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Fusing small resource states into a larger, fully connected graph-state is essential for scalable photonic quantum computing. Theoretical analysis reveals that this can only be achieved when the success probability of the fusion gate surpasses a specific percolation threshold of 58.98% by using three-photon GHZ states as resource states. However, such an implementation of a fusion gate has never been experimentally realized before. Here, we successfully demonstrate a boosted fusion gate with a theoretical success probability of 75%, using deterministically generated auxiliary states. The success probability is experimentally measured to be 71.0(7)%. We further demonstrate the effectiveness of the boosted fusion gate by fusing two Bell states with a fidelity of 67(2)%. Our work paves a crucial path toward scalable linear optical quantum computing., Comment: 5 pages, 4 figures

An important aspect in categorizing topological phases is whether the system is spinless or spinful, given that these classes exhibit distinct symmetry algebras, leading to disparate topological classifications. By utilizing the projective presentation strategy, the topological phases of spinless (or spinful) systems can be emulated using spinful (or spinless) systems augmented with gauge fields. In this study, we propose to implement the topological phases safeguarded by the unique projective space-time (PT) symmetry inherent to spinful models, using synthetic spinless alkaline-earth-like atoms. Employing the separation of orbital and nuclear-spin degrees of freedom, the model is configured as a rectangular tube penetrated by a uniform magnetic flux through each plaquette, which simulates a spinless ladder endowed with projective PT symmetry satisfying the algebraic properties of a spinful model. For interacting topological phases with inter-orbital spin-exchange interactions, which also adhere to PT symmetry, the four-fold degeneracy of edge modes is split into two pairs of edge modes with two-fold degeneracy. We map the complete phase diagram in the end and discover that these interacting topological phases ultimately evolve into distinct charge-density-wave phases via spontaneous symmetry breaking., Comment: 7 pages+6 figures

We study the chiral transport of interacting bosons in a two-leg flux ladder with on-site interactions. Focusing on the flux-induced chiral current along the two legs, we show that, counter-intuitively, on-site interactions can reverse the direction of the chiral flow. For a Bose-Einstein condensate whose dynamical evolution is driven by the Gross-Pitaevskii equation under the mean-field approximation, this reversal can be understood as an interaction-induced dynamic occupation inversion, under which single-particle band with opposing chirality becomes heavily populated in the dynamics. This chirality inversion also persists in the two-body dynamics with strong quantum fluctuations beyond the mean-field regime, as demonstrated through time-dependent density-matrix renormalization group and exact diagonalization analyses. Herein, besides the band-occupation-inversion mechanism, we find that the formation of two-body bound states with opposite chirality contributes significantly to the reversed chiral transport. Our discovery highlights the significance of correlation effects in quantum transport, and can be readily demonstrated using cold atoms., Comment: 7 pages+3 figures

Assembling increasingly larger-scale defect-free optical tweezer-trapped atom arrays is essential for quantum computation and quantum simulations based on atoms. Here, we propose an AI-enabled, rapid, constant-time-overhead rearrangement protocol, and we experimentally assemble defect-free 2D and 3D atom arrays with up to 2024 atoms with a constant time cost of 60 ms. The AI model calculates the holograms for real-time atom rearrangement. With precise controls over both position and phase, a high-speed spatial light modulator moves all the atoms simultaneously. This protocol can be readily used to generate defect-free arrays of tens of thousands of atoms with current technologies, and become a useful toolbox for quantum error correction.

Despite the significant progress in superconducting quantum computation over the past years, quantum state measurement still lags nearly an order of magnitude behind quantum gate operations in speed and fidelity. The main challenge is that the strong coupling and readout signal used to probe the quantum state may also introduce additional channels which may cause qubit state transitions. Here, we design a novel architecture to implement the long-sought longitudinal interaction scheme between qubits and resonators. This architecture not only provides genuine longitudinal interaction by eliminating residual transversal couplings, but also introduces proper nonlinearity to the resonator that can further minimize decay error and measurement-induced excitation error. Our experimental results demonstrate a measurement fidelity of 99.8% in 202 ns without the need for any first-stage amplification. After subtracting the residual preparation errors, the pure measurement fidelity is above 99.9%. Our scheme is compatible with the multiplexing readout scheme and can be used for quantum error correction.

In the relentless pursuit of quantum computational advantage, we present a significant advancement with the development of Zuchongzhi 3.0. This superconducting quantum computer prototype, comprising 105 qubits, achieves high operational fidelities, with single-qubit gates, two-qubit gates, and readout fidelity at 99.90%, 99.62% and 99.18%, respectively. Our experiments with an 83-qubit, 32-cycle random circuit sampling on Zuchongzhi 3.0 highlight its superior performance, achieving one million samples in just a few hundred seconds. This task is estimated to be infeasible on the most powerful classical supercomputers, Frontier, which would require approximately $6.4\times 10^9$ years to replicate the task. This leap in processing power places the classical simulation cost six orders of magnitude beyond Google's SYC-67 and SYC-70 experiments [Nature 634, 328(2024)], firmly establishing a new benchmark in quantum computational advantage. Our work not only advances the frontiers of quantum computing but also lays the groundwork for a new era where quantum processors play an essential role in tackling sophisticated real-world challenges.

