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Planar, two-dimensional, two-colour, time-resolved laser-induced incandescence (2D-2C-TiRe-LII) is employed to investigate the formation of soot in a standard methane laminar diffusion flame for the first time. The work builds on previous developments in 2D LII by time-resolving the signal decay by shifting the gating time of ICCD cameras. The two-colour configuration allows application of the technique to extract the initial temperature of soot particles immediately after the laser pulse, instead of relying on estimates of the soot absorption coefficient, thus allowing higher accuracy in the determination of very small particle sizes produced in methane flames, using a minimum error approach. The technique is combined with a previous work on Continuous Wave Laser Cavity Extinction (CW-LCE) to allow absolute measurements of sub-ppm low soot volume fractions with very small particle sizes.

Multi-pass cavity line-of-sight extinction (MPC-LOSE) and laser- induced incandescence (LII) techniques are deployed to measure the soot volume fraction in a series of nitrogen-diluted flames, which produce only ppm volume mass fractions of soot. The separate suppression effects on soot formation of direct fuel dilution and indirect effects of temperature and res- idence time are interpreted by using a numerically calculated flow velocity and temperature field using a one-step fast chemistry model. The experi- mentally determined rate of soot formation is shown to obey approximately the same function of the local temperature for all dilution cases. The results show that a simple one-step reaction model using previously measured acti- vation energies can account for the dilution effect with good accuracy. The results show that the direct effect of dilution on concentration is comparable to the effects of changing the temperature estimated local temperature and residence time.

This work presents simultaneous 2D temperature and velocity measurements on a heated jet using two non-intensified cameras to realize thermographic PIV. In contrast to previous studies which use separate PIV cameras and LIP cameras, the present experiment uses only a double-pulsed UV laser and two low-speed CCD cameras running in double-frame mode, greatly simplifying the setup. The intensity ratio is calculated based on the image pair recorded at two spectral lines for thermography, while the cross-correlation is performed over the two consecutive frames for PIV. A method is proposed to correct for the effects of non-uniform spatial distribution of laser fluence on the intensity ratio, by including the laser fluence into the calibration function. The laser sheet energy profiles are measured and the intensity ratio is translated into temperature according to the local laser fluence and two-colour ratio. The temperature accuracy using this technique is estimated as 3 K at 410 K, by comparing the mean temperature field with the result provided by a thermocouple. Simultaneous 2D temperature and velocity fields are presented for a simple heated jet, demonstrating the expected similarities. The demonstration shows the potential of thermographic PIV in the investigation fundamental problems on turbulent flows, and shows that the technique can be improved through the availability of a dual-cavity UV laser.

Accurate measurement techniques for in situ determination of soot are necessary to understand and monitor the process of soot particle production. One of these techniques is line-of-sight extinction, which is a fast, low-cost and quantitative method to investigate the soot volume fraction in flames. However, the extinction-based technique suffers from relatively high measurement uncertainty due to low signal-to-noise ratio, as the single-pass attenuation of the laser beam intensity is often insufficient. Multi-pass techniques can increase the sensitivity, but may suffer from low spatial resolution. To overcome this problem, we have developed a high spatial resolution laser cavity extinction technique to measure the soot volume fraction from low-soot-producing flames. A laser beam cavity is realised by placing two partially reflective concave mirrors on either side of the laminar diffusion flame under investigation. This configuration makes the beam convergent inside the cavity, allowing a spatial resolution within 200 μm, whilst increasing the absorption by an order of magnitude. Three different hydrocarbon fuels are tested: methane, propane and ethylene. The measurements of soot distribution across the flame show good agreement with results using laser-induced incandescence (LII) in the range from around 20 ppb to 15 ppm.

The generation of a temperature disturbance in a flow is accompanied by the production of acoustic waves (direct noise), and of an entropy perturbation. If this entropy perturbation is accelerated or decelerated (as is the case through a nozzle or flow restriction), additional acoustic waves are generated (indirect noise). Several studies have demonstrated this mechanism in controlled conditions by using Entropy Wave Generators, in which entropy waves are generated and convected through a nozzle, leading to direct and indirect noise. An analytical analysis of the direct and indirect noise produced by the generation and acceleration of entropy waves in a reflective environment is presented. The e ect of reverberation (repeated acoustic reflections) on low-frequency perturbations (characteristic of Entropy Wave Generators) is determined analytically. These results are then implemented in a set of limit cases, showing the limit behaviours of such systems. The analytical model is applied to the case of the Cambridge Entropy Wave Generator experiment, in which entropy waves are generated by an electric heater and accelerated through a subsonic ori ce plate. Due to the clear time separation of direct and indirect noise in the experimental results, direct and indirect noise transfer functions can be extracted from the experimental data for the rst time, and compared directly with existing theoretical models. The backward-propagating indirect noise generated at an ori ce plate is shown to be signi cantly higher than predicted by existing theoretical models for isentropic nozzles., EPSRC EP/K02924X/1.

