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Laser technