Search

A long-term measurement was conducted to search for $\alpha$, double-$\alpha$ and double-$\beta$ decays with $\gamma$ quanta emission in naturally occurring osmium isotopes. This study took advantage of two ultra-low background HPGe detectors and one ultra-low background BEGe detector at the Gran Sasso National Laboratory (LNGS) of the INFN. Over almost 5 years of data were taken using high-purity osmium samples of approximately 173 g. The half-life limits set for a decays of $^{184}$Os to the first $2^+$ 103.6 keV excited level of $^{180}$W ($T_{1/2} > 9.3 \times 10^{15}$ yr) and of $^{186}$Os to the first $2^+$ 100.1 keV of $^{182}$W ($T_{1/2} > 4.8 \times 10^{17}$ yr) exceed substantially the present theoretical predictions that are at level of $T_{1/2} \sim (0.6 - 3) \times 10^{15}$ yr for $^{184}$Os and $T_{1/2} \sim (0.3 - 2) \times 10^{17}$ yr for $^{186}$Os. New half-life limits on the 2EC and EC$\beta^+$ decay of $^{184}$Os to the ground and excited levels of $^{184}$W were set at level of $T_{1/2} > 10^{16} - 10^{17}$ yr; a lower limit on the $2\beta^-$ decay of $^{192}$Os to the $2^+$ 316.5 keV excited level of $^{192}$Pt was estimated as $T_{1/2} > 6.1 \times 10^{20}$ yr. The half-life limits for $2\alpha$ decay of $^{189}$Os and $^{192}$Os were set for the first time at level of $T_{1/2} > 10^{20}$ yr., Comment: 38 pages, 17 figures, 5 tables

A search for full energy depositions from bosonic keV-scale dark matter candidates of masses between 65 keV and 1021 keV has been performed with data collected during Phase II of the GERmanium Detector Array (GERDA) experiment. Our analysis includes direct dark matter absorption as well as dark Compton scattering. With a total exposure of 105.5 kg yr, no evidence for a signal above the background has been observed. The resulting exclusion limits deduced with either Bayesian or Frequentist statistics are the most stringent direct constraints in the major part of the 140-1021 keV mass range. As an example, at a mass of 150 keV the dimensionless coupling of dark photons and axion-like particles to electrons has been constrained to $\alpha$'/$\alpha$ < 8.7x10$^{-24}$ and g$_{ae}$ < 3.3x10$^{-12}$ at 90% credible interval (CI), respectively. Additionally, a search for peak-like signals from beyond the Standard Model decays of nucleons and electrons is performed. We find for the inclusive decay of a single neutron in $^{76}$Ge a lower lifetime limit of $\tau_n$ > 1.5x10$^{24}$ yr and for a proton $\tau_p$ > 1.3x10$^{24}$ yr at 90% CI. For the electron decay e$^-\rightarrow\nu_e\gamma$ a lower limit of $\tau_e$ > 5.4x10$^{25}$ yr at 90% CI has been determined., Comment: 20 pages, 12 figures, 7 tables

The GERmanium Detector Array (GERDA) experiment operated enriched high-purity germanium detectors in a liquid argon cryostat, which contains 0.33% of $^{36}$Ar, a candidate isotope for the two-neutrino double-electron capture (2$\nu$ECEC) and therefore for the neutrinoless double-electron capture (0$\nu$ECEC). If detected, this process would give evidence of lepton number violation and the Majorana nature of neutrinos. In the radiative 0$\nu$ECEC of $^{36}$Ar, a monochromatic photon is emitted with an energy of 429.88 keV, which may be detected by the GERDA germanium detectors. We searched for the $^{36}$Ar 0$\nu$ECEC with GERDA data, with a total live time of 4.34 yr (3.08 yr accumulated during GERDA Phase II and 1.26 yr during GERDA Phase I). No signal was found and a 90% C.L. lower limit on the half-life of this process was established T$_{1/2}$ > 1.5x10$^{22}$ yr, Comment: 10 pages, 5 figures, 1 table

The Golden (British Columbia, Canada) meteorite fall occurred on Oct 4, 2021 at 0534 UT with the first recovered fragment (1.3 kg) landing on an occupied bed. The meteorite is an unbrecciated, low-shock (S2) ordinary chondrite of intermediate composition, typed as an L/LL5. From noble gas measurements the cosmic ray exposure age is 25 Ma while gas retention ages are all >2 Ga. Short-lived radionuclides and noble gas measurements of the pre-atmospheric size overlap with estimates from infrasound and lightcurve modelling producing a preferred pre-atmospheric mass of 70-200 kg. The orbit of Golden has a high inclination (23.5 degs) and is consistent with delivery from the inner main belt. The highest probability (60%) of an origin is from the Hungaria group. We propose that Golden may originate among the background S-type asteroids found interspersed in the Hungaria region. The current collection of 18 L and LL chondrite orbits shows a strong preference for origins in the inner main belt, suggesting multiple parent bodies may be required to explain the diversity in CRE ages and shock states., Comment: 92 Pages, 20 Tables, 21 Figures, plus 3 appendices, accepted in Meteoritics and Planetary Science Oct 26 2023

