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A morphing wing model is used to improve aircraft performance. To obtain the desired airfoils, electrical actuators are used, which are installed inside of the wing to morph its upper surface in order to obtain its desired shape. In order to achieve this objective, a robust position controller is needed. In this research, a design and test validation of a controller based on neural networks is presented. This controller was composed by a position controller and a current controller to manage the current consumed by the electrical actuators to obtain its desired displacement. The model was tested and validated using simulation and experimental tests. The results obtained with the proposed controller were compared to the results given by the PID controller. Wind tunnel tests were conducted in the Price-Païdoussis Wind Tunnel at the LARCASE laboratory in order to calculate the pressure coefficient distribution on an ATR-42 morphing wing model for different flow conditions. The pressure coefficients obtained experimentally were compared with their numerical values given by XFoil software.

Within the frame of the European Aerosol Cloud Climate and Air Quality Interactions (EUCAARI) project, the Météo-France aircraft ATR-42 performed 22 research flights over central Europe and the North Sea during the intensive observation period in May 2008. For the campaign, the ATR-42 was equipped to study the aerosol physical, chemical, hygroscopic and optical properties, as well as cloud microphysics. For the 22 research flights, retroplume analyses along the flight tracks were performed with FLEXPART in order to classify air masses into five sectors of origin, allowing for a qualitative evaluation of emission influence on the respective air parcel. This study shows that the extensive aerosol parameters (aerosol mass and number concentrations) show vertical decreasing gradients and in some air masses maximum mass concentrations (mainly organics) in an intermediate layer (1–3 km). The observed mass concentrations (in the boundary layer (BL): between 10 and 30 μg m−3; lower free troposphere (LFT): 0.8 and 14 μg m−3) are high especially in comparison with the 2015 European norms for PM2.5 (25 μg m−3) and with previous airborne studies performed over England (Morgan et al., 2009; McMeeking et al., 2012). Particle number size distributions show a larger fraction of particles in the accumulation size range in the LFT compared to BL. The chemical composition of submicron aerosol particles is dominated by organics in the BL, while ammonium sulphate dominates the submicron aerosols in the LFT, especially in the aerosol particles originated from north-eastern Europe (~ 80%), also experiencing nucleation events along the transport. As a consequence, first the particle CCN acting ability, shown by the CCN/CN ratio, and second the average values of the scattering cross sections of optically active particles (i.e. scattering coefficient divided by the optical active particle concentration) are increased in the LFT compared to BL.

Aerosol properties were studied during an intensive airborne measurement campaign that took place at Rotterdam in Netherlands in May 2008 within the framework of the European Aerosol Cloud Climate and Air Quality Interactions project (EUCAARI). The objective of this study is to illustrate seven events of new particle formation (NPF) observed with two Condensation Particle Counters (CPCs) operated on board the ATR-42 research aircraft in airsectors around Rotterdam, and to provide information on the spatial extent of the new particle formation phenomenon based on 1-s resolution measurements of ultra-fine particle (in the size range 3–10 nm diameter, denoted N3-10 hereafter) concentrations. The results show that particle production occurred under the influence of different air mass origins, at different day times and over the North Sea as well as over the continent. The number concentration of freshly nucleated particles (N3-10) varied between 5000 and 100 000 cm−3 within the boundary layer (BL). Furthermore the vertical extension for all nucleation events observed on the ATR-42 never exceeded the upper limit of the BL. The horizontal extent of N3-10 could not be delimited due to inflexible flight plans which could not be modified to accommodate real-time results. However, the NPF events were observed over geographically large areas; typically the horizontal extension was about 100 km and larger.

The fast determination of aerodynamic parameters such as pressure distributions, lift, drag and moment coefficients from the known airflow conditions (angles of attack, Mach and Reynolds numbers) in real time is still not easily achievable by numerical analysis methods in aerodynamics and aeroelasticity. A flight parameters control system is proposed to solve this problem. This control system is based on new optimisation methodologies using Neural Networks (NNs) and Extended Great Deluge (EGD) algorithms. Validation of these new methodologies is realised by experimental tests using a wing model installed in a wind tunnel and three different transducer systems (a FlowKinetics transducer, an AEROLAB PTA transducer and multitube manometer tubes) to determine the pressure distribution. For lift, drag and moment coefficients, the results of our approach are compared to the XFoil aerodynamics software and the experimental results for different angles of attack and Mach numbers. The main purpose of this new proposed control system is to improve, in this paper, wing aerodynamic performance, and in future to apply it to improve aircraft aerodynamic performance. [ABSTRACT FROM PUBLISHER]

A morphing wing model is used to improve aircraft performance. To obtain the desired airfoils, electrical actuators are used, which are installed inside of the wing to morph its upper surface in order to obtain its desired shape. In order to achieve this objective, a robust position controller is needed. In this research, a design and test validation of a controller based on neural networks is presented. This controller was composed by a position controller and a current controller to manage the current consumed by the electrical actuators to obtain its desired displacement. The model was tested and validated using simulation and experimental tests. The results obtained with the proposed controller were compared to the results given by the PID controller. Wind tunnel tests were conducted in the Price-Païdoussis Wind Tunnel at the LARCASE laboratory in order to calculate the pressure coefficient distribution on an ATR-42 morphing wing model for different flow conditions. The pressure coefficients obtained experimentally were compared with their numerical values given by XFoil software. [ABSTRACT FROM AUTHOR]

Aerosol properties were studied during an intensive airborne measurement campaign that took place at Rotterdam in Netherlands in May 2008 within the framework of the European Aerosol Cloud Climate and Air Quality Interactions project (EUCAARI). The objective of this study is to illustrate seven events of new particle formation (NPF) observed with two Condensation Particle Counters (CPCs) operated on board the ATR-42 research aircraft in airsectors around Rotterdam, and to provide information on the spatial extent of the new particle formation phenomenon based on 1-s resolution measurements of ultra-fine particle (in the size range 3-10 nm diameter, denoted N3-10 hereafter) concentrations. The results show that particle production occurred under the influence of different air mass origins, at different day times and over the North Sea as well as over the continent. The number concentration of freshly nucleated particles (N3-10) varied between 5000 and 100 000 cm-3 within the boundary layer (BL). Furthermore the vertical extension for all nucleation events observed on the ATR-42 never exceeded the upper limit of the BL. The horizontal extent of N3-10 could not be delimited due to inflexible flight plans which could not be modified to accommodate real-time results. However, the NPF events were observed over geographically large areas; typically the horizontal extension was about 100 km and larger. [ABSTRACT FROM AUTHOR]

. Within the frame of the European Aerosol Cloud Climate and Air Quality Interactions (EUCAARI) project the Météo-France aircraft ATR-42 performed 22 research flights, over central Europe and the North Sea during the intensive observation period in May 2008. For the campaign, the ATR-42 was equipped in order to study aerosol physical, chemical and optical properties, as well as cloud microphysics. During the campaign, continental air masses from Eastern and Western Europe were encountered, along with polar and Scandinavian air masses. For the 22 research flights, retroplume analyses along the flight tracks were performed with FLEXPART in order to classify air masses into five sectors of origin which allows for a qualitative evaluation of emission influence on the respective air parcel. In the polluted boundary layer (BL), typical concentrations of particles with diameters larger than 10nm (N10) are of the order of 5000-6000cm-3, whereas N10 concentrations of clean air masses were lower than 1300 cm-3. The detection of the largest particle number concentrations occurred in air masses coming from Polar and Scandinavian regions for which an elevated number of nucleation mode (25-28 nm) particles was observed and attributed to new particle formation over open sea. In the free troposphere (FT), typical observed N10 are of the order of 900cm10 in polluted air masses and 400-600 cm10 in clean air masses, respectively. In both layers, the chemical composition of submicron aerosol particles is dominated by organic matter and nitrate in polluted air masses, while, sulphate and ammonium followed by organics dominate the submicron aerosols in clean air masses. The highest CCN/CN ratios were observed within the polar air masses while the CCN concentration values are the highest within the polluted air masses. Within the five air mass sectors defined and the two layers (BL and FT), observations have been distinguished into anticyclonic (first half of May 2008) and cyclonic conditions (second half of May 2008). Strong relationships between meteorological conditions and physical, chemical as well as optical properties are found. [ABSTRACT FROM AUTHOR]

