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As its next step in space exploration, the National Aeronautics and Space Administration (NASA) revealed plans to establish a permanent human presence on Mars. Habitat outfitting, i.e., the technology to provide the crew with the necessary equipment to perform mission tasks as well as a comfortable, safe, and livable habitable volume, has not been fully explored yet. This study proposes that, rather than shipping prefabricated outfitting elements to Mars, habitat outfitting can be realized by in-situ construction using cyanobacteria and fungi as building agents. A synthetic lichen system, composed of diazotrophic cyanobacteria and filamentous fungi, can be created to produce abundant biominerals (CaCO3) and biopolymers, which will glue Martian regolith into consolidated building blocks. These self-growing building blocks can be assembled into various structures, such as floors, walls, partitions, and furniture.

We calculate from first principles the electron-phonon coupling strength in ferromagnetic iron-cobalt Fe$_{1-x}$Co$_x$ alloys for compositions ranging from $x=0$ to $x=0.75$. We find strong, spin-dependent variation of the electron-phonon coupling strength with alloy composition. The minimum of the electron-phonon interaction is found near the composition $x=0.25$. We analyze the variation of the electron-phonon interaction with composition, as a function of electron spin, density of states, electron-phonon matrix elements, and phonon frequencies. Our results are in good qualitative agreement with magnetization dynamics experiments.

A six-night optical turbulence monitoring campaign has been carried at Cerro Paranal observatory in February and March, 2023 to facilitate the development and characterisation of two novel atmospheric site monitoring instruments - the ring-image next generation scintillation sensor (RINGSS) and 24-hour Shack Hartmann image motion monitor (24hSHIMM) in the context of providing optical turbulence monitoring support for upcoming 20-40m telescopes. Alongside these two instruments, the well-characterised Stereo-SCIDAR and 2016-MASS-DIMM were operated throughout the campaign to provide data for comparison. All instruments obtain estimates of optical turbulence profiles through statistical analysis of intensity and wavefront angle-of-arrival fluctuations from observations of stars. Contemporaneous measurements of the integrated turbulence parameters are compared and the ratios, bias, unbiased root mean square error and correlation of results from each instrument assessed. Strong agreement was observed in measurements of seeing, free atmosphere seeing and coherence time. Less correlation is seen for isoplanatic angle, although the median values agree well. Median turbulence parameters are further compared against long-term monitoring data from Paranal instruments. Profiles from the three small-telescope instruments are compared with the 100-layer profile from the stereo-SCIDAR. It is found that the RINGSS and SHIMM offer improved accuracy in characterisation of the vertical optical turbulence profile over the MASS-DIMM. Finally, the first results of continuous optical turbulence monitoring at Paranal are presented which show a strong diurnal variation and predictable trend in the seeing. A value of 2.65" is found for the median daytime seeing., Comment: Accepted in MNRAS

Materials with high thermal conductivity are needed to conduct heat away from hot spots in power electronics and optoelectronic devices. Cubic boron arsenide (c-BAs) has a high thermal conductivity due to its special phonon dispersion relation. Previous experimental studies of c-BAs report a room-temperature thermal conductivity between 1000 and 1300 watts per meter-kelvin. We synthesized high purity c-BAs single crystals with room-temperature thermal conductivity of 1500 watts per meter-kelvin. We observed its thermal conductivity to be proportional to the inverse square of temperature between 300 and 600 kelvin, a stronger dependence than predicted by state-of-the-art theory., Comment: 14 pages, 3 figures

Using the Boltzmann transport equation (BTE), we study the evolution of nonequilibrium carrier distributions in simple ($sp$) metals, assumed to have been instantaneously excited by an ultrafast laser pulse with photon energy $h \nu$. The mathematical structure of the BTE scattering integrals reveals that $h \nu$ is a natural energy scale for describing the dynamics. Normalizing all energy quantities by $h \nu$ leads to a set of three unitless parameters -- $\beta / \delta$, $\gamma$, and $\alpha$ -- that control the relaxation dynamics: $\beta / \delta$ is the normalized ratio of electron-phonon to electron-electron scattering strengths, $\gamma$ is the normalized phonon (lattice) temperature, and $\alpha$ is the normalized absorbed energy density. Using this theory, we systematically investigate relaxation times for the high-energy part of the distribution ($\tau_H$), energy transfer to the phonon subsystem ($\tau_E$), and intracarrier thermalization ($\tau_{th}$). In the linear region of response (valid when $\alpha$ is sufficiently small), we offer heuristic descriptions of each of these relaxation times as functions of $\beta / \delta$ and $\gamma$. Our results as a function of excitation level $\alpha$ show that many ultrafast experimental investigations lie in a transition region between low excitation (where the relaxation times are independent of $\alpha$) and high excitation (where the two-temperature model of carrier dynamics is valid). Approximate boundaries that separate these three regions are described by simple expressions involving the normalized parameters of our model., Comment: 26 pages, 11 figures, and Supplemental Material. arXiv admin note: substantial text overlap with arXiv:2210.09422