Accurate long-distance ranging is crucial for diverse applications, including satellite formation flying, very-long-baseline interferometry, gravitational-wave observatory, geographical research, etc. The integration of the time-of-flight mesurement with phase interference in dual-comb method enables high-precision ranging with a rapid update rate and an extended ambiguity range. Pioneering experiments have demonstrated unprecedented precision in ranging, achieving 5 nm @ 60 ms for 1.1 m and 200 nm @ 0.5 s for 25 m. However, long-distance ranging remains technically challenging due to high transmission loss and noise. In this letter, we propose a two-way dual-comb ranging (TWDCR) approach that enables successful ranging over a distance of 113 kilometers. We employ air dispersion analysis and synthetic repetition rate technique to extend the ambiguity range of the inherently noisy channel beyond 100 km. The achieved ranging precision is 11.5 $\mu$m @ 1.3 ms, 681 nm @ 1 s, and 82 nm @ 21 s, as confirmed through a comparative analysis of two independent systems. The advanced long-distance ranging technology is expected to have immediate implications for space research initiatives, such as the space telescope array and the satellite gravimetry., Comment: 21 pages, 5 figures, 1 table

We propose hardware-efficient schemes for implementing logical H and S gates transversally on rotated surface codes with reconfigurable neutral atom arrays. For logical H gates, we develop a simple strategy to rotate code patches efficiently with two sets of 2D-acousto-optic deflectors (2D-AODs). Our protocol for logical S gates utilizes the time-dynamics of the data and ancilla qubits during syndrome extraction (SE). In particular, we break away from traditional schemes where transversal logical gates take place between two SE rounds and instead embed our fold-transversal logical operation inside a single SE round, leveraging the fact that data and ancilla qubits can be morphed to an unrotated surface code state at half-cycle. Under circuit noise, we observe the performance of our S gate protocol is on par with the quantum memory. Together with transversal logical CNOT gates, our protocols complete a transversal logical Clifford gate set on rotated surface codes and admit efficient implementation on neutral atom array platforms.

String breaking is a fundamental concept in gauge theories, describing the decay of a flux string connecting two charges through the production of particle-antiparticle pairs. This phenomenon is particularly important in particle physics, notably in Quantum Chromodynamics, and plays a crucial role in condensed matter physics. However, achieving a theoretical understanding of this non-perturbative effect is challenging, as conventional numerical approaches often fall short and require substantial computational resources. On the experimental side, studying these effects necessitates advanced setups, such as high-energy colliders, which makes direct observation difficult. Here, we report an experimental investigation of the string breaking mechanism in a one-dimensional U(1) lattice gauge theory using an optical lattice quantum simulator. By deterministically preparing initial states of varying lengths with fixed charges at each end, and adiabatically tuning the mass and string tension, we observed in situ microscopic confined phases that exhibit either string or brokenstring states. Further analysis reveals that string breaking occurs under a resonance condition, leading to the creation of new particle-antiparticle pairs. These findings offer compelling evidence of string breaking and provide valuable insights into the intricate dynamics of lattice gauge theories. Our work underscores the potential of optical lattices as controllable quantum simulators, enabling the exploration of complex gauge theories and their associated phenomena., Comment: 12 pages, (5+3) figures

Owing to its repeater-like rate-loss scaling, twin-field quantum key distribution (TF-QKD) has repeatedly exhibited in laboratory its superiority for secure communication over record fiber lengths. Field trials pose a new set of challenges however, which must be addressed before the technology's roll-out into real-world. Here, we verify in field the viability of using independent optical frequency combs -- installed at sites separated by a straight-line distance of 300~km -- to achieve a versatile TF-QKD setup that has no need for optical frequency dissemination and thus enables an open and network-friendly fiber configuration. Over 546 and 603 km symmetric links, we record a finite-size secure key rate (SKR) of 0.53~bit/s and an asymptotic SKR of 0.12 bit/s, respectively. Of practical importance, the setup is demonstrated to support 44~km fiber asymmetry in the 452 km link. Our work marks an important step towards incorporation of long-haul fiber links into large quantum networks., Comment: To appear in Physical Review Applied

In the context of quantum electrodynamics, the decay of false vacuum leads to the production of electron-positron pair, a phenomenon known as the Schwinger effect. In practical experimental scenarios, producing a pair requires an extremely strong electric field, thus suppressing the production rate and making this process very challenging to observe. Here we report an experimental investigation, in a cold-atom quantum simulator, of the effect of the background field on pair production from the infinite-mass vacuum in a $1+1$D $\mathrm{U}(1)$ lattice gauge theory. The ability to tune the background field allows us to study pair production in a large production rate regime. Furthermore, we find that the energy spectrum of the time-evolved observables in the zero mass limit displays excitation peaks analogous to bosonic modes in the Schwinger model. Our work opens the door to quantum-simulation experiments that can controllably tune the production of pairs and manipulate their far-from-equilibrium dynamics.

