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Generation and preservation of quantum entanglement are among the primary tasks in quantum information processing. State stabilization via quantum bath engineering offers a resource-efficient approach to achieve this objective. However, current methods for engineering dissipative channels to stabilize target entangled states often require specialized hardware designs, complicating experimental realization and hindering their compatibility with scalable quantum computation architectures. In this work, we propose and experimentally demonstrate a stabilization protocol readily implementable in the mainstream integrated superconducting quantum circuits. The approach utilizes a Raman process involving a resonant (or nearly resonant) superconducting qubit array and their dedicated readout resonators to effectively emerge nonlocal dissipative channels. Leveraging individual controllability of the qubits and resonators, the protocol stabilizes two-qubit Bell states with a fidelity of $90.7\%$, marking the highest reported value in solid-state platforms to date. Furthermore, by extending this strategy to include three qubits, an entangled $W$ state is achieved with a fidelity of $86.2\%$, which has not been experimentally investigated before. Notably, the protocol is of practical interest since it only utilizes existing hardware common to standard operations in the underlying superconducting circuits, thereby facilitating the exploration of many-body quantum entanglement with dissipative resources.

Superconducting qubits are a promising platform for building fault-tolerant quantum computers, with recent achievement showing the suppression of logical error with increasing code size. However, leakage into non-computational states, a common issue in practical quantum systems including superconducting circuits, introduces correlated errors that undermine QEC scalability. Here, we propose and demonstrate a leakage reduction scheme utilizing tunable couplers, a widely adopted ingredient in large-scale superconducting quantum processors. Leveraging the strong frequency tunability of the couplers and stray interaction between the couplers and readout resonators, we eliminate state leakage on the couplers, thus suppressing space-correlated errors caused by population propagation among the couplers. Assisted by the couplers, we further reduce leakage to higher qubit levels with high efficiency (98.1%) and low error rate on the computational subspace (0.58%), suppressing time-correlated errors during QEC cycles. The performance of our scheme demonstrates its potential as an indispensable building block for scalable QEC with superconducting qubits., Comment: 25 pages, 15 figures

As quantum circuits become more integrated and complex, additional error sources that were previously insignificant start to emerge. Consequently, the fidelity of quantum gates benchmarked under pristine conditions falls short of predicting their performance in realistic circuits. To overcome this problem, we must improve their robustness against pertinent error models besides isolated fidelity. Here we report the experimental realization of robust quantum gates in superconducting quantum circuits based on a geometric framework for diagnosing and correcting various gate errors. Using quantum process tomography and randomized benchmarking, we demonstrate robust single-qubit gates against quasi-static noise and spatially-correlated noise in a broad range of strengths, which are common sources of coherent errors in large-scale quantum circuit. We also apply our method to non-static noises and to realize robust two-qubit gates. Our work provides a versatile toolbox for achieving noise-resilient complex quantum circuits., Comment: 6 pages, 4 figures plus Supplementary Information

As the basis for generating multi-particle quantum correlations, inter-particle interaction plays a crucial role in collective quantum phenomena, quantum phase transitions, and quantum information processing. It can profoundly alter the band structure of quantum many-body systems and give rise to exotic topological phenomena. Conventional topological pumping, which has been well demonstrated in driven linear or noninteracting systems, may break down in the presence of strong interaction. However, the interplay between band topology and interaction could also induce emergent topological pumping of interacting particles, but its experimental realization has proven challenging. Here we demonstrate interaction-induced topological pumping in a solid-state quantum system comprising an array of 36 superconducting qubits. With strong interaction inherent in the qubits and site-resolved controllability of the lattice potential and hopping strength, we realize the topological Thouless pumping of single and two bounded particles. Beyond these topological phenomena with linear or noninteracting counterparts, we also observe topologically resonant tunneling and asymmetric edge-state transport of interacting particles. Our work creates a paradigm for multi-particle topological effects, and provides a new pathway to the study of exotic topological phenomena, many-body quantum transport, and quantum information transfer., Comment: 8+29 pages, 4+24 figures

