Search

The deployment of molten salt reactors requires validation of the computational tools used to support the licensing process. The Molten Salt Reactor Experiment (MSRE), built and operated in the 196...

The impact of replacing Zircaloy with FeCrAl, a candidate enhanced accident-tolerant fuel cladding material, was evaluated for 10 × 10 boiling water reactor fuel bundles. Results from a series of full-core parametric studies estimated that replacing UO2/Zircaloy with UO2/FeCrAl would require an average enrichment increase of 0.6% 235U throughout the fuel lattice with the cladding and channel box thicknesses halved and fuel pellet diameter increased. Full-core results indicated that UO2/FeCrAl models with these geometric/enrichment specifications matched the base UO2/Zircaloy cycle length of 527 effective full power days. Optimization studies of the full-core design established loading and control blade patterns for both Zircaloy and FeCrAl models. A side study was conducted modeling a hybrid fuel bundle consisting of FeCrAl cladding and a SiC/Ni/Cr channel box. By halving the cladding thickness, the enrichment level required was less than that of the Zircaloy base case design after performing loading pattern optimization of the hybrid bundle core. Lastly, the thermomechanical performance of a Zircaloy-cladded fuel rod was compared to that of a FeCrAl system. Results from this analysis show that, if starting from the same fuel-cladding gap thickness, a FeCrAl-clad fuel rod operates with a greater average fuel centerline temperature, comparable axial elongation and radial displacement, and longer time to gap closure compared to a Zircaloy-clad fuel rod. This fuel performance analysis was primarily based on the commercial Kanthal APMT FeCrAl alloy but also used available data for the C35M FeCrAl alloy developed at Oak Ridge National Laboratory.

Critical experiments using an insertion zone with FLiBe salt performed at the LR-0 reactor at Research Centre Řež (RC Řež) have been compared to application models for solid-fueled, fluoride-salt-cooled high-temperature reactor (FHR) and liquid-fueled molten salt reactor (MSR) concepts using sensitivity and uncertainty (S/U) analysis techniques. These experiments support FHR and MSR advanced reactor concepts by informing on neutron spectral effects and nuclear data uncertainties related to fluoride salts. The FLiBe salt in the LR-0 experiments is from the Oak Ridge National Laboratory Molten Salt Reactor Experiment and is enriched to greater than 99.99% 7Li. This work is part of a broader collaboration between the United States and the Czech Republic on MSR and FHR technology. Results from the S/U analyses for FHR and MSR models indicated the most significant potential source of eigenvalue bias due to nuclear data within the FLiBe salt is radiative capture in 7Li. Other smaller but potentially significant contributions come from 19F, 6Li, and other 7Li reactions. Similarity comparisons of the RC Řež LR-0 experiments and FHR and MSR application models indicate that the LR-0 FLiBe experiments could be useful as candidate benchmarks for low-enriched uranium–fueled application models. However, sensitivity differences observed included both spectral effects, due to the LR-0 reactor being moderated by water instead of graphite and fluoride salt, and sensitivity magnitude effects driven by the amount of FLiBe inserted and its location. New experiments with refined designs to increase the volume and importance of salt in the system could provide improved data. Results also demonstrate that salt systems using thorium and/or 233U fuel will require additional experiments with relevant driver fuels. Increased contributions from the graphite moderator and 19F and covariance between reactions such as 233U fission and 233U radiative capture indicate higher uncertainty contributions from the salt and significant differences in contributions from the fuel species due to underlying uncertainties in their nuclear data.

Research on molten salt reactor (MSR) neutronics continues in Research Centre Rez (Czech Republic) with experimental work being conducted using fluoride salt that was originally used in the Molten Salt Reactor Experiment (MSRE). Previous results identified significant variations in the neutron spectrum measured in LiF-NaF salt. These variations could originate from the fluorine description in current nuclear data sets. Subsequent experiments were performed to try to confirm this phenomenon. Therefore, another fluorine-rich compound, Teflon, was used for testing. Critical experiments showed slight discrepancies in C/E-1 for both compounds, Teflon and FLIBE, and systematic overestimation of criticality was observed in calculations. Different nuclear data libraries were used for data set testing. For Teflon, the overestimation is higher when using JENDL-3.3, JENDL-4, and RUSFOND-2010 libraries, all three of which share the same inelastic-to-elastic scattering cross section ratio. Calculations using other libraries (ENDF/B-VII.1, ENDF/B-VII.0, JEFF-3.2, JEFF-3.1, and CENDL-3.1) tend to be closer to the experimental value. Neutron spectrum measurement in both substances revealed structure similar to that seen in previous measurements using LiF-NaF salt, which indicates that the neutron spectrum seems to be strongly shaped by fluorine. Discrepancies between experimental and calculational results seem to be larger in the neutron energy range of 100–1300 keV than in higher energies. In the case of neutron spectrum calculation, none of the tested libraries gives overall better results than the others.