Borexino could efficiently distinguish between alpha and beta radiation in its liquid scintillator by the characteristic time profile of their scintillation pulse. This alpha/beta discrimination, first demonstrated at the tonne scale in the Counting Test Facility prototype, was used throughout the lifetime of the experiment between 2007 and 2021. With this method, alpha events are identified and subtracted from the beta-like solar neutrino events. This is particularly important in liquid scintillator as alpha scintillation is quenched many-fold. In Borexino, the prominent Po-210 decay peak was a background in the energy range of electrons scattered from Be-7 solar neutrinos. Optimal alpha-beta discrimination was achieved with a "multi-layer perceptron neural network", which its higher ability to leverage the timing information of the scintillation photons detected by the photomultiplier tubes. An event-by-event, high efficiency, stable, and uniform pulse shape discrimination was essential in characterising the spatial distribution of background in the detector. This benefited most Borexino measurements, including solar neutrinos in the \pp chain and the first direct observation of the CNO cycle in the Sun. This paper presents the key milestones in alpha/beta discrimination in Borexino as a term of comparison for current and future large liquid scintillator detectors, Comment: 13 pages, 14 figures

We present the measurement of the two-neutrino double-$\beta$ decay rate of $^{76}$Ge performed with the GERDA Phase II experiment. With a subset of the entire GERDA exposure, 11.8 kg$\cdot$yr, the half-life of the process has been determined: $T^{2\nu}_{1/2} = (2.022 \pm 0.018_{stat} \pm 0.038_{sys})\times10^{21}$ yr. This is the most precise determination of the $^{76}$Ge two-neutrino double-$\beta$ decay half-life and one of the most precise measurements of a double-$\beta$ decay process. The relevant nuclear matrix element can be extracted: $M^{2\nu}_{\text{eff}} = (0.101\pm0.001).$, Comment: 7 pages, 4 figures, 2 tables

We search for tri-nucleon decays of $^{76}$Ge in the dataset from the GERmanium Detector Array (GERDA) experiment. Decays that populate excited levels of the daughter nucleus above the threshold for particle emission lead to disintegration and are not considered. The ppp-, ppn-, and pnn-decays lead to $^{73}$Cu, $^{73}$Zn, and $^{73}$Ga nuclei, respectively. These nuclei are unstable and eventually proceed by the beta decay of $^{73}$Ga to $^{73}$Ge (stable). We search for the $^{73}$Ga decay exploiting the fact that it dominantly populates the 66.7 keV $^{73m}$Ga state with half-life of 0.5 s. The nnn-decays of $^{76}$Ge that proceed via $^{73m}$Ge are also included in our analysis. We find no signal candidate and place a limit on the sum of the decay widths of the inclusive tri-nucleon decays that corresponds to a lower lifetime limit of 1.2x10$^{26}$ yr (90% credible interval). This result improves previous limits for tri-nucleon decays by one to three orders of magnitude., Comment: 8 pages, 9 figures, 3 tables

We report the first measurement of CNO solar neutrinos by Borexino that uses the Correlated Integrated Directionality (CID) method, exploiting the sub-dominant Cherenkov light in the liquid scintillator detector. The directional information of the solar origin of the neutrinos is preserved by the fast Cherenkov photons from the neutrino scattered electrons, and is used to discriminate between signal and background. The directional information is independent from the spectral information on which the previous CNO solar neutrino measurements by Borexino were based. While the CNO spectral analysis could only be applied on the Phase-III dataset, the directional analysis can use the complete Borexino data taking period from 2007 to 2021. The absence of CNO neutrinos has been rejected with >5{\sigma} credible level using the Bayesian statistics. The directional CNO measurement is obtained without an external constraint on the $^{210}$Bi contamination of the liquid scintillator, which was applied in the spectral analysis approach. The final and the most precise CNO measurement of Borexino is then obtained by combining the new CID-based CNO result with an improved spectral fit of the Phase-III dataset. Including the statistical and the systematic errors, the extracted CNO interaction rate is $R(\mathrm{CNO})=6.7^{+1.2}_{-0.8} \, \mathrm{cpd/100 \, tonnes}$. Taking into account the neutrino flavor conversion, the resulting CNO neutrino flux at Earth is $\Phi_\mathrm{CNO}=6.7 ^{+1.2}_{-0.8} \times 10^8 \, \mathrm{cm^{-2} s^{-1}}$, in agreement with the high metallicity Standard Solar Models. The results described in this work reinforce the role of the event directional information in large-scale liquid scintillator detectors and open up new avenues for the next-generation liquid scintillator or hybrid neutrino experiments.