Neutral atom array has emerged as a promising platform for quantum computation due to its high-fidelity two-qubit gate, arbitrary connectivity and remarkable scalability. However, achieving fault-tolerant quantum computing with neutral atom necessitates careful consideration of the errors inherent to these systems. One typical error is the leakage from Rydberg states during the implementation of multi-qubit gates, which induces two-qubit error chain and degrades the error distance. To address this, researchers have proposed an erasure conversion protocol that employs fast leakage detection and continuous atomic replacement to convert leakage errors into benign erasure errors. While this method achieves a favorable error distance de = d, its applicability is restricted to certain atom species. In this work, we present a novel approach to manage Rydberg leakage errors in measurement-based quantum computation (MBQC). From a hardware perspective, we utilize practical experimental techniques along with an adaptation of the Pauli twirling approximation (PTA) to mitigate the impacts of leakage errors, which propagate similarly to Pauli errors without degrading the error distance. From a decoding perspective, we leverage the inherent structure of topological cluster states and final leakage detection information to locate propagated errors from Rydberg leakage. This approach eliminates the need for mid-circuit leakage detection, while maintaining an error distance de = d and achieving a high threshold of 3.4% per CZ gate for pure leakage errors under perfect final leakage detection. Furthermore, in the presence of additional Pauli errors, our protocol demonstrates comparable logical error rates to the erasure conversion method within a reasonable range of physical errors., Comment: 9+5 pages, 6+2 figures. Comments welcome - v2 The newest version has updated error model to handle coherent error in no-jump evolution. The updated error model has better error propagation and performance. Core conclusion about error distance is unchanged

Differential absorption Lidar (DIAL) in the ultraviolet (UV) region is an effective approach for monitoring tropospheric ozone. 4H-SiC single-photon detectors (SPDs) are emergent devices for UV single-photon detection. Here, we demonstrate a 4H-SiC SPD-based ozone DIAL. We design and fabricate the 4H-SiC single-photon avalanche diode with a beveled mesa structure and optimized layer thickness. An active quenching circuit with a quenching time of 1.03 ns is developed to significantly mitigate the afterpulsing effect while enhancing the maximum count rate. After characterization, the SPD exhibits excellent performance with a photon detection efficiency of 16.6% at 266 nm, a dark count rate of 138 kcps, a maximum count rate of 13 Mcps, and an afterpulse probability of 2.7% at room temperature. Then, we apply two 4H-SiC SPDs in an ozone DIAL. The measured ozone concentrations at altitudes of 1-3.5 km agree well with the results of a commercial ozone DIAL. Our work provides an alternative solution for general UV Lidar applications., Comment: Accepted by Applied Physics Letters

In 1927, during the fifth Solvay Conference, Einstein and Bohr described a double-slit interferometer with a "movable slit" that can detect the momentum recoil of one photon. Here, we report a faithful realization of the Einstein-Bohr interferometer using a single atom in an optical tweezer, cooled to the motional ground state in three dimensions. The single atom has an intrinsic momentum uncertainty comparable to a single photon, which serves as a movable slit obeying the minimum Heisenberg uncertainty principle. The atom's momentum wavefunction is dynamically tunable by the tweezer laser power, which enables observation of an interferometric visibility reduction at a shallower trap, demonstrating the quantum nature of this interferometer. We further identify classical noise due to atom heating and precession, illustrating a quantum-to-classical transition., Comment: 18 pages, 4 figures

Topological phases at quantum criticality attract much attention recently. Here we numerically study the interaction-induced phase transitions at around the topological quantum critical points of an extended Su-Schrieffer-Heeger (SSH) chain with next-nearest-neighbor hopping. This extended SSH model shows topological phase transitions between the topologically trivial and nontrivial critical phases when interaction is absent. So long as the interaction terms are turned on, the topologically nontrivial (trivial) critical phases are driven into topologically nontrivial (trivial) insulator phases with finite energy gaps. Particularly, we find the trivial insulator phase is further driven to the nontrivial insulator phase, through interaction-induced topological phase transition, although interaction generally is harmful to nontrivial topology. The stability of trivial insulator phase against interaction tends to vanish at the multicritical point that separates the trivial and nontrivial critical phases. Our work provides a concrete example for manifesting the impact of interaction on topological quantum criticality., Comment: 6 pages, 4 figures

Quantum money is the first invention in quantum information science, promising advantages over classical money by simultaneously achieving unforgeability, user privacy, and instant validation. However, standard quantum money relies on quantum memories and long-distance quantum communication, which are technologically extremely challenging. Quantum "S-money" tokens eliminate these technological requirements while preserving unforgeability, user privacy, and instant validation. Here, we report the first full experimental demonstration of quantum S-tokens, proven secure despite errors, losses and experimental imperfections. The heralded single-photon source with a high system efficiency of 88.24% protects against arbitrary multi-photon attacks arising from losses in the quantum token generation. Following short-range quantum communication, the token is stored, transacted, and verified using classical bits. We demonstrate a transaction time advantage over intra-city 2.77 km and inter-city 60.54 km optical fibre networks, compared with optimal classical cross-checking schemes. Our implementation demonstrates the practicality of quantum S-tokens for applications requiring high security, privacy and minimal transaction times, like financial trading and network control. It is also the first demonstration of a quantitative quantum time advantage in relativistic cryptography, showing the enhanced cryptographic power of simultaneously considering quantum and relativistic physics., Comment: 74 pages, 6 figures

