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Low-loss high-speed switches are an integral component of future photonic quantum technologies, with applications in state generation, multiplexing, and the implementation of quantum gates. Phase modulation is one method of achieving this switching, but existing optical phase modulators either achieve high bandwidth or low loss, but not both. We demonstrate fast ($100\,\mathrm{MHz}$ bandwidth), low-loss ($83\pm2\%$ transmission) phase shifting ($\Delta\phi = (0.90\pm0.05)\pi$) in a signal field, induced by a control field, and mediated by the two-photon $5S_{1/2} \rightarrow{} 5P_{3/2} \rightarrow{} 5D_{5/2}$ transition in $^{87}\text{Rb}$ vapour. We discuss routes to enhance both performance and scalability for application to a range of quantum and classical technologies., Comment: 10 pages, 6 figures, this version includes more detailed simulation with collaborators from Imperial College London

Adding or subtracting a single quantum of excitation to a thermal state of a bosonic system has the counter-intuitive effect of approximately doubling its mean occupation. We perform the first experimental demonstration of this effect outside optics by implementing single-phonon addition and subtraction to a thermal state of a mechanical oscillator via Brillouin optomechanics in an optical whispering-gallery microresonator. Using a detection scheme that combines single-photon counting and optical heterodyne detection, we observe this doubling of the mechanical thermal fluctuations to a high precision. The capabilities of this joint click-dyne detection scheme adds a significant new dimension for optomechanical quantum science and applications.

A remarkable aspect of quantum theory is that certain measurement outcomes are entirely unpredictable to all possible observers. Such quantum events can be harnessed to generate numbers whose randomness is asserted based upon the underlying physical processes. We formally introduce, design and experimentally demonstrate an ultrafast optical quantum random number generator that uses a totally untrusted photonic source. While considering completely general quantum attacks, we certify and generate in real-time random numbers at a rate of $8.05\,$Gb/s with a rigorous security parameter of $10^{-10}$. Our security proof is entirely composable, thereby allowing the generated randomness to be utilised for arbitrary applications in cryptography and beyond. To our knowledge, this represents the fastest composably secure source of quantum random numbers ever reported., Comment: 37 pages, 7 figures. New substantial material has been added and the title was modified accordingly

Quantum memories are essential for large-scale quantum information networks. Along with high efficiency, storage lifetime and optical bandwidth, it is critical that the memory add negligible noise to the recalled signal. A common source of noise in optical quantum memories is spontaneous four-wave mixing. We develop and implement a technically simple scheme to suppress this noise mechanism by means of quantum interference. Using this scheme with a Raman memory in warm atomic vapour we demonstrate over an order of magnitude improvement in noise performance. Furthermore we demonstrate a method to quantify the remaining noise contributions and present a route to enable further noise suppression. Our scheme opens the way to quantum demonstrations using a broadband memory, significantly advancing the search for scalable quantum photonic networks., Comment: 6 pages, 5 figures plus Supplementary Material

Strong light-matter interactions are critical for quantum technologies based on light, such as memories or nonlinear interactions. Solid state materials will be particularly important for such applications, because of the relative ease of fabrication of components. Silicon vacancy centers (SiV) in diamond feature especially narrow inhomogeneous spectral lines, which are rare in solid materials. Here, we demonstrate resonant coherent manipulation, stimulated Raman adiabatic passage, and strong light-matter interaction via four-wave mixing of a weak signal field in an ensemble of SiV centers.

Quantum memory capable of storage and retrieval of flying photons on demand is crucial for developing quantum information technologies. However, the devices needed for long-distance links are quite different from those envisioned for local processing. Here, we present the first hybrid quantum memory enabled network by demonstrating the interconnection and simultaneous operation of two types of quantum memory: an atomic-ensemble-based memory and an all-optical loop memory. The former generates and stores single atomic excitations that can then be converted to single photons; and the latter maps incoming photons in and out on demand, at room-temperature and with a broad acceptance bandwidth. Interfacing these two types of quantum memories, we observe a well-preserved quantum cross-correlation, reaching a value of 22, and a violation of the Cauchy-Schwarz inequality up to 549 standard deviations. Furthermore, we demonstrate the creation and storage of a fully operable heralded photon chain state that can achieve memory-built-in combining, swapping, splitting, tuning and chopping single photons in a chain temporally. Such a quantum network allows atomic excitations to be generated, stored, and converted to broadband photons, which are then transferred to the next node, stored, and faithfully retrieved, all at high speed and in a programmable fashion., Comment: 14 pages, 10 figures, 1 table

