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We identify and characterize a new class of fingering instabilities in liquid metals; these instabilities are unexpected due to the large interfacial tension of metals. Electrochemical oxidation lowers the effective interfacial tension of a gallium-based liquid metal alloy to values approaching zero, thereby inducing drastic shape changes, including the formation of fractals. The measured fractal dimension ($D = 1.3 \pm 0.05$) places the instability in a different universality class than other fingering instabilities. By characterizing changes in morphology and dynamics as a function of droplet volume and applied electric potential, we identify the three main forces involved in this process: interfacial tension, gravity, and oxidative stress. Importantly, we find that electrochemical oxidation can generate compressive interfacial forces that oppose the tensile forces at a liquid interface. Thus, the surface oxide layer not only induces instabilities, but ultimately provides a physical barrier that halts the instabilities at larger positive potentials. Controlling the competition between surface tension and oxidative (compressive) stresses at the interface is important for the development of reconfigurable electronic, electromagnetic, and optical devices that take advantage of the metallic properties of liquid metals.

Developing quantitative methods for characterizing structural properties of force chains in densely packed granular media is an important step toward understanding or predicting large-scale physical properties of a packing. A promising framework in which to develop such methods is network science, which can be used to translate particle locations and force contacts to a graph in which particles are represented by nodes and forces between particles are represented by weighted edges. Applying network-based community-detection techniques to extract force chains opens the door to developing statistics of force chain structure, with the goal of identifying shape differences across packings, and providing a foundation on which to build predictions of bulk material properties from mesoscale network features. Here, we discuss a trio of related but fundamentally distinct measurements of mesoscale structure of force chains in arbitrary 2D packings, including a novel statistic derived using tools from algebraic topology, which together provide a tool set for the analysis of force chain architecture. We demonstrate the utility of this tool set by detecting variations in force chain architecture with pressure. Collectively, these techniques can be generalized to 3D packings, and to the assessment of continuous deformations of packings under stress or strain., Comment: 13 pages, 5 figures

This paper reports on a theoretical analysis of the rich variety of spatio-temporal patterns observed recently in inclined layer convection at medium Prandtl number when varying the inclination angle $\gamma$ and the Rayleigh number $R$. The present numerical investigation of the inclined layer convection system is based on the standard Oberbeck-Boussinesq equations. The patterns are shown to originate from a complicated competition of buoyancy-driven and shear-flow driven pattern forming mechanisms. The former are expressed as \rm{longitudinal} convection rolls with their axes oriented parallel to the incline, the latter as perpendicular \rm{transverse} rolls. Along with conventional methods to study roll patterns and their stability, we employ direct numerical simulations in large spatial domains, comparable with the experimental ones. As a result, we determine the phase diagram of the characteristic complex 3D convection patterns above onset of convection in the $\gamma-R$ plane, and find that it compares very well with the experiments. In particular we demonstrate that interactions of specific Fourier modes, characterized by a resonant interaction of their wavevectors in the layer plane, are key to understanding the pattern morphologies., Comment: 26 pages, 20 figures, 1 table. Changes in this version: extensive restructuring according to reviewer comments and modification to order of authors

Force chains form heterogeneous physical structures that can constrain the mechanical stability and acoustic transmission of granular media. However, despite their relevance for predicting bulk properties of materials, there is no agreement on a quantitative description of force chains. Consequently, it is difficult to compare the force-chain structures in different materials or experimental conditions. To address this challenge, we treat granular materials as spatially-embedded networks in which the nodes (particles) are connected by weighted edges that represent contact forces. We use techniques from community detection, which is a type of clustering, to find sets of closely connected particles. By using a geographical null model that is constrained by the particles' contact network, we extract chain-like structures that are reminiscent of force chains. We propose three diagnostics to measure these chain-like structures, and we demonstrate the utility of these diagnostics for identifying and characterizing classes of force-chain network architectures in various materials. To illustrate our methods, we describe how force-chain architecture depends on pressure for two very different types of packings: (1) ones derived from laboratory experiments and (2) ones derived from idealized, numerically-generated frictionless packings. By resolving individual force chains, we quantify statistical properties of force-chain shape and strength, which are potentially crucial diagnostics of bulk properties (including material stability). These methods facilitate quantitative comparisons between different particulate systems, regardless of whether they are measured experimentally or numerically., Comment: 15 pages, 13 figures, and 2 appendices