Within the European Aerosol Cloud Climate and Air Quality Interactions (EUCAARI) project, the Meteo France research aircraft ATR-42 was operated from Rotterdam airport during May 2008, to perform scientific flights dedicated to the investigation of aerosol-cloud interactions. Therein, the objective of this study is to illustrate the impact of cloud processing on the aerosol particles physical and chemical properties. The presented results are retrieved from measurements during a double-flight mission from Rotterdam (Netherlands) to Newcastle (UK) and back using data measured with compact Time of Flight Aerosol Mass Spectrometer (cToF-AMS) and Scanning Mobility Particle Sizer (SMPS). Cloud-related measurements during these flights were performed over the North Sea within as well as in close vicinity of a marine stratocumulus cloud layer. Particle physical and chemical properties observed in the close vicinity (V), below and above the stratocumulus cloud show strong differences. Firstly, measurements at constant altitude above the cloud layer show decreasing mass concentrations with decreasing horizontal distance (210-0 km) to the cloud layer by a factor up to 7, whereas below the cloud and by same means of distance, the mass concentrations merely decrease by a factor of 2 on average. Secondly, the averaged aerosol size distributions, observed above and below the cloud layer, are of bimodal character with pronounced minima between Aitken and accumulation mode which is potentially the consequence of cloud processing. Finally, the chemical composition of aerosol particles is strongly dependent on the location relative to the cloud layer (vicinity or below/above cloud). In general, the nitrate and organic fractions decrease with decreasing distance to the cloud, in the transit from cloud-free conditions towards the cloud boundaries. The decrease of nitrate and organic compounds ranges at a factor of three to ten, affecting sulfate and ammonium compounds to be increasingly abundant in the aerosol chemical composition while approaching the cloud layer. Finally, the chemical composition of non-refractory evaporated cloud droplets measured within the cloud shows increased fractions of nitrate and organics (with respect to concentrations found below clouds), but also large amounts of sulfate, thus, related to activation of particles, made up of soluble compounds. [ABSTRACT FROM AUTHOR]

An international field experiment took place in the Swiss Jura in January 2021 as a milestone of the European ICE GENESIS project (www.ice-genesis.eu/), which aims to better measure, understand, and model the ice/snow particle properties and mechanisms responsible for icing of rotor-craft and aircraft. The field campaign was designed to collect observations of clouds and snowfall at a prescribed range of temperatures (−10° to +2°C). The suite of in situ and remote sensing instruments included airborne probes and imagers on board a SAFIRE ATR-42 aircraft, able to sample liquid and ice particles from the micron to the millimeter size range, as well as icing sensors and cameras. Two 95 GHz Doppler cloud radars were installed on the SAFIRE ATR-42, while six Doppler weather radars operating at frequencies ranging from 10 to 95 GHz (and one lidar) were ground based. An operational polarimetric weather radar in nearby France (Montancy) complements the coverage. Finally, observations of standard meteorological variables as well as high-resolution pictures of falling snowflakes from a multiangle snowflake camera were collected at the ground level. The campaign showed its full potential during five (multihourly) flights where precipitation was monitored from cloud to ground. The originality of this campaign resides in the targeted specific temperature range for snowfall and in the synchronization between the ground-based remote sensing and the aircraft trajectories designed to maximize the collection of in situ observations within the column above the radar systems. [ABSTRACT FROM AUTHOR]

To understand tropospheric air pollution at regional and global scales, the SPIRIT (SPectromètre Infra-Rouge In situ Toute altitude) airborne instrument was developed and used on aircraft to measure volume mixing ratios of carbon monoxide (CO), an important indicator of air pollution, during the last decade. SPIRIT provides high-quality CO measurements with 1 σ precision of 0.3 ppbv at a time resolution of 1.6 s thanks to the coupling of a quantum cascade laser to a Robert optical multi-pass cell. It can be operated on different aircraft such as Falcon-20 and ATR-42 from the German Aerospace Agency (DLR) and from SAFIRE (CNRS-CNES-Météo France). With support from various projects, measurements were taken for more than 200 flight hours over three continents (Europe, Asia, and Africa), including two intercontinental transects (Europe–Asia and Europe–Africa). Levels of CO and its spatial distribution are briefly discussed and compared between different regions/continents. CO generally decreases with altitude except in some cases, indicating the important contribution of long-distance transport to CO levels. A 3D trajectory mapped by CO level was plotted for each flight and is presented in this study (which includes a Supplement). The database is archived in the AERIS database (10.25326/440), the French national center for atmospheric observations (Catoire et al., 2023). In addition, it could help to validate model performance and satellite measurements. For instance, the database covers measurements at high-latitude regions (i.e., Kiruna, Sweden, 68 ∘ N), where satellite measurements are still challenging, and at low-latitude regions (West Africa and Southeast Asia), where in situ data are scarce and satellites need more validation by airborne measurements. [ABSTRACT FROM AUTHOR]

A shallow cumulus cloud transition from a sugar to flower type of organization occurred under a layer of mineral dust on 2 February 2020, during the multinational Atlantic Tradewind Ocean‐Atmosphere Mesoscale Interaction Campaign (ATOMIC) and the Elucidating the Role of Clouds‐Circulation Coupling in Climate (EUREC4A) campaigns. Lagrangian large eddy simulations following an airmass trajectory along the tradewinds are used to explore radiative impacts of the diel cycle and mineral dust on the sugar‐to‐flower (S2F) cloud transition. The large‐scale meteorological forcing is derived from the European Center for Medium‐Range Weather Forecasts Reanalysis Fifth Generation and based on aerosol measurements from the U.S. Ronald H. Brown Research Vessel and the French ATR‐42 Research Aircraft during the field campaigns. A 12‐hr delay in the diel cycle accelerates the S2F transition at night, leading to more cloud liquid water and precipitation. The aggregated clouds generate more and stronger cold pools, which alter the original mechanism responsible for the organization. Although there is still mesoscale moisture convergence in the cloud layer, the near‐surface divergence associated with cold pools transports the subcloud moisture to the drier surrounding regions. New convection forms along the cold‐pool edges, generating new flower clouds. The modulation of the surface radiative budget by free‐tropospheric mineral dust poses a less dramatic effect on the S2F transition. Mineral dust releases longwave radiation, reducing the cloud amount at night, and absorbs shortwave radiation during the day, cooling the boundary‐layer temperature and increasing the overall cloud amount. Cloud‐top radiative heating because of more clouds strengthens the mesoscale organization, enlarging the aggregate areas, and increasing the cloud amount further. Plain Language Summary: During a joint field study called ATOMIC and EUREC4A, a transition between two cloud systems took place during the day on 2 February 2020. Very small and shallow clouds called "sugar" transitioned into deeper and wider cloud aggregates called "flowers." A dense mineral‐dust layer was also observed above the tradewind cumulus cloud field, likely modulating the radiation interacting with the clouds. High‐resolution simulations are applied to help understand the same cloud transition as if it had taken place at night, and to explore the impacts of mineral dust on the transition. A 12‐hr delay in the daily cycle such that the transition occurs at night affects the cloud transition more significantly than when the transition occurs during the day under a layer of mineral dust. The cloud transition that occurs at night produces more clouds and rain. The mineral dust blocks the solar radiation and cools the air beneath during the day, but does not change the cloud and rain amount as much. Key Points: The transition from sugar to flowers occurs more rapidly at night, producing more cloud and rain, with stronger organization and cold poolsPrecipitation and cold pools weaken the mechanism of cloud aggregation as they transport moisture to drier regions to form new convectionMineral dust above the clouds modulates radiative fluxes below leading to weaker mesoscale organization at night but stronger during the day [ABSTRACT FROM AUTHOR]

Profiles of eddy momentum flux divergence are calculated as the residual in the momentum budget constructed from airborne circular dropsonde arrays (∼$$ \sim $$220 km) for 13 days during the EUREC4$$ {}^4 $$A/ATOMIC field campaign. The observed dynamical forcing averaged over all flights agrees broadly with European Centre for Medium‐Range Weather Forecasts (ECMWF) Integrated Forecasting System (IFS) forecasts. In the direction of the flow, a mean flux divergence (friction) exists over a 1.5‐km deep Ekman layer, and a mean flux convergence (acceleration) is present near cloud tops. The friction is countergradient between 1 and 1.5 km, where vertical wind shear exceeds the observed thermal wind. From the frictional profile, a 10‐m momentum flux of ∼$$ \sim $$0.1 N·$$ \cdotp $$m−2$$ {}^{-2} $$ is derived, in line with Saildrone turbulence measurements. A momentum flux divergence in the cross‐wind direction is pronounced near the surface and acts to veer the wind, opposing the friction‐induced cross‐isobaric wind turning. Weaker friction and upper‐level acceleration of easterly flow are observed when stronger winds and more vigorous convection prevail. Turbulence measurements on board the SAFIRE ATR‐42 aircraft and the Uncrewed Aircraft System (UAS) RAAVEN reveal pronounced spatial variability of momentum fluxes, with a non‐negligible contribution of mesoscales (5–30 km). The findings highlight the nontrivial impact of turbulence, convection, and mesoscale flows in the presence of diverse cloud fields on the depth and strength of the frictional layer. [ABSTRACT FROM AUTHOR]

