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The quantum tunneling and emission of a single constituent nucleon provide a beautifully simple and unique window into the complex properties of atomic nuclei at the extreme edge of nuclear existence. In particular, for odd-odd proton emitting nuclides, the associated decay energy and partial half-life can be used to probe the correlations between the valence neutrons and protons which have been theoretically predicted to favour a new type of nuclear superfluidity, isoscalar neutron-proton pairing, for which the experimental “smoking gun" remains elusive. In the present work, proton emission from the lanthanum isotope 11657La59, 23 neutrons away from the only stable isotope 13957La82, is reported. 116La nuclei were synthesised in the fusion-evaporation reaction 58Ni(64Zn, p5n)116La and identified via their proton radioactivity using the mass spectrometer MARA (Mass Analysing Recoil Apparatus) and the silicon detectors placed at its focal plane. Comparisons of the measured proton energy (Ep = 718 ± 9 keV) and half-life (T1/2 = 50 ± 22 ms) with values calculated using the Universal Decay Law approach indicate that the proton is emitted with an orbital angular momentum l = 2 and that its emission probability is enhanced relative to its closest, less exotic, odd-even lanthanum isotope (11757La60) while the proton-emission Q-value is lower. We propose this to be a possible signature for the presence of strong neutron-proton pair correlations in this exotic, neutron deficient system. The observations of γ decays from isomeric states in 116La and 117La are also reported. peerReviewed

The mean lifetimes of the lowest energy 2+, 8+ and 9− states in 166Os have been measured using the recoil distance Doppler-shift method in conjunction with a selective recoil-decay tagging technique. These measurements extend studies into the most neutron-deficient mass region accessible to current experimental methods. The B(E2; 2+ → 0+) = 7(2) W.u. extracted from these measurements is markedly lower than those observed in the heavier even-mass Os isotopes. The 8+ and 9− states yield reduced transition probabilities that are consistent with single-particle transitions. While these values may indicate a departure from collective structure, the level scheme and the underlying nuclear configurations can also be interpreted in terms of a simple collective picture. This contrasting behaviour suggests an intriguing dichotomy in the description of heavy transitional nuclei. peerReviewed

A low-energy branch is under development for the MARA vacuum-mode recoil separator at the Accelerator Laboratory of the University of Jyväskylä. This development will allow for the study of proton-rich nuclei through laser ionisation spectroscopy and mass measurements. After stopping and extraction from a buffer gas cell, the ions of interest will be accelerated and transported to dedicated experimental setups by an ion transport system consisting of several focusing, accelerating and mass-separating elements. This article presents the current design and simulations for the ion transport. peerReviewed

An experiment has been performed to study excited states in the neutron-deficient nucleus 175Ir via the use of the JUROGAM II high-purity germanium detector array and the RITU gas-filled separator at JYFL, Jyväskylä. By using isomer tagging, an isomeric state with a half-life of 6.58(15) μs has been observed in 175Ir for the first time. It has been established that the isomer decays via a 45.2 (E1)–26.1 (M1) keV cascade to new states below the previously reported ground state in 175Ir with Iπ = (5/2−). We now reassign this (5/2−) state to the isomeric state discovered in this study. peerReviewed

Fine structure in the α decay of high-spin states in 156Lu and 158Ta has been identified by means of αγ - coincidence analysis. One new α decay from 156Lu and two from 158Ta were identified, one of which was found to populate a previously unknown state in 154Lu. The hindrance-factor systematics from all four odd-odd, N = 85 nuclei with known α-decaying, πh11/2 coupled states were reviewed and are discussed. These proved consistent with the previously assigned (πh11/2νh9/2 )10+ configuration of the α-decaying state in 156Lu, which differs from the (πh11/2ν f7/2 )9+ assignments in the other three nuclei. peerReviewed

Lifetime measurements have been performed using the 98 Mo ( 86 Kr , 4 n ) 180 Pt reaction at a beam energy of 380 MeV, and the recoil distance Doppler-shift method. In a second experiment the 168 Yb ( 16 O , 4 n ) 180 Pt reaction at a beam energy of 88 MeV using the Ge-gated γ − γ fast timing technique was used to determine lifetimes. Lifetimes of the four lowest yrast states of 180 Pt have been determined. The experimental data are compared to calculations within the framework of the interacting boson model and the general collective model. Both models predict a deformed ground state and are consistent with all the remaining experimental results. peerReviewed