The fuel cycle performance and core design of the Transatomic Power liquid-fueled molten salt reactor concept is analyzed. This advanced reactor concept uses configurable zirconium hydride moderator rod assemblies to shift the neutron spectrum in the core from intermediate at beginning of life to thermal at end of life. With a harder spectrum during the early years of reactor operation, this spectral shift design drives captures in fertile 238U. The converted fissile plutonium makes up over 50% of the fissile material in the fuel salt over the last half (∼15 years) of reactor operation. A softer spectrum late in reactor life helps drive the fuel to a burnup of 90 GWd/MTU. Continuously changing physics necessitates time-dependent analyses resolved over long timescales (i.e., months to years), as this concept does not meet an equilibrium condition. The spectral shift and molten salt reactor material feeds and removals enable this concept to perform better in fuel cycle metrics, increasing resource utilization by more than 50% compared with a typical light water reactor (i.e., from ∼0.6% to ∼1%). These metrics are compared to similar fuel cycles using alternate technologies. Additional core design and analysis challenges associated with the spectral shift and use of molten salt reactor technology are identified and discussed.

Fully ceramic microencapsulated (FCM) fuel is a proposed fuel type for improved accident performance in LWRs (Light Water Reactors) that involves TRISO (TRistructural-ISOtropic) particles embedded in a nano-powder sintered silicon carbide (SiC) matrix. The TRISO particles contain a spherical fuel kernel ranging from 500 to 800 µm in diameter. The kernel and buffer layer are then coated with three layers, each of which is 30–40 µm thick, composed of dense inner pyrolytic carbon (IPyC), chemically vapor deposited silicon carbide (SiC) layer, and an outer pyrolytic carbon (OPyC) layer. These TRISO particles are then embedded in a fully dense sintered SiC matrix with an expected particle packing fraction of about 35–40% by volume. As is the case for gas reactor applications, the release of radioactivity into the coolant is dependent on the integrity of the silicon carbide layer of the TRISO particles, in addition to the SiC matrix. In this work, we report on fuel performance modeling of TRISO-bearing FCM fuel using the BISON code to simulate the thermo-mechanical behavior of this fuel in a prototypic LWR environment. This paper considers the effects of embedding a TRISO particle in the SiC pellet matrix and includes a discussion of the irradiation-induced dimensional change in the pyrolytic carbon (PyC) layers of the TRISO particle. Additionally, methods were developed to simulate a FCM pellet containing a large number of discrete and independent particles. Future work will report on developing an interface debonding model, a fracture model, and a radionuclide transport model.

Interest in circulating fuel reactors (CFRs), particularly molten salt reactors (MSRs) of the fluid fuel type, has been growing in the last two decades. Starting with a resurgence of interest in Eu...

The Consortium for Advanced Simulation of Light Water Reactors (CASL) aims to provide high-fidelity multiphysics simulations of light water nuclear reactors. To accomplish this, CASL is developing the Virtual Environment for Reactor Applications (VERA), which is a suite of code packages for thermal hydraulics, neutron transport, fuel performance, and coolant chemistry. As VERA continues to grow and expand, there has been an increased focus on incorporating fuel performance analysis methods. One of the primary goals of CASL is to estimate local cladding failure probability through pellet-clad interaction, which consists of both pellet-clad mechanical interaction (PCMI) and stress corrosion cracking. Estimating clad failure is important to preventing release of fission products to the primary system and accurate estimates could prove useful in establishing less conservative power ramp rates or when considering load-follow operations. While this capability is being pursued through several different approaches, the procedure presented in this article focuses on running independent fuel performance calculations with BISON using a file-based one-way coupling based on multicycle output data from high fidelity, pin-resolved coupled neutron transport–thermal hydraulics simulations. This type of approach is consistent with traditional fuel performance analysis methods, which are typically separate from core simulation analyses. A more tightly coupled approach is currently being developed, which is the ultimate target application in CASL. Recent work simulating 12 cycles of Watts Bar Unit 1 with VERA core simulator are capitalized upon, and quarter-core BISON results for parameters of interest to PCMI (maximum centerline fuel temperature, maximum clad hoop stress, and minimum gap size) are presented for Cycles 1–3. Based on these results, this capability demonstrates its value and how it could be used as a screening tool for gathering insight into PCMI, singling out limiting rods for further, more detailed analysis.