From 23 January to 13 February 2020, 20 ATR-42 scientific flights were conducted in the framework of the EUREC4A field campaign over the tropical Atlantic, off the coast of Barbados (13 ∘ 30 ′ N, - 58 ∘ 30 ′ W). By means of a sideway-pointing lidar, these flights allowed us to retrieve the optical properties of the aerosols found in the sub-cloud layer and below the trade wind inversion. Two distinct periods with significant aerosol contents were identified in relationship with the so-called trade wind and tropical regimes, respectively. For these two regimes, mixings of two air mass types encompassing dust and carbonaceous aerosols have been highlighted. Both were mainly from West Africa with similar optical contributions and linked to dust uptake above Sahara and biomass burning between Guinea-Bissau and Côte d'Ivoire. In the tropical transport regime, the wind within the planetary boundary layer is stronger and favours a contribution of marine aerosols (sulfate and sea salt aerosol components) in shallower aerosol layers than for the trade wind transport regime. The latter is responsible for advecting dust–biomass-burning-aerosol mixtures in the deeper, well-mixed layer, in part due to the complex interactions of the easterly flow from West Africa with mid-latitude dynamics. The aerosol vertical structures appear to be well reproduced using atmospheric composition reanalyses from CAMS when comparing with lidar-derived vertical profiles. The competition between the two types of transport regimes leads to strong heterogeneity in the optical properties of the horizontal aerosol field. Our study highlights the transport regime under which a significant mixture of dust and biomass burning aerosols from West Africa can be observed over the Caribbean and Barbados in particular, namely the trade wind regime. [ABSTRACT FROM AUTHOR]

To understand tropospheric air pollution at regional and global scales, the SPIRIT airborne instrument (SPectromètre Infra- Rouge In situ Toute altitude) was developed and used on aircraft to measure volume mixing ratios of carbon monoxide (CO), an important indicator of air pollution, during the last decade. SPIRIT could provide high-quality CO measurements with 1σ precision of 0.3 ppbv at a time resolution of 1.6 s thanks to the coupling of a quantum cascade laser to a Robert multi-pass cell. It can be operated on different aircraft such as Falcon-20 and ATR-42 from DLR (Germany) and SAFIRE (CNRS-CNES- Météo France). With support from various projects, more than 200 flight hours measurements were conducted over three continents (Europe, Asia, and Africa), including two inter-continental measurements (Europe-Asia and Europe-Africa). Levels of CO and its horizontal and vertical distribution are briefly discussed and compared between different regions/continents. CO generally decreases with altitude except for the measurements in high-latitude regions, indicating the important contribution of long-distance transport to CO levels at high-latitude regions. A 3D trajectory mapped by CO level was plotted for each flight and presented in this study. The database is archived on the AERIS database (https://doi.org/10.25326/440), the French national center for atmospheric observations (Catoire et al., 2023). Besides, it could help to validate model performances and satellite measurements. For instance, the database covers measurements at high-latitude regions (i.e., Kiruna, Sweden, 68°N) where satellite measurements are still challengeable and at low-latitude regions (West Africa and South-East Asia) where in situ data are scarce and satellites need more validation by airborne measurements. [ABSTRACT FROM AUTHOR]

Ozone data retrieved in the Arctic region from infrared radiance spectra recorded by the Infrared Atmospheric Sounding Interferometer (IASI) on board the MetOp-A European satellite are presented. They are compared with in situ and lidar observations obtained during a series of aircraft measurement campaigns as part of the International Polar Year POLARCAT activities in spring and summer 2008. Different air masses were sampled during the campaigns including clean air, polluted plumes originating from anthropogenic sources, forest fire plumes from the three northern continents, and stratospheric-influenced air masses. The comparison between IASI O3 [0-8km], [0-12 km] partial columns and profiles with collocated aircraft observations is achieved by taking into account the different sensitivity and geometry of the sounding instruments. A detailed analysis is provided and the agreement is discussed in terms of vertical sensitivity and surface properties at the location of the observations. Overall, IASI O3 profiles are found to be in relatively good agreement with smoothed in situ and lidar profiles in the free troposphere with differences of less than 40% (25% over sea for both seasons) and 10%, respectively. The correlation between IASI O3 retrieved partial columns and the smoothed aircraft partial columns is good with DC8 in situ data in spring over North America (r = 0.68), and over Greenland with ATR-42 lidar measurements in summer (r = 0.67). Correlations with other data are less significant highlighting the difficulty of IASI to capture precisely the O3 variability in the Arctic upper troposphere and lower stratosphere (UTLS). This is particularly noted in comparison with the [0-12 km] partial columns. The IASI [0-8 km] partial columns display a low negative bias (by less than 26% over snow) compared to columns derived from in situ measurements. Despite the relatively high biases of the IASI retrievals in the Arctic UTLS, our analysis shows that IASI can be used to identify, using O3 / CO ratios, stratospheric intrusions. [ABSTRACT FROM AUTHOR]

While the Sahelian belt in West Africa stretches in the border between the global hot-spots of mineral dust and biomass burning aerosols, the presence of West African Monsoon is expected to create significant vertical and temporal variations in the regional aerosol properties through transport and mixing of particles from various sources (mineral dust, biomass burning, sulfates, sea salt). In order to improve our understanding of the evolution of the aerosolcloud system over such region across the onset of the summer monsoon, the French ATR-42 research aircraft was deployed in Niamey, Niger (13°30′ N, 02°05′ E) in summer 2006, during the three special observation periods (SOPs) of the African Monsoon Multidisciplinary Analysis (AMMA) project. These three SOPs covered both dry and wet periods before and after the onset of the Western African Monsoon. State of the art physico-chemical aerosol measurements on the ATR-42 showed a notable seasonal transition in averaged number size distributions where (i) the Aitken mode is dominating over the accumulation mode during the dry season preceding the monsoon arrival and (ii) the accumulation mode increasingly gained importance after the onset of theWest African monsoon and even dominated the Aitken mode after the monsoon had fully developed. The parameters for the mean log-normal distributions observed in respective layers characterized by the different wind regimes (monsoon layer, SAL, free troposphere) are presented, together with the major particle compositions found in the accumulation mode particles. Thereby, results of this study should facilitate radiative transfer calculations, validation of satellite remote sensors, and detailed transport modeling by partners within and outside the AMMA community. Extended analysis of the chemical composition of single aerosol particles by a transmission electron microscope (TEM) coupled to an energy dispersive X-ray spectrometer (EDX) revealed dominance of mineral dust (aluminosilicate) even in the submicron particle size range during the dry period, gradually replaced by prevailing biomass burning and sulfate particles, after the onset of the monsoon period. The spatial and temporal evolution from SOP1 to SOP2a1 and SOP2a2 of the particle physical and chemical properties and associated aerosol hygroscopic properties are remarkably consistent. [ABSTRACT FROM AUTHOR]

From 23 January to 13 February 2020, 20 manned research flights were conducted over the tropical Atlantic, off the coast of Barbados (13∘30′ N, 58∘30′ W), to characterize the trade-wind clouds generated by shallow convection. These flights were conducted as part of the international EUREC 4 A (Elucidating the role of cloud–circulation coupling in climate) field campaign. One of the objectives of these flights was to characterize the trade-wind cumuli at their base for a range of meteorological conditions, convective mesoscale organizations and times of the day, with the help of sidewards-staring remote sensing instruments (lidar and radar). This paper presents the datasets associated with horizontal lidar measurements. The lidar sampled clouds from a lateral window of the aircraft over a range of about 8 km, with a horizontal resolution of 15 m, over a rectangle pattern of 20 km by 130 km. The measurements made possible the characterization of the size distribution of clouds near their base and the presence of dust-like aerosols within and above the marine boundary layer. This paper presents the measurements and the different levels of data processing, ranging from the raw Level 1 data (10.25326/57; Chazette et al., 2020c) to the Level 2 and Level 3 processed data that include a horizontal cloud mask (10.25326/58; Chazette et al., 2020b) and aerosol extinction coefficients (10.25326/59; Chazette et al., 2020a). An intermediate level, companion to Level 1 data (Level 1.5), is also available for calibrated and geolocalized data (10.25326/57; Chazette et al., 2020c). [ABSTRACT FROM AUTHOR]