A differential-plunger device was used to measure the lifetimes of the lowest states in the πg7/2 ⊗ νh11/2 rotational band in doubly odd 112I with the 58Ni(58Ni, 3pn) reaction. A differential decay curve method was performed using the fully shifted and degraded γ -ray intensity measurements as a function of target-to-degrader distance. The lifetimes of the lowest three states in the πg7/2 ⊗ νh11/2 band in 112I were measured to be 124(30), 130(25), and 6.5(5) ps, respectively. As the lifetimes of successive excited states in a rotational band are expected to decrease with increasing excitation energy, these measurements suggest that the order of the transitions in the established band in 112I may need revising and that the state tentatively assigned to be (7−) may not belong to the rotational band. peerReviewed

Excited states above the 17+ isomeric state in the proton-rich nucleus 152Tm were established by employing the recoil-isomer tagging technique. Data were collected using the JUROGAM gamma-ray array and the GREAT spectrometer together with the recoil ion transport unit (RITU) gas-filled recoil separator and analyzed to identify the prompt and delayed γ decays from the levels in 152Tm. Shell-model calculations, either in a large valence space or in a reduced model space with five protons in the π0h11/2 orbital and one neutron in the ν1f7/2 orbital, agree with the observed energies of the yrast levels up to angular momentum J = 21. The observation of near degeneracies in the energy spectrum can be attributed to specific components of the proton-neutron interaction. The isomeric decay of the 17+ level is not reproduced in the shell-model calculations as it arises from a delicate balance between hindrance due to seniority selection rules and enhancement due to configuration mixing peerReviewed

A multiparticle spin-trap isomeric state having a half-life of 179(4) ns and lying 2601 keV above the yrast 10 + state in 156 Lu has been discovered. The 156 Lu nuclei were produced by bombarding isotopically enriched 106 Cd targets with beams of 58 Ni ions, separated in flight using the gas-filled separator RITU and their decays were measured using the GREAT spectrometer. Analysis of the main decay path that populates yrast states observed previously suggests a spin-parity assignment of 19 − for the isomeric state, which is consistent with isomeric states identified in the N = 85 isotones. Comparison with other decay paths in 156 Lu indicates that the [ π h − 1 11 / 2 ⊗ ν h 9 / 2 ] 10 + state at the bottom of the yrast sequence is likely to be the α -decaying isomeric state, with the [ π h − 1 11 / 2 ⊗ ν f 7 / 2 ] 9 + state lying 62 keV above it. The relative ordering of the lowest-lying 9 + and 10 + states is inverted in 156 Lu compared with its odd-odd isotones. peerReviewed

Fine structure in the α decay of high-spin isomers in 155Lu(25/2−) and 156Hf (8+) has been studied for the first time using αγ -coincidence analysis. Three new α decays from 155Lu(25/2−) and two from 156Hf (8+) have been identified, populating seniority s > 1 states in the N = 82 nuclei 151Tm and 152Yb, respectively. The reduced hindrance factors of the α decays support the previous configuration assignments of the populated states. This is the first observation of states with excitation energy greater than 1.5 MeV being populated following α decay in nuclei outside of the 208Pb region. peerReviewed

Using fusion-evaporation reactions, a gas-filled recoil separator, recoil-gating technique and recoil-isomer decay tagging technique we have extended the level scheme of 203 At ( N = 118 ) significantly. We have observed an isomeric [ τ = 14.1 ( 3 ) μ s ] state with a spin and parity of 29 / 2 + . The isomeric state is suggested to originate from the π ( h 9 / 2 ) ⊗ ∣ ∣ 202 Po ; 11 − ⟩ coupling, and it is depopulated through 286 keV E 2 and 366 keV E 3 transitions. In addition, we have observed a cascade of magnetic-dipole transitions which is suggested to be generated by the shears mechanism. peerReviewed