Engineering demonstration reactors are nuclear reactors built to establish proof of concept for technology options that have never been built. Examples of engineering demonstration reactors include Peach Bottom 1 for high temperature gas-cooled reactors and the Experimental Breeder Reactor-II for sodium-cooled fast reactors. Engineering demonstrations have historically played a vital role in advancing the technology readiness level of reactor concepts. This paper details a preconceptual design for a fluoride salt-cooled engineering demonstration reactor. The fluoride salt-cooled high-temperature reactor (FHR) demonstration reactor (DR) is a concept for a salt-cooled reactor with 100 megawatts of thermal output. It would use tristructural-isotropic (TRISO) particle fuel in compacts within prismatic graphite blocks. FLiBe (2 7LiF-BeF2) is the reference primary coolant. The FHR DR is designed to be small, simple, and affordable. Development of the FHR DR is an intermediate step to enable near-term commercial FHRs. The design philosophy of the FHR DR was focused on safety, near-term deployment, and flexibility. Lower risk technologies are purposely included in the initial FHR DR design to ensure that the reactor can be built, licensed, and operated as an engineering demonstration with minimal risk and cost. These technologies include TRISO particle fuel, replaceable core structures, and consistent structural material selection for core structures and the primary and intermediate loops, and tube-and-shell primary-to-intermediate heat exchangers. Important capabilities to be demonstrated by building and operating the FHR DR include: • core design methodologies, • heat exchanger performance (including passive decay heat removal), • pump performance, • reactivity control, • salt chemistry control to maximize plant life, • salt procurement, handling, maintenance and ultimate disposal, and • tritium management. Non-nuclear separate and integral test efforts (e.g., heated salt loops or loops using simulant fluids) are necessary to develop the technologies that will be demonstrated in the FHR DR.

Current interest in advanced nuclear energy and molten salt reactor (MSR) concepts has enhanced interest in building the tools necessary to analyze these systems. A Python script known as ChemTriton has been developed to simulate equilibrium MSR fuel cycle performance by modeling the changing isotopic composition of an irradiated fuel salt using SCALE for neutron transport and depletion calculations. Improved capabilities in ChemTriton include a generic geometry capable of modeling multi-zone and multi-fluid systems, enhanced time-dependent feed and separations, and a critical concentration search. Although more generally applicable, the capabilities developed to date are illustrated in this paper in three applied problems: (1) simulating the startup of a thorium-based MSR fuel cycle (a likely scenario requires the first of these MSRs to be started without available 233U); (2) determining the effect of the removal of different fission products on MSR operations; and (3) obtaining the equilibrium concentration of a mixed-oxide light-water reactor fuel in a two-stage fuel cycle with a sodium fast reactor. The third problem is chosen to demonstrate versatility in an application to analyze the fuel cycle of a non-MSR system. In the first application, the initial fuel salt compositions fueled with different sources of fissile material are made feasible after (1) removing the associated nonfissile actinides after much of the initial fissile isotopes have burned and (2) optimizing the thorium concentration to maintain a critical configuration without significantly reducing breeding capability. In the second application, noble metal, volatile gas, and rare earth element fission products are shown to have a strong negative effect on criticality in a uranium-fueled thermal-spectrum MSR; their removal significantly increases core lifetime (by 30%) and fuel utilization. In the third application, the fuel of a mixed-oxide light-water reactor approaches an equilibrium composition after 20 depletion steps, demonstrating the potential for the longer time scales required to achieve equilibrium for solid-fueled systems over liquid fuel systems. This time to equilibrium can be reduced by starting with an initial fuel composition closer to that of the equilibrium fuel, reducing the need to handle time-dependent fuel compositions.