Volcanic emissions can significantly affect the Earth's radiation budget by emitting aerosol particles and gas‐phase species that can result in the new particle formation (NPF). These particles can scatter solar radiation or modify cloud properties, with consequences on health, weather, and climate. To our knowledge, this is the first dedicated study detailing how gas‐phase precursors emitted from volcanic plumes can influence the NPF. A series of airborne measurements were performed around the Etna and Stromboli volcanoes within the framework of the CLerVolc and STRAP projects. The ATR‐42 aircraft was equipped with a range of instrumentation allowing the measurement of particle number concentration in diameter range above 2.5 nm and gaseous species to investigate the aerosol dynamics and the processes governing the NPF and their growth within the volcanic plumes. We demonstrate that NPF occurs within the volcanic plumes in the free troposphere (FT) and boundary layer (BL). Typically, the NPF events were more pronounced in the FT, where the condensational sink was up to two orders of magnitude smaller and the temperature was ~20 °C lower than in the BL. Within the passive volcanic plume, the concentration of sulfur dioxide, sulfuric acid, and N2.5 were as high as 92 ppbV, 5.65 × 108 and 2.4 × 105 cm−3, respectively. Using these measurements, we propose a new parameterization for NPF rate (J2.5) within the passive volcanic plume in the FT. These results can be incorporated into mesoscale models to better assess the impact of the particle formed by natural processes, that is, volcanic plumes, on climate. Key Points: New particle formation was evidenced to occur within different volcanic plumes of Etna and Stromboli and was more pronounced in the free troposphereThe growth of the newly formed particles to the CCN active size was observed to occur within the volcanic plumes in different ratesA novel parameterization rate of new particle formation within the Etna's volcanic passive plume was proposed based on the actual measurements [ABSTRACT FROM AUTHOR]

The western Mediterranean atmosphere is impacted by a variety of aerosol sources, producing a complex and variable mixture of natural and anthropogenic particles, with different chemical and physical properties. Satellite sensors provide a useful global coverage of aerosol parameters but through indirect measurements that require careful validation. Here we present the results of a long-term regional scale analysis of the full dataset (March 2005 and October 2013) of POLDER-3/PARASOL ocean operational retrievals of the total, fine, and coarse aerosol optical depth (AOD, AOD F , and AOD C), Ångström exponent (AE), and the spherical or non-spherical partition of coarse-mode AOD (AOD CS and AOD CNS), respectively. The evaluation is performed using data from 17 coastal and insular ground-based AERONET sites on one side, and airborne vertical profiles of aerosol extinction and number size distribution obtained by the SAFIRE ATR-42 aircraft operated in the area during summer 2012 and 2013 on the other side. This study provides the first regional evaluation of uncertainties of the POLDER-3 products, and highlights their quality. The POLDER-3 Ångström exponent, representing AOD spectral dependence in link with the aerosol particle size distribution, is biased towards small values. This bias, however, does not prevent using AE for classifying the regional aerosol laden air masses. AOD F corresponds to particles smaller than 0.6–0.8 µm in diameter and appears suitable to monitor the aerosol submicron fraction from space. We also provide an original validation of POLDER-3 AOD C and its spherical or non-spherical partition, which shows agreement within 25 % with AERONET shape retrievals when the aerosol coarse fraction dominates. [ABSTRACT FROM AUTHOR]

Carbon fiber (CF) is highly valued for its exceptional strength-to-weight relation, making it best for energy-efficient applications in aerospace, automotive, and construction sectors. Recent advancements in CF technology have reduced production costs, enhancing market growth. Carbon fiber-reinforced polymer (CFRP) composites offer benefits such as fatigue resistance, weight reduction, stiffness, and corrosion resistance. The choice of matrix material, particularly thermoplastics, impacts CFRP properties, with thermoplastics favored for recyclability and mass production. Fabrication techniques like filament winding and resin transfer molding ensure precise CF alignment but have complexities. Additive manufacturing (AM) methods, such as FDM, DLP, and SLA, provide design flexibility and efficiency. Recycling approaches, including thermal, mechanical, and chemical methods, address CFRP waste. This review offers an overview of AM technologies in CFRP manufacturing, focusing on advancements in continuous, short, and nano carbon fiber composites, their properties, manufacturing methods, and recycling techniques, as well as their applications and topological optimization. [ABSTRACT FROM AUTHOR]

Atmospheric aerosols impact the Earth's climate system directly by scattering and absorbing solar radiation, and it is important to characterise the aerosol optical properties in detail. This study reports the development and validation of an airborne dual-wavelength cavity-attenuated phase-shift (CAPS) single monitor, named A2S2 (Aerosol Absorption Spectral Sizer), based on the commercial CAPS single-scattering albedo monitor (CAPS-PM SSA ; Aerodyne), to simultaneously measure the aerosol optical scattering and extinction at both 450 and 630 nm wavelengths. Replaced pressure and temperature sensors and an additional flow control system were incorporated into the A2S2 for its utilisation on board research aircraft measuring within the troposphere. The evaluation of A2S2 characteristics was performed in the laboratory and included the investigation of the signal-to-noise ratio, validation of performance at various pressure levels, optical closure studies and intercomparing with the currently validated techniques. The chamber experiments show that the A2S2 can perform measurements at sample pressures as low as 550 hPa and at sample temperatures as high as 315 K. Based on the Allan analysis results, we have evaluated that the minimum detection limit of the measurements shows that the measurements have a limit accuracy of ∼ 2 Mm-1 at 450 nm and ∼ 1 Mm-1 at 630 nm for 1 Hz measurements of both scattering coefficients (σsca) and extinction coefficients (σext). The optical closure study with size-selected polystyrene latex (PSL) particles shows that the truncation error of the A2S2 is negligible for particles with particle volume diameter (Dp) < 200 nm, while, for the larger sub-micrometre particles, the measurement uncertainty of A2S2 increases but remains less than 20 %. The average factors to correct the truncation error are 1.13 and 1.05 for 450 and 630 nm, respectively. A simplified truncation correction, dependent on the scattering Ångström exponent (SAE), was developed to rectify truncation errors of the future A2S2 field measurement data. The σsca and σext measured by the A2S2 show good agreement with the concurrent measured results from the nephelometer and the CAPS particle extinction monitor (CAPS-PM ex). The absorption coefficient (σabs) derived through the extinction-minus-scattering (EMS) method by the A2S2 also corresponds with the results obtained from the aethalometer. The A2S2 was successfully deployed during an aircraft measurement campaign (Atmospheric ChemistRy Of the Suburban foreSt – ACROSS) conducted in the vicinity of Paris and the surrounding regions. The average SSA measured during the entire ACROSS flight campaign is 0.86 and 0.88 at 450 and 630 nm, respectively, suggesting that light-absorbing organic aerosols play a significant role. The average SAE and absorption Ångström exponent (AAE) varied due to measurements in various pollution conditions. The results presented in this study indicate that the A2S2 instrument is reliable for measuring aerosol σsca and σext at both blue and red wavelengths, and it stands as a viable substitute for future airborne evaluations of aerosol optical properties. [ABSTRACT FROM AUTHOR]

Ozone data retrieved in the Arctic region from infrared radiance spectra recorded by the Infrared Atmospheric Sounding Interferometer (IASI) on board the MetOp-A European satellite are presented. They are compared with in situ and lidar observations obtained during a series of aircraft measurement campaigns as part of the International Polar Year (IPY) POLARCAT activities in spring and summer 2008. Different air masses were sampled during the campaigns including clean air, polluted plumes originating from anthropogenic sources, forest fire plumes from the three northern continents, and stratospheric-influenced air masses. The comparison between IASI O3 [0-8 km], [0-12 km] partial columns and profiles with collocated aircraft observations is achieved by taking into account the different sensitivity and geometry of the sounding instruments. A detailed analysis is provided and the agreement is discussed in terms of information content and surface properties at the location of the observations. Overall, IASI O3 profiles are found to be in relatively good agreement in the free troposphere with smoothed in situ and lidar profiles with differences less than 40% (25% over the sea for both seasons) and 10 %, respectively. The correlation between IASI O3 retrieved partial columns and the smoothed aircraft partial columns is good with DC-8 in situ data in spring over North American forest fire regions (r = 0.68), and over Greenland with ATR-42 lidar measurements in summer (r =0.67). Correlations with other data are less significant highlighting the difficulty with which IASI is able to capture O3 variability in the Arctic upper troposphere and lower stratosphere (UTLS) with sufficient precision as noted in comparison with the [0-12 km] partial columns. However the [0-8 km] partial columns show good results with IASI which displays a negative bias (maximum of 26% over snow) compared to columns derived from in situ measurements. Despite these difficulties in the Arctic UTLS, this work also shows that IASI can be used to study particular cases where stratospheric intrusions are present using a O3/CO ratio diagnostic. [ABSTRACT FROM AUTHOR]

Within the framework of the POLARCAT-France campaign, aerosol physical, chemical and optical properties over Greenland were measured onboard the French ATR-42 research aircraft. The origins of CO excess peaks detected in the aircraft measurements then have been identified through FLEXPART simulations. The study presented here focuses particularly on the characterization of air masses transported from the North American continent to Greenland. Air masses that picked up emissions from Canadian boreal forest fires as well as from the cities on the American east coast were identified and selected for a detailed study. Measurements of CO concentrations, aerosol chemical composition, aerosol number size distributions, aerosol volume volatile fractions and aerosol light absorption (mainly from black carbon) are used in order to study the relationship between CO enhancement (ΔCO), aerosol particle concentrations and number size distributions. Aerosol number size distributions (normalised with their respective ΔCO) are in good agreement with previous studies. Nonetheless, wet scavenging may have occurred along the pathway between the emission sources and Greenland leading to a less pronounced accumulation mode in the POLARCAT data. Chemical analyses from mass spectrometry show that submicrometer aerosol particles are mainly composed of sulphate and organics. The observed bimodal (Aitken and accumulation) aerosol number size distributions show a significant enhancement in Aitken mode particles. Furthermore, results from the thermodenuder analysis demonstrate the external mixture of boreal fire (BF) air masses from North America (NA). This is particularly observed in the accumulation mode, containing a volume fraction of up to 25-30% of refractory material at the applied temperature of 280 °C. NA anthropogenic air masses with only 6% refractory material in the accumulation mode can be clearly distinguished from BF air masses. Overall, during the campaign rather small amounts of black carbon from the North American continent were transported towards Greenland during the summer POLARCAT observation period, which also is a valuable finding with respect to potential climate impacts of black carbon in the Arctic. [ABSTRACT FROM AUTHOR]

