1. Magnetic excitations in infinite-layer nickelates
- Author
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Lu, H., Rossi, M., Nag, A., Osada, M., Li, D. F., Lee, K., Wang, B. Y., Garcia-Fernandez, M., Agrestini, S., Shen, Z. X., Been, E. M., Moritz, B., Devereaux, T. P., Zaanen, J., Hwang, H. Y., Zhou, Ke-Jin, and Lee, W. S.
- Subjects
Condensed Matter - Superconductivity ,Condensed Matter - Strongly Correlated Electrons - Abstract
The discovery of superconductivity in infinite-layer nickelates brings us tantalizingly close to a new material class that mirrors the cuprate superconductors. Here, we report on magnetic excitations in these nickelates, measured using resonant inelastic x-ray scattering (RIXS) at the Ni L3-edge, to shed light on the material complexity and microscopic physics. Undoped NdNiO2 possesses a branch of dispersive excitations with a bandwidth of approximately 200 meV, reminiscent of strongly-coupled, antiferromagnetically aligned spins on a square lattice, despite a lack of evidence for long range magnetic order. The significant damping of these modes indicates the importance of coupling to rare-earth itinerant electrons. Upon doping, the spectral weight and energy decrease slightly, while the modes become overdamped. Our results highlight the role of Mottness in infinite-layer nickelates., Comment: This is the initially submitted version before revising for reviewers' comments. The peer-reviewed version has been accepted at Science and will be published soon
- Published
- 2021
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