Search

Cryogenic phonon-scintillation detectors (CPSD) for rare event search experiments require reliable, efficient and robust photon detectors that can resolve individual photons in a scintillation event.

Application of CaMoO4 as a scintillation target in cryogenic rare event searches relies on the understanding of scintillation properties of the material at the temperatures at which these detectors operate. We devised and implemented a detection module with a low-temperature photomultiplier from Hamamatsu (model R8520-06) powered by a Cockcroft-Walton generator. The detector module containing the CaMoO4 crystal was placed in a 3He/4He dilution refrigerator and used to measure scintillation characteristics of CaMoO4 in the millikelvin temperature range. At the lowest temperature achieved, the energy resolution of CaMoO4 for 122 keV from a 57Co source is found to be 30% (FWHM), and the fast and slow decay constants are 40.6+-0.8 us and 3410+-50 us, respectively. The temperature variation of the CaMoO4 decay kinetics is discussed in terms of a three-level model of the emission center

Studies of the X-ray luminescence and scintillation properties of a SrMoO4 crystal as function of temperature down to T=10 K have been carried out. The luminescence in SrMoO4 is quenched at room temperature, but below T<200 K the crystal exhibits a broad emission band with a maximum at a wavelength of 520 nm. The emission is attributed to the radiative decay of self-trapped excitons and defects acting as traps for the exactions at low temperatures. Such complex character of radiative decay is reflected in the kinetics which contains several components plus a contribution from delayed recombination at low temperatures. The temperature dependence of scintillation light output of SrMoO4 was studied. Comparing with a reference ZnWO4 crystal measured under the same experimental conditions it was found that the light output of SrMoO4 is 15+-5%. It is suggested, therefore, that there is scope for optimisation of strontium molybdate for application as scintillator in cryogenic rare event searches

Caesium iodide is one of the more extensively studied scintillators. Here we present X-ray luminescence spectra, scintillation light output and decay curves as function of temperature, from room temperature down to below 10 K. Features of the observed intrinsic luminescence are explained in terms of radiative recombination of on- and off-centre STE. A model permitting interpretation of the dynamics of luminescence changes in CsI with temperature is suggested. This model includes adiabatic potential energy surfaces (APES) associated with singlet and triplet states of self-trapped excitons (STE) and explains the variation of the luminescence spectra with temperature as a result of re-distribution in the population between on- and off-centre STE. The temperature dependence of the scintillation light yield is discussed in the framework of the Onsager mechanism.

Simulations of photon propagation in scintillation detectors were performed with the aim to find the optimal scintillator geometry, surface treatment, and shape of external reflector in order to achieve maximum light collection efficiency for detector configurations that avoid direct optical coupling, a situation that is commonly found in cryogenic scintillating bolometers in experimental searches for double beta decay and dark matter. To evaluate the light collection efficiency of various geometrical configurations we used the ZEMAX ray-tracing software. It was found that scintillators in the shape of a triangular prism with an external mirror shaped as truncated cone gives the highest light collection efficiency. The results of the simulations were confirmed by carrying out measurements of the light collection efficiencies of CaWO4 crystal scintillators. A comparison of simulated and measured values of light output shows good agreement

High light collection efficiency is an important requirement in any application of scintillation detectors. The purpose of this study is to investigate the possibility for improving this parameter in cryogenic scintillation bolometers, which can be considered as a promising detectors in experiments investigating neutrinoless double beta decay and dark matter. Energy resolutions and relative pulse amplitudes of scintillation detectors using ZnWO4 scintillation crystals of different shapes (cylinder 20 mm in dimater by 20 mm and hexagonal prism with diagonal 20 mm and height 20 mm), reflector materials and shapes, optical contact and surface properties (polished and diffused) were measured at room temperature. Propagation of optical photons in these experimental conditions was simulated using Geant4 and ZEMAX codes. The results of the simulations are found to be in good agreement with each other and with direct measurements of the crystals. This could be applied to optimize the geometry of scintillation detectors used in the cryogenic experiments., Comment: 12 pages, 8 figures, 1 Table