A nuclear fuel cycle systems modeling and code-to-code comparison effort was coordinated across multiple national laboratories to verify the tools needed to perform fuel cycle analyses of the transition from a once-through nuclear fuel cycle to a sustainable potential future fuel cycle. For this verification study, a simplified example transition scenario was developed to serve as a test case for the four systems codes involved (DYMOND, VISION, ORION, and MARKAL), each used by a different laboratory participant. In addition, all participants produced spreadsheet solutions for the test case to check all the mass flows and reactor/facility profiles on a year-by-year basis throughout the simulation period. The test case specifications describe a transition from the current US fleet of light water reactors to a future fleet of sodium-cooled fast reactors that continuously recycle transuranic elements as fuel. After several initial coordinated modeling and calculation attempts, it was revealed that most of the differences in code results were not due to different code algorithms or calculation approaches, but due to different interpretations of the input specifications among the analysts. Therefore, the specifications for the test case itself were iteratively updated to remove ambiguity and to help calibrate interpretations. In addition, a fewmore » corrections and modifications were made to the codes as well, which led to excellent agreement between all codes and spreadsheets for this test case. Although no fuel cycle transition analysis codes matched the spreadsheet results exactly, all remaining differences in the results were due to fundamental differences in code structure and/or were thoroughly explained. As a result, the specifications and example results are provided so that they can be used to verify additional codes in the future for such fuel cycle transition scenarios.« less

Molten salt reactors (MSRs) represent a class of reactors that use liquid salt, usually fluoride based or chloride based, as either a coolant with a solid fuel (such as fluoride salt–cooled high-te...

Thorium has great potential to stretch nuclear fuel reserves because of its natural abundance and because it is possible to breed the 232Th isotope into a fissile fuel (233U). Various scenarios exi...

As the core simulator capabilities in the Virtual Environment for Reactor Applications (VERA) have become more mature and stable, increased attention has been focused on coupling Bison to provide fuel performance simulations. This technique has been a very important driver for the pellet-clad interaction challenge problem being addressed by the Consortium for Advanced Simulation of Light Water Reactors (CASL). In this article, two coupling approaches are demonstrated on quarter core problems based on Watts Bar Nuclear Plant Unit 1, Cycle 1: (1) an inline approach in which a one-way coupling is used between neutronics/thermal hydraulics (through MPACT/CTF) and fuel performance (through Bison) but no fuel temperature information is passed back to MPACT/CTF, and (2) a two-way approach (coupled) in which the fuel temperature is passed from Bison to MPACT/CTF. In both approaches, power and temperature distributions from MPACT/CTF are used to inform the Bison simulations for each rod in the core. The demonstrations presented here are the first integrated fuel performance simulations in VERA, which opens many possibilities for future work, including applications to accident-tolerant fuel efforts and transient simulations, which are of critical importance to CASL. These demonstrations also highlight the potential to move away from the current Bison-informed fuel temperature lookup table approach, which is the default in MPACT/CTF simulations, if performance improvements are made in the near future.

This paper presents analyses of possible reactor representations of a nuclear fuel cycle with continuous recycling of thorium and produced uranium (mostly U-233) with thorium-only feed. The analysis was performed in the context of a U.S. Department of Energy effort to develop a compendium of informative nuclear fuel cycle performance data. The objective of this paper is to determine whether intermediate spectrum systems, having a majority of fission events occurring with incident neutron energies between 1 eV and 105 eV, perform as well as fast spectrum systems in this fuel cycle. The intermediate spectrum options analyzed include tight lattice heavy or light water-cooled reactors, continuously refueled molten salt reactors, and a sodium-cooled reactor with hydride fuel. All options were modeled in reactor physics codes to calculate their lattice physics, spectrum characteristics, and fuel compositions over time. Based on these results, detailed metrics were calculated to compare the fuel cycle performance. These metrics include waste management and resource utilization, and are binned to accommodate uncertainties. The performance of the intermediate systems for this self-sustaining thorium fuel cycle was similar to a representative fast spectrum system. However, the number of fission neutrons emitted per neutron absorbed limits performance in intermediate spectrum systems.