We report a single-stage bi-directional interface capable of linking Sr+ trapped ion qubits in a long-distance quantum network. Our interface converts photons between the Sr+ emission wavelength at 422 nm and the telecoms C-band to enable low-loss transmission over optical fiber. We have achieved both up- and down-conversion at the single photon level with efficiencies of 9.4% and 1.1% respectively. Furthermore we demonstrate noise levels that are low enough to allow for genuine quantum operation in the future., Comment: 5 pages, 4 figures

The heat engine, a machine that extracts useful work from thermal sources, is one of the basic theoretical constructs and fundamental applications of classical thermodynamics. The classical description of a heat engine does not include coherence in its microscopic degrees of freedom. By contrast, a quantum heat engine might possess coherence between its internal states. Although the Carnot efficiency cannot be surpassed, and coherence can be performance degrading in certain conditions, it was recently predicted that even when using only thermal resources, internal coherence can enable a quantum heat engine to produce more power than any classical heat engine using the same resources. Such a power boost therefore constitutes a quantum thermodynamic signature. It has also been shown that the presence of coherence results in the thermodynamic equivalence of different quantum heat engine types, an effect with no classical counterpart. Microscopic heat machines have been recently implemented with trapped ions, and proposals for heat machines using superconducting circuits and optomechanics have been made. When operated with standard thermal baths, however, the machines implemented so far have not demonstrated any inherently quantum feature in their thermodynamic quantities. Here we implement two types of quantum heat engines by use of an ensemble of nitrogen-vacancy centres in diamond, and experimentally demonstrate both the coherence power boost and the equivalence of different heat-engine types. This constitutes the first observation of quantum thermodynamic signatures in heat machines.

Photonics offers a route to fast and distributed quantum computing in ambient conditions, provided that photon sources and logic gates can be operated deterministically. Quantum memories, capable of storing and re-emitting photons on demand, enable quasi-deterministic operations by synchronising stochastic events. We recently interfaced a Raman-type quantum memory with a travelling-wave heralded photon source. Here we discuss the trade-space for the spectral characteristics of such sources, and we present measurements of our source, which represents a practical compromise enabling passive stability, high brightness in a single-pass configuration, high purity and good matching to our Cs vapour memory.

We present a composable security proof, valid against arbitrary attacks and including finite-size effects, for a high dimensional time-frequency quantum key distribution (TFQKD) protocol based upon spectrally entangled photons. Previous works have focused on TFQKD schemes as it combines the impressive loss tolerance of single-photon QKD with the large alphabets of continuous variable (CV) schemes, which enables the potential for more than one bit of secret key per transmission. However, the finite-size security of such schemes has only been proven under the assumption of collective Gaussian attacks. Here, by combining recent advances in entropic uncertainty relations for CVQKD with decoy state analysis, we derive a composable security proof that predicts key rates on the order of Mbits/s over metropolitan distances (40km or less) and maximum transmission distances of up to 140km., Comment: 12 pages, 3 figures

We show that cold Rydberg gases enable an efficient six-wave mixing process where terahertz or microwave fields are coherently converted into optical fields and vice versa. This process is made possible by the long lifetime of Rydberg states, the strong coupling of millimeter waves to Rydberg transitions and by a quantum interference effect related to electromagnetically induced transparency (EIT). Our frequency conversion scheme applies to a broad spectrum of millimeter waves due to the abundance of transitions within the Rydberg manifold, and we discuss two possible implementations based on focussed terahertz beams and millimeter wave fields confined by a waveguide, respectively. We analyse a realistic example for the interconversion of terahertz and optical fields in rubidium atoms and find that the conversion efficiency can in principle exceed 90\%., Comment: 11 pages, 6 figures and supplementary information