Using CaWO$_4$ crystals as cryogenic calorimeters, the CRESST experiment searches for nuclear recoils caused by the scattering of potential Dark Matter particles. A reliable identification of a potential signal crucially depends on an accurate background model. In this work we introduce an improved normalisation method for CRESST's model of the electromagnetic backgrounds. Spectral templates, based on Geant4 simulations, are normalised via a Bayesian likelihood fit to experimental background data. Contrary to our previous work, no assumption of partial secular equilibrium is required, which results in a more robust and versatile applicability. Furthermore, considering the correlation between all background components allows us to explain 82.7% of the experimental background within [1 keV, 40 keV], an improvement of 18.6% compared to our previous method., Comment: 24 pages, 14 figures, submitted to EPJC

$^{180m}$Ta is the longest-lived metastable state presently known. Its decay has not been observed yet. In this work, we report a new result on the decay of \mTa obtained with a $2015.12$-g tantalum sample measured for $527.7$ d with an ultra-low background HPGe detector in the STELLA laboratory of the Laboratori Nazionali del Gran Sasso (LNGS), in Italy. Before the measurement, the sample has been stored deep-underground for ten years, resulting in subdominant background contributions from cosmogenically activated $^{182}$Ta. We observe no signal in the regions of interest and set half-life limits on the process for the two channels EC and $\beta^-$: $T_{1/2,~\mathrm{EC}} > 1.6 \times 10^{18}$ yr and $T_{1/2,~\beta^-} > 1.1\times 10^{18}$ yr ($90$\% C.\,I.), respectively. We also set the limit on the $\gamma$ de-excitation / IC channel: $T_{1/2,~\mathrm{IC}} > 4.1 \times 10^{15}$ yr ($90$\% C.\,I.). These are, as of now, the most stringent bounds on the decay of $^{180m}$Ta worldwide. Finally, we test the hypothetical scenarios of de-excitation of $^{180m}$Ta by cosmological Dark Matter and constrain new parameter space for strongly-interacting dark-matter particle with mass up to $10^5$ GeV., Comment: 9 pages, 7 figures, 4 tables

In this work, we present novel Machine Learning and Differentiable Programming enhanced calibration techniques used to improve the energy resolution of the Silicon Drift Detectors (SDDs) of the VIP-2 underground experiment at the Gran Sasso National Laboratory (LNGS). We achieve for the first time a Full Width at Half Maximum (FWHM) in VIP-2 below 180 eV at 8 keV, improving around 10 eV on the previous state-of-the-art. SDDs energy resolution is a key parameter in the VIP-2 experiment, which is dedicated to searches for physics beyond the standard quantum theory, targeting Pauli Exclusion Principle (PEP) violating atomic transitions. Additionally, we show that this method can correct for potential miscalibrations, requiring less fine-tuning with respect to standard methods., Comment: Submitted to Measurement Science and Technology

The first detailed study on the performance of a ZnO-based cryogenic scintillating bolometer as a detector to search for rare processes in zinc isotopes was performed. A 7.2 g ZnO low-temperature detector, containing more than 80\% of zinc in its mass, exhibits good energy resolution of baseline noise 1.0--2.7 keV FWHM at various working temperatures resulting in a low-energy threshold for the experiment, 2.0--6.0 keV. The light yield for $\beta$/$\gamma$ events was measured as 1.5(3) keV/MeV, while it varies for $\alpha$ particles in the range of 0.2--3.0 keV/MeV. The detector demonstrate an effective identification of the $\beta$/$\gamma$ events from $\alpha$ events using time-properties of only heat signals. %(namely, Rise time parameter). The radiopurity of the ZnO crystal was evaluated using the Inductively Coupled Plasma Mass Spectrometry, an ultra-low-background High Purity Ge $\gamma$-spectrometer, and bolometric measurements. Only limits were set at the level of $\mathcal{O}$(1--100) mBq/kg on activities of \Nuc{K}{40}, \Nuc{Cs}{137} and daughter nuclides from the U/Th natural decay chains. The total internal $\alpha$-activity was calculated to be 22(2) mBq/kg, with a major contribution caused by 6(1) mBq/kg of \Nuc{Th}{232} and 12(2) mBq/kg of \Nuc{U}{234}. Limits on double beta decay (DBD) processes in \Nuc{Zn}{64} and \Nuc{Zn}{70} isotopes were set on the level of $\mathcal{O}(10^{17}$--$10^{18})$ yr for various decay modes profiting from 271 h of acquired background data in the above-ground lab. This study shows a good potential for ZnO-based scintillating bolometers to search for DBD processes of Zn isotopes, especially in \Nuc{Zn}{64}, with the most prominent spectral features at $\sim$10--20 keV, like the two neutrino double electron capture. A 10 kg-scale experiment can reach the experimental sensitivity at the level of $\mathcal{O}(10^{24})$ yr., Comment: Prepared for submission to JINST; 27 pages, 9 figures, and 7 tables