A study analyzed the neutronics of alternate cladding materials in a pressurized water reactor (PWR) environment. Austenitic type 310 (310SS) and 304 stainless steels, ferritic Fe-20Cr-5Al (FeCrAl) and APMT™ alloys, and silicon carbide (SiC)-based materials were considered and compared with Zircaloy-4. SCALE 6.1 was used to analyze the associated neutronics penalty/advantage, changes in reactivity coefficients, and spectral variations once a transition in the cladding was made. In the cases examined, materials containing higher absorbing isotopes invoked a reduction in reactivity due to an increase in neutron absorption in the cladding. Higher absorbing materials produced a harder neutron spectrum in the fuel pellet, leading to a slight increase in plutonium production. A parametric study determined the geometric conditions required to match cycle length requirements for each alternate cladding material in a PWR. A method for estimating the end of cycle reactivity was implemented to compare each model to that of standard Zircaloy-4 cladding. By using a thinner cladding of 350 μm and keeping a constant outer diameter, austenitic stainless steels require an increase of no more than 0.5 wt% enriched 235U to match fuel cycle requirements, while the required increase for FeCrAl was about 0.1%. When modeling SiC (with slightly lowermore » thermal absorption properties than that of Zircaloy), a standard cladding thickness could be implemented with marginally less enriched uranium (~0.1%). Moderator temperature and void coefficients were calculated throughout the depletion cycle. Nearly identical reactivity responses were found when coolant temperature and void properties were perturbed for each cladding material. By splitting the pellet into 10 equal areal sections, relative fission power as a function of radius was found to be similar for each cladding material. FeCrAl and 310SS cladding have a slightly higher fission power near the pellet’s periphery due to the harder neutron spectrum in the system, causing more 239Pu breeding. An economic assessment calculated the change in fuel pellet production costs for use of each cladding. Furthermore, implementing FeCrAl alloys would increase fuel pellet production costs about 15% because of increased 235U enrichment and the additional UO2 pellet volume enabled by using thinner cladding.« less

This study evaluated the neutronics and some of the fuel cycle characteristics of using uranium-based fully ceramic microencapsulated (FCM) fuel in a pressurized water reactor (PWR). Specific PWR l...

© 2016, American Nuclear Society. All rights reserved. Externally driven subcritical systems are closely associated with thorium, partially because thorium has no naturally occurring fissile isotopes. Both accelerator-driven systems (ADSs) and fusion-driven systems have been proposed. This paper highlights key literature related to the use of thorium in externally driven systems (EDSs) and builds upon this foundation to identify potential roles for EDSs in thorium fuel cycles. In fuel cycles with natural thorium feed and no enrichment, the potential roles are (1) a once-through breed-and-burn fuel cycle and (2) a fissile breeder (mainly233U) to support a fleet of critical reactors. If enriched uranium is used in the fuel cycle in addition to thorium, EDSs may be used to burn transuranic material. These fuel cycles were evaluated in the recently completed U.S. Department of Energy Evaluation and Screening of nuclear fuel cycle options relative to the current once-through commercial nuclear fuel cycle in the United States. The evaluation was performed with respect to nine specified high-level criteria, such as waste management and resource utilization. Each of these fuel cycles presents significant potential benefits per unit energy generation compared to the present once-through uranium fuel cycle. A parametric study indicates that fusion-fission-hybrid systems perform better than ADSs in some missions due to a higher neutron source relative to the energy required to produce it. However, both potential externally driven technology choices face significant development and deployment challenges. In addition, there are significant challenges associated with the use of thorium fuel and with the transition from a uranium-based fuel cycle to a thorium-based fuel cycle.

The fluoride salt-cooled high-temperature reactor (FHR) demonstration reactor (DR) is a concept for a salt-cooled reactor with 100 megawatts of thermal output (MWt). It would use tristructural-isotropic (TRISO) particle fuel within prismatic graphite blocks. FLiBe (2 LiF-BeF2) is the reference primary coolant. The FHR DR is designed to be small, simple, and affordable. Development of the FHR DR is a necessary intermediate step to enable near-term commercial FHRs. Lower risk technologies are purposely included in the initial FHR DR design to ensure that the reactor can be built, licensed, and operated within an acceptable budget and schedule. These technologies include TRISO particle fuel, replaceable core structural material, the use of that same material for the primary and intermediate loops, and tube-and-shell primary-to-intermediate heat exchangers. Several preconceptual and conceptual design efforts that have been conducted on FHR concepts bear a significant influence on the FHR DR design. Specific designs include the Oak Ridge National Laboratory (ORNL) advanced high-temperature reactor (AHTR) with 3400/1500 MWt/megawatts of electric output (MWe), as well as a 125 MWt small modular AHTR (SmAHTR) from ORNL. Other important examples are the Mk1 pebble bed FHR (PB-FHR) concept from the University of California, Berkeley (UCB), and an FHR testmore » reactor design developed at the Massachusetts Institute of Technology (MIT). The MIT FHR test reactor is based on a prismatic fuel platform and is directly relevant to the present FHR DR design effort. These FHR concepts are based on reasonable assumptions for credible commercial prototypes. The FHR DR concept also directly benefits from the operating experience of the Molten Salt Reactor Experiment (MSRE), as well as the detailed design efforts for a large molten salt reactor concept and its breeder variant, the Molten Salt Breeder Reactor. The FHR DR technology is most representative of the 3400 MWt AHTR concept, and it will demonstrate key operational features of that design. The FHR DR will be closely scaled to the SmAHTR concept in power and flows, so any technologies demonstrated will be directly applicable to a reactor concept of that size. The FHR DR is not a commercial prototype design, but rather a DR that serves a cost and risk mitigation function for a later commercial prototype. It is expected to have a limited operational lifetime compared to a commercial plant. It is designed to be a low-cost reactor compared to more mature advanced prototype DRs. A primary reason to build the FHR DR is to learn about salt reactor technologies and demonstrate solutions to remaining technical gaps.« less