Extractant design in liquid-liquid extraction (LLE) is a research frontier of metal ion separations that typically focuses on the direct extractant-metal interactions. However, a more detailed understanding of energetic drivers of separations beyond primary metal coordination is often lacking, including the role of solvent in the extractant phase. In this work, we propose a new mechanism for enhancing metal-complexant energetics with nanostructured solvents. Using molecular dynamics simulations with umbrella sampling, we find that the organic solvent can reshape the energetics of the extractant's intramolecular conformational landscape. We calculate free energy profiles of different conformations of a representative bidentate extractant, n-octyl(phenyl)-N,N-diisobutyl carbamoyl methyl phosphinoxide (CMPO), in four different solvents: dodecane, tributyl phosphate (TBP), and dry and wet ionic liquid (IL) 1-ethyl-3-methylimidazolium bis(trifluoromethylsulfonyl)imide ([EMIM][Tf_2N]). By promoting reorganization of the extractant molecule into its binding conformation, our findings reveal how particular solvents can ameliorate this unfavorable step of the metal separation process. In particular, the charge alternating nanodomains formed in ILs substantially reduce the free energy penalty associated with extractant reorganization. Importantly, using alchemical free energy calculations, we find that this stabilization persists even when we explicitly include the extracted cation. These findings provide insight into the energic drivers of metal ion separations and potentially suggest a new approach to designing effective separations using a molecular-level understanding of solvent effects.

The inverse Faraday effect is an opto-magnetic phenomenon that describes the ability of circularly polarized light to induce magnetism in solids. The capability of light to control magnetic order in solid state materials and devices is of interest for a variety of applications, such as magnetic recording, quantum computation and spintronic technologies. However, significant gaps in understanding about the effect persist, such as what material properties govern the magnitude of the effect in metals. In this work, we report time-resolved measurements of the specular inverse Faraday effect in non-magnetic metals, i.e., the magneto-optic Kerr effect induced by circularly polarized light. We measure this specular inverse Faraday effect in Cu, Pd, Pt, W, Ta, and Au at a laser wavelength of 783 nm. For Ta and W, we investigate both {\alpha} and \{beta} phases. We observe that excitation of these metals with circularly polarized light induces significant circular dichroism. This nonlinear magneto-optical response to circularly polarized light is an order of magnitude larger in {\alpha}-W than other metals, e.g., Pt, Au, and is greater than nearly all other reported values for IFE in other materials. Our results benchmark the range of IFE that can be observed in non-magnetic metals and provide insight into what material properties govern the inverse Faraday effect in metals.

We report an investigation of the bulk optical, bulk acoustic, and surface acoustic phonons in thin films of turbostratic boron nitride (t-BN) and cubic boron nitride (c-BN) grown on B-doped polycrystalline and single-crystalline diamond (001) and (111) substrates. The characteristics of different types of phonons were determined using Raman and Brillouin-Mandelstam light scattering spectroscopies. The atomic structure of the films was determined using high-resolution transmission electron microscopy (HRTEM) and correlated with the Raman and Brillouin-Mandelstam spectroscopy data. The HRTEM analysis revealed that the cubic boron nitride thin films consisted of a mixture of c-BN and t-BN phases, with c-BN being the dominant phase. It was found that while visible Raman spectroscopy provided information for characterizing the t-BN phase, it faced challenges in differentiating the c-BN phase either due to the presence of high-density defects or the overlapping of the Raman features with those from the B-doped diamond substrates. In contrast, Brillouin-Mandelstam spectroscopy clearly distinguishes the bulk longitudinal and surface acoustic phonons of the c-BN thin films grown on diamond substrates. Additionally, the angle-dependent surface Brillouin-Mandelstam scattering data show the peaks associated with the Rayleigh surface acoustic waves, which have higher phase velocities in c-BN films on diamond (111) substrates. These findings provide valuable insights into the phonon characteristics of the c-BN and diamond interfaces and have important implications for the thermal management of electronic devices based on ultra-wide-band-gap materials., Comment: 27 pages; 4 figures