The Workshop on results of the Project Kosmomikrofizyka-2 (Astroparticle Physics) of the National Academy of Sciences (NAS) of Ukraine "Astrophysical and cosmological problems of invisible mass and dark energy in the Universe" was held on November 21-22, 2012 in the Institute for Nuclear Research, Kyiv, Ukraine (http://lpd.kinr.kiev.ua/kmf12). This Project was carried out during three years (2010-2012) by scientists from various universities and institutes of the National Academy of Sciences of Ukraine; it was a logical continuation of the previous scientific program of the NAS of Ukraine "Researches of structure and composition of the Universe, hidden mass and dark energy (Kosmomikrofizyka)" in 2007-2009. These programs were devoted to theoretical and experimental investigations in astronomy, astrophysics, cosmology, physics of atomic nuclei and particle physics, which are related with the problems of dark matter and dark energy in the Universe., Comment: Proceedings of the Workshop on results of the Project Kosmomikrofizyka-2 (Astroparticle Physics) of the National Academy of Sciences of Ukraine, November 21-22, 2012, Institute for Nuclear Research, Kyiv, Ukraine. 94 pages, 29 figures, 5 tables (in English, Ukrainian, Russian)

The use of 40Ca100MoO in experimental searches for neutrinoless double beta decay (0{\nu}DBD) relies on knowledge of fundamental scintillation properties of the material. In this work we determine the absolute light yield of calcium molybdate using Monte-Carlo refractive index matching technique (MCRIM). The MCRIM technique is a combination of experiment and simulations that allows the absolute light yield of scintillators to be determined by taking into account effects of refraction, scattering and absorption in the material. The light collection efficiency of the scintillator-detector assembly was simulated using the ZEMAX ray-tracing software. By tuning the optical parameters of the scintillation crystal, a model was derived that gives good agreement with the experimental results. It is shown that the light collection efficiency of scintillators increases with transmittance and scattering due to an enhanced probability for photons to escape the crystal volume. Using MCRIM, the absolute light yield for the 40Ca100MoO4 scintillator was found to be 7.5+-1.2 ph/keV at room temperature. Comparative measurements using a CaWO4 scintillator as a reference show good agreement with this result. In that way, the study demonstrated the potential of the MCRIM technique as a tool for quantitative characterization of scintillation materials.

Future cryogenic experiments searching for rare events require reliable, efficient and robust techniques for the detection of photons at temperatures well below that to which low-temperature photomultipliers (PMT) were characterised. Motivated by this we investigated the feasibility of a low-temperature PMT for the detection of scintillation from crystalline scintillators at T = 6 K. The scintillation module was composed of a CaWO4 scintillator and a low-temperature PMT D745B from ET Enterprises. The PMT responsivity was studied at T=290, 77 and 6 K using gamma-quanta from 241Am (60 keV) and 57Co (122 and 136 keV) sources. We have shown that the low-temperature PMT retains its single photon counting ability even at cryogenic temperatures. At T = 6 K, the response of the PMT decreases to 51 +- 13 % and 27 +- 6 % when assessed in photon counting and pulse height mode, respectively. Due to the light yield increase of the CaWO4 scintillating crystal the overall responsivity of the scintillation modules CaWO4+PMT is 94 +- 15 % (photon counting) and 48 +- 8 % (pulse height) when cooling to T = 6 K. The dark count rate was found to be 20 s-1. The energy resolution of the module remains similar to that measured at room temperature using either detection mode. It is concluded that commercially available low-temperature PMT are well suited for detection of scintillation light at cryogenic temperatures.

