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C4F7N/CO2 mixture has been widely studied as an environmental-friendly insulating gas expected to replace sulfur hexafluoride (SF6) in high-voltage equipment. In high-voltage power systems, the medium dielectric characteristics under switching impulse (SI) voltage are an important factor in insulation coordination. Nevertheless, few studies on this aspect of C4F7N/CO2 mixture have been reported. This article investigates the surface flashover of a cylindrical insulator in a C4F7N/CO2 mixture under switching voltage. The effects of molar fraction, gas pressure, creepage distance, and insulator materials on surface flashover voltage are studied in a uniform field. The result shows that the increase of flashover voltage indicates a saturation trend with the increase of C4F7N molar fraction and pressure, respectively. The dielectric strength of 13% C4F7N/87% CO2 relative to SF6 can reach at least 84%. The limiting factors of the flashover voltage increase under high pressure are preliminarily discussed. Additionally, the empirical formula on the critical flashover electrical field has been obtained, which can provide a reference for insulation design for environment-friendly gas insulation equipment. [ABSTRACT FROM AUTHOR]