While West Africa is recognized as being one of the global hot-spots of atmospheric aerosols, the presence of West African Monsoon is expected to create significant spatial and temporal variations in the regional aerosol properties through mixing particles from various sources (mineral dust, biomass burning, sulfates, sea salt). To improve our understanding of the complexity of the aerosol-cloud system in that region, the African Monsoon Multidisciplinary Analysis (AMMA) project has been launched, providing valuable data sets of in-situ and remote sensing measurements including satellites for extended modeling. The French ATR-42 research aircraft was deployed in Niamey, Niger (13°300 N, 02°050 E) in summer 2006, during the three special observation periods (SOPs) of AMMA. These three SOPs covered both dry and wet periods before and after the onset of the Western African Monsoon. State of the art physico-chemical aerosol measurements on the ATR-42 showed a notable seasonal transition in averaged number size distributions where (i) the Aitken mode is dominating over the accumulation mode during the dry season preceding the monsoon arrival and (ii) the accumulation mode increasingly gained importance after the onset of the West African monsoon and even dominated the Aitken mode after the monsoon had fully developed. An extended analysis of the vertical dependence of size spectra, comparing the three observation periods, revealed that the decreasing concentration of the Aitken mode particles, as we move from SOP1 (June) to SOP2a1 (July), and SOP2a2 (August), was less pronounced in the monsoon layer as compared to the overlying Saharan dust layer and free troposphere. In order to facilitate to all partners within the AMMA community radiative transfer calculations, validation of satellite remote sensors, and detailed transport modeling, the parameters describing the mean log-normally fitted number size distributions as a function of altitude and special observation periods were summarized and subsequently related to simultaneously performed measurements of major aerosol particle chemical composition. Extended TEM-EDX analysis of the chemical composition of single aerosol particles revealed dominance of mineral dust (aluminosilicate) even in the submicron particle size range during the dry period, gradually replaced by prevailing biomass burning and sulfate particles, after the onset the monsoon period. The spatial and temporal evolution from SOP1 to SOP2a1 and SOP2a2 of the particle physical and chemical properties and associated aerosol hygroscopic properties are remarkably consistent. [ABSTRACT FROM AUTHOR]

A large dataset of reactive trace gases was collected for the first time over West Africa during the African Monsoon Multidisciplinary Analysis (AMMA) field experiment in August 2006. Volatile Organic Compounds (VOC from C5-C9) were measured onboard the two French aircrafts the ATR-42 and the Falcon-20 by a new instrument AMOVOC. The goal of this study is (i) to characterize VOC distribution in the tropical region of West Africa (ii) to determine the impact of deep convection on VOC distribution and chemistry in the tropical upper troposphere (UT) and (iii) to characterize its spatial and temporal extensions. Experimental strategy consisted in sampling at altitudes between 0 and 12 km downwind of Mesoscale Convective Systems (MCS) and at cloud base. Biogenic and anthropogenic VOC distribution in West Africa is clearly affected by North to South emission gradient. Isoprene, the most abundant VOC, is at maximum level over the forest (1.26 ppb) while benzene reaches its maximum over the urban areas (0.11 ppb). First, a multiple physical and chemical tracers approach using CO, O3 and relative humidity was implemented to distinguish between convective and non-convective air masses. Then, additional tools based on VOC observations (tracer ratios, proxy of emissions and photochemical clocks) were adapted to characterize deep convection on a chemical, spatial and temporal basis. VOC vertical profiles show a "C-shaped" trend indicating that VOC-rich air masses are transported from the sur face to the UT by deep convective systems. VOC mixing ratios in convective outflow are up to two times higher than background levels even for reactive and short-lived VOC (e.g. isoprene up to 0.19 ppb at 12 km-altitude) and are dependent on surface emission type. As a consequence, UT air mass reactivity increases from 0.52 s-1 in non-convective conditions to 0.95 s-1 in convective conditions. Fractions of boundary layer air contained in convective outflow are estimated to be 40±15%. Vertical transport timescale is calculated to be 25±10 min. These results characterize deep convection occurring over West Africa and provide relevant information for tropical convection parameterization in regional/global models. [ABSTRACT FROM AUTHOR]

From 23 January to 13 February 2020, twenty ATR-42 scientific flights were conducted in the framework of the EUREC4A field campaign over the tropical Atlantic, off the coast of Barbados (-58°30'°W 13°30' N). By means of a side-pointing lidar, these flights allowed to retrieve the optical properties of the aerosols found in the sub-cloud layer and below the trade winds inversion. Two distinct periods with significant aerosol contents were identified in relationship with the so-called trade wind and tropical regimes, respectively. A very strong spatial heterogeneity of the aerosol field has been highlighted at the airborne measurements scale of a few tens of kilometres. This heterogeneity, difficult to capture using spaceborne instruments, can be related to the highly variable relative humidity field and the fractional cloud cover encountered during all the flights. [ABSTRACT FROM AUTHOR]

The Chemistry-Aerosol Mediterranean Experiment (ChArMEx; http://charmex.lsce.ipsl.fr) is a collaborative research program federating international activities to investigate Mediterranean regional chemistry-climate interactions. A special observing period (SOP-1a) including intensive airborne measurements was performed in the framework of the Aerosol Direct Radiative Impact on the regional climate in the MEDiterranean region (ADRIMED) project during the Mediterranean dry season over the western and central Mediterranean basins, with a focus on aerosol-radiation measurements and their modeling. The SOP-1a took place from 11 June to 5 July 2013. Airborne measurements were made by both the ATR-42 and F-20 French research aircraft operated from Sardinia (Italy) and instrumented for in situ and remote-sensing measurements, respectively, and by sounding and drifting balloons, launched in Minorca. The experimental setup also involved several ground-based measurement sites on islands including two ground-based reference stations in Corsica and Lampedusa and secondary monitoring sites in Minorca and Sicily. Additional measurements including lidar profiling were also performed on alert during aircraft operations at EARLINET/ACTRIS stations at Granada and Barcelona in Spain, and in southern Italy. Remote-sensing aerosol products from satellites (MSG/SEVIRI, MODIS) and from the AERONET/PHOTONS network were also used. Dedicated meso-scale and regional modeling experiments were performed in relation to this observational effort. We provide here an overview of the different surface and aircraft observations deployed during the ChArMEx/ADRIMED period and of associated modeling studies together with an analysis of the synoptic conditions that determined the aerosol emission and transport. Meteorological conditions observed during this campaign (moderate temperatures and southern flows) were not favorable to producing high levels of atmospheric pollutants or intense biomass burning events in the region. However, numerous mineral dust plumes were observed during the campaign, with the main sources located in Morocco, Algeria and Tunisia, leading to aerosol optical depth (AOD) values ranging between 0.2 and 0.6 (at 440 nm) over the western and central Mediterranean basins. One important point of this experiment concerns the direct observations of aerosol extinction onboard the ATR-42, using the CAPS system, showing local maxima reaching up to 150Mm-1 within the dust plume. Non-negligible aerosol extinction (about 50Mm-1) has also been observed within the marine boundary layer (MBL). By combining the ATR-42 extinction coefficient observations with absorption and scattering measurements, we performed a complete optical closure revealing excellent agreement with estimated optical properties. This additional information on extinction properties has allowed calculation of the dust single scattering albedo (SSA) with a high level of confidence over the western Mediterranean. Our results show a moderate variability from 0.90 to 1.00 (at 530 nm) for all flights studied compared to that reported in the literature on this optical parameter. Our results underline also a relatively low difference in SSA with values derived near dust sources. In parallel, active remote-sensing observations from the surface and onboard the F-20 aircraft suggest a complex vertical structure of particles and distinct aerosol layers with sea spray and pollution located within the MBL, and mineral dust and/or aged North American smoke particles located above (up to 6–7 km in altitude). Aircraft and balloon-borne observations allow one to investigate the vertical structure of the aerosol size distribution showing particles characterized by a large size (> 10 μm in diameter) within dust plumes. In most of cases, a coarse mode characterized by an effective diameter ranging between 5 and 10 μm, has been detected above the MBL. In terms of shortwave (SW) direct forcing, in situ surface and aircraft observations have been merged and used as inputs in 1-D radiative transfer codes for calculating the aerosol direct radiative forcing (DRF). Results show significant surface SW instantaneous forcing (up to -90Wm-2 at noon). Aircraft observations provide also original estimates of the vertical structure of SW and LW radiative heating revealing significant instantaneous values of about 5° K per day in the solar spectrum (for a solar angle of 30°) within the dust layer. Associated 3-D modeling studies from regional climate (RCM) and chemistry transport (CTM) models indicate a relatively good agreement for simulated AOD compared with observations from the AERONET/PHOTONS network and satellite data, especially for long-range dust transport. Calculations of the 3-D SW (clear-sky) surface DRF indicate an average of about -10 to -20Wm-2 (for the whole period) over the Mediterranean Sea together with maxima (-50Wm-2) over northern Africa. The top of the atmosphere (TOA) DRF is shown to be highly variable within the domain, due to moderate absorbing properties of dust and changes in the surface albedo. Indeed, 3-D simulations indicate negative forcing over the Mediterranean Sea and Europe and positive forcing over northern Africa. Finally, a multiyear simulation, performed for the 2003 to 2009 period and including an ocean–atmosphere (O–A) coupling, underlines the impact of the aerosol direct radiative forcing on the sea surface temperature, O–A fluxes and the hydrological cycle over the Mediterranean. [ABSTRACT FROM AUTHOR]