Lawrence Livermore National Laboratory is currently developing a hybrid fusion-fission nuclear energy system, called LIFE, to generate power and burn nuclear waste. We utilize inertial confinement ...

Molten salt with dissolved uranium is being considered for the Laser Inertial Confinement Fusion Fission Energy (LIFE) fission blanket as a backup in case a solid-fuel version cannot meet the performance objectives, for example because of radiation damage of the solid materials. Molten salt is not damaged by radiation and therefore could likely achieve the desired high burnup (>99%) of heavy atoms of 238 U. A perceived disadvantage is the possibility that the circulating molten salt could lend itself to misuse (proliferation) by making separation of fissile material easier than for the solid-fuel case. The molten salt composition being considered is the eutectic mixture of 73 mol% LiF and 27 mol% UF4, whose melting point is 490°C. The use of 232 Th as a fuel is also being studied. ( 232 Th does not produce Pu under neutron irradiation.) The temperature of the molten salt would be ~550°C at the inlet (60°C above the solidus temperature) and ~650°C at the outlet. Mixtures of U and Th are being considered. To minimize corrosion of structural materials, the molten salt would also contain a small amount (~1 mol%) of UF3. The same beryllium neutron multiplier could be used as in the solid fuel case; alternatively, a liquid lithium or liquid lead multiplier could be used. Insuring that the solubility of Pu 3+ in the melt is not exceeded is a design criterion. To mitigate corrosion of the steel, a refractory coating such as tungsten similar to the first wall facing the fusion source is suggested in the highneutron-flux regions; and in low-neutron-flux regions, including the piping and heat exchangers, a nickel alloy, Hastelloy, would be used. These material choices parallel those made for the Molten Salt Reactor Experiment (MSRE) at ORNL. The nuclear performance is better than the solid fuel case. At the beginning of life, the tritium breeding ratio is unity and the plutonium plus 233 U

This work focuses on ATF concepts being researched at Oak Ridge National Laboratory (ORNL), expanding on previous studies of using alternate cladding materials in pressurized water reactors (PWRs). The neutronic performance of two leading alternate cladding materials were assessed in boiling water reactors (BWRs): iron-chromium-aluminum (FeCrAl) cladding, and silicon carbide (SiC)-based composite cladding. This report fulfills ORNL Milestone M3FT-15OR0202332 within the fiscal year 2015 (FY15)

Technology implimentation plan for FeCrAl development under the FCRD Advanced Fuel program. The document describes the activities required to get FeCrAl clad ready for LTR testing