Characterisation of atmospheric optical turbulence is crucial for the design and operation of modern ground-based optical telescopes. In particular, the effective application of adaptive optics correction on large and extremely large telescopes relies on a detailed knowledge of the prevailing atmospheric conditions, including the vertical profile of the optical turbulence strength and the atmospheric coherence timescale. The Differential Image Motion Monitor (DIMM) has been employed as a facility seeing monitor at many astronomical observing sites across the world for several decades, providing a reliable estimate of the seeing angle. Here we present the Shack-Hartmann Image Motion Monitor (SHIMM), which is a development of the DIMM instrument, in that it exploits differential image motion measurements of bright target stars. However, the SHIMM employs a Shack-Hartmann wavefront sensor in place of the two-hole aperture mask utilised by the DIMM. This allows the SHIMM to provide an estimate of the seeing, unbiased by shot noise or scintillation effects. The SHIMM also produces a low-resolution (three-layer) measure of the vertical turbulence profile, as well as an estimate of the coherence timescale. The SHIMM is designed as a low-cost, portable, instrument. It is comprised of off-the-shelf components so that it is easy to duplicate and well-suited for comparisons of atmospheric conditions within and between different observing sites. Here, the SHIMM design and methodology for estimating key atmospheric parameters will be presented, as well as initial field test results with comparisons to the Stereo-SCIDAR instrument., Comment: Published in MNRAS

PCANet and its variants provided good accuracy results for classification tasks. However, despite the importance of network depth in achieving good classification accuracy, these networks were trained with a maximum of nine layers. In this paper, we introduce a residual compensation convolutional network, which is the first PCANet-like network trained with hundreds of layers while improving classification accuracy. The design of the proposed network consists of several convolutional layers, each followed by post-processing steps and a classifier. To correct the classification errors and significantly increase the network's depth, we train each layer with new labels derived from the residual information of all its preceding layers. This learning mechanism is accomplished by traversing the network's layers in a single forward pass without backpropagation or gradient computations. Our experiments on four distinct classification benchmarks (MNIST, CIFAR-10, CIFAR-100, and TinyImageNet) show that our deep network outperforms all existing PCANet-like networks and is competitive with several traditional gradient-based models.

We report what is believed to be the first example of fully continuous, 24-hour vertical monitoring of atmospheric optical turbulence. This is achieved using a novel instrument, the 24-hour Shack-Hartmann Image Motion Monitor (24hSHIMM). Optical turbulence is a fundamental limitation for applications such as free-space optical communications, where it limits the achievable bandwidth, and ground-based optical astronomy, restricting the observational precision. Knowledge of the turbulence enables us to select the best sites, design optical instrumentation and optimise the operation of ground-based optical systems. The 24hSHIMM estimates the vertical optical turbulence coherence length, time, angle and Rytov variance from the measurement of a four-layer vertical turbulence profile and a wind speed profile retrieved from meteorological forecasts. To illustrate our advance we show the values of these parameters recorded during a 35-hour, continuous demonstration of the instrument. Due to its portability and ability to work in stronger turbulence, the 24hSHIMM can also operate in urban locations, providing the field with a truly continuous, versatile turbulence monitor for all but the most demanding of applications., Comment: Accepted in Optics Express

The Earth's turbulent atmosphere results in speckled and blurred images of astronomical objects when observed by ground based visible and near-infrared telescopes. Adaptive optics (AO) systems are employed to reduce these atmospheric effects by using wavefront sensors (WFS) and deformable mirrors. Some AO systems are not fast enough to correct for strong, fast, high turbulence wind layers leading to the wind butterfly effect, or wind-driven halo, reducing contrast capabilities in coronagraphic images. Estimating the effective wind speed of the atmosphere allows us to calculate the atmospheric coherence time. This is not only an important parameter to understand for site characterization but could be used to help remove the wind butterfly in post processing. Here we present a method for estimating the atmospheric effective wind speed from spatio-temporal covariance maps generated from pseudo open-loop (POL) WFS data. POL WFS data is used as it aims to reconstruct the full wavefront information when operating in closed-loop. The covariance maps show how different atmospheric turbulent layers traverse the telescope. Our method successfully recovered the effective wind speed from simulated WFS data generated with the soapy python library. The simulated atmospheric turbulence profiles consist of two turbulent layers of ranging strengths and velocities. The method has also been applied to Gemini Planet Imager (GPI) AO WFS data. This gives insight into how the effective wind speed can affect the wind-driven halo seen in the AO image point spread function. In this paper, we will present results from simulated and GPI WFS data., Comment: 7 pages, 6 figures