The Chemistry-Aerosol Mediterranean Experiment (ChArMEx; http://charmex.lsce.ipsl. fr) is a collaborative research program federating international activities to investigate Mediterranean regional chemistry-climate interactions. A special observing period (SOP-1a) including intensive airborne measurements was performed in the framework of the Aerosol Direct Radiative Forcing on the Mediterranean Climate (ADRIMED) project during the Mediterranean dry season over the western and central Mediterranean basins, with a focus on aerosol-radiation measurements and their modeling. The SOP-1a took place from 11 June to 5 July 2013. Airborne measurements were made by both the ATR-42 and F-20 French research aircraft operated from Sardinia (Italy) and instrumented for in situ and remote-sensing measurements, respectively, and by sounding and drifting balloons, launched in Minorca. The experimental setup also involved several ground-based measurement sites on islands including two ground-based reference stations in Corsica and Lampedusa and secondary monitoring sites in Minorca and Sicily. Additional measurements including lidar profiling were also performed on alert during aircraft operations at EARLINET/ACTRIS stations at Granada and Barcelona in Spain, and in southern Italy. Remote sensing aerosol products from satellites (MSG/SEVIRI, MODIS) and from the AERONET/PHOTONS network were also used. Dedicated meso-scale and regional modelling experiments were performed in relation to this observational effort. We provide here an overview of the different surface and aircraft observations deployed during the ChArMEx/ADRIMED period and of associated modeling studies together with an analysis of the synoptic conditions that determined the aerosol emission and transport. Meteorological conditions observed during this campaign (moderate temperatures and southern flows) were not favorable to produce high level of atmospheric pollutants nor intense biomass burning events in the region. However, numerous mineral dust plumes were observed during the campaign with main sources located in Morocco, Algeria and Tunisia, leading to aerosol optical depth (AOD) values ranging between 0.2 to 0.6 (at 440 nm) over the western and central Mediterranean basins. Associated aerosol extinction values measured on-board the ATR-42 within the dust plume show local maxima reaching up to 150 Mm-1. Non negligible aerosol extinction (about 50 Mm-1) was also been observed within the Marine Boundary Layer (MBL). By combining ATR-42 extinction, absorption and scattering measurements, a complete optical closure has been made revealing excellent agreement with estimated optical properties. Associated calculations of the dust single scattering albedo (SSA) have been conducted, which show a moderate variability (from 0.90 to 1.00 at 530 nm). In parallel, active remote-sensing observations from the surface and onboard the F-20 aircraft suggest a complex vertical structure of particles and distinct aerosol layers with sea-salt and pollution located within the MBL, and mineral dust and/or aged north American smoke particles located above (up to 6-7 km in altitude). Aircraft and balloon-borne observations show particle size distributions characterized by large aerosols (> 10 μm in diameter) within dust plumes. In terms of shortwave (SW) direct forcing, in-situ surface and aircraft observations have been merged and used as inputs in 1-D radiative transfer codes for calculating the direct radiative forcing (DRF). Results show significant surface SW instantaneous forcing (up to -90 Wm-2 at noon). Associated 3-D modeling studies from regional climate (RCM) and chemistry transport (CTM) models indicate a relatively good agreement for simulated AOD compared with measurements/observations from the AERO NET/PHOTONS network and satellite data, especially for long-range dust transport. Calculations of the 3-D SW (clear-sky) surface DRF indicate an average of about -10 to -20 Wm-2 (for the whole period) over the Mediterranean Sea together with maxima (-50 W m-2) over northern Africa. The top of the atmosphere (TOA) DRF is shown to be highly variable within the domain, due to moderate absorbing properties of dust and changes in the surface albedo. Indeed, 3-D simulations indicate negative forcing over the Mediterranean Sea and Europe and positive forcing over northern Africa. [ABSTRACT FROM AUTHOR]

From 23 January to 13 February 2020, twenty ATR-42 flights were conducted over the tropical Atlantic, off the coast of Barbados (-58°30' W 13°30' N), to characterize the trade-wind clouds generated by shallow convection. These flights were conducted as part of the international EUREC4A (Elucidating the role of clouds-circulation coupling in climate) field campaign. One of the objectives of these flights was to characterize the trade-wind cumuli at their base for a range of meteorological conditions, convective mesoscale organizations and times of the day, with the help of sidewards staring remote sensing (lidar and radar). This paper presents the datasets associated with horizontal lidar measurements. The lidar sampled clouds from a lateral window of the aircraft over a range of about 8 km, with a horizontal resolution of 15 to 30 m, over a rectangle pattern of 20 km by 130 km. The measurements made it possible to characterize the size distribution of clouds near their base, and the presence of dust-like aerosols within and above the marine boundary layer. This paper presents the measurements and the different levels of data processing, ranging from raw level 1 data (https://doi.org/10.25326/57; Chazette et al., 2020c) to level 2 and 3 processed data that include an horizontal cloud mask (https://doi.org/10.25326/58; Chazette et al., 2020b) and aerosol extinction coefficients (https://doi.org/10.25326/59; Chazette et al., 2020a). An intermediate level, companion to the level 1 data (level 1.5), is also available for calibrated and geolocalized data (https://doi.org/10.25326/57; Chazette et al., 2020c). [ABSTRACT FROM AUTHOR]

Naturally available, stable, and heavy water molecules such as HDO and H 218 O have a lower saturation vapour pressure than the most abundant light water molecule H 216 O; therefore, these heavy water molecules preferentially condense and rain out during cloud formation. Stable water isotope observations thus have the potential to provide information on cloud processes in the trade-wind region, in particular when combined with high-resolution model simulations. In order to evaluate this potential, nested COSMO iso (isotope-enabled Consortium for Small Scale Modelling;) simulations with explicit convection and horizontal grid spacings of 10, 5, and 1 km were carried out in this study over the tropical Atlantic for the time period of the EUREC 4 A (Elucidating the role of clouds-circulation coupling in climate;) field experiment. The comparison to airborne in situ and remote sensing observations shows that the three simulations are able to distinguish between different mesoscale cloud organisation patterns as well as between periods with comparatively high and low rain rates. Cloud fraction and liquid water content show a better agreement with aircraft observations with higher spatial resolution, because they show strong spatial variations on the scale of a few kilometres. A low-level cold-dry bias, including too depleted vapour in the subcloud and cloud layer and too enriched vapour in the free troposphere, is found in all three simulations. Furthermore, the simulated secondary isotope variable d -excess in vapour is overestimated compared to observations. Special attention is given to the cloud base level, which is the formation altitude of shallow cumulus clouds. The temporal variability of the simulated isotope variables at cloud base agrees reasonably well with observations, with correlations of the flight-to-flight data as high as 0.7 for δ2 H and d -excess. A close examination of isotopic characteristics under precipitating clouds, non-precipitating clouds, clear-sky and dry-warm patches at the altitude of cloud base shows that these different environments are represented faithfully in the model with similar frequencies of occurrence, isotope signals, and specific-humidity anomalies as found in the observations. Furthermore, it is shown that the δ2 H of cloud base vapour at the hourly timescale is mainly controlled by mesoscale transport and not by local microphysical processes, while the d -excess is mainly controlled by large-scale drivers. Overall, this evaluation of COSMO iso , including the isotopic characterisation of different cloud base environments, suggests that the simulations can be used for investigating the role of atmospheric circulations on different scales for controlling the formation of shallow cumulus clouds in the trade-wind region, as will be done in part 2 of this study. [ABSTRACT FROM AUTHOR]