A quantum network provides an infrastructure connecting quantum devices with revolutionary computing, sensing, and communication capabilities. As the best-known application of a quantum network, quantum key distribution (QKD) shares secure keys guaranteed by the laws of quantum mechanics. A quantum satellite constellation offers a solution to facilitate the quantum network on a global scale. The Micius satellite has verified the feasibility of satellite quantum communications, however, scaling up quantum satellite constellations is challenging, requiring small lightweight satellites, portable ground stations and real-time secure key exchange. Here we tackle these challenges and report the development of a quantum microsatellite capable of performing space-to-ground QKD using portable ground stations. The quantum microsatellite features a payload weighing approximately 23 kg, while the portable ground station weighs about 100 kg. These weights represent reductions by more than an order and two orders of magnitude, respectively, compared to the Micius satellite. Additionally, we multiplex bidirectional satellite-ground optical communication with quantum communication, enabling key distillation and secure communication in real-time. Using the microsatellite and the portable ground stations, we demonstrate satellite-based QKD with multiple ground stations and achieve the sharing of up to 0.59 million bits of secure keys during a single satellite pass. The compact quantum payload can be readily assembled on existing space stations or small satellites, paving the way for a satellite-constellation-based quantum and classical network for widespread real-life applications., Comment: 40 pages, 8 figures

Nonlocality, evidenced by the violation of Bell inequalities, not only signifies entanglement but also highlights measurement incompatibility in quantum systems. Utilizing the generalized Clauser-Horne-Shimony-Holt (CHSH) Bell inequality, our high-efficiency optical setup achieves a loophole-free violation of $2.0132$. This result provides a device-independent lower bound on entanglement, quantified as the entanglement of formation at $0.0159$. Moreover, by tuning the parameters of the generalized Bell inequality, we enhance the estimation of measurement incompatibility, which is quantified by an effective overlap of $4.3883 \times 10^{-5}$. To explore the intricate interplay among nonlocality, entanglement, and measurement incompatibility, we generate mixed states, allowing for flexible modulation of entanglement via fast switching among the four Bell states using Pockels cells, achieving a fidelity above $99.10\%$. Intriguingly, our results reveal a counterintuitive relationship where increasing incompatibility initially boosts nonlocality but eventually leads to its reduction. Typically, maximal nonlocality does not coincide with maximal incompatibility. This experimental study sheds light on the optimal management of quantum resources for Bell-inequality-based quantum information processing., Comment: 15 pages, 9 figures

The entangled photons are crucial resources for quantum communications and networking. Here, we present an ultra-bright polarization-entangled photon source based on a periodically poled lithium niobate waveguide designed for practical quantum communication networks. Using a 780 nm pump laser, the source achieves a pair generation rate of 2.4 $\times 10^{10}$ pairs/s/mW. This work has achieved a directly measured power of 17.9 nW in entangled photon generation with a 3.2 mW pump power. Based on this, we demonstrate the practicality of the source by conducting quantum key distribution experiments over long-distance fiber links, achieving the applicable secure key rates of up to 440.80 bits/s over 200 km with 62 dB loss and reaching a maximum secure key generation distance of 404 km. These results demonstrate the potential of wavelength-multiplexed polarization-entangled photon sources for high-speed, long-distance quantum communication, positioning them as key components for future large-scale quantum networks., Comment: 18 pages, 6 figures

The emergence of quantum mechanics and general relativity has transformed our understanding of the natural world significantly. However, integrating these two theories presents immense challenges, and their interplay remains untested. Recent theoretical studies suggest that the single-photon interference covering huge space can effectively probe the interface between quantum mechanics and general relativity. We developed an alternative design using unbalanced Michelson interferometers to address this and validated its feasibility over an 8.4 km free-space channel. Using a high-brightness single-photon source based on quantum dots, we demonstrated single-photon interference along this long-distance baseline. We achieved a phase measurement precision of 16.2 mrad, which satisfied the measurement requirements for a gravitational redshift at the geosynchronous orbit by five times the standard deviation. Our results confirm the feasibility of the single-photon version of the Colella-Overhauser-Werner experiment for testing the quantum effects in curved spacetime., Comment: 22 pages, 6 figures

Frequency tunable qubit plays a significant role for scalable superconducting quantum processors. The state-of-the-art room-temperature electronics for tuning qubit frequency suffers from unscalable limit, such as heating problem, linear growth of control cables, etc. Here we propose a scalable scheme to tune the qubit frequency by using in situ superconducting circuit, which is based on radio frequency superconducting quantum interference device (rf-SQUID). We demonstrate both theoretically and experimentally that the qubit frequency could be modulated by inputting several single pulses into rf-SQUID. Compared with the traditional scheme, our scheme not only solves the heating problem, but also provides the potential to exponentially reduce the number of cables inside the dilute refrigerator and the room-temperature electronics resource for tuning qubit frequency, which is achieved by a time-division-multiplex (TDM) scheme combining rf-SQUID with switch arrays. With such TDM scheme, the number of cables could be reduced from the usual $\sim 3n$ to $\sim \log_2{(3n)} + 1$ for two-dimensional quantum processors comprising $n$ qubits and $\sim 2n$ couplers. Our work paves the way for large-scale control of superconducting quantum processor., Comment: 9 pages, 6 figures