Lifetimes of the first excited 2þ and 4þ states in the extremely neutron-deficient nuclide 172Pt have been measured for the first time using the recoil-distance Doppler shift and recoil-decay tagging techniques. An unusually low value of the ratio BðE2∶4þ 1 → 2þ 1 Þ=BðE2∶2þ 1 → 0þ gsÞ ¼ 0.55ð19Þ was found, similar to a handful of other such anomalous cases observed in the entire Segr´e chart. The observation adds to a cluster of a few extremely neutron-deficient nuclides of the heavy transition metals with neutron numbers N ≈ 90–94 featuring the effect. No theoretical model calculations reported to date have been able to explain the anomalously low BðE2∶4þ 1 → 2þ 1 Þ=BðE2∶2þ 1 → 0þ gsÞ ratios observed in these cases. Such low values cannot, e.g., be explained within the framework of the geometrical collective model or by algebraic approaches within the interacting boson model framework. It is proposed that the group of BðE2∶4þ 1 → 2þ 1 Þ=BðE2∶2þ 1 → 0þ gs) ratios in the extremely neutron-deficient even-even W, Os, and Pt nuclei around neutron numbers N ≈ 90–94 reveal a quantum phase transition from a seniority-conserving structure to a collective regime as a function of neutron number. Although a system governed by seniority symmetry is the only theoretical framework for which such an effect may naturally occur, the phenomenon is highly unexpected for these nuclei that are not situated near closed shells.

The level structure of 136Nd has been investigated using the 100Mo(40Ar, 4n) reaction and the JUROGAM II+RITU+GREAT setup. The level scheme has been extended significantly. Many new bands have been identified both at low and high spin, among which are five nearly degenerate bands interpreted as chiral partners. Excitation energies, spins, and parities of the previously known bands are revised and firmly established, and some previously known bands have been revised. Configurations are assigned to the observed bands based on cranked Nilsson-Strutinsky calculations. The band structure of 136Nd is now clarified and the various types of single-particle and collective excitations are well understood. peerReviewed

The excited states of the proton emitter 151Lu were reinvestigated in a recoil-decay tagging experiment at the Accelerator Laboratory of the University of Jyväskylä (JYFL). The level scheme built on the ground state of 151Lu was updated with five new γ -ray transitions. Large-scale shell model calculations were carried out in the model space consisting of the neutron and proton orbitals 0g7/2, 1d5/2, 1d3/2, 2s1/2, and 0h11/2 with the optimized monopole interaction in order to interpret the experimental level scheme of 151Lu. It is found that the excitation energies of states above the 27/2− and 23/2+ isomeric levels in 151Lu can be sensitive to excitations from g7/2 and d5/2 to single-particle orbitals above N = Z = 64. peerReviewed

Lifetimes of excited states in the yrast band of the neutron-deficient nuclide 166W have been measured utilizing the DPUNS plunger device at the target position of the JUROGAM II γ -ray spectrometer in conjunction with the RITU gas-filled separator and the GREAT focal-plane spectrometer. Excited states in 166W were populated in the 92Mo(78Kr,4p) reaction at a bombarding energy of 380 MeV. The measurements reveal a low value for the ratio of reduced transitions probabilities for the lowest-lying transitions B(E2; 4+ → 2+)/B(E2; 2+ → 0+) = 0.33(5), compared with the expected ratio for an axially deformed rotor (B4/2 = 1.43). peerReviewed

The very neutron-deficient isobars 179Pb and 179Tl have been produced using the fusion-evaporation reactions 104Pd(78Kr,xpyn), where x≤1 and y≥2. The gas-filled separator RITU was employed to transport and separate the recoiling nuclei of interest from the scattered beam and unwanted products. The GREAT spectrometer was used to study the decay properties through α−α and α−γ correlations, which has allowed the ground state of 179Pb to be assigned as Iπ=9/2−. The decay of 179Pb was measured to have an α-particle energy and half-life of Eα=7348(5)keV and t1/2=2.7(2) ms, respectively. A search for a νi13/2 state in 179Pb was performed, but only a limit of excitation energy and half-life was obtained. In 179Tl a t1/2=114+18−10 ns isomeric state, likely at an excitation energy of 904.5(9) keV, was identified and is tentatively assigned to be a 9/2− proton intruder state. peerReviewed

A newly observed isomeric intruder ½ + state [ T ½ = 3.5 ( 6 ) ms ] is identified in 203 At using a gas-filled recoil separator and fusion-evaporation reactions. The isomer is depopulated through a cascade of E 3 and mixed M 1 / E 2 transitions to the 9 / 2 − ground state, and it is suggested to originate from the π ( s ½ ) − 1 configuration. In addition, the structures above the ½ + state in 203 At and 197 At are studied using in-beam γ -ray spectroscopy, recoil-decay tagging, and recoil-isomer decay tagging methods. The ½ + state is fed from 3 / 2 + and 5 / 2 + states, and the origin of these states are discussed. peerReviewed