The search for neutrino events in correlation with gravitational wave (GW) events for three observing runs (O1, O2 and O3) from 09/2015 to 03/2020 has been performed using the Borexino data-set of the same period. We have searched for signals of neutrino-electron scattering with visible energies above 250 keV within a time window of 1000 s centered at the detection moment of a particular GW event. The search was done with three visible energy thresholds of 0.25, 0.8 and 3.0 MeV.Two types of incoming neutrino spectra were considered: the mono-energetic line and the spectrum expected from supernovae. The same spectra were considered for electron antineutrinos detected through inverse beta-decay (IBD) reaction. GW candidates originated by merging binaries of black holes (BHBH), neutron stars (NSNS) and neutron star and black hole (NSBH) were analysed separately. Additionally, the subset of most intensive BHBH mergers at closer distances and with larger radiative mass than the rest was considered. In total, follow-ups of 74 out of 93 gravitational waves reported in the GWTC-3 catalog were analyzed and no statistically significant excess over the background was observed. As a result, the strongest upper limits on GW-associated neutrino and antineutrino fluences for all flavors (\nu_e, \nu_\mu, \nu_\tau) have been obtained in the (0.5 - 5.0) MeV neutrino energy range., Comment: 13 pages, 8 figures

A search for rare decays of gadolinium isotopes was performed with an ultra-low background high-purity germanium detector at Gran Sasso Underground Laboratory (Italy). A 198 g Gd$_2$O$_3$ powder sample was measured for 63.8 d with a total Gd exposure of 12.6 kg$\times$d. $^{152}$Gd is the most promising isotope for resonant neutrinoless double electron capture which could significantly enhance the decay rate over other neutrinoless double beta decay processes. The half-life for this decay was constrained to $>4.2\times10^{12}$ yr (90\% credibility). This limit is still orders of magnitude away from theoretical predictions but it is the first established limit on the transition paving the way for future experiments. In addition, other rare alpha and double beta decay modes were investigated in $^{152}$Gd, $^{154}$Gd, and $^{160}$Gd with half-life limits in the range of $10^{17-20}$ yr., Comment: fixed typos and minor text changes

The ability to detect liquid argon scintillation light from within a densely packed high-purity germanium detector array allowed the GERDA experiment to reach an exceptionally low background rate in the search for neutrinoless double beta decay of $^{76}$Ge. Proper modeling of the light propagation throughout the experimental setup, from any origin in the liquid argon volume to its eventual detection by the novel light read-out system, provides insight into the rejection capability and is a necessary ingredient to obtain robust background predictions. In this paper, we present a model of the GERDA liquid argon veto, as obtained by Monte Carlo simulations and constrained by calibration data, and highlight its application for background decomposition.

Radioactivity was recently discovered as a source of decoherence and correlated errors for the real-world implementation of superconducting quantum processors. In this work, we measure levels of radioactivity present in a typical laboratory environment (from muons, neutrons, and gamma's emitted by naturally occurring radioactive isotopes) and in the most commonly used materials for the assembly and operation of state-of-the-art superconducting qubits. We develop a GEANT-4 based simulation to predict the rate of impacts and the amount of energy released in a qubit chip from each of the mentioned sources. We finally propose mitigation strategies for the operation of next-generation qubits in a radio-pure environment.

A 510 day long-term measurement of a 45.3 g platinum foil acting as the sample and high voltage contact in an ultra-low-background high purity germanium detector was performed at Laboratori Nazionali del Gran Sasso (Italy). The data was used for a detailed study of double beta decay modes in natural platinum isotopes. Limits are set in the range $\mathcal{O}(10^{14} - 10^{19})$ yr (90% C.L.) for several double beta decay transitions to excited states confirming, and partially extending existing limits. The highest sensitivity of the measurement, greater than $10^{19}$ yr, was achieved for the two neutrino and neutrinoless double beta decay modes of the isotope $^{198}$Pt. Additionally, novel limits for inelastic dark matter scattering on $^{195}$Pt are placed up to mass splittings of approximately 500 keV. We analyze several techniques to extend the sensitivity and propose a few approaches for future medium-scale experiments with platinum-group elements., Comment: 15 pages, 3 figures, updated from journal review

A search for Beyond the Standard Model double-$\beta$ decay modes of $^{76}$Ge has been performed with data collected during the Phase II of the GERmanium Detector Array (GERDA) experiment, located at Laboratori Nazionali del Gran Sasso of INFN (Italy). Improved limits on the decays involving Majorons have been obtained, compared to previous experiments with $^{76}$Ge, with half-life values on the order of 10$^{23}$ yr. For the first time with $^{76}$Ge, limits on Lorentz invariance violation effects in double-$\beta$ decay have been obtained. The isotropic coefficient $\mathring{a}_\text{of}^{(3)}$, which embeds Lorentz violation in double-$\beta$ decay, has been constrained at the order of $10^{-6}$ GeV. We also set the first experimental limits on the search for light exotic fermions in double-$\beta$ decay, including sterile neutrinos.