A semiempirical theory for the excitation and subsequent relaxation of nonthermal electrons is described. The theory, which is applicable to ultrafast-laser excited metals, is based on the Boltzmann transport equation for the carrier distribution function $f(\epsilon,t)$ and includes electron-phonon, electron-electron, and electron-photon scattering integrals in forms that explicitly depend on the electronic density of states. Electron-phonon coupling is treated by extending the theory of Allen [Phys. Rev. Lett. 59, 1460 (1987)] to include highly-excited nonthermal electron distributions, and is used to determine the energy transfer rate between a nonthermal electron subsystem and a thermal phonon subsystem. Electron-electron scattering is treated with a simple energy-conserving electron-electron scattering integral. The electron-photon integral assumes photon absorption is phonon assisted. We apply the theory to analyze prior ultrafast thermionic emission, two-color photoemission, and electronic inelastic light (Raman) scattering experiments on Au. These analyses show that getting the details of $f(\epsilon,t)$ is necessary for proper interpretation of each experiment. Together, the photoemission and Raman-scattering analyses indicate an electron excited 1 eV above the Fermi level has an electron-electron scattering time in the range of 25 to 55 fs., Comment: 26 pages, 5 figures; 1 page Supplemental Material

We report the results of the investigation of bulk and surface acoustic phonons in the undoped and boron-doped single-crystal diamond films using the Brillouin-Mandelstam light scattering spectroscopy. The evolution of the optical phonons in the same set of samples was monitored with Raman spectroscopy. It was found that the frequency and the group velocity of acoustic phonons decrease non-monotonically with the increasing boron doping concentration, revealing pronounced phonon softening. The change in the velocity of the shear horizontal and the high-frequency pseudo-longitudinal acoustic phonons in the degenerately doped diamond, as compared to the undoped diamond, was as large as ~15% and ~12%, respectively. As a result of boron doping, the velocity of the bulk longitudinal and transverse acoustic phonons decreased correspondingly. The frequency of the optical phonons was unaffected at low boron concentration but experienced a strong decrease at the high doping level. The density-functional-theory calculations of the phonon band structure for the pristine and highly-doped sample confirm the phonon softening as a result of boron doping in diamond. The obtained results have important implications for thermal transport in heavily doped diamond, which is a promising material for ultra-wide-band-gap electronics., Comment: 27 pages; 5 figures

The thermal properties of amorphous materials have attracted significant attention due to their technological importance in electronic devices. Additionally, the disorder-induced breakdown of the phonon gas model makes vibrational transport in amorphous materials a topic of fundamental interest. In the past few decades, theoretical concepts such as propagons, diffusons, and locons have emerged to describe different types of vibrational modes in disordered solids. But experiments can struggle to accurately determine which types of vibrational states carry the majority of the heat. In the present study, we use nanoscale laser flash measurements (front/back time-domain thermoreflectance) to investigate thermal transport mechanisms in amorphous Ge and amorphous Si thin-films. We observe a nearly linear relationship between the amorphous film's thermal resistance and the film's thickness. The slope of the film's thermal resistance vs. thickness corresponds to a thickness-independent thermal conductivity of 0.4 and 0.6 W/(m-K) for a-Ge and a-Si, respectively. This result reveals that the majority of heat currents in amorphous Si and Ge thin films prepared via RF sputtering at room temperature are carried by diffusons and/or propagons with mean free paths less than a few nanometers.

Time-domain thermoreflectance (TDTR) is a well-established pump/probe method for measuring thermal conductivity and interface conductance of multilayers. Interpreting signals in a TDTR experiment requires a thermal model.In standard front/front TDTR experiments, both pump and probe beams typically irradiate the surface of a multilayer. As a result, existing thermal models for interpreting thermoreflectance experiments assume the pump and probe beams both interact with the surface layer. Here, we present a frequency-domain solution to the heat-diffusion equation of a multilayer in response to nonhomogenous laser heating. This model allows analysis of experiments where the pump and probe beams irradiate opposite sides of a multilayer. We call such a geometry a front/back experiment to differentiate such experiments from standard TDTR experiments. As an example, we consider a 60nm amorphous Si film. We consider how signals differ in a front/front vs. front/back geometry and compare thermal model predictions to experimental data.