The new neutron-deficient nuclei 240Es and 236Bk were synthesised at the gas-filled recoil separator RITU. They were identified by their radioactive decay chains starting from 240Es produced in the fusion–evaporation reaction 209Bi(34S,3n)240Es. Half-lives of 6(2) sand 22+13−6swere obtained for 240Es and 236Bk, respectively. Two groups of αparticles with energies Eα=8.19(3) MeVand 8.09(3) MeVwere unambiguously assigned to 240Es. Electron-capture delayed fission branches with probabilities of 0.16(6)and 0.04(2)were measured for 240Es and 236Bk, respectively. These new data show a continuation of the exponential increase of ECDF probabilities in more neutron-deficient isotopes. peerReviewed

The structure of the low- and medium-spin levels of the 211Po nucleus have been studied with in-beam γ-ray spectroscopy with the 208Pb(α,n)211Po fusion-evaporation reaction. The level scheme was further extended with levels of the configurations π(h9/2)22+−4+⊗νg9/2, π(h9/2)28+⊗νg9/2, π(h9/2)22+−4+⊗νi11/2, π(h9/2)22+−4+⊗νj15/2, π(h9/2f7/2)8+⊗νg9/2, and π(h9/2)20+⊗ν(g9/2)20+(s1/2)−1. The single-particle neutron states νd5/2 and νs1/2 were also identified. Furthermore, a number of states feeding the low-spin structures were added. peerReviewed

The evolution of collectivity with spin along the yrast line in the neutron-deficient nucleus 112Te has been studied by measuring the reduced transition probability of excited states in the yrast band. In particular, the lifetimes of the 4+ and 6+ excited states have been determined by using the recoil distance Doppler-shift method. The results are discussed using both large-scale shell-model and total Routhian surface calculations. peerReviewed

The lifetime of the (11/2+) state in the band above the proton-emitting (3/2+) state in 113Cs has been measured to be τ = 24(6) ps from a recoil-decay-tagged differential-plunger experiment. The measured lifetime was used to deduce the deformation of the states using wave functions from a nonadiabatic quasiparticle model to independently calculate both proton-emission and electromagnetic γ -ray transition rates as a function of deformation. The only quadrupole deformation, which was able to reproduce the experimental excitation energies of the states, the electromagnetic decay rate of the (11/2+) state and the proton-emission rate of the (3/2+) state, was found to be β2 = 0.22(6). This deformation is in agreement with the earlier proton emission studies which concluded that 113Cs was best described as a deformed proton emitter, however, it is now more firmly supported by the present measurement of the electromagnetic transition rate. peerReviewed

The level scheme of the neutron-deficient nuclide 168Os has been extended and mean lifetimes of excited states have been measured by the recoil distance Doppler-shift method using the JUROGAM γ -ray spectrometer in conjunction with the IKP Koln plunger device. The ¨ 168Os γ rays were measured in delayed coincidence with recoiling fusion-evaporation residues detected at the focal plane of the RITU gas-filled separator. The ratio of reduced transition probabilities B(E2; 4+ 1 → 2+ 1 )/B(E2; 2+ 1 → 0+ 1 ) is measured to be 0.34(18), which is very unusual for collective band structures and cannot be reproduced by interacting boson model (IBM-2) calculations based on the SkM* energy-density functional. peerReviewed

Excited states in the neutron-deficient N=84 nuclide 155Lu have been populated by using the 102Pd(58Ni,αp) reaction. The 155Lu nuclei were separated by using the gas-filled recoil ion transport unit (RITU) separator and implanted into the Si detectors of the gamma recoil electron alpha tagging (GREAT) spectrometer. Prompt γ-ray emissions measured at the target position using the JUROGAM Ge detector array were assigned to 155Lu through correlations with α decays measured in GREAT. Structures feeding the (11/2−) and (25/2−)α-decaying states have been revised and extended. Shell-model calculations have been performed and are found to reproduce the excitation energies of several of the low-lying states observed to within an average of 71 keV. In particular, the seniority inversion of the 25/2− and 27/2− states is reproduced. peerReviewed