Quantum teleportation~\cite{Bennett1993} is of both fundamental interest and great practical importance in quantum information science. To date, quantum teleportation has been implemented in various physical systems~\cite{Pirandola2015}, among which superconducting qubits are of particular practical significance as they emerge as a leading system to realize large-scale quantum computation~\cite{Arute2019,Wu2021}. Nevertheless, the number of superconducting qubits on the same chip is severely limited by the available chip size, the cooling power, and the wiring complexity. Realization of quantum teleportation and remote computation over qubits on distant superconducting chips is a key quantum communication technology to scaling up the system through a distributed quantum computational network~\cite{Gottesman1999,Eisert2000,Jiang2007,Kimble2008,Monroe2014}. However, this goal has not been realized yet in experiments due to the technical challenge of making a quantum interconnect between distant superconducting chips and the inefficient transfer of flying microwave photons over the lossy interconnects~\cite{Kurpiers2018,Axline2018,Campagne2018,Magnard2020}. Here we demonstrate deterministic teleportation of quantum states and entangling gates between distant superconducting chips connected by a 64-meter-long cable bus featuring an ultralow loss of 0.32~dB/km at cryogenic temperatures, where high fidelity remote entanglement is generated via flying microwave photons utilizing time-reversal-symmetry~\cite{Cirac1997,Korotkov2011}. Apart from the fundamental interest of teleporting macroscopic superconducting qubits over a long distance, our work lays a foundation to realization of large-scale superconducting quantum computation through a distributed computational network~\cite{Gottesman1999,Eisert2000,Jiang2007,Kimble2008,Monroe2014}.

Scaling is now a key challenge in superconducting quantum computing. One solution is to build modular systems in which smaller-scale quantum modules are individually constructed and calibrated, and then assembled into a larger architecture. This, however, requires the development of suitable interconnects. Here, we report low-loss interconnects based on pure aluminium coaxial cables and on-chip impedance transformers featuring quality factors up to $8.1 \times 10^5$, which is comparable to the performance of our transmon qubits fabricated on single-crystal sapphire substrate. We use these interconnects to link five quantum modules with inter-module quantum state transfer and Bell state fidelities up to 99\%. To benchmark the overall performance of the processor, we create maximally-entangled, multi-qubit Greenberger-Horne-Zeilinger (GHZ) states. The generated inter-module four-qubit GHZ state exhibits 92.0\% fidelity. We also entangle up to 12 qubits in a GHZ state with $55.8 \pm 1.8\%$ fidelity, which is above the genuine multipartite entanglement threshold of 1/2. These results represent a viable modular approach for large-scale superconducting quantum processors.

Gate-based quantum computation has been extensively investigated using quantum circuits based on qubits. In many cases, such qubits are actually made out of multilevel systems but with only two states being used for computational purpose. While such a strategy has the advantage of being in line with the common binary logic, it in some sense wastes the ready-for-use resources in the large Hilbert space of these intrinsic multi-dimensional systems. Quantum computation beyond qubits (e.g., using qutrits or qudits) has thus been discussed and argued to be more efficient than its qubit counterpart in certain scenarios. However, one of the essential elements for qutrit-based quantum computation, two-qutrit quantum gate, remains a major challenge. In this work, we propose and demonstrate a highly efficient and scalable two-qutrit quantum gate in superconducting quantum circuits. Using a tunable coupler to control the cross-Kerr coupling between two qutrits, our scheme realizes a two-qutrit conditional phase gate with fidelity 89.3% by combining simple pulses applied to the coupler with single-qutrit operations. We further use such a two-qutrit gate to prepare an EPR state of two qutrits with a fidelity of 95.5%. Our scheme takes advantage of a tunable qutrit-qutrit coupling with a large on:off ratio. It therefore offers both high efficiency and low cross talk between qutrits, thus being friendly for scaling up. Our work constitutes an important step towards scalable qutrit-based quantum computation., Comment: 15 pages, 12 figures

Implementing quantum algorithms on realistic hardware requires translating high-level global operations into sequences of native elementary gates, a process known as quantum compiling. Physical limitations, such as constraints in connectivity and gate alphabets, often result in unacceptable implementation costs. To enable successful near-term applications, it is crucial to optimize compilation by exploiting the potential capabilities of existing hardware. Here, we implement a resource-efficient construction for a quantum version of AND logic that can reduce the cost, enabling the execution of key quantum circuits. On a high-scalability superconducting quantum processor, we demonstrate low-depth synthesis of high-fidelity generalized Toffoli gates with up to 8 qubits and Grover's search algorithm in a search space of up to 64 entries; both are the largest such implementations in scale to date. Our experimental demonstration illustrates a scalable implementation of simplifying quantum algorithms, paving the way for larger, more meaningful quantum applications on noisy devices.

Geometric phases accompanying adiabatic quantum evolutions can be used to construct robust quantum control for quantum information processing due to their noise-resilient feature. A significant development along this line is to construct geometric gates using nonadiabatic quantum evolutions to reduce errors due to decoherence. However, it has been shown that nonadiabatic geometric gates are not necessarily more robust than dynamical ones, in contrast to an intuitive expectation. Here we experimentally investigate this issue for the case of nonadiabatic holonomic quantum computation~(NHQC) and show that conventional NHQC schemes cannot guarantee the expected robustness due to a cross coupling to the states outside the computational space. We implement a different set of constraints for gate construction in order to suppress such cross coupling to achieve an enhanced robustness. Using a superconducting quantum circuit, we demonstrate high-fidelity holonomic gates whose infidelity against quasi-static transverse errors can be suppressed up to the fourth order, instead of the second order in conventional NHQC and dynamical gates. In addition, we explicitly measure the accumulated dynamical phase due to the above mentioned cross coupling and verify that it is indeed much reduced in our NHQC scheme. We further demonstrate a protocol for constructing two-qubit NHQC gates also with an enhanced robustness., Comment: 14 pages, 14 figures