The thermal conductivity of boron arsenide (BAs) is believed to be influenced by phonon scattering selection rules due to its special phonon dispersion. Compression of BAs leads to significant changes in phonon dispersion, which allows for a test of first principles theories for how phonon dispersion affects three- and four-phonon scattering rates. This study reports the thermal conductivity of BAs from 0 to 30 GPa. Thermal conductivity vs. pressure of BAs is measured by time-domain thermoreflectance with a diamond anvil cell. In stark contrast to what is typical for nonmetallic crystals, BAs is observed to have a pressure independent thermal conductivity below 30 GPa. The thermal conductivity of nonmetallic crystals typically increases upon compression. The unusual pressure independence of thermal conductivity of BAs shows the important relationship between phonon dispersion properties and three- and four-phonon scattering rates.

We report the magneto optic Kerr effect (MOKE) angle of Au magnetically excited by spin accumulation. We perform time resolved polar MOKE measurements on Au/Co heterostructures. In our experiment, the ultrafast optical excitation of the Co drives spin accumulation into an adjacent Au layer. The spin accumulation, together with spin-orbit coupling, leads to non-zero terms in the off-diagonal conductivity tensor of Au, which we measure by recording the polarization and ellipticity of light reflected from the Au surface for photon energies between 1.3 and 3.1 eV. At energies near the interband transition threshold of Au, the Kerr rotation per A/m exceeds 1 urad. Typical values for Kerr rotation per moment in transition ferromagnetic metals like Ni are < 10 nrad per A/m, while predicted values for heavy metals like Pt or W are < 13 nrad per A/m. The exceptional sensitivity of the optical properties of Au to spin magnetic moments make Au to be an exceptionally sensitive optical magnetometer, with potential applications in the development of optospintronic technologies.

Recent investigations have advanced the understanding of how structure-property relationships in ferromagnetic metal alloys affect the magnetization dynamics on nanosecond time-scales. A similar understanding for magnetization dynamics on femto- to pico-second time-scales does not yet exist. To address this, we perform time-resolved magneto optic Kerr effect (TRMOKE) measurements of magnetization dynamics in Co-Fe alloys on femto- to nano-second regimes. We show that Co-Fe compositions that exhibit low Gilbert damping parameters also feature prolonged ultrafast demagnetization upon photoexcitation. We analyze our experimental TR-MOKE data with the three-temperature-model (3TM) and the Landau-Lifshitz-Gilbert equation. These analyses reveal a strong compositional dependence of the dynamics across all time-scales on the strength of electron-phonon interactions. Our findings are beneficial to the spintronics and magnonics community, and will aid in the quest for energy-efficient magnetic storage applications.

We investigate picosecond spin-currents across Au/iron-garnet interfaces in response to ultrafast laser heating of the electrons in the Au film. In the picoseconds after optical heating, interfacial spin currents occur due to an interfacial temperature difference between electrons in the metal and magnons in the insulator. We report measurements of this interfacial longitudinal spin Seebeck effect between Au and rare-earth iron-garnet insulators, i.e. RE$_3$ Fe$_5$O$_{12}$, where RE is Y, Eu, Tb, Tm. We use time domain thermoreflectance (TDTR) measurements to characterize the thermal response of the bilayer to ultrafast optical heating. We use time-resolved magneto-optic Kerr effect (TR-MOKE) measurements of the Au layer to measure the time-evolution of spin accumulation in the Au film. We observe a spin Seebeck effect between Au/TmIG that is three times larger than for an Au/YIG bilayer. The interfacial thermal conductance between electrons in the Au and magnons in the TmIG layer is ~ 3 $\frac{MW}{m^2 K}$.

To better understand the many effects of temperature on the optical properties of metals, we experimentally and theoretically quantify the electron vs. phonon contributions to the thermoreflectance spectra of gold. We perform a series of pump/probe measurements on nanoscale Pt/Au bilayers at wavelengths between 400 and 1000 nm. At all wavelengths, we find that changes in phonon temperature, not electron temperature, are the primary contributor to the thermoreflectance of Au. The thermoreflectance is most sensitive to the electron temperature at wavelength of ~480 nm due to interband transitions between d-states and the Fermi-level. In the near infrared, the electron temperature is responsible for only ~2% of the total thermoreflectance. We also compute the thermoreflectance spectra of Au from first principles. Our calculations further confirm that phonon temperature dominates thermoreflectance of Au. Most of Au's thermoreflectance is due to the effect of the phonon population on electron lifetime., Comment: 30 pages, 5 figures, 7 supplemental figures

