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Under future net zero emission policies, reductions in emissions of ozone (O3) precursors are expected to alter the temporal and spatial distribution of tropospheric O3. In this study, we quantify changes in the tropospheric O3 budget, spatiotemporal distribution of surface O3 in East Asia and the contributions from regional emissions, intercontinental transport and climate change between the present day and 2060 under a net zero scenario, using the NCAR Community Earth System Model (CESM) with online tagging of O3 and its precursors. The results reveal that the global tropospheric O3 burden is likely to decrease by more than 20 %, from 316 Tg in present day to 247 Tg in 2060, under a net zero scenario. The burden of stratospheric O3 in the troposphere is expected to increase from 69 to 77 Tg. The mean lifetime of tropospheric O3 increases by 2 days, ~10 %. Changes in climate under a net zero pathway are relatively small, and only lead to small increases in tropospheric O3. Over East China, surface O3 increases in winter, due to the weakened titration of O3 by NO associated with reduced anthropogenic NO emissions, and to enhanced stratospheric input. In summer, surface O3 decreases by more than 30 ppbv, and peak concentrations shift from July to May. Local contributions from anthropogenic emissions to surface O3 over East Asia are highest in summer, but drop substantially, from 30 % to 14 %, under a net zero scenario. The contribution of biogenic sources is enhanced, and forms the dominant contributor to future surface O3, especially in summer, ~40 %. This enhanced contribution is mainly due to the increased O3 production efficiency under lower anthropogenic precursor emissions. Over Eastern China, local anthropogenic contributions decrease from 50 % to 30 %. The decreases in surface O3 are strongly beneficial, and are more than sufficient to counteract the increases in surface O3 observed in China over recent years. This study thus highlights the important co-benefits of net zero policies that target climate change in addressing surface O3 pollution over East Asia.

The strong economic growth in China in recent decades, together with meteorological factors, has resulted in serious air pollution problems, in particular over large industrialized areas with high population density. To reduce the concentrations of pollutants, air pollution control policies have been successfully implemented, resulting in the gradual decrease of air pollution in China during the last decade, as evidenced from both satellite and ground-based measurements. The aims of the Dragon 4 project “Air quality over China” were the determination of trends in the concentrations of aerosols and trace gases, quantification of emissions using a top-down approach and gain a better understanding of the sources, transport and underlying processes contributing to air pollution. This was achieved through (a) satellite observations of trace gases and aerosols to study the temporal and spatial variability of air pollutants; (b) derivation of trace gas emissions from satellite observations to study sources of air pollution and improve air quality modeling; and (c) study effects of haze on air quality. In these studies, the satellite observations are complemented with ground-based observations and modeling.