CRESST is a leading direct detection sub-$\mathrm{GeVc}^{-2}$ dark matter experiment. During its second phase, cryogenic bolometers were used to detect nuclear recoils off the $\mathrm{CaWO}_4$ target crystal nuclei. The previously established electromagnetic background model relies on secular equilibrium (SE) assumptions. In this work, a validation of SE is attempted by comparing two likelihood-based normalisation results using a recently developed spectral template normalisation method based on Bayesian likelihood. We find deviations from SE; further investigations are necessary to determine their origin., Comment: Part of special issue: ICRM-LLRMT22 8th International Conference on Radionuclide Metrology - Low Level Radioactivity Measurement and Techniques, 6 pages, 3 figures

We present an improved measurement of the CNO solar neutrino interaction rate at Earth obtained with the complete Borexino Phase-III dataset. The measured rate R$_{\rm CNO}$ = $6.7^{+2.0}_{-0.8}$ counts/(day$ \cdot$ 100 tonnes), allows us to exclude the absence of the CNO signal with about 7$\sigma$ C.L. The correspondent CNO neutrino flux is $6.6^{+2.0}_{-0.9} \times 10^8$ cm$^{-2}$ s$^{-1}$, taking into account the neutrino flavor conversion. We use the new CNO measurement to evaluate the C and N abundances in the Sun with respect to the H abundance for the first time with solar neutrinos. Our result of $N_{\rm CN}$ = $(5.78^{+1.86}_{-1.00})\times10^{-4}$ displays a $\sim$2$\sigma$ tension with the "low metallicity" spectroscopic photospheric measurements. On the other hand, our result used together with the $^7$Be and $^8$B solar neutrino fluxes, also measured by Borexino, permits to disfavour at 3.1$\sigma$ C.L. the "low metallicity" SSM B16-AGSS09met as an alternative to the "high metallicity" SSM B16-GS98., Comment: 8 pages, 6 figures

Since the beginning of 2012, the Borexino collaboration has been reporting precision measurements of the solar neutrino fluxes, emitted in the proton-proton chain and in the Carbon-Nitrogen-Oxygen cycle. The experimental sensitivity achieved in Phase-II and Phase-III of the Borexino data taking made it possible to detect the annual modulation of the solar neutrino interaction rate due to the eccentricity of Earth's orbit, with a statistical significance greater than 5$\sigma$. This is the first precise measurement of the Earth's orbital parameters based solely on solar neutrinos and an additional signature of the solar origin of the Borexino signal. The complete periodogram of the time series of the Borexino solar neutrino detection rate is also reported, exploring frequencies between one cycle/year and one cycle/day. No other significant modulation frequencies are found. The present results were uniquely made possible by Borexino's decade-long high-precision solar neutrino detection., Comment: 12 pages, 10 figures

The GERmanium Detector Array (GERDA) collaboration searched for neutrinoless double-$\beta$ decay in $^{76}$Ge using isotopically enriched high purity germanium detectors at the Laboratori Nazionali del Gran Sasso of INFN. After Phase I (2011-2013), the experiment benefited from several upgrades, including an additional active veto based on LAr instrumentation and a significant increase of mass by point-contact germanium detectors that improved the half-life sensitivity of Phase II (2015-2019) by an order of magnitude. At the core of the background mitigation strategy, the analysis of the time profile of individual pulses provides a powerful topological discrimination of signal-like and background-like events. Data from regular $^{228}$Th calibrations and physics data were both considered in the evaluation of the pulse shape discrimination performance. In this work, we describe the various methods applied to the data collected in GERDA Phase II corresponding to an exposure of 103.7 kg$\cdot$yr. These methods suppress the background by a factor of about 5 in the region of interest around Q$_{\beta\beta}$ = 2039 keV, while preserving (81$\pm$3)% of the signal. In addition, an exhaustive list of parameters is provided which were used in the final data analysis.

We report the measurement of sub-MeV solar neutrinos through the use of their associated Cherenkov radiation, performed with the Borexino detector at the Laboratori Nazionali del Gran Sasso. The measurement is achieved using a novel technique that correlates individual photon hits of events to the known position of the Sun. In an energy window between 0.54 MeV to 0.74 MeV, selected using the dominant scintillation light, we have measured 10887$^{+2386}_{-2103} (\mathrm{stat.})\pm 947 (\mathrm{syst.})$ ($68\%$ confidence interval) solar neutrinos out of 19904 total events. This corresponds to a $^{7}$Be neutrino interaction rate of 51.6$^{+13.9}_{-12.5}$ counts/(day$\cdot$ 100 ton), which is in agreement with the Standard Solar Model predictions and the previous spectroscopic results of Borexino. The no-neutrino hypothesis can be excluded with $>$5$\sigma$ confidence level. For the first time, we have demonstrated the possibility of utilizing the directional Cherenkov information for sub-MeV solar neutrinos, in a large-scale, high light yield liquid scintillator detector. This measurement provides an experimental proof of principle for future hybrid event reconstruction using both Cherenkov and scintillation signatures simultaneously., Comment: 6 pages, 4 figures, short letter of arXiv:2109.04770

The selection of low-radioactive construction materials is of the utmost importance for rare-event searches and thus critical to the XENONnT experiment. Results of an extensive radioassay program are reported, in which material samples have been screened with gamma-ray spectroscopy, mass spectrometry, and $^{222}$Rn emanation measurements. Furthermore, the cleanliness procedures applied to remove or mitigate surface contamination of detector materials are described. Screening results, used as inputs for a XENONnT Monte Carlo simulation, predict a reduction of materials background ($\sim$17%) with respect to its predecessor XENON1T. Through radon emanation measurements, the expected $^{222}$Rn activity concentration in XENONnT is determined to be 4.2$\,(^{+0.5}_{-0.7})\,\mu$Bq/kg, a factor three lower with respect to XENON1T. This radon concentration will be further suppressed by means of the novel radon distillation system.