Two scenarios are typically envisioned for thorium fuel cycles: 'open' cycles based on irradiation of {sup 232}Th and fission of {sup 233}U in situ without reprocessing or 'closed' cycles based on irradiation of {sup 232}Th followed by reprocessing, and recycling of {sup 233}U either in situ or in critical fission reactors. This study evaluates a third option based on the possibility of breeding fissile material in a fusion-fission hybrid reactor and burning the same fuel in a critical reactor without any reprocessing or reconditioning. This fuel cycle requires the hybrid and the critical reactor to use the same fuel form. TRISO particles embedded in carbon pebbles were selected as the preferred form of fuel and an inertial laser fusion system featuring a subcritical blanket was combined with critical pebble bed reactors, either gas-cooled or liquid-salt-cooled. The hybrid reactor was modeled based on the earlier, hybrid version of the LLNL Laser Inertial Fusion Energy (LIFE1) system, whereas the critical reactors were modeled according to the Pebble Bed Modular Reactor (PBMR) and the Pebble Bed Advanced High Temperature Reactor (PB-AHTR) design. An extensive neutronic analysis was carried out for both the hybrid and the fission reactors in order to track the fuelmore » composition at each stage of the fuel cycle and ultimately determine the plant support ratio, which has been defined as the ratio between the thermal power generated in fission reactors and the fusion power required to breed the fissile fuel burnt in these fission reactors. It was found that the maximum attainable plant support ratio for a thorium fuel cycle that employs neither enrichment nor reprocessing is about 2. This requires tuning the neutron energy towards high energy for breeding and towards thermal energy for burning. A high fuel loading in the pebbles allows a faster spectrum in the hybrid blanket; mixing dummy carbon pebbles with fuel pebbles enables a softer spectrum in the critical reactors. This combination consumes about 20% of the thorium initially loaded in the hybrid reactor ({approx}200 GWd/tHM), partially during hybrid operation, but mostly during operation in the critical reactor. The plant support ratio is low compared to the one attainable using continuous fuel chemical reprocessing, which can yield a plant support ratio of about 20, but the resulting fuel cycle offers better proliferation resistance as fissile material is never separated from the other fuel components.« less

This study focused on creating a new tristructural isotropic (TRISO) coated particle fuel performance model and demonstrating the integration of this model into an existing system of neutronics and heat transfer codes, creating a user-friendly option for including fuel performance analysis within system design optimization and system-level trade-off studies. The end product enables both a deeper understanding and better overall system performance of nuclear energy systems limited or greatly impacted by TRISO fuel performance. A thorium-fueled hybrid fusion-fission Laser Inertial Fusion Energy (LIFE) blanket design was used for illustrating the application of this new capability and demonstrated both the importance of integrating fuel performance calculations into mainstream design studies and the impact that this new integrated analysis had on system-level design decisions.A new TRISO fuel performance model named TRIUNE was developed and verified and validated during this work with a novel methodology established for simulating the actual lifetime of a TRISO particle during repeated passes through a pebble bed. In addition, integrated self-consistent calculations were performed for neutronics depletion analysis, heat transfer calculations, and then fuel performance modeling for a full parametric study that encompassed over 80 different design options that went through all three phases of analysis. Lastly, side studies were performed that included a comparison of thorium and depleted uranium (DU) LIFE blankets as well as some uncertainty quantification work to help guide future experimental work by assessing what material properties in TRISO fuel performance modeling are most in need of improvement.A recommended thorium-fueled hybrid LIFE engine design was identified with an initial fuel load of 20MT of thorium, 15% TRISO packing within the graphite fuel pebbles, and a 20cm neutron multiplier layer with beryllium pebbles in flibe molten salt coolant. It operated at a system power level of 2000 MWth, took about 3.5 years to reach full plateau power, and was capable of an End of Plateau burnup of 38.7 %FIMA if considering just the neutronic constraints in the system design; however, fuel performance constraints led to a maximum credible burnup of 12.1 %FIMA due to a combination of internal gas pressure and irradiation effects on the TRISO materials (especially PyC) leading to SiC pressure vessel failures. The optimal neutron spectrum for the thorium-fueled blanket options evaluated seemed to favor a hard spectrum (low but non-zero neutron multiplier thicknesses and high TRISO packing fractions) in terms of neutronic performance but the fuel performance constraints demonstrated that a significantly softer spectrum would be needed to decrease the rate of accumulation of fast neutron fluence in order to improve the maximum credible burnup the system could achieve.

The Laser Inertial Fusion Energy (LIFE) concept is being developed to operate as either a pure fusion or hybrid fusion-fission system. The hybrid version is designed to generate power and burn both...