The adoption of hybrid–electric propulsion, allowing us to partially replace fuel with batteries and to reduce aircraft in-flight emissions, represents one of the main investigated solutions to mitigate the aviation climate impact. Despite its environmental potential being appealing for a practical application, two main drawbacks limit the actual implementation of this technology: first, the low gravimetric energy density of the batteries restricts hybrid–electric aircraft payload and range capabilities; second, the production of electricity is currently not entirely based on renewable energy sources, hence a non-direct emissions budget may limit the benefit in terms of overall decarbonization. When designing hybrid–electric aircraft, even projecting its actual entry into service in the next decades, it is necessary to take these limitations into account depending on both the more reliable technological forecasts on the development of electric components and on the estimates of electricity production. A proper analysis of the figure of merits related to the operation of such an aircraft, therefore, becomes crucial in assessing the impact related to its introduction into service. In this context, trade-offs between different performance metrics may be needed to efficiently exploit the environmental benefits of such an advanced concept, while limiting the possible drawbacks coming from its utilisation. This paper provides a performance analysis of hybrid–electric aircraft through an assessment of the relevant figures of merit characterizing its operations. In particular, direct and non-direct emissions, climate impact, ground pollution, operating costs, fuel consumption, weight, and a combination of these figures of merit allow us to define a proper development perimeter in which a possible (future) hybrid–electric aircraft can express its maximum potential towards all the aspects of its utilisation. The trade-off analyses provided in this paper allow us to identify more effective paths for the actual development of hybrid–electric aircraft, highlighting the impact of the selected design variables on the performance metrics, and bringing to light also the possible related limitations. [ABSTRACT FROM AUTHOR]

There is a need for improved wind measurements inside the planetary boundary layer (PBL), including the capability to sample turbulent flow. Airborne Doppler lidar (ADL) provides unique capabilities for spatially resolved and targeted wind measurements in the PBL. However, ADL wind profiling in the PBL is challenging, as turbulence violates the flow homogeneity assumption used in wind profile retrieval and thereby introduces error in the retrieved wind profiles. As turbulence is a dominant source of error it is necessary to investigate and optimize ADL wind profiling capabilities in turbulent PBL flow. This study investigates the potential of a novel multiple-fixed-beam ADL system design to provide improved wind information in turbulent PBL flow compared to traditional single-scanning-beam ADL systems. To achieve this, an LES-based (LES: large eddy simulation) airborne Doppler lidar simulator presented in is employed and extended in this study. Results show that a multiple-fixed-beam system with settings comparable to those of commonly used single-scanning-beam systems offers distinct advantages. Advantages include overall reduced wind profile retrieval error due to turbulence and improved spatial representation alongside higher wind profile availability. The study also offers insight into the dependence of the retrieval error on system setup parameters and retrieval parameters for both fixed-beam and scanning-beam systems. When using a fixed-beam system, an order of magnitude higher wind profile resolution appears possible compared to traditional scanning systems at comparable retrieval accuracy. Thus, using multiple-fixed-beam systems opens the door to better sampling of turbulent PBL flow. Overall, the simulator provides a cost-effective tool to investigate and optimize wind profile error characteristics due to turbulence and to optimize system setup and retrieval strategies for ADL wind profiling in turbulent flow. [ABSTRACT FROM AUTHOR]

This research paper delves into the longitudinal wind tunnel tests conducted on the 19-passengers aircraft model of the Italian PROSIB project. The concept is an innovative small air transport airplane with distributed propellers and hybrid-electric powerplant. The primary objective was to assess its stability and control characteristics in power-off conditions. In addition to the usual investigation of the aircraft components, the study introduced a belly-mounted pod, which served as a battery storage unit, and explored two distinct tail configurations: a body-mounted (low) tail and a T-tail (high). The results obtained from these tests generally confirmed the anticipated characteristics of the aircraft design. The experiments provided data on aerodynamic forces and moments, giving useful indications on the effects of a belly-mounted battery storage unit and tail layout on the aircraft stability and control characteristics. This information could be used by aircraft designers to size an airplane of the same class. [ABSTRACT FROM AUTHOR]

The MEGAPOLI (Megacities: Emissions, urban, regional and Global Atmospheric POLlution and climate effects, and Integrated tools for assessment and mitigation) experiment took place in July 2009. The aim of this campaign was to study the aging and reactions of aerosol and gas-phase emissions in the city of Paris. Three ground-based measurement sites and several mobile platforms including instrument equipped vehicles and the ATR-42 aircraft were involved. We present here the variations in particle- and gas-phase species over the city of Paris, using a combination of high-time resolution measurements aboard the ATR-42 aircraft. Particle chemical composition was measured using a compact time-of-flight aerosol mass spectrometer (C-ToF-AMS), giving detailed information on the non-refractory submicron aerosol species. The mass concentration of black carbon (BC), measured by a particle absorption soot photometer (PSAP), was used as a marker to identify the urban pollution plume boundaries. Aerosol mass concentrations and composition were affected by air-mass history, with air masses that spent longest time over land having highest fractions of organic aerosol and higher total mass concentrations. The Paris plume is mainly composed of organic aerosol (OA), BC, and nitrate aerosol, as well as high concentrations of anthropogenic gas-phase species such as toluene, benzene, and NOx. Using BC and CO as tracers for air-mass dilution, we observe the ratio of ΔOA/ΔBC and ΔOA/ΔCO increase with increasing photochemical age (-log(NOx/NOy)). Plotting the equivalent ratios of different organic aerosol species (LV-OOA, SV-OOA, and HOA) illustrate that the increase in OA is a result of secondary organic aerosol (SOA) formation. Within Paris the changes in the ΔOA/ΔCO are similar to those observed during other studies in London, Mexico City, and in New England, USA. Using the measured SOA volatile organic compounds (VOCs) species together with organic aerosol formation yields, we were able to predict ~ 50 % of the measured organics. These airborne measurements during the MEGAPOLI experiment show that urban emissions contribute to the formation of OA and have an impact on aerosol composition on a regional scale. [ABSTRACT FROM AUTHOR]

To understand tropospheric air pollution at regional and global scales, the SPIRIT (SPectromètre Infra-Rouge In situ Toute altitude) airborne instrument was developed and used on aircraft to measure volume mixing ratios of carbon monoxide (CO), an important indicator of air pollution, during the last decade. SPIRIT provides high-quality CO measurements with 1σ precision of 0.3 ppbv at a time resolution of 1.6 s thanks to the coupling of a quantum cascade laser to a Robert optical multi-pass cell. It can be operated on different aircraft such as Falcon-20 and ATR-42 from the German Aerospace Agency (DLR) and from SAFIRE (CNRS-CNES-Météo France). With support from various projects, measurements were taken for more than 200 flight hours over three continents (Europe, Asia, and Africa), including two intercontinental transects (Europe–Asia and Europe–Africa). Levels of CO and its spatial distribution are briefly discussed and compared between different regions/continents. CO generally decreases with altitude except in some cases, indicating the important contribution of long-distance transport to CO levels. A 3D trajectory mapped by CO level was plotted for each flight and is presented in this study (which includes a Supplement). The database is archived in the AERIS database (https://doi.org/10.25326/440), the French national center for atmospheric observations (Catoire et al., 2023). In addition, it could help to validate model performance and satellite measurements. For instance, the database covers measurements at high-latitude regions (i.e., Kiruna, Sweden, 68∘ N), where satellite measurements are still challenging, and at low-latitude regions (West Africa and Southeast Asia), where in situ data are scarce and satellites need more validation by airborne measurements.