Excited states in the neutron-deficient odd-odd proton-unbound nuclide 158Ta have been investigated in two separate experiments. In the first experiment, 166Ir nuclei were produced in the reactions of 380 MeV 78Kr ions with an isotopically enriched 92Mo target. The α-decay chain of the 9+ state in 166Ir was analyzed. Fine structure in the α decay of the 9+ state in 162Re established a 66 keV difference in excitation energy between the lowest-lying 9+ and 10+ states in 158Ta. Higher-lying states in 158Ta were populated in the reactions of 255 MeV 58Ni ions with an isotopically enriched 102Pd target. Gamma-ray decay paths that populate, depopulate, and bypass a 19− isomeric state have been identified. The general features of the deduced level scheme are discussed and the prospects for observing proton emission branches from excited states are considered. peerReviewed

The extremely neutron-deficient isotope 178Pb has been produced. The GREAT spectrometer at the focal plane position of the gas-filled separator RITU was used to study the α decay of 178Pb and its α-decay chain through α-α correlations. The α decay was measured to have an energy and half-life of Eα= 7610(30) keV and t1/2 = 0.21+0.21 −0.08 ms, respectively. The half-life is consistent with recent theoretical calculations using the Coulomb and proximity potential model. The α-decay reduced width and hindrance factor for 178Pb were deduced and correspond to an unhindered l = 0 transition. In addition, the mass excess of 178Pb and the α-decay Q value were calculated from the experimental results and compared to theoretical values. peerReviewed

Lifetimes of excited states in the neutron-deficient odd-odd nucleus 166Re have been measured for the first time using the recoil distance Doppler-shift method. The measured lifetime for the (8−) state; τ = 480 (80) ps, enabled an assessment of the multipolarities of the γ rays depopulating this state. Information on electromagnetic transition strengths were deduced for the γ -ray transitions from the (9−), (10−), and (11−) states, and in the case of the (10−) and (11−) states limits on the B(M1) and B(E2) strengths were estimated. The results are compared with total Routhian surface predictions and semiclassical calculations. Tilted-axis cranking calculations based on a relativistic mean-field approach (TAC-RMF) have also been performed in order to test the possibility of magnetic rotation in the 166Re nucleus. While the TAC-RMF calculations predict a quadrupole-deformed nuclear shape with similar β2 deformation as obtained by using the TRS model, it was found that the experimental electromagnetic transition rates are in better agreement with a collective-rotational description. peerReviewed

The α decay of 222Th populating the low-lying J π = 3− state, and also a proposed 1− state, in 218Ra has been observed. The observations suggest an excitation energy of 853 keV for the 1− state, which is 60 keV above the 3− state. The hindrance factors of these α decays give a possible boundary to the region of ground-state octupole deformation in the light-actinide nuclei. The relative positions of the J π = 1− and 3− states suggest they are produced by an octupole-vibrational mechanism, as opposed to α clustering or rotations of a reflection-asymmetric octupole-deformed shape. peerReviewed

A non-reference based method to determine internal conversion coefficients using the SAGE spectrometer is carried out for transitions in the nuclei of 154Sm, 152Sm and 166Yb. The Normalised-Peak-to-Gamma method is in general an efficient tool to extract internal conversion coefficients. However, in many cases the required well-known reference transitions are not available. The data analysis steps required to determine absolute internal conversion coefficients with the SAGE spectrometer are presented. In addition, several background suppression methods are introduced and an example of how ancillary detectors can be used to select specific reaction products is given. The results obtained for ground-state band E2 transitions show that the absolute internal conversion coefficients can be extracted using the methods described with a reasonable accuracy. In some cases of less intense transitions only an upper limit for the internal conversion coefficient could be given. peerReviewed

The excited states of 201At were studied and an isomeric 29/2 + state [T1/2 = 3.39(9) μs] was identified by using a fusion-evaporation reaction, a gas-filled recoil separator, and recoil gating techniques. The 29/2 + state is suggested to originate from the π(h9/2) ⊗ |200Po;11− configuration, and it decays through the 269- and 339-keV E2- and E3-type transitions, respectively. Moreover, a cascade of magnetic dipole transitions that is suggested to originate from a shears band was observed by using recoil-gated γ − γ (−γ ) coincidence techniques. peerReviewed

In the search for the fully aligned 27− state in 140Nd predicted by cranked Nilsson-Strutinsky calculations, new close-to-spherical high-spin states have been discovered. Both the close-to-spherical and the triaxial calculated states are in good agreement with the experimental results, supporting the existence of shape coexistence up to very high spins. Shell-model calculations using a newly developed effective interaction for the 50 N ,Z 82 mass region are in good agreement with the observed spherical states. The comparison between the experimental and calculated level energies allowed the relative energy to be established between several proton and neutron orbitals at high energy and spins. peerReviewed