Quantum Computational Superiority boasts rapid computation and high energy efficiency. Despite recent advances in classical algorithms aimed at refuting the milestone claim of Google's sycamore, challenges remain in generating uncorrelated samples of random quantum circuits. In this paper, we present a groundbreaking large-scale system technology that leverages optimization on global, node, and device levels to achieve unprecedented scalability for tensor networks. This enables the handling of large-scale tensor networks with memory capacities reaching tens of terabytes, surpassing memory space constraints on a single node. Our techniques enable accommodating large-scale tensor networks with up to tens of terabytes of memory, reaching up to 2304 GPUs with a peak computing power of 561 PFLOPS half-precision. Notably, we have achieved a time-to-solution of 14.22 seconds with energy consumption of 2.39 kWh which achieved fidelity of 0.002 and our most remarkable result is a time-to-solution of 17.18 seconds, with energy consumption of only 0.29 kWh which achieved a XEB of 0.002 after post-processing, outperforming Google's quantum processor Sycamore in both speed and energy efficiency, which recorded 600 seconds and 4.3 kWh, respectively.

Random quantum circuit sampling serves as a benchmark to demonstrate quantum computational advantage. Recent progress in classical algorithms, especially those based on tensor network methods, has significantly reduced the classical simulation time and challenged the claim of the first-generation quantum advantage experiments. However, in terms of generating uncorrelated samples, time-to-solution, and energy consumption, previous classical simulation experiments still underperform the \textit{Sycamore} processor. Here we report an energy-efficient classical simulation algorithm, using 1432 GPUs to simulate quantum random circuit sampling which generates uncorrelated samples with higher linear cross entropy score and is 7 times faster than \textit{Sycamore} 53 qubits experiment. We propose a post-processing algorithm to reduce the overall complexity, and integrated state-of-the-art high-performance general-purpose GPU to achieve two orders of lower energy consumption compared to previous works. Our work provides the first unambiguous experimental evidence to refute \textit{Sycamore}'s claim of quantum advantage, and redefines the boundary of quantum computational advantage using random circuit sampling., Comment: This work was completed on August 2023. A further 50x improvement has been achieved and will be posted on arXiv shortly

Single-photon sources are essential for quantum networks, enabling applications ranging from quantum key distribution (QKD) to the burgeoning quantum internet. Despite the remarkable advancements, the current reliance of QKD on attenuated coherent (laser) light sources has imposed a fundamental limit on the secret key rate (SKR). This constraint is primarily attributable to the scarcity of single-photon components within coherent light, confined by an inherent upper bound of 1/e. Here, we report high-rate QKD using a high-efficiency single-photon source, enabling an SKR transcending the fundamental rate limit of coherent light. We developed an on-demand, bright semiconductor quantum-dot single-photon source with an efficiency of 0.71(2), exceeding the inherent bound of coherent light by approximately 2.87 dB. Implementing narrow-bandwidth filtering and random polarization modulation, we conducted a field QKD trial over a 14.6(1.1)-dB-loss free-space urban channel, achieving an SKR of 0.00108 bits per pulse. This surpasses the practical limit of coherent-light-based QKD by 2.53 dB. Our findings conclusively demonstrate the superior performance of nanotechnology-based single-photon sources over coherent light for QKD applications, marking a pivotal stride towards the realization of a global quantum internet., Comment: 22 pages, 5 figures, 1 Table

Finding accurate ground state energy of a many-body system has been a major challenge in quantum chemistry. The integration of classic and quantum computers has shed new light on resolving this outstanding problem. Here we propose QiankunNet-VQE, a transformer based language models enforced with quantum computing to learn and generate quantum states. It has been implemented using up to 12 qubits and attaining an accuracy level competitive with state-of-the-art classical methods. By leveraging both quantum and classical resources, this scheme overcomes the limitations of variational quantum eigensolver(VQE) without the need for cumbersome error mitigation. Moreover, QiankunNet-VQE provides a different route to achieve a practical quantum advantage for solving many-electron Schr\"odinger equation without requiring extremely precise preparation and measurement of the ground-state wavefunction on quantum computer.

To make practical quantum algorithms work, large-scale quantum processors protected by error-correcting codes are required to resist noise and ensure reliable computational outcomes. However, a major challenge arises from defects in processor fabrication, as well as occasional losses or cosmic rays during the computing process, all of which can lead to qubit malfunctions and disrupt error-correcting codes' normal operations. In this context, we introduce an automatic adapter to implement the surface code on defective lattices. Unlike previous approaches, this adapter leverages newly proposed bandage-like super-stabilizers to save more qubits when defects are clustered, thus enhancing the code distance and reducing super-stabilizer weight. For instance, in comparison with earlier methods, with a code size of 27 and a random defect rate of 2\%, the disabled qubits decrease by $1/3$, and the average preserved code distance increases by 63\%. This demonstrates a significant reduction in overhead when handling defects using our approach, and this advantage amplifies with increasing processor size and defect rates. Our work presents a low-overhead, automated solution to the challenge of adapting the surface code to defects, an essential step towards scaling up the construction of large-scale quantum computers for practical applications.

