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In contrast to the high performances of long-range, high-speed optical information transfer, optical information processing remains outperformed by electronic microprocessing. The two mains reasons are the lack of gain medium that hampers the development of an optical analogue of the transistor and the lack of compactness of the approaches proposed so far. Here, we demonstrate a new concept of the design of all-optical elementary computing units based on the shaping of plasmonic modal landscape in micrometric on-chip 2D cavities to realize reconfigurable Arithmetic and Logic Units (ALU). Our interconnect-free devices perform multi-bit logic gate functions in a single cavity without ALU cascading, therefore obviating loss in vias and so the need for gain to restore the binary signal. Moreover, an astute cavity design allows to reconfigure a single cavity into multiple logic functions, including a first full adder. The main challenge on the way to increasing the functional Boolean complexity is the design of the cavity shape and of the excitation/detection parameters for which an approach based on artificial intelligence will be implemented.

ITO is a transparent conductive material commonly used in everyday life and for its potential in material research. In nonlinear optics for instance, ITO has shown great capabilities for harmonic generation in its epsilon-near-zero configuration. In this article, we demonstrate a completely new nonlinear behaviour from ITO thin layers. After a Ga-Focused Ion Beam (FIB) milling of the thin film, we observe nonlinear photoluminescence produced for tightly focused femtosecond pulses. The signal shares strong similarities with that commonly detected from noble metals. We show that the arising of this nonlinear photoluminescence originates from the radiative decay of metal-like hot electron distribution in the material and is associated to a modification of the optical properties by the Ga ions.

We aim at controlling the spatial distribution of nonlinear photoluminescence in a shaped micrometer-size crystalline gold flake. Interestingly, the underlying surface plasmon modal landscape sustained by this mesoscopic structure can be advantageously used to generate nonlinear photoluminescence (nPL) in remote locations away from the excitation spot. By controlling the modal pattern, we show that the delocalized nonlinear photoluminescence intensity can be redistributed spatially. This is first accomplished by changing the polarization orientation of the pulsed laser excitation in order to select a subset of available surface plasmon modes within a continuum. We then propose a second approach to redistribute the nPL within the structure by implementing a phase control of the plasmon interference pattern arising from a coherent two-beam excitation. Control and engineering of the nonlinear photoluminescence spatial extension is a prerequisite for deploying the next generation of plasmonic-enabled integrated devices relying on hot carriers.