The search for neutrino events in correlation with several of the most intense fast radio bursts (FRBs) has been performed using the Borexino data. We have searched for signals with visible energies above $250$~keV within a time window of $\pm$1000~s corresponding to the detection time of a particular FRB. We also applied an alternative approach based on searching for specific shapes of neutrino-electron scattering spectra in the full exposure spectrum of the Borexino detector. In particular, two incoming neutrino spectra were considered: the monoenergetic line and the spectrum expected from supernovae. The same spectra were considered for electron antineutrinos detected through the inverse beta-decay reaction. No statistically significant excess over the background was observed. As a result, the strongest upper limits on FRB-associated neutrino fluences of all flavors have been obtained in the $0.5 - 50$~MeV neutrino energy range., Comment: 14 pages, 10 figures

Roger Penrose proposed that a spatial quantum superposition collapses as a back-reaction from spacetime, which is curved in different ways by each branch of the superposition. In this sense, one speaks of gravity-related wave function collapse. He also provided a heuristic formula to compute the decay time of the superposition $\mathord{-}$ similar to that suggested earlier by Lajos Di\'osi, hence the name Di\'osi-Penrose model. The collapse depends on the effective size of the mass density of particles in the superposition, and is random: this randomness shows up as a diffusion of the particles' motion, resulting, if charged, in the emission of radiation. Here, we compute the radiation emission rate, which is faint but detectable. We then report the results of a dedicated experiment at the Gran Sasso underground laboratory to measure this radiation emission rate. Our result sets a lower bound on the effective size of the mass density of nuclei, which is about three orders of magnitude larger than previous bounds. This rules out the natural parameter-free version of the Di\'osi-Penrose model., Comment: 66 pages, 7 figures

Poly Ethylene Naphthalate (PEN) is an industrial polymer plastic which is investigated as a low background, transparent, scintillating and wavelength shifting structural material. PEN scintillates in the blue region and has excellent mechanical properties both at room and cryogenic temperatures. Thus, it is an ideal candidate for active structural components in experiments for the search of rare events like neutrinoless double-beta decay or dark matter recoils. Such optically active structures improve the identification and rejection efficiency of background events, like this improving the sensitivity of experiments. This paper reports on the production of radiopure and transparent PEN plates These structures can be used to mount germanium detectors operating in cryogenic liquids (LAr, LN). Thus, as first application PEN holders will be used to mount the Ge detectors in the LEGEND-200 experiment. The whole process from cleaning the raw material to testing the PEN active components under final operational conditions is reported.

The spectral shape of forbidden beta-decays is a crucial benchmark for nuclear physics calculations and has important implications also for astroparticle physics experiments. Among the interesting isotopes in this field, $^{115}$In is an excellent candidate, being a primordial nuclide featuring a good compromise among Q-value (497.954 keV) and half-life (4.41$\times$10$^{14}$ yr). In this paper, we propose to exploit a cryogenic calorimeter based on In$_2$O$_3$ crystal to perform a high-precision measurement of the $\beta$-decay energy spectrum, discussing also the results obtained within a preliminary test of this crystal and the next steps to improve the detector performance.

In the global landscape of neutrinoless double beta ($0\nu\beta\beta$) decay search, the use of semiconductor germanium detectors provides many advantages. The excellent energy resolution, the negligible intrinsic radioactive contamination, the possibility of enriching the crystals up to 88% in the $^{76}$Ge isotope as well as the high detection efficiency, are all key ingredients for highly sensitive $0\nu\beta\beta$ decay search. The MAJORANA and GERDA experiments successfully implemented the use of germanium (Ge) semiconductor detectors, reaching an energy resolution of $2.53 \pm 0.08$ keV at the Q$_{\beta\beta}$ and an unprecedented low background level of $5.2 \times 10^{-4}$ cts/(keV$\cdot$kg$\cdot$yr), respectively. In this paper, we will review the path of $0\nu\beta\beta$ decay search with Ge detectors from the original idea of E. Fiorini et al. in 1967, to the final recent results of the GERDA experiment setting a limit on the half-life of $^{76}$Ge $0\nu\beta\beta$ decay at $T_{1/2} > 1.8 \times 10^{26}$ yr (90\% C.L.). We will then present the LEGEND project designed to reach a sensitivity to the half-life up to $10^{28}$ yr and beyond, opening the way to the exploration of the normal ordering region., Comment: 28 pages, 15 figures