Excited states in the neutron-deficient nuclei 163 75 Re88 and 165 75 Re90 were populated in the 106Cd(60Ni, p2nγ ) and 92Mo(78Kr, 3p2nγ ) fusion-evaporation reactions at bombarding energies of 270 and 380 MeV, respectively. γ rays were detected at the target position using the JUROGAM spectrometer while recoiling ions were separated in-flight by the RITU gas-filled recoil separator and implanted in the GREAT spectrometer. The energy level schemes for 163Re and 165Re were identified using recoil-decay correlation techniques. At low spin, the yrast bands of these isotopes consist of signature partner bands based on a single πh11/2 quasiproton configuration. The bands display large energy splitting consistent with the soft triaxial shape typical of transitional nuclei above N = 82. The configurations of the excited states are proposed within the framework of the cranked shell model. peerReviewed

A dipole band of six transitions built upon a firmly established I π = 31/2− isomeric state has been identified in 189Pb using recoil-isomer tagging. This is the lightest odd-mass Pb nucleus in which a dipole band is known. The dipole nature of the new transitions has been confirmed through angular-intensity arguments. The evolution of the excitation energy and the aligned-angular momentum of the states in the new dipole band are compared with those of dipole bands in heavier, odd-mass lead isotopes. This comparison suggests that the new band in 189Pb is based upon a π[s−2 1/2h9/2i13/2]11− ⊗ ν[i −1 13/2+ ]13/2+ configuration. However, the increased aligned-angular momentum in 189Pb may suggest evidence for a reduced repulsive proton/neutron-hole interaction compared to dipole bands in the heavier mass isotopes. peerReviewed

Excited states have been studied in the deformed proton emitter 113Cs. Gamma-ray transitions have been unambiguously assigned to 113Cs by correlation with its characteristic proton decay, using the method of recoil-decay tagging. Two previously identified rotational bands have been observed and extended to tentative spins of 45/2 and 51/2 h¯, with excitation energies over 8 MeV above the lowest state. These are the highest angular momenta and excitation energies observed to date in any nucleus beyond the proton drip-line. Transitions in the bands have been rearranged compared to previous work. A study of aligned angular momenta, in comparison to the predictions of Woods–Saxon cranking calculations, is consistent with the most intense band being based on the π g7/2[422]3/2+ configuration, which would contradict the earlier πh11/2 assignment, and with the second band being based on the πd5/2[420]1/2+ configuration. The data suggest that the band based upon the πh11/2 configuration is not observed. peerReviewed

Excited states in the highly neutron-deficient nucleus 162W have been investigated via the 92Mo(78Kr, 2α) 162W reaction. Prompt γ rays were detected by the JUROGAM II high-purity germanium detector array and the recoiling fusion-evaporation products were separated by the recoil ion transport unit (RITU) gas-filled recoil separator and identified with the gamma recoil electron alpha tagging (GREAT) spectrometer at the focal plane of RITU. γ rays from 162W were identified uniquely using mother-daughter and mother-daughter-granddaughter α-decay correlations. The observation of a rotational-like ground-state band is interpreted within the framework of total Routhian surface (TRS) calculations, which suggest an axially symmetric ground-state shape with a γ -soft minimum at β2 ≈ 0.15. Quasiparticle alignment effects are discussed based on cranked shell model calculations. New measurements of the 162W ground-state α-decay energy and half-life were also performed. The observed α-decay energy agrees with previous measurements. The half-life of 162W was determined to be t1/2 = 990(30) ms. This value deviates significantly from the currently adopted value of t1/2 = 1360(70) ms. In addition, the α-decay energy and half-life of 166Os were measured and found to agree with the adopted values. peerReviewed

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Excited states in the neutron-deficient nucleus 161 72Hf89 have been populated using the 118Sn(48Ti,5n) 161Hf and 110Pd(56Fe,5n) 161Hf fusion-evaporation reactions at 240 and 270 MeV, respectively. The level scheme for 161Hf has been extended with the observation of new band structures and an I π = (13/2+) isomeric state with a half-life of 4.8(2) μs has been identified. The decay path from this isomer to the (7/2−) ground state is established. The yrast band, based on the (13/2+) isomeric state, is extended up to (73/2+) and side band structures are identified up to (69/2−) and (55/2−). Quasiparticle assignments for these rotational structures are made on the basis of their alignment properties and Woods-Saxon cranked shell-model calculations. peerReviewed