section ratios σ(0+,T=1)/σ(1+,T=0). They are compared with second-order distorted-wave born approximation (DWBA) calculations. The enhancement of the ground-state to ground-state pair transfer cross-section close to mid-shell, in 52Fe, points towards a superfluid phase in the isovector channel. For the “deuteron-like” transfer, very low cross-sections to the first (J=1+, T=0) state were observed both for 56Ni(p,3He) and 52Fe(p,3He) and are related to a strong hindrance of this channel due to spin-orbit effect. No evidence for an isoscalar deuteron-like condensate is observed.

The properties of nuclei with extreme neutron–to–proton ratios, far from those naturally occurring on Earth, are key to understand nuclear forces and how nucleons hold together to form nuclei. 7H, with six neutrons and a single proton, is the nuclear system with the most unbalanced neutron–to–proton ratio known so far. However, its sheer existence and properties are still a challenge for experimental efforts and theoretical models. Here we report experimental evidences on the formation of 7H as a resonance, detected with independent observables, and the first measurement of the structure of its ground state. The resonance is found at ∼0.7 MeV above the 3H+4n mass, with a narrow width of ∼0.2 MeV and a 1/2+ spin and parity. These data are consistent with a 7H as a 3H core surrounded by an extended four-neutron halo, with a unique four-neutron decay and a relatively long half-life thanks to neutron pairing; a prime example of new phenomena occurring in what would be the most pure-neutron nuclear matter we can access in the laboratory.

States in the N=35 and 37 isotopes 55,57Ca have been populated by direct proton-induced nucleon removal reactions from 56,58Sc and 56Ca beams at the RIBF. In addition, the (p,2p) quasi-free single-proton removal reaction from 56Ca was studied. Excited states in 55K, 55Ca, and 57Ca were established for the first time via in-beam γ-ray spectroscopy. Results for the proton and neutron removal reactions from 56Ca to states in 55K and 55Ca for the level energies, excited state lifetimes, and exclusive cross sections agree well with state-of-the-art theoretical calculations using different approaches. The observation of a short-lived state in 57Ca suggests a transition in the calcium isotopic chain from single-particle dominated states at N=35 to collective excitations at N=37.

The nuclear structure of 51Ar, an uncharted territory so far, was studied by the (p,2p) reaction using γ-ray spectroscopy for the bound states and the invariant mass method for the unbound states. Two peaks were detected in the γ-ray spectrum and six peaks were observed in the 50Ar+n relative energy spectrum. Comparing the results to our shell-model calculations, two bound and six unbound states were established. Three of the unbound states could only be placed tentatively due to the low number of counts in the relative energy spectrum of events associated with the decay through the first excited state of 50Ar. The low cross sections populating the two bound states of 51Ar could be interpreted as a clear signature for the presence of significant subshell closures at neutron numbers 32 and 34 in argon isotopes. It was also revealed that due to the two valence holes, unbound collective states coexist with individual-particle states in 51Ar.

The first investigation of the single-particle structure of the bound states of 17C, via the d(16C,p) transfer reaction, has been undertaken. The measured angular distributions confirm the spin-parity assignments of 1/2+ and 5/2+ for the excited states located at 217 and 335 keV, respectively. The spectroscopic factors deduced for these states exhibit a marked single-particle character, in agreement with shell model and particle-core model calculations, and combined with their near degeneracy in energy provide clear evidence for the absence of the N=14 sub-shell closure. The very small spectroscopic factor found for the 3/2+ ground state is consistent with theoretical predictions and indicates that the ν1d3/2 strength is carried by unbound states. With a dominant ℓ=0 valence neutron configuration and a very low separation energy, the 1/2+ excited state is a one-neutron halo candidate.

We report on the first γ-ray spectroscopy of 51,53K produced via the 52,54Ca(p,2p) reactions at ∼250 MeV/nucleon. Unambiguous final-state angular-momentum assignments were achieved for beam intensities down to few particles per second by using a new technique based on reaction vertex tracking combined with a thick liquid-hydrogen target. Through γ-ray spectroscopy and exclusive parallel momentum distribution analysis, 3/2+ ground states and 1/2+ first excited states in 51,53K were established quantifying the natural ordering of the 1d3/2 and 2s1/2 proton-hole states that are restored at N = 32 and 34. State-of-the-art ab initio calculations and shell-model calculations with improved phenomenological effective interactions reproduce the present data and predict consistently the increase of the E(1/21+) - E(3/21+) energy differences towards N = 40. Keywords: Spectroscopy, Shell evolution, 51K, 53K

Excited states in the N=40 isotone 62Ti were populated via the 63V(p,2p)62Ti reaction at ∼200 MeV/nucleon at the Radioactive Isotope Beam Factory and studied using γ-ray spectroscopy. The energies of the 21+→0gs+ and 41+→21+ transitions, observed here for the first time, indicate a deformed 62Ti ground state. These energies are increased compared to the neighboring 64Cr and 66Fe isotones, suggesting a small decrease of quadrupole collectivity. The present measurement is well reproduced by large-scale shell-model calculations based on effective interactions, while ab initio and beyond mean-field calculations do not yet reproduce our findings. The shell-model calculations for 62Ti show a dominant configuration with four neutrons excited across the N=40 gap. Likewise, they indicate that the N=40 island of inversion extends down to Z=20, disfavoring a possible doubly magic character of the elusive 60Ca. Keywords: Shell evolution, Radioactive beams, Gamma-ray spectroscopy