An increasing number of applications of scintillators at low temperatures, particularly in cryogenic experiments searching for rare events, has motivated the investigation of scintillation properties of materials over a wide temperature range. This paper provides an overview of the latest results on the study of luminescence, absorption and scintillation properties of materials selected for rare event searches so far. These include CaWO4, ZnWO4, CdWO4, MgWO4, CaMoO4, CdMoO4, Bi4Ge3O12, CaF2, MgF2, ZnSe and AL2O3-Ti. We discuss the progress achieved in research and development of these scintillators, both in material preparation and in the understanding of scintillation mechanisms, as well as the underlying physics. To understand the origin of the performance limitation of self-activated scintillators we employed a semi-empirical model of conversion of high energy radiation into light and made appropriate provision for effects of temperature and energy transfer. We conclude that the low-temperature value of the light yield of some modern scintillators, namely CaWO4, CdWO4 and Bi4Ge3O12, is close to the theoretical limit. Finally, we discuss the advantages and limitations of different materials with emphasis on their application as cryogenic phonon-scintillation detectors (CPSD) in rare event search experiments.

The CRESST experiment aims for a detection of dark matter in the form of WIMPs. These particles are expected to scatter elastically off the nuclei of a target material, thereby depositing energy on the recoiling nucleus. CRESST uses scintillating CaWO4 crystals as such a target. The energy deposited by an interacting particle is primarily converted to phonons which are detected by transition edge sensors. In addition, a small fraction of the interaction energy is emitted from the crystals in the form of scintillation light which is measured in coincidence with the phonon signal by a separate cryogenic light detector for each target crystal. The ratio of light to phonon energy permits the discrimination between the nuclear recoils expected from WIMPs and events from radioactive backgrounds which primarily lead to electron recoils. CRESST has shown the success of this method in a commissioning run in 2007 and, since then, further investigated possibilities for an even better suppression of backgrounds. Here, we report on a new class of background events observed in the course of this work. The consequences of this observation are discussed and we present the current status of the experiment., Comment: Proceedings of the 13th International Workshop on Low Temperature Detectors, 4 pages, 3 figures

CRESST-II, standing for Cryogenic Rare Events Search with Superconducting Thermometers phase II, is an experiment searching for Dark Matter. In the LNGS facility in Gran Sasso, Italy, a cryogenic detector setup is operated in order to detect WIMPs by elastic scattering off nuclei, generating phononic lattice excitations and scintillation light. The thermometers used in the experiment consist of a tungsten thin-film structure evaporated onto the CaWO4 absorber crystal. The process of evaporation causes a decrease in the scintillation light output. This, together with the need of a big-scale detector production for the upcoming EURECA experiment lead to investigations for producing thermometers on smaller crystals which are glued onto the absorber crystal. In our Run 31 we tested composite detectors for the first time in the Gran Sasso setup. They seem to produce higher light yields as hoped and could provide an additional time based discrimination mechanism for low light yield clamp events., Comment: Proceedings of the Thirteenth International Workshop on Low Temperature Detectors 4 pages, 9 figures

We measure and explain scintillator non-proportionality and gamma quenching of CaWO4 at low energies and low temperatures. Phonons that are created following an interaction in the scintillating crystal at temperatures of 15mK are used for a calorimetric measurement of the deposited energy, and the scintillation light is measured with a separate cryogenic light detector. Making use of radioactivity intrinsic to the scintillating crystal, the scintillator non-proportionality is mapped out to electron energies <5keV. The observed behavior is in agreement with a simple model based on Birks' law and the stopping power dE/dx for electrons. We find for Birks' constant $k_B=(18.5\pm0.7)$nm/keV in CaWO4. Gamma lines allow a measurement of the reduced light yield of photons with respect to electrons, as expected in the presence of scintillator non-proportionality. In particular, we show that gamma-induced events in CaWO4 give only about 90 percent of the light yield of electrons, at energies between 40keV and 80keV., Comment: 5 pages, 5 figures