Long baseline diffraction-limited optical aperture synthesis technology by interferometry plays an important role in scientific study and practical application. In contrast to amplitude (phase) interferometry, intensity interferometry -- which exploits the quantum nature of light to measure the photon bunching effect in thermal light -- is robust against atmospheric turbulence and optical defects. However, a thermal light source typically has a significant divergence angle and a low average photon number per mode, forestalling the applicability over long ranges. Here, we propose and demonstrate active intensity interferometry for super-resolution imaging over the kilometer range. Our scheme exploits phase-independent multiple laser emitters to produce the thermal illumination and uses an elaborate computational algorithm to reconstruct the image. In outdoor environments, we image two-dimension millimeter-level targets over 1.36 kilometers at a resolution of 14 times the diffraction limit of a single telescope. High-resolution optical imaging and sensing are anticipated by applying long-baseline active intensity interferometry in general branches of physics and metrology., Comment: 42 pages, 11 figures

In this work, we give a hybrid quantum-classical algorithm for solving electronic structure problems of molecules using only linear quantum optical systems. The variational ansatz we proposed is a hybrid of non-interacting Boson dynamics and classical computational chemistry methods, specifically, the Hartree-Fock method and the Configuration Interaction method. The Boson part is built by a linear optical interferometer which is easier to realize compared with the well-known Unitary Coupled Cluster (UCC) ansatz composed of quantum gates in conventional VQE and the classical part is merely classical processing acting on the Hamiltonian. We called such ansatzes Boson Sampling-Classic (BS-C). The appearance of permanents in the Boson part has its physical intuition to provide different kinds of resources from commonly used single-, double-, and higher-excitations in classical methods and the UCC ansatz to exploring chemical quantum states. Such resources can help enhance the accuracy of methods used in the classical parts. We give a scalable hybrid homodyne and photon number measurement procedure for evaluating the energy value which has intrinsic abilities to mitigate photon loss errors and discuss the extra measurement cost induced by the no Pauli exclusion principle for Bosons with its solutions. To demonstrate our proposal, we run numerical experiments on several molecules and obtain their potential energy curves reaching chemical accuracy., Comment: 15 pages, 5 figures

Quantum randomness relies heavily on the accurate characterization of the generator implementation, where the device imperfection or inaccurate characterization can lead to incorrect entropy estimation and practical bias, significantly affecting the reliability of the generated randomness. Measurement-device-independent (MDI) quantum random number generation (QRNG) endeavors to produce certified randomness, utilizing uncharacterized and untrusted measurement devices that are vulnerable to numerous attack schemes targeting measurement loopholes. However, existing implementations have shown insufficient performance thus far. Here, we propose a high-speed MDI-QRNG scheme based on a robust measurement tomography approach against the imperfection of single-photon sources. Compared with the conventional approach, the decoy-state method is introduced to obtain more accurate tomography results and a tighter lower bound of randomness. Finally, by using a high-speed time-bin encoding system, we experimentally demonstrated the scheme and obtained a reliable min-entropy lower bound of $7.37 \times 10^{-2}$ bits per pulse, corresponding to a generation rate over 23 Mbps, which substantially outperforms the existing realizations and makes a record in discrete-variable semi-device-independent QRNGs., Comment: 20 pages, 9 figures, including appendixes. Accepted for publication in Quantum Science and Technology

Quantum key distribution is a cornerstone of quantum technology, offering information-theoretical secure keys for remote parties. With many quantum communication networks established globally, the mode-pairing protocol stands out for its efficacy over inter-city distances using simple setups, emerging as a promising solution. In this study, we employ the mode-pairing scheme into existing inter-city fiber links, conducting field tests across distances ranging from tens to about a hundred kilometers. Our system achieves a key rate of $1.217$ kbit/s in a $195.85$ km symmetric link and $3.089$ kbit/s in a $127.92$ km asymmetric link without global phase locking. The results demonstrate that the mode-pairing protocol can achieve key rates comparable to those of a single quantum link between two trusted nodes on the Beijing-Shanghai backbone line, effectively reducing the need for half of the trusted nodes. These field tests confirm the mode-pairing scheme's adaptability, efficiency, and practicality, positioning it as a highly suitable protocol for quantum networks., Comment: 15 pages, 5 figures, 6 tables

We report on an experimental simulation of the spin-1 Heisenberg model with composite bosons in a one-dimensional chain based on the two-component Bose-Hubbard model. Exploiting our site-and spin-resolved quantum gas microscope, we observed faster superexchange dynamics of the spin-1 system compared to its spin-1/2 counterpart, which is attributed to the enhancement effect of multi-bosons. We further probed the non-equilibrium spin dynamics driven by the superexchange and single-ion anisotropy terms, unveiling the linear expansion of the spin-spin correlations, which is limited by the Lieb-Robinson bound. Based on the superexchange process, we prepared and verified the entangled qutrits pairs with these composite spin-1 bosons, potentially being applied in qutrit-based quantum information processing.