A liquid droplet resting on a soft gel substrate can deform that substrate to the point of material failure, whereby fractures develop on the gel surface that propagate outwards from the contact-line in a starburst pattern. In this paper, we characterize i) the initiation process in which the number of arms in the starburst is controlled by the ratio of surface tension contrast to the gel's elastic modulus and ii) the propagation dynamics showing that once fractures are initiated they propagate with a universal power law $L\propto t^{3/4}$. We develop a model for crack initiation by treating the gel as a linear elastic solid and computing the deformations within the substrate from the liquid/solid wetting forces. The elastic solution shows that both the location and magnitude of the wetting forces are critical in providing a quantitative prediction for the number of fractures and, hence, an interpretation of the initiation of capillary fractures. This solution also reveals that the depth of the gel is an important factor in the fracture process, as it can help mitigate large surface tractions; this finding is confirmed with experiments. We then develop a model for crack propagation by considering the transport of an inviscid fluid into the fracture tip of an incompressible material, and find that a simple energy-conservation argument can explain the observed material-independent power law. We compare predictions for both linear elastic and neo-Hookean solids finding that the latter better explains the observed exponent.

We investigate the origins of the widely-observed "en passant" crack pattern which forms through interactions between two approaching cracks. A rectangular elastic plate is notched on each long side and then subjected to quasistatic uniaxial strain from the short side. The two cracks propagate along approximately straight paths until they pass each other, after which they curve and release a lenticular fragment. We find that for materials with diverse mechanical properties, the shape of this fragment has an aspect ratio of 2:1, with the length scale set by the initial crack offset $s$ and the time scale set by the ratio of $s$ to the pulling velocity. The cracks have a universal square root shape which we understand using a simple geometric model of the crack-crack interaction.

Experimental and theoretical investigations of undulation patterns in high-pressure, inclined layer gas convection at a Prandtl number near unity are reported. Particular focus is given to the competition between the spatiotemporal chaotic state of undulation chaos and stationary patterns of ordered undulations. In experiments a competition and bistability between the two states is observed, with ordered undulations most prevalent at higher Rayleigh number. The spectral pattern entropy, spatial correlation lengths, and defect statistics are used to characterize the competing states. The experiments are complemented by a theoretical analysis of the Oberbeck-Boussinesq equations. The stability region of the ordered undulation as a function of their wavevectors and the Rayleigh number is obtained with Galerkin techniques. In addition, direct numerical simulations are used to investigate the spatiotemporal dynamics. In the simulations both ordered undulations and undulation chaos were observed dependent on initial conditions. Experiment and theory are found to agree well., Comment: Reduced-resolution figures

We present experimental evidence that the motion of point defects in thermal convection patterns in an inclined fluid layer is well-described by Tsallis statistics with an entropic index $q \approx 1.5$. The dynamical properties of the defects (anomalous diffusion, shape of velocity distributions, power law decay of correlations) are in good agreement with typical predictions of nonextensive models, over a range of driving parameters.

We report experiments on defect-tracking in the state of undulation chaos observed in thermal convection of an inclined fluid layer. We characterize the ensemble of defect trajectories according to their velocities, relative positions, diffusion, and gain and loss rates. In particular, the defects exhibit incidents of rapid transverse motion which result in power law distributions for a number of quantitative measures. We examine connections between this behavior and L\'evy flights and anomalous diffusion. In addition, we describe time-reversal and system size invariance for defect creation and annihilation rates., Comment: (21 pages, 17 figures)

We investigate a novel bursting state in inclined layer thermal convection in which convection rolls exhibit intermittent, localized, transverse bursts. With increasing temperature difference, the bursts increase in duration and number while exhibiting a characteristic wavenumber, magnitude, and size. We propose a mechanism which describes the duration of the observed bursting intervals and compare our results to bursting processes in other systems., Comment: 4 pages, 8 figures

We report experimental results on the defect turbulent state of undulation chaos in inclined layer convection of a fluid withPrandtl number $\approx 1$. By measuring defect density and undulation wavenumber, we find that the onset of undulation chaos coincides with the theoretically predicted onset for stable, stationary undulations. At stronger driving, we observe a competition between ordered undulations and undulation chaos, suggesting bistability between a fixed-point attractor and spatiotemporal chaos. In the defect turbulent regime, we measured the defect creation, annihilation, entering, leaving, and rates. We show that entering and leaving rates through boundaries must be considered in order to describe the observed statistics. We derive a universal probability distribution function which agrees with the experimental findings., Comment: 4 pages, 5 figures

We report experiments on thermally driven convection in an inclined layer of large aspect ratio in a fluid of Prandtl number $\sigma \approx 1$. We observed a number of new nonlinear, mostly spatio-temporally chaotic, states. At small angles of inclination we found longitudinal rolls, subharmonic oscillations, Busse oscillations, undulation chaos, and crawling rolls. At larger angles, in the vicinity of the transition from buoyancy- to shear-driven instability, we observed drifting transverse rolls, localized bursts, and drifting bimodals. For angles past vertical, when heated from above, we found drifting transverse rolls and switching diamond panes., Comment: For MPEG movies, see http://milou.msc.cornell.edu/ILCmovies