Quantum light-matter interfaces are at the heart of photonic quantum technologies. Quantum memories for photons, where non-classical states of photons are mapped onto stationary matter states and preserved for subsequent retrieval, are technical realizations enabled by exquisite control over interactions between light and matter. The ability of quantum memories to synchronize probabilistic events makes them a key component in quantum repeaters and quantum computation based on linear optics. This critical feature has motivated many groups to dedicate theoretical and experimental research to develop quantum memory devices. In recent years, exciting new applications, and more advanced developments of quantum memories, have proliferated. In this review, we outline some of the emerging applications of quantum memories in optical signal processing, quantum computation, and nonlinear optics. We review recent experimental and theoretical developments, and their impacts on more advanced photonic quantum technologies based on quantum memories., Comment: Review paper. Comments are welcome!

Alkali-filled hollow-core fibres are a promising medium for investigating light-matter interactions, especially at the single-photon level, due to the tight confinement of light and high optical depths achievable by light-induced atomic desorption. However, until now these large optical depths could only be generated for seconds at most once per day, severely limiting the practicality of the technology. Here we report the generation of highest observed transient ($>10^5$ for up to a minute) and highest observed persistent ($>2000$ for hours) optical depths of alkali vapours in a light-guiding geometry to date, using a caesium-filled Kagom\'e-type hollow-core photonic crystal fibre. Our results pave the way to light-matter interaction experiments in confined geometries requiring long operation times and large atomic number densities, such as generation of single-photon-level nonlinearities and development of single photon quantum memories., Comment: Author Accepted version

We report a comprehensive approach to analysing continuous-output photon detectors. We employ principal component analysis to maximise the information extracted, followed by a novel noise-tolerant parameterised approach to the tomography of PNRDs. We further propose a measure for rigorously quantifying a detector's photon-number-resolving capability. Our approach applies to all detectors with continuous-output signals. We illustrate our methods by applying them to experimental data obtained from a transition-edge sensor (TES) detector., Comment: 5 pages, 3 figures, also includes supplementary information

We develop a scheme for time-frequency encoded continuous-variable cluster-state quantum computing using quantum memories. In particular, we propose a method to produce, manipulate and measure 2D cluster states in a single spatial mode by exploiting the intrinsic time-frequency selectivity of Raman quantum memories. Time-frequency encoding enables the scheme to be extremely compact, requiring a number of memories that is a linear function of only the number of different frequencies in which the computational state is encoded, independent of its temporal duration. We therefore show that quantum memories can be a powerful component for scalable photonic quantum information processing architectures., Comment: 5 pages, 6 figures, and supplementary information. Updated to be consistent with published version

We adopt the beam splitter model for losses to analyse the performance of a recent compact continuous-variable entanglement distillation protocol [Phys. Rev. Lett. 108, 060502, (2012)] implemented using realistic quantum memories. We show that the decoherence undergone by a two-mode squeezed state while stored in a quantum memory can strongly modify the results of the preparatory step of the protocol. We find that the well-known method for locally increasing entanglement, phonon subtraction, may not result in entanglement gain when losses are taken into account. Thus, we investigate the critical number $m_c$ of phonon subtraction attempts from the matter modes of the quantum memory. If the initial state is not de-Gaussified within $m_c$ attempts, the protocol should be restarted to obtain any entanglement increase. Moreover, the condition $m_c>1$ implies an additional constraint on the subtraction beam splitter interaction transmissivity, viz. it should be about 50% for a wide range of protocol parameters. Additionally, we consider the average entanglement rate, which takes into account both the unavoidable probabilistic nature of the protocol and its possible failure as a result of a large number of unsuccessful subtraction attempts. We find that a higher value of the average entanglement can be achieved by increasing the subtraction beam splitter interaction transmissivity. We conclude that the compact distillation protocol with the practical constraints coming from realistic quantum memories allows a feasible experimental realization within existing technologies., Comment: 9 pages, 8 figures. Updated version for publication