The counterflow superfluidity (CSF) was predicted two decades ago. Counterintuitively, while both components in the CSF have fluidity, their correlated counterflow currents cancel out leading the overall system to an incompressible Mott insulator. However, realizing and identifying the CSF remain challenging due to the request on extreme experimental capabilities in a single setup. Here, we observe the CSF in a binary Bose mixture in optical lattices. We prepare a low-entropy spin-Mott state by conveying and merging two spin-1/2 bosonic atoms at every site and drive it adiabatically to the CSF at $\sim$ 1 nK. Antipair correlations of the CSF are probed though a site- and spin-resolved quantum gas microscope in both real and momentum spaces. These techniques and observations provide accessibility to the symmetry-protected topological quantum matters., Comment: 13 pages, 10 figures

The fermionic Hubbard model (FHM)[1], despite its simple form, captures essential features of strongly correlated electron physics. Ultracold fermions in optical lattices[2, 3] provide a clean and well-controlled platform for simulating FHM. Doping its antiferromagnetic ground state at half filling, various exotic phases are expected to arise in the FHM simulator, including stripe order[4], pseudogap[5], and d-wave superconductors[6], offering valuable insights into high-temperature superconductivity[7{9]. Although notable progress, such as the observation of antiferromagnetic correlations over short[10] and extended distances[11], has been obtained, the antiferromagnetic phase has yet to be realized due to the significant challenges of achieving low temperatures in a large and uniform quantum simulator. Here, we report the observation of the antiferromagnetic phase transition in a three-dimensional fermionic Hubbard system comprising lithium-6 atoms in a uniform optical lattice with approximately 800,000 sites. When the interaction strength, temperature, and doping concentration are finely tuned to approach their respective critical values, sharp increases in the spin structure factor (SSF) are observed. These observations can be well described by a power-law divergence, with a critical exponent of 1.396 from the Heisenberg universality class[12]. At half filling and with optimal interaction strength, the measured SSF reaches 123(8), signifying the establishment of an antiferromagnetic phase. Our results set the stage for exploring the low-temperature phase diagram of FHM.

Fractional quantum Hall (FQH) states, known for their robust topological order and the emergence of non-Abelian anyons, have captured significant interest due to the appealing applications in fault-tolerant quantum computing. Bottom-up approach on an engineered quantum platform will provide opportunities to operate FQH states without external magnetic field and enhance local and coherent manipulation of these exotic states. Here we demonstrate a lattice version of photon FQH state using a programmable on-chip platform based on photon blockade and engineering gauge fields on a novel two-dimensional circuit quantum electrodynamics (QED) system. We first observe the effective photon Lorentz force and butterfly spectrum in the artificial gauge field, a prerequisite for FQH states. After adiabatic assembly of Laughlin FQH wavefunction of 1/2 filling factor from localized photons, we observe strong density correlation and chiral topological flow among the FQH photons. We then verify the unique features of FQH states in response to external fields, including the incompressibility of generating quasiparticles and the smoking-gun signature of fractional quantum Hall conductivity. Our work represents a significant advance in the bottom-up creation and manipulation of novel strongly correlated topological quantum matter composed of photons and opens up possibilities for fault-tolerant quantum information devices., Comment: 8 pages, 6 figures

In this work, we give a polynomial-time quantum algorithm for solving the ground states of a class of classically hard Hamiltonians. The mechanism of the exponential speedup that appeared in our algorithm comes from dissipation in open quantum systems. To utilize the dissipation, we introduce a new idea of treating vectorized density matrices as pure states, which we call the vectorization picture. By doing so, the Lindblad master equation (LME) becomes a Schr\"odinger equation with non-Hermitian Hamiltonian. The steady state of the LME, therefore, corresponds to the ground states of a special class of Hamiltonians. The runtime of the LME has no dependence on the overlap between the initial state and the ground state. For the input part, given a Hamiltonian, under plausible assumptions, we give a polynomial-time classical procedure to judge and solve whether there exists LME with the desired steady state. For the output part, we propose a novel measurement strategy to extract information about the ground state from the original steady density matrix. We show that the Hamiltonians that can be efficiently solved by our algorithms contain classically hard instances assuming $\text{P}\neq \text{BQP}$. We also discuss possible exponential complexity separations between our algorithm and previous quantum algorithms without using the vectorization picture., Comment: 19 pages, 4 figures,big revision compared before