A search for alpha and double beta decays of ytterbium isotopes was performed with an ultra-low background high purity germanium detector at Gran Sasso Underground Laboratory (Italy). A 194.7 g Yb$_2$(C$_2$O$_4$)$_3$ powder sample was measured for 11.3~d with a total Yb exposure of 1.25 kg$\times$d. Half-life limits for $\alpha$-decay modes of $^{168}$Yb, $^{170}$Yb, $^{171}$Yb, $^{172}$Yb, $^{173}$Yb, $^{174}$Yb and $^{176}$Yb into the first excited states have been obtained between $6\times10^{14}$ yr and $2\times10^{16}$ yr. These are the first experimental constraints of these decay modes. Double electron capture of $^{168}$Yb and double beta decay of $^{176}$Yb into the first excited 2$^+$ and 0$^+$ states could be excluded with limits between $1\times10^{14}$ yr to $8\times10^{16}$ yr. This improves the experimental information on some of the decay modes compared to previous constraints.

Liquid scintillator detectors play a central role in the detection of neutrinos from various sources. In particular, it is the only technique used so far for the precision spectroscopy of sub-MeV solar neutrinos, as demonstrated by the Borexino experiment at the Gran Sasso National Laboratory in Italy. The benefit of a high light yield, and thus a low energy threshold and a good energy resolution, comes at the cost of the directional information featured by water Cherenkov detectors, measuring $^8$B solar neutrinos above a few MeV. In this paper we provide the first directionality measurement of sub-MeV solar neutrinos which exploits the correlation between the first few detected photons in each event and the known position of the Sun for each event. This is also the first signature of directionality in neutrinos elastically scattering off electrons in a liquid scintillator target. This measurement exploits the sub-dominant, fast Cherenkov light emission that precedes the dominant yet slower scintillation light signal. Through this measurement, we have also been able to extract the rate of $^{7}$Be solar neutrinos in Borexino. The demonstration of directional sensitivity in a traditional liquid scintillator target paves the way for the possible exploitation of the Cherenkov light signal in future kton-scale experiments using liquid scintillator targets. Directionality is important for background suppression as well as the disentanglement of signals from various sources., Comment: 19 pages, 15 Figures, revised version after comments from PRD Referees, shorter letter submitted with the title: "First Directional Measurement of sub-MeV Solar Neutrinos with Borexino"

We propose the construction of LEGEND-1000, the ton-scale Large Enriched Germanium Experiment for Neutrinoless $\beta \beta$ Decay. This international experiment is designed to answer one of the highest priority questions in fundamental physics. It consists of 1000 kg of Ge detectors enriched to more than 90% in the $^{76}$Ge isotope operated in a liquid argon active shield at a deep underground laboratory. By combining the lowest background levels with the best energy resolution in the field, LEGEND-1000 will perform a quasi-background-free search and can make an unambiguous discovery of neutrinoless double-beta decay with just a handful of counts at the decay $Q$ value. The experiment is designed to probe this decay with a 99.7%-CL discovery sensitivity in the $^{76}$Ge half-life of $1.3\times10^{28}$ years, corresponding to an effective Majorana mass upper limit in the range of 9-21 meV, to cover the inverted-ordering neutrino mass scale with 10 yr of live time.

Cosmogenic radio-nuclei are an important source of background for low-energy neutrino experiments. In Borexino, cosmogenic $^{11}$C decays outnumber solar $pep$ and CNO neutrino events by about ten to one. Highly efficient identification of this background is mandatory for these neutrino analyses. We present here the details of the most consolidated strategy, used throughout Borexino solar neutrino measurements. It hinges upon finding the space-time correlations between $^{11}$C decays, the preceding parent muons and the accompanying neutrons. This article describes the working principles and evaluates the performance of this Three-Fold Coincidence (TFC) technique in its two current implementations: a hard-cut and a likelihood-based approach. Both show stable performances throughout Borexino Phases II (2012-2016) and III (2016-2020) data sets, with a $^{11}$C tagging efficiency of $\sim$90 % and $\sim$63-66 % of the exposure surviving the tagging. We present also a novel technique that targets specifically $^{11}$C produced in high-multiplicity during major spallation events. Such $^{11}$C appear as a burst of events, whose space-time correlation can be exploited. Burst identification can be combined with the TFC to obtain about the same tagging efficiency of $\sim$90 % but with a higher fraction of the exposure surviving, in the range of $\sim$66-68 %., Comment: 21 pages, 14 figures (but 15 files, one figure being made of 2 images), 3 tables