Scalable quantum information processing requires the ability to tune multi-qubit interactions. This makes the precise manipulation of quantum states particularly difficult for multi-qubit interactions because tunability unavoidably introduces sensitivity to fluctuations in the tuned parameters, leading to erroneous multi-qubit gate operations. The performance of quantum algorithms may be severely compromised by coherent multi-qubit errors. It is therefore imperative to understand how these fluctuations affect multi-qubit interactions and, more importantly, to mitigate their influence. In this study, we demonstrate how to implement dynamical-decoupling techniques to suppress the two-qubit analogue of the dephasing on a superconducting quantum device featuring a compact tunable coupler, a trending technology that enables the fast manipulation of qubit--qubit interactions. The pure-dephasing time shows an up to ~14 times enhancement on average when using robust sequences. The results are in good agreement with the noise generated from room-temperature circuits. Our study further reveals the decohering processes associated with tunable couplers and establishes a framework to develop gates and sequences robust against two-qubit errors., Comment: 19 pages, 14 figures

Graphene is an attractive material for broadband photodetection but suffers from weak light absorption. Coating graphene with quantum dots can significantly enhance light absorption and create extraordinarily high photo gain. This high gain is often explained by the classical gain theory which is unfortunately an implicit function and may even be questionable. In this work, we managed to derive explicit gain equations for hybrid graphene-quantum-dot photodetectors. Due to the work function mismatch, lead sulfide (PbS) quantum dots coated on graphene will form a surface depletion region near the interface of quantum dots and graphene. Light illumination narrows down the surface depletion region, creating a photovoltage that gates the graphene. As a result, high photo gain in graphene is observed. The explicit gain equations are derived from the theoretical gate transfer characteristics of graphene and the correlation of the photovoltage with the light illumination intensity. The derived explicit gain equations fit well with the experimental data, from which physical parameters are extracted., Comment: 14 pages, 6 figures

Quantum simulation can be implemented in pure digital or analog ways, each with their pros and cons. By taking advantage of the universality of a digital route and the efficiency of analog simulation, hybrid digital-analog approaches can enrich the possibilities for quantum simulation. We use a unique hybrid approach to experimentally perform a quantum simulation of phase-controlled dynamics resulting from a closed-contour interaction (CCI) within certain multi-level systems in superconducting quantum circuits. Due to symmetry constraints, such systems cannot host an inherent CCI. Nevertheless, by assembling analog modules corresponding to their natural evolutions and specially designed digital modules constructed from standard quantum logic gates, we can bypass such constraints and realize an effective CCI in these systems. Based on this realization, we demonstrate a variety of related and interesting phenomena, including phase-controlled chiral dynamics, separation of chiral enantiomers, and a new mechanism to generate entangled states based on CCI., Comment: 13 pages, 11 figures

Higher-order topological phases give rise to new bulk and boundary physics, as well as new classes of topological phase transitions. While the realization of higher-order topological phases has been confirmed in many platforms by detecting the existence of gapless boundary modes, a direct determination of the higher-order topology and related topological phase transitions through the bulk in experiments has still been lacking. To bridge the gap, in this work we carry out the simulation of a two-dimensional second-order topological phase in a superconducting qubit. Owing to the great flexibility and controllability of the quantum simulator, we observe the realization of higher-order topology directly through the measurement of the pseudo-spin texture in momentum space of the bulk for the first time, in sharp contrast to previous experiments based on the detection of gapless boundary modes in real space. Also through the measurement of the evolution of pseudo-spin texture with parameters, we further observe novel topological phase transitions from the second-order topological phase to the trivial phase, as well as to the first-order topological phase with nonzero Chern number. Our work sheds new light on the study of higher-order topological phases and topological phase transitions., Comment: 8+8 pages; 4+7 figures

Stimulated Raman adiabatic passage (STIRAP) is a widely-used technique of coherent state-to-state manipulation for many applications in physics, chemistry, and beyond. The adiabatic evolution of the state involved in STIRAP, called adiabatic passage, guarantees its robustness against control errors, but also leads to problems of low efficiency and decoherence. Here we propose and experimentally demonstrate an alternative approach, termed stimulated Raman "user-defined" passage (STIRUP), where a parameterized state is employed for constructing desired evolutions to replace the adiabatic passage in STIRAP. The user-defined passages can be flexibly designed for optimizing different objectives for different tasks, e.g. minimizing leakage error. To experimentally benchmark its performance, we apply STIRUP to the task of coherent state transfer in a superconducting Xmon qutrit. We found that STIRUP completed the transfer more then four times faster than STIRAP with enhanced robustness, and achieved a fidelity of 99.5%, which is the highest among all recent experiments based on STIRAP and its variants. In practice, STIRUP differs from STIRAP only in the design of driving pulses; therefore, most existing applications of STIRAP can be readily implemented with STIRUP., Comment: 5 pages, 4 figures