The MEGAPOLI experiment took place in July 2009. The aim of this campaign was to study the aging and reactions of aerosol and gas-phase emissions in the city of Paris. Three ground-based measurement sites and several mobile platforms including instrument equipped vehicles and the ATR-42 aircraft were involved. We present here the variations in particle- and gas-phase species over the city of Paris using a combination of high-time resolution measurements aboard the ATR-42 aircraft. Particle chemical composition was measured using a compact time-of-flight aerosol mass spectrometer (C-ToF-AMS) giving detailed information of the non-refractory submicron aerosol species. The mass concentration of BC, measured by a particle absorption soot photometer (PSAP), was used as a marker to identify the urban pollution plume boundaries. Aerosol mass concentrations and composition were affected by air-mass history, with air masses that spent longest time over land having highest fractions of organic aerosol and higher total mass concentrations. The Paris plume is mainly composed of organic aerosol (OA), black carbon and nitrate aerosol, as well as high concentrations of anthropogenic gas-phase species such as toluene, benzene, and NOx. Using BC and CO as tracers for air-mass dilution, we observe the ratio of ΔOA/Δ BC and ΔOA/Δ CO increase with increasing photochemical age (-log(NOx/NOy)). Plotting the equivalent ratios for the Positive Matrix Factorization (PMF) resolved species (LV-OOA, SV-OOA, and HOA) illustrate that the increase in OA is a result of secondary organic aerosol (SOA). Within Paris the changes in the ΔOA/Δ CO are similar to those observed during other studies in Mexico city, Mexico and in New England, USA. Using the measured VOCs species together with recent organic aerosol formation yields we predicted ~50% of the measured organics. These airborne measurements during the MEGAPOLI experiment show that urban emissions contribute to the formation of OA, and have an impact on aerosol composition on a regional scale. They provide a quantitative measure of this impact in terms of urban plume composition and evolution relative to background aerosol composition. [ABSTRACT FROM AUTHOR]

Ozone pollution transported to the Arctic is a significant concern because of the rapid, enhanced warming in high northern latitudes, which is caused, in part, by shortlived climate forcers, such as ozone. Long-range transport of pollution contributes to background and episodic ozone levels in the Arctic. However, the extent to which plumes are photochemically active during transport, particularly during the summer, is still uncertain. In this study, regional chemical transport model simulations are used to examine photochemical production of ozone in air masses originating from boreal fire and anthropogenic emissions over North America and during their transport toward the Arctic during early July 2008. Model results are evaluated using POLARCAT aircraft data collected over boreal fire source regions in Canada (ARCTAS-B) and several days downwind over Greenland (POLARCAT-France and POLARCAT-GRACE). Model results are generally in good agreement with the observations, except for certain trace gas species over boreal fire regions, in some cases indicating that the fire emissions are too low. Anthropogenic and biomass burning pollution (BB) from North America was rapidly uplifted during transport east and north to Greenland where pollution plumes were observed in the mid- and upper troposphere during POLARCAT. A model sensitivity study shows that CO levels are in better agreement with POLARCAT measurements (fresh and aged fire plumes) upon doubling CO emissions from fires. Analysis of model results, using ΔO3/ΔCO enhancement ratios, shows that pollution plumes formed ozone during transport towards the Arctic. Fresh anthropogenic plumes have averageΔO3/ΔCO enhancement ratios of 0.63 increasing to 0.92 for aged anthropogenic plumes, indicating additional ozone production during aging. Fresh fire plumes are only slightly enhanced in ozone (ΔO3/ΔCO=0.08), but form ozone downwind with ΔO3/ΔCO of 0.49 for aged BB plumes (model-based run). We estimate that aged anthropogenic and BB pollution together made an important contribution to ozone levels with an average contribution for latitudes > 55° N of up to 6.5 ppbv (18 %) from anthropogenic pollution and 3 ppbv (5.2 %) from fire pollution in the model domain in summer 2008. [ABSTRACT FROM AUTHOR]

We deployed an aerosol mass spectrometer during the POLARCAT (Polar Study using Aircraft, Remote Sensing, Surface Measurements and Models, of Climate, Chemistry, Aerosols, and Transport) summer campaign in Greenland in June/July 2008 on the research aircraft ATR-42. Online size resolved chemical composition data of submicron aerosol were collected up to 7.6 km altitude in the region 60 to 71° N and 40 to 60°W. Biomass burning (BB) and fossil fuel combustion (FF) plumes originating from North America, Asia, Siberia and Europe were sampled. Transport pathways of detected plumes included advection below 700 hPa, air mass uplifting in warm conveyor belts, and high altitude transport in the upper troposphere. By means of the Lagrangian particle dispersion model FLEXPART, trace gas analysis of O3 and CO, particle size distributions and aerosol chemical composition 48 pollution events were identified and classified into five chemically distinct categories. Aerosol from North American BB consisted of 22% particulate sulphate, while with increasing anthropogenic and Asian influence aerosol in Asian FF dominated plumes was composed of up to 37% sulphate category mean value. Overall, it was found that the organic matter fraction was larger (85 %) in pollution plumes than for background conditions (71 %). Despite different source regions and emission types the particle oxygen to carbon ratio of all plume classes was around 1 indicating low-volatility highly oxygenated aerosol. The volume size distribution of out-of-plume aerosol showed markedly smaller modes than all other distributions with two Aitken mode diameters of 24 and 43 nm and a geometric standard deviation σg of 1.12 and 1.22, respectively, while another very broad mode was found at 490 nm (σg =2.35). Nearly pure BB particles from North America exhibited an Aitken mode at 66 nm (σg =1.46) and an accumulation mode diameter of 392 nm (σg =1.76). An aerosol lifetime, including all processes from emission to detection, in the range between 7 and 11 days was derived for North American emissions. [ABSTRACT FROM AUTHOR]

We report on airborne Differential Optical Absorption Spectroscopy (DOAS) measurements of aerosol extinction and NO2 tropospheric profiles performed off the North coast of Norway in April 2008. The DOAS instrument was installed on the Satire ATR-42 aircraft during the POLARCAT-France spring campaign and recorded scattered light spectra in near-limb geometry using a scanning telescope. We use O4 slant column measurements to derive the aerosol extinction at 360 nm. Regularization is based on the maximum a posteriori solution, for which we compare a linear and a logarithmic approach. The latter inherently constrains the solution to positive values and yields aerosol extinction profiles more consistent with independently measured size distributions. We present results from two soundings performed on 8 April 2008 above 71°N, 22°E and on 9 April 2008 above 70°N, 17.8°E. The first profile shows aerosol extinction and NO2 in the marine boundary layer with respective values of 0.04±0.005 km-1 and 1.9±0.3 x 109 molec cm-3. A second extinction layer of 0.01±0.003 km-1 is found at 4km altitude where the NO2 concentration is 0.32±0.2 x 109 molec cm-3. During the second sounding, clouds prevent retrieval of profile parts under 3 km altitude but a layer with enhanced extinction (0.025±0.005 km-1) and NO2 (1.95±0.2 x 109 molec cm-3) is clearly detected at 4 km altitude. From CO and ozone in-situ measurements complemented by back-trajectories, we interpret the measurements in the free troposphere as, for the first sounding, a mix between stratospheric and polluted air from Northern Europe and for the second sounding, polluted air from Central Europe containing NO2. Considering the boundary layer measurements of the first flight, modeled source regions indicate closer sources, especially the Kola Peninsula smelters, which can explain the NO2 enhancement not correlated with a CO increase at the same altitude. [ABSTRACT FROM AUTHOR]

We performed airborne measurements of aerosol particle concentration, composition, size distribution and optical properties over Western Africa in the corridor 2-17° N and 3-5 E. Data were collected on board the French ATR-42 research aircraft in June-July 2006 as part of the African Monsoon Multidisciplinary Analysis (AMMA) intensive field phases in June-July 2006 using the AVIRAD airborne aerosol sampling system. The aerosol vertical distribution was documented on an almost daily basis. In particular, the vertical distribution of mineral dust emitted locally by Mesoscale Convective Systems (MSC) was distinguished from that of mineral dust that was transported from the Saharan by the African Easterly Jet (AEJ). Mineral dust emitted in the Sahel by convection-driven erosion was mostly confined in the boundary layer. One episode of injection of Sahelian mineral dust in the AEJ was observed. The elemental composition was found to be an element of difference between episodes, whereas the volume size distribution was more uniform. For non-mixed dust, the single scattering albedo ranged between 0.88-0.93 at 370 nm and between 0.91-0.99 at 950 nm, lower values being observed for Sahelian dust. In correspondence, the imaginary part of the complex refractive index varied between 0.002-0.004 at 370 nm and between 0.001-0.002 at 950 nm. [ABSTRACT FROM AUTHOR]

The calibration of the CloudSat spaceborne cloud radar has been thoroughly assessed using very accurate internal link budgets before launch, comparisons with predicted ocean surface backscatter at 94 GHz, direct comparisons with airborne cloud radars, and statistical comparisons with ground-based cloud radars at different locations of the world. It is believed that the calibration of CloudSat is accurate to within 0.5--1 dB. In the present paper it is shown that an approach similar to that used for the statistical comparisons with ground-based radars can now be adopted the other way around to calibrate other ground-based or airborne radars against CloudSat and/or to detect anomalies in long time series of ground-based radar measurements, provided that the calibration of CloudSat is followed up closely (which is the case). The power of using CloudSat as a global radar calibrator is demonstrated using the Atmospheric Radiation Measurement cloud radar data taken at Barrow, Alaska, the cloud radar data from the Cabauw site, Netherlands, and airborne Doppler cloud radar measurements taken along the CloudSat track in the Arctic by the Radar System Airborne (RASTA) cloud radar installed in the French ATR-42 aircraft for the first time. It is found that the Barrow radar data in 2008 are calibrated too high by 9.8 dB, while the Cabauw radar data in 2008 are calibrated too low by 8.0 dB. The calibration of the RASTA airborne cloud radar using direct comparisons with CloudSat agrees well with the expected gains and losses resulting from the change in configuration that required verification of the RASTA calibration. [ABSTRACT FROM AUTHOR]