Double-beta processes in $^{184}$Os and $^{192}$Os were searched for over 15851 h at the Gran Sasso National Laboratory (LNGS) of the I.N.F.N. by using a 118 g ultra-pure osmium sample installed on the endcap of a 112 cm$^3$ ultra-low-background broad-energy germanium detector. New limits on double-electron capture and electron capture with positron emission in $^{184}$Os were set at the level of $\lim T_{1/2} \sim 10^{16}-10^{17}$ yr. In particular the $2\nu$2K and $2\nu$KL decays of $^{184}$Os to the ground state of $^{184}$W are restricted as $T_{1/2}\geq3.0\times 10^{16}$ yr and $T_{1/2}\geq2.0\times 10^{16}$ yr, respectively. A lower limit on the half-life for the double-beta decay of $^{192}$Os to the first excited level of $^{192}$Pt was set as $\lim T_{1/2}=2.0\times 10^{20}$ yr at 90\% C.L., Comment: 22 pages, 9 figures, 2 tables

Borexino is a liquid scintillator detector located at the Laboratori Nazionale del Gran Sasso, Italy with the main goal to measure solar neutrinos. The experiment recently provided the first direct experimental evidence of CNO-cycle neutrinos in the Sun, rejecting the no-CNO signal hypothesis with a significance greater than 5$\sigma$ at 99\%C.L. The intrinsic $^{210}$Bi is an important background for this analysis due to its similar spectral shape to that of CNO neutrinos. $^{210}$Bi can be measured through its daughter $^{210}$Po which can be distinguished through an event-by-event basis via pulse shape discrimination. However, this required reducing the convective motions in the scintillator that brought additional $^{210}$Po from peripheral sources. This was made possible through the thermal insulation and stabilization campaign performed between 2015 and 2016. This article will explain the strategy and the different methods performed to extract the $^{210}$Bi upper limit in Phase-III (Jul 2016- Feb 2020) of the experiment through the analysis of $^{210}$Po in the cleanest region of the detector called the Low Polonium Field., Comment: Contribution to the 2021 Neutrinos session of the 55th Rencontres de Moriond

Neutrinos are elementary particles which are known since many years as fundamental messengers from the interior of the Sun. The Standard Solar Model, which gives a theoretical description of all nuclear processes which happen in our star, predicts that roughly 99% of the energy produced is coming from a series of processes known as the "pp chain". Such processes have been studied in detail over the last years by means of neutrinos, thanks also to the important measurements provided by the Borexino experiment. The remaining 1% is instead predicted to come from a separate loop-process, known as the "CNO cycle". This sub-dominant process is theoretically well understood, but has so far escaped any direct observation. Another fundamental aspect is that the CNO cycle is indeed the main nuclear engine in stars more massive than the Sun. In 2020, thanks to the unprecedented radio-purity and temperature control achieved by the Borexino detector over recent years, the first ever detection of neutrinos from the CNO cycle has been finally announced. The milestone result confirms the existence of this nuclear fusion process in our Universe. Here, the details of the detector stabilization and the analysis techniques adopted are reported., Comment: 7 pages, 3 figures. Contribution to the 2021 Neutrinos session of the 55th Rencontres de Moriond

Neutrinoless double-$\beta$ decay of $^{76}$Ge is searched for with germanium detectors where source and detector of the decay are identical. For the success of future experiments it is important to increase the mass of the detectors. We report here on the characterization and testing of five prototype detectors manufactured in inverted coaxial (IC) geometry from material enriched to 88% in $^{76}$Ge. IC detectors combine the large mass of the traditional semi-coaxial Ge detectors with the superior resolution and pulse shape discrimination power of point contact detectors which exhibited so far much lower mass. Their performance has been found to be satisfactory both when operated in vacuum cryostat and bare in liquid argon within the GERDA setup. The measured resolutions at the Q-value for double-$\beta$ decay of $^{76}$Ge (Q$_{\beta\beta}$ = 2039 keV) are about 2.1 keV full width at half maximum in vacuum cryostat. After 18 months of operation within the ultra-low background environment of the GERmanium Detector Array (GERDA) experiment and an accumulated exposure of 8.5 kg$\cdot$yr, the background index after analysis cuts is measured to be $4.9^{+7.3}_{-3.4}\times 10^{-4}$ counts /(keV$\cdot$kg$\cdot$yr) around Q$_{\beta\beta}$. This work confirms the feasibility of IC detectors for the next-generation experiment LEGEND., Comment: 13 pages, 12 figures, submitted to EPJC

The GERmanium Detector Array (GERDA) collaboration searched for neutrinoless double-$\beta$ decay in $^{76}$Ge with an array of about 40 high-purity isotopically-enriched germanium detectors. The experimental signature of the decay is a monoenergetic signal at Q$_{\beta\beta}$ = 2039.061(7)keV in the measured summed energy spectrum of the two emitted electrons. Both the energy reconstruction and resolution of the germanium detectors are crucial to separate a potential signal from various backgrounds, such as neutrino-accompanied double-$\beta$ decays allowed by the Standard Model. The energy resolution and stability were determined and monitored as a function of time using data from regular $^{228}$Th calibrations. In this work, we describe the calibration process and associated data analysis of the full GERDA dataset, tailored to preserve the excellent resolution of the individual germanium detectors when combining data over several years., Comment: 12 pages, 7 figures