We find that in BaTiO$_3$ the phonon angular momentum is dominantly pointing in directions perpendicular to the electrical polarization. Therefore, external electric field in ferroelectric BaTiO$_3$ does not control only the direction of electrical polarization, but also the direction of phonon angular momentum. This finding opens up the possibility for electric-field control of physical phenomena that rely on phonon angular momentum. We construct an intuitive model, based on our first-principles calculations, that captures the origin of the relationship between phonon angular momentum and electric polarization.

Many questions are still open regarding the physical mechanisms behind the magnetic switching in GdFeCo alloys by single optical pulses. Phenomenological models suggest a femtosecond scale exchange relaxation between sublattice magnetization as the driving mechanism for switching. The recent observation of thermally induced switching in GdFeCo by using both several picosecond optical laser pulse as well as electric current pulses has questioned this previous understanding. This has raised the question of whether or not the same switching mechanics are acting at the femo- and picosecond scales. In this work, we aim at filling this gap in the understanding of the switching mechanisms behind thermal single-pulse switching. To that end, we have studied experimentally thermal single-pulse switching in GdFeCo alloys, for a wide range of system parameters, such as composition, laser power and pulse duration. We provide a quantitative description of the switching dynamics using atomistic spin dynamics methods with excellent agreement between the model and our experiments across a wide range of parameters and timescales, ranging from femtoseconds to picoseconds. Furthermore, we find distinct element-specific damping parameters as a key ingredient for switching with long picosecond pulses and argue, that switching with pulse durations as long as 15 picoseconds is possible due to a low damping constant of Gd. Our findings can be easily extended to speed up dynamics in other contexts where ferrimagnetic GdFeCo alloys have been already demonstrated to show fast and energy-efficient processes, e.g. domain-wall motion in a track and spin-orbit torque switching in spintronics devices.

Reducing energy dissipation while increasing speed in computation and memory is a long-standing challenge for spintronics research. In the last 20 years, femtosecond lasers have emerged as a tool to control the magnetization in specific magnetic materials at the picosecond timescale. However, the use of ultrafast optics in integrated circuits and memories would require a major paradigm shift. An ultrafast electrical control of the magnetization is far preferable for integrated systems. Here we demonstrate reliable and deterministic control of the out-of-plane magnetization of a 1 nm-thick Co layer with single 6 ps-wide electrical pulses that induce spin-orbit torques on the magnetization. We can monitor the ultrafast magnetization dynamics due to the spin-orbit torques on sub-picosecond timescales, thus far accessible only by numerical simulations. Due to the short duration of our pulses, we enter a counter-intuitive regime of switching where heat dissipation assists the reversal. Moreover, we estimate a low energy cost to switch the magnetization, projecting to below 1fJ for a (20 nm)^3 cell. These experiments prove that spintronic phenomena can be exploited on picosecond time-scales for full magnetic control and should launch a new regime of ultrafast spin torque studies and applications., Comment: Includes article + supplementary information. Latest version uses full name of the first author. Nature Electronics (2020)

We report results of investigation of the phonon and thermal properties of the exfoliated films of layered single crystals of antiferromagnetic FePS3 and MnPS3 semiconductors. The Raman spectroscopy was conducted using three different excitation lasers with the wavelengths of 325 nm (UV), 488 nm (blue), and 633 nm (red). The resonant UV-Raman spectroscopy reveals new spectral features, which are not detectable via visible Raman light scattering. The thermal conductivity of FePS3 and MnPS3 thin films was measured by two different techniques: the steady-state Raman optothermal and transient time-resolved magneto-optical Kerr effect. The Raman optothermal measurements provided the orientation-average thermal conductivity of FePS3 to be 1.35 W/mK at room temperature. The transient measurements revealed that the through-plane and in-plane thermal conductivity of FePS3 is 0.85 W/mK and 2.7 W/mK, respectively. The films of MnPS3 have higher thermal conductivity of 1.1 W/mK through-plane and 6.3 W/mK in-plane. The data obtained by both techniques reveal strong thermal anisotropy of the films and the dominant contribution of phonons to heat conduction. Our results are important for the proposed applications of the antiferromagnetic semiconductor thin films in spintronic devices., Comment: 43 pages, 8 figures