The low-lying unbound level structure of the halo nucleus 19C has been investigated using single-neutron knockout from 20C on a carbon target at 280 MeV/nucleon. The invariant mass spectrum, derived from the momenta of the forward going beam velocity 18C fragment and neutrons, was found to be dominated by a very narrow near threshold (Erel=0.036(1) MeV) peak. Two less strongly populated resonance-like features were also observed at Erel=0.84(4) and 2.31(3) MeV, both of which exhibit characteristics consistent with neutron p-shell hole states. Comparisons of the energies, measured cross sections and parallel momentum distributions to the results of shell-model and eikonal reaction calculations lead to spin-parity assignments of 5/21+ and 1/21− for the levels at Ex=0.62(9) and 2.89(10) MeV with Sn=0.58(9) MeV. Spectroscopic factors were also deduced and found to be in reasonable accord with shell-model calculations. The valence neutron configuration of the 20C ground state is thus seen to include, in addition to the known 1s1/22 component, a significant 0d5/22 contribution. The level scheme of 19C, including significantly the 1/21− cross-shell state, is well accounted for by the YSOX shell-model interaction developed from the monopole-based universal interaction.

We present an investigation of the structure of 13Be obtained via a kinematically complete measurement of the (p,pn) reaction in inverse kinematics at 265 MeV/nucleon. The relative energy spectrum of 13Be is compared to Transfer-to-the-Continuum calculations which use as structure inputs the overlaps of the 14Be ground-state wave function, computed in a three-body model, with the unbound states of the 13Be residual nucleus. The key role of neutron p-wave orbital in the interpretation of the low-relative-energy part of the spectrum is discussed. Keywords: Quasi-free scattering, Borromean nuclei, Three-body model, Resonances

The interaction cross sections (σI) of the very neutron-rich carbon isotopes 19C, 20C and 22C have been measured on a carbon target at 307, 280, and 235 MeV/nucleon, respectively. A σI of 1.280±0.023 b was obtained for 22C, significantly larger than for 19,20C, supporting the halo character of 22C. A 22C root-mean-squared matter radius of 3.44±0.08 fm was deduced using a four-body Glauber reaction model. This value is smaller than an earlier estimate (of 5.4±0.9 fm) derived from a σI measurement on a hydrogen target at 40 MeV/nucleon. These new, higher-precision σI data provide stronger constraints for assessing the consistency of theories describing weakly bound nuclei.

The Isoscalar Giant Monopole Resonance (ISGMR) and the Isoscalar Giant Dipole Resonance (ISGDR) compression modes have been studied in the doubly-magic unstable nucleus 56Ni. They were measured by inelastic α-particle scattering in inverse kinematics at 50 MeV/u with the MAYA active target at the GANIL facility. The centroid of the ISGMR has been obtained at Ex=19.1±0.5 MeV. Evidence for the low-lying part of the ISGDR has been found at Ex=17.4±0.7 MeV. The strength distribution for the dipole mode shows similarity with the prediction from the Hartree–Fock (HF) based random-phase approximation (RPA) [1]. These measurements confirm inelastic α-particle scattering as a suitable probe for exciting the ISGMR and the ISGDR modes in radioactive isotopes in inverse kinematics.

One-neutron knockout from 24O leading to the first excited state in 23O has been measured for a proton target at a beam energy of 62 MeV/nucleon. The decay energy spectrum of the neutron unbound state of 23O was reconstructed from the measured four momenta of the 22O fragment and emitted neutron. A sharp peak was found at Edecay=50±3 keV, corresponding to an excited state in 23O at 2.78±0.11 MeV, as observed in previous measurements. The longitudinal momentum distribution for this state was consistent with d-wave neutron knockout, providing support for a Jπ assignment of 5/2+. The associated spectroscopic factor was deduced to be C2S(0d5/2)=4.1±0.4 by comparing the measured cross section (σ−1nexp=61±6 mb) with a distorted wave impulse approximation calculation. Such a large occupancy for the neutron 0d5/2 orbital is in line with the N=16 shell closure in 24O.

The Billotron is a device designed and built by the LPC Caen to illustrate the methods with which physicists are able to study the basic structure of matter, in particular the nucleus of the atom. [ABSTRACT FROM AUTHOR]

The behavior of the nuclear shell structure far away from the valley of stability is discussed in this paper with an emphasis on the N = 20 magic number. Two experimental examples, namely g-spectroscopy of 27Ne by 1H(28Ne, 27Ne) reaction and single-particle spectroscopy of 23O by 22O(d, p)23O* - 22O+n process in inverse kinematics, are shown providing indirect indication and a direct evidence for the extreme decrease of the N = 20 shell gap and, consequently, the vanishing N = 20 magicity. [ABSTRACT FROM AUTHOR]