The goals of the Laser Inertial Fusion Fission Energy (LIFE) is to use fusion neutrons to fission materials with no enrichment and minimum processing and have greatly reduced wastes that are not of interest to making weapons. Fusion yields expected to be achieved in NIF a few times per day are called for with a high reliable shot rate of about 15 per second. We have found that the version of LIFE using TRISO fuel discussed in other volumes of this series can be modified by replacing the molten-flibe-cooled TRISO fuel zone with a molten salt in which the same actinides present in the TRISO particles are dissolved in the molten salt. Molten salts have the advantage that they are not subject to radiation damage, and hence overcome the radiation damage effects that may limit the lifetime of solid fuels such as TRISO-containing pebbles. This molten salt is pumped through the LIFE blanket, out to a heat exchanger and back into the blanket. To mitigate corrosion, steel structures in contact with the molten salt would be plated with tungsten or nickel. The salt will be processed during operation to remove certain fission products (volatile and noble and semi-noble fission products),more » impurities and corrosion products. In this way neutron absorbers (fission products) are removed and neutronics performance of the molten salt is somewhat better than that of the TRISO fuel case owing to the reduced parasitic absorption. In addition, the production of Pu and rare-earth elements (REE) causes these elements to build up in the salt, and leads to a requirement for a process to remove the REE during operation to insure that the solubility of a mixed (Pu,REE)F3 solid solution is not exceeded anywhere in the molten salt system. Removal of the REE will further enhance the neutronics performance. With molten salt fuels, the plant would need to be safeguarded because materials of interest for weapons are produced and could potentially be removed.« less

The Laser Inertial Confinement Fusion Fission Energy (LIFE) Program being developed at Lawrence Livermore National Laboratory (LLNL) aims to design a hybrid fission-fusion subcritical nuclear engine that uses a laser-driven Inertial Confinement Fusion (ICF) system to drive a subcritical fission blanket. This combined fusion-fission hybrid system could be used for generating electricity, material transmutation or incineration, or other applications. LIFE does not require enriched fuel since it is a sub-critical system and LIFE can sustain power operation beyond the burnup levels at which typical fission reactors need to be refueled. In light of these factors, numerous options have been suggested and are being investigated. Options being investigated include fueling LIFE engines with spent nuclear fuel to aid in disposal/incineration of commercial spent nuclear fuel or using depleted uranium or thorium fueled options to enhance proliferation resistance and utilize non-fissile materials [1]. LIFE engine blanket designs using a molten salt fuel system represent one area of investigation. Possible applications of a LIFE engine with a molten salt blanket include uses as a spent nuclear fuel burner, fissile fuel breeding platform, and providing a backup alternative to other LIFE engine blanket designs using TRISO fuel particles in case the TRISO particles aremore » found to be unable to withstand the irradiation they will be subjected to. These molten salts consist of a mixture of LiF with UF{sub 4} or ThF{sub 4} or some combination thereof. Future systems could look at using PuF{sub 3} or PuF{sub 4} as well, though no work on such system with initial plutonium loadings has been performed for studies documented in this report. The purpose of this report is to document preliminary neutronics design studies performed to support the development of a molten salt blanket LIFE engine option, as part of the LIFE Program being performed at Lawrence Livermore National laboratory. Preliminary design studies looking at fast ignition and hot spot ignition fusion options are documented, along with limited scoping studies performed to investigate other options of interest that surfaced during the main design effort. Lastly, side studies that were not part of the main design effort but may alter future work performed on LIFE engine designs are shown. The majority of all work reported in this document was performed during the Molten Salt Fast Ignition Moderator Study (MSFIMS) which sought to optimize the amount of moderator mixed into the molten salt region in order to produce the most compelling design. The studies in this report are of a limited scope and are intended to provide a preliminary neutronics analysis of the design concepts described herein to help guide decision processes and explore various options that a LIFE engine with a molten salt blanket might enable. None of the designs shown in this report, even reference cases selected for detailed description and analysis, have been fully optimized. The analyses were performed primarily as a neutronics study, though some consultation was made regarding thermal-hydraulic and structural concerns during both scoping out an initial model and subsequent to identifying a neutronics-based reference case to ensure that the design work contained no glaring mechanical or thermal issues that would preclude its feasibility. Any analyses and recommendations made in this report are either primarily or solely from the point of view of LIFE neutronics and ignore other fundamental issues related to molten salt fuel blankets such as chemical processing feasibility and political feasibility of a molten salt system.« less

This study establishes a procedure for constructing explicit and adjoint-based implicit sensitivities with MCNP5. Using these methods, an instantaneous sensitivity-based uncertainty analysis is performed on the depleted uranium hybrid LIFE (Laser Inertial Fusion Energy) blanket. Explicit sensitivities and uncertainties are calculated for (n, 2n), tritium production, fission, and radiative capture reaction rates during the fuel lifecycle. Nuclear data uncertainties and Monte Carlo counting precision are compared in a convergence study and the compounding of the two is quantified to gauge the validity of the analysis. A multi-group cross-section library is generated for adjoint calculations and selected adjoint distributions are shown and discussed.