The CRESST experiment monitors 300g CaWO_4 crystals as targets for particle interactions in an ultra low background environment. In this paper, we analyze the background spectra that are recorded by three detectors over many weeks of data taking. Understanding these spectra is mandatory if one wants to further reduce the background level, and allows us to cross-check the calibration of the detectors. We identify a variety of sources, such as intrinsic contaminations due to primordial radioisotopes and cosmogenic activation of the target material. In particular, we detect a 3.6keV X-ray line from the decay of 41-Ca with an activity of (26\pm4)\mu Bq, corresponding to a ratio 41-Ca/40-Ca=(2.2\pm0.3)\times10^{-16}., Comment: 7 pages, 12 figures

The alpha decay of $\n{{}^{210}Po}$ is a dangerous background to rare event searches. Here, we describe observations related to this alpha decay in the Cryogenic Rare Event Search with Superconducting Thermometers (CRESST). We find that lead nuclei show a scintillation light yield in our $\n{CaWO_4}$ crystals of $0.0142\pm0.0013$ relative to electrons of the same energy. We describe a way to discriminate this source of nuclear recoil background by means of a scintillating foil, and demonstrate its effectiveness. This leads to an observable difference in the pulse shape of the light detector, which can be used to tag these events. Differences in pulse shape of the phonon detector between lead and electron recoils are also extracted, opening the window to future additional background suppression techniques based on pulse shape discrimination in such experiments., Comment: 5 pages, 9 figures

The CRESST cryogenic direct dark matter search at Gran Sasso, searching for WIMPs via nuclear recoil, has been upgraded to CRESST-II by several changes and improvements.We present the results of a commissioning run carried out in 2007. The basic element of CRESST-II is a detector module consisting of a large (~ 300 g) CaWO_4 crystal and a very sensitive smaller (~ 2 g) light detector to detect the scintillation light from the CaWO_4.Information from light-quenching factor studies allows the definition of a region of the energy-light yield plane which corresponds to tungsten recoils. A neutron test is reported which supports the principle of using the light yield to identify the recoiling nucleus. Data obtained with two detector modules for a total exposure of 48 kg-days are presented. Judging by the rate of events in the "all nuclear recoils" acceptance region the apparatus shows a factor ~ten improvement with respect to previous results, which we attribute principally to the presence of the neutron shield. In the "tungsten recoils" acceptance region three events are found, corresponding to a rate of 0.063 per kg-day. Standard assumptions on the dark matter flux, coherent or spin independent interactions,then yield a limit for WIMP-nucleon scattering of 4.8 \times 10^{-7}pb, at M{WIMP} ~50 GeV., Comment: 10 pages, 9 figs No essential changes in content. Minor errors corrected. Sentence added at end of introduction concerning increased sensitivity. Best limit on plots at M=50 GeV. Text labelling of candidate events corrected

We present first competitive results on WIMP dark matter using the phonon-light-detection technique. A particularly strong limit for WIMPs with coherent scattering results from selecting a region of the phonon-light plane corresponding to tungsten recoils. The observed count rate in the neutron band is compatible with the rate expected from neutron background. CRESST is presently being upgraded with a 66 channel SQUID readout system, a neutron shield and a muon veto system. This results in a significant improvement in sensitivity., Comment: 6 pages, 3 figures, to be published in the proceedings of the 5th International Workshop on the Identification and Detection of Dark Matter IDM 2004, Edinburgh, Sept. 2004, World Scientific

The natural alpha decay of 180W has been unambiguously detected for the first time. The alpha peak is found in a (gamma,beta and neutron)-free background spectrum. This has been achieved by the simultaneous measurement of phonon and light signals with the CRESST cryogenic detectors. A half-life of T1/2 = (1.8 +- 0.2) x 10^18 y and an energy release of Q = (2516.4 +- 1.1 (stat.) +- 1.2 (sys.)) keV have been measured. New limits are also set on the half-lives of the other naturally occurring tungsten isotopes., Comment: Submitted to Physical Review C Revised version