Solid-state qubits with a photonic interface is very promising for quantum networks. Color centers in silicon carbide have shown excellent optical and spin coherence, even when integrated with membranes and nano-structures. Additionally, nuclear spins coupled with electron spins can serve as long-lived quantum memories. Pioneering work in previous has realized the initialization of a single nuclear spin and demonstrated its entanglement with an electron spin. In this paper, we report the first realization of single-shot readout for a nuclear spin in SiC. We obtain a deterministic readout fidelity of 98.2% with a measurement duration of 1.13 ms. With a dual-step readout scheme, we obtain a readout fidelity as high as 99.5% with a success efficiency of 89.8%. Our work complements the experimental toolbox of harnessing both electron and nuclear spins in SiC for future quantum networks., Comment: 5 pages, 4 figures

Surface currents emerge in superconductors exposed to magnetic fields, and are a key signature of the Meissner effect. Analogously, chiral dynamics were observed in quantum simulators under synthetic Abelian gauge fields. The flexible control of these simulators also facilitates the engineering of non-Abelian gauge fields, but their impact on the chiral dynamics remains elusive. Here, by employing the cutting-edge momentum-lattice technique, we implement a synthetic SU(2) gauge field in a spinful 1D ladder and study the rich chiral dynamics therein. We confirm the non-Abelian nature of the synthetic potential by observing the non-Abelian Aharonov-Bohm effect on a single plaquette. More importantly, the chiral current along the two legs of the ladder is observed to be spin-dependent and highly tunable through the parameters of the gauge potential. We experimentally map out different dynamic regimes of the chiral current, and reveal the underlying competition between overlaying flux ladders with distinct spin compositions. Our experiment demonstrates the dramatic impact of non-Abelian gauge fields on the system dynamics, paving the way for future studies of exotic synthetic gauge fields on the versatile platform of momentum lattices., Comment: 6 pages, 4 figures

The manipulation of particle transport in synthetic quantum matter is an active research frontier for its theoretical importance and potential applications. Here we experimentally demonstrate an engineered topological transport in a synthetic flat-band lattice of ultracold $^{87}$Rb atoms. We implement a quasi-one-dimensional rhombic chain with staggered flux in the momentum space of the atomic condensate and observe biased local oscillations that originate from the interplay of the staggered flux and flat-band localization under the mechanism of Aharonov-Bohm caging. Based on these features, we design and experimentally confirm a state-dependent chiral transport under the periodic modulation of the synthetic flux. We show that the phenomenon is topologically protected by the winding of the Floquet Bloch bands of a coarse-grained effective Hamiltonian. The observed chiral transport offers a strategy for efficient quantum device design where topological robustness is ensured by fast Floquet driving and flat-band localization., Comment: 5 pages, 3 figures

Bell's theorem states that quantum mechanical description on physical quantity cannot be fully explained by local realistic theories, and lays solid basis for various quantum information applications. Hardy's paradox is celebrated to be the simplest form of Bell's theorem concerning its "All versus Nothing" way to test local realism. However, due to experimental imperfections, existing tests of Hardy's paradox require additional assumptions of experimental systems, which constitute potential loopholes for faithfully testing local realistic theories. Here, we experimentally demonstrate Hardy's nonlocality through a photonic entanglement source. By achieving a detection efficiency of $82.2\%$, a quantum state fidelity of $99.10\%$ and applying high speed quantum random number generators for measurement setting switching, the experiment is implemented in a loophole-free manner. During $6$ hours of running, a strong violation of $P_{\text{Hardy}}=4.646\times 10^{-4}$ up to $5$ standard deviations is observed with $4.32\times 10^{9}$ trials. A null hypothesis test shows that the results can be explained by local realistic theories with an upper bound probability of $10^{-16348}$. These testing results present affirmative evidence against local realism, and provide an advancing benchmark for quantum information applications based on Hardy's paradox.

Quantum key distribution (QKD) holds the potential to establish secure keys over long distances. The distance of point-to-point QKD secure key distribution is primarily impeded by the transmission loss inherent to the channel. In the quest to realize a large-scale quantum network, increasing the QKD distance under current technology is of great research interest. Here we adopt the 3-intensity sending-or-not-sending twin-field QKD (TF-QKD) protocol with the actively-odd-parity-pairing method. The experiment demonstrates the feasibility of secure QKD over a 1002 km fibre channel considering the finite size effect. The secure key rate is $3.11\times10^{-12}$ per pulse at this distance. Furthermore, by optimizing parameters for shorter fiber distances, we conducted performance tests on key distribution for fiber lengths ranging from 202 km to 505 km. Notably, the secure key rate for the 202 km, the normal distance between major cities, reached 111.74 kbps., Comment: 18 pages, 3 figures

Photon loss is the biggest enemy for scalable photonic quantum information processing. This problem can be tackled by using quantum error correction, provided that the overall photon loss is below a threshold of 1/3. However, all reported on-demand and indistinguishable single-photon sources still fall short of this threshold. Here, by using tailor shaped laser pulse excitation on a high-quantum efficiency single quantum dot deterministically coupled to a tunable open microcavity, we demonstrate a high-performance source with a single-photon purity of 0.9795(6), photon indistinguishability of 0.986(16), and an overall system efficiency of 0.717(20), simultaneously. This source for the first time reaches the efficiency threshold for scalable photonic quantum computing. With this source, we further demonstrate 1.87(13) dB intensity squeezing, and consecutive 40-photon events with 1.67 mHz count rate.