The generation of large multiphoton quantum states - for applications in computing, metrology, and simulation - requires a network of high-efficiency quantum memories capable of storing broadband pulses. Integrating these memories into a fibre offers a number of advantages towards realising this goal: strong light-matter coupling at low powers, simplified alignment, and compatibility with existing photonic architectures. Here, we introduce a large-core kagome-structured hollow-core fibre as a suitable platform for an integrated fibre-based quantum memory with a warm atomic vapour. We demonstrate, for the first time, efficient optical pumping in a hollow-core photonic-crystal fibre with a warm atomic vapour, where (90 $\pm$ 1)% of atoms are prepared in the ground state. We measure high optical depths (3$\times 10^{4}$) and, also, narrow homogeneous linewidths that do not exhibit significant transit-time broadening. Our results establish that kagome fibres are suitable for implementing a broadband, room-temperature quantum memory., Comment: 10 pages, 4 figures

Subtracting photons from a two-mode squeezed state is a well-known method to increase entanglement. We analyse different strategies of local photon subtraction from a two-mode squeezed state in terms of entanglement gain and success probability. We develop a general framework that incorporates imperfections and losses in all stages of the process: before, during, and after subtraction. By combining all three effects into a single efficiency parameter, we provide analytical and numerical results for subtraction strategies using photon-number-resolving and threshold detectors. We compare the entanglement gain afforded by symmetric and asymmetric subtraction scenarios across the two modes. For a given amount of loss, we identify an optimised set of parameters, such as initial squeezing and subtraction beam splitter transmissivity, that maximise the entanglement gain rate. We identify regimes for which asymmetric subtraction of different Fock states on the two modes outperforms symmetric strategies. In the lossless limit, subtracting a single photon from one mode always produces the highest entanglement gain rate. In the lossy case, the optimal strategy depends strongly on the losses on each mode individually, such that there is no general optimal strategy. Rather, taking losses on each mode as the only input parameters, we can identify the optimal subtraction strategy and required beam splitter transmissivities and initial squeezing parameter. Finally, we discuss the implications of our results for the distillation of continuous-variable quantum entanglement., Comment: 13 pages, 11 figures. Updated version for publication

We introduce a new protocol in continuous variable entanglement distillation that requires only linear temporal and constant physical or spatial resources.Compared with the existing protocols, our protocol uses atom-photon entanglement to substitute for atom-atom entanglement in existing protol, which will not only save the number of quantum memories, but also has the advantages in operation efficiency and temporal saving. The distillation can be realized by a fixed model of iterations, in which only three quantum memories and photon detectors are required., Comment: 5 pages,6 figures

Large-scale quantum-correlated networks could transform technologies ranging from communications and cryptography to computation, metrology, and simulation of novel materials. Critical to achieving such quantum enhancements is distributing high-quality entanglement between distant nodes. This is made possible in the unavoidable presence of decoherence by entanglement distillation. However, current versions of this protocol are prohibitively costly in terms of resources. We introduce a new scheme for continuous-variable entanglement distillation that requires only linear temporal and constant physical or spatial resources, both of which are exponential improvements over existing protocols. Our scheme uses a fixed module - an entanglement distillery - comprising only four quantum memories of at most 50 % storage efficiency and allowing a feasible experimental implementation. Tangible quantum advantages are obtained by using non-ideal quantum memories outside their conventional role of storage. By creating, storing and processing information in the same physical space, the scheme establishes a potentially valuable technique for designing stable, scalable protocols across different quantum technologies., Comment: 5 + 3 figures, 5 + 4 pages

Loss is a critical roadblock to achieving photonic quantum-enhanced technologies. We explore a modular platform for implementing integrated photonics experiments and consider the effects of loss at different stages of these experiments, including state preparation, manipulation and measurement. We frame our discussion mainly in the context of quantum sensing and focus particularly on the use of loss-tolerant Holland-Burnett states for optical phase estimation. In particular, we discuss spontaneous four-wave mixing in standard birefringent fibre as a source of pure, heralded single photons and present methods of optimising such sources. We also outline a route to programmable circuits which allow the control of photonic interactions even in the presence of fabrication imperfections and describe a ratiometric characterisation method for beam splitters which allows the characterisation of complex circuits without the need for full process tomography. Finally, we present a framework for performing state tomography on heralded states using lossy measurement devices. This is motivated by a calculation of the effects of fabrication imperfections on precision measurement using Holland-Burnett states., Comment: 19 pages, 7 figures