The recent discovery of 2D magnets has revealed various intriguing phenomena due to the coupling between spin and other degree of freedoms (such as helical photoluminescence, nonreciprocal SHG). Previous research on the spin-phonon coupling effect mainly focuses on the renormalization of phonon frequency. Here we demonstrate that the Raman polarization selection rules of optical phonons can be greatly modified by the magnetic ordering in 2D magnet CrI$_3$. For monolayer samples, the dominant A$\rm_{1g}$ peak shows abnormally high intensity in the cross polarization channel at low temperature, which is forbidden by the selection rule based on the lattice symmetry. While for bilayer, this peak is absent in the cross polarization channel for the layered antiferromagnetic (AFM) state and reappears when it is tuned to the ferromagnetic (FM) state by an external magnetic field. Our findings shed light on exploring the emergent magneto-optical effects in 2D magnets., Comment: 15 pages, 4 figures

The recent discovery of the interfacial superconductivity (SC) of the Bi2Te3/Fe1+yTe heterostructure has attracted extensive studies due to its potential as a novel platform for trapping and controlling Majorana fermions. Here we present studies of another topological insulator (TI)/Fe1+yTe heterostructure, Sb2Te3/Fe1+yTe, which also enjoys an interfacial two-dimensional SC. The results of transport measurements support that the reduction of excess Fe concentration of the Fe1+yTe layer not only increases the fluctuation of its antiferromagnetic (AFM) order but also enhances the quality of the SC of this heterostructure system. On the other hand, the interfacial SC of this heterostructure was found to have a wider-ranging TI-layer thickness dependence than that of the Bi2Te3/Fe1+yTe heterostructure, which is believed to be attributed to the much higher bulk conductivity of Sb2Te3 that enhances indirect coupling between its top and bottom topological surface states (TSSs). Our results provide the evidence of the interplay among the AFM order, itinerant carries from the TSSs and the induced interfacial SC of the TI/Fe1+yTe heterostructure system., Comment: 28 pages, 5 figures

We perform Raman spectroscopy studies on $\alpha$-RuCl$_3$ at room temperature to explore its phase transitions of magnetism and chemical bonding under pressures. The Raman measurements resolve two critical pressures, about $p_1=1.1$~GPa and $p_2=1.7$~GPa, involving very different intertwining behaviors between the structural and magnetic excitations. With increasing pressures, a stacking order phase transition of $\alpha$-RuCl$_3$ layers develops at $p_1=1.1$~GPa, indicated by the new Raman phonon modes and the modest Raman magnetic susceptibility adjustment. The abnormal softening and splitting of the Ru in-plane Raman mode provide direct evidence of the in-plane dimerization of the Ru-Ru bonds at $p_2=1.7$~GPa. The Raman susceptibility is greatly enhanced with pressure increasing and sharply suppressed after the dimerization. We propose that the system undergoes Mott collapse at $p_2=1.7$~GPa and turns into a dimerized correlated band insulator. Our studies demonstrate competitions between Kitaev physics, magnetism, and chemical bondings in Kitaev compounds., Comment: 7 pages, 4 figures

When a quantum system is driven adiabatically through a parametric cycle in a degenerate Hilbert space, the state would acquire a non-Abelian geometric phase, which is stable and forms the foundation for holonomic quantum computation (HQC). However, in the adiabatic limit, the environmental decoherence becomes a significant source of errors. Recently, various non-adiabatic HQC schemes have been proposed, but all at the price of increased sensitivity to control errors. Alternatively, there exist theoretical proposals for speeding up HQC by the technique of "shortcut to adiabaticity" (STA), but no experimental demonstration has been reported so far, as these proprosals involve a complicated control of four energy levels simultaneously. Here we propose and experimentally demonstrate that HQC via shortcut to adiabaticity can be constructed with only three energy levels, using a superconducting qubit in a scalable architecture. With this scheme, all holonomic single-qubit operations can be realized non-adiabatically through a single cycle of state evolution. As a result, we are able to experimentally benchmark the stability of STA+HQC against NHQC in the same platform. The flexibility and simplicity of our scheme makes it also implementable on other systems, such as nitrogen-vacancy center, quantum dots, and nuclear magnetic resonance., Comment: 6 pages, 4 figures