Quasi-instantaneous Mie scattering measurements were conducted to determine the flame surface location using two orthogonal planes to obtain the 3D orientation and measurement of 3D flame surface density (FSD) on a stabilised piloted Bunsen burner with turbulence levels of 1 to 2.5 times the laminar flame speed. A double-pulsed 527 nm high-frequency laser (part of a high-frequency particle image velocimetry dual-head setup) was split into two separated laser beams through a polarizer to generate laser sheets at 3 kHz on a vertical plane and a horizontal plane. The vertical plane across the centerline of the Bunsen-stabilized flame was kept constant, whilst the height of the horizontal plane was adjusted from the base of the flame for different heights. The flame edge was defined as the location where droplet tracers disappear, and calculated based on the local change in the number density of the flame edge. Projections of the flame normal vector onto two measurement planes were used to calculate directing angles on each plane, and the 3D FSD was estimated based on the measured angles at the intersecting lines of two planes. A comparison of the 2D to 3D FSD magnitudes was made, for cases with and without mean angle corrections. The results show that the 2D FSD approximations are lower than the 3D measurements by a factor of 20-30% if uncorrected, and up to 28% after corrections.

We review the state of the art in measurements and simulations of the behavior of premixed laminar and turbulent flames, subject to differential diffusion, stretch and curvature. The first part of the paper reviews the behavior of premixed laminar flames subject to flow stretch, and how it affects the accuracy of measurements of unstrained laminar flame speeds in stretched and spherically propagating flames. We then examine how flow field stretch and differential diffusion interact with flame propagation, promoting or suppressing the onset of thermodiffusive instabilities. Secondly, we survey the methodology for and results of measurements of turbulent flame speeds in the light of theory, and identify issues of consistency in the definition of mean flame speeds, and their corresponding mean areas. Data for methane at a single operating condition are compared for a range of turbulent conditions, showing that fundamental issues that have yet to be resolved for Bunsen and spherically propagating flames. Finally, we consider how the laminar flame scale response of flames to flow perturbations interacting with differential diffusion leads to very different outcomes to the overall sensitivity of the burning rate to turbulence, according to numerical simulations (DNS). The paper concludes with opportunities for future measurements and model development, including the perennial recommendation for robust archival databases of experimental and DNS results for future testing of models.

© 2018 The Combustion Institute. Biodiesel and blends with petroleum diesel have shown their potential as renewable alternative fuels for engines, with additional benefits of low particulate matter and low sulfate emissions. In this paper we measure the soot volume fraction produced by three different methyl esters processed biodiesels (extracted from palm (PME), soy (SME) and coconut (CME)), and their blends with petroleum diesel, in a series of co-flow stabilized laminar pool flames, using laser induced-incandescence (LII) and laser extinction optical methods. The soot volume fraction measurement results show that all neat biodiesels produce only up to 33% of the total soot volume compared to pure diesel, and that the total soot volume correlates directly with the degree of unsaturation of the biodiesels. Blending leads to approximately linear behaviour of total soot volume, with a shift in slope with smaller sensitivity towards neat diesel.

Indirect noise generated by the acceleration of synthetic compositional and entropic perturbations through non-isentropic nozzles is measured experimentally. A physics-based analytical low-order model to evaluate the indirect noise generated by non-isentropic compact nozzles is developed and validated with experimental measurements. A one-dimensional model for describing the waves generated by the addition of mass, momentum, energy and species to a steady flow in an entropy and composition wave generator is presented. The transfer functions describing the multiple reflections of acoustic waves in an enclosed environment are derived. This analytical framework allows unambiguous identification and isolation of the experimental direct and indirect noise generated by the injection of helium, methane, argon or carbon dioxide into a flow duct. Experimental data show that entropic and compositional noise make a significant contribution to the overall pressure traces acquired in the entropy generator. Moreover, it is demonstrated that the isentropic modelling assumption is inadequate to capture the experimental behaviour, while the analytical model for non-isentropic nozzles successfully describes the direct and indirect noise transfer functions. The disregard for the compositional contribution and the unjustified use of the isentropic assumption can provide significantly inaccurate noise predictions. This work shows that compositional noise, as well as non-isentropicity in the system, should be considered in future thermoacoustic and combustion noise models.

The present research deals with a hybrid combustion of aluminum/boron dust particles in a heterogeneous quiescent reaction medium with spatially discrete heat sources. A developed thermal model is employed to estimate flame propagation speed in a reaction medium. The burning velocity and minimum ignition energy are studied parametrically as a function of dust concentration and particle diameter for different percentages of boron powder in a hybrid mixture of aluminum/boron dust cloud. The model shows that the addition of boron powder as a component of the mixture decreases the burning rate and causes a higher amount of minimum ignition energy needed for ignition, owing to the role of boron as a heat sink. Comparison of the simulation results with the available experimental data shows that the model captures the flame propagation speed as a function of particle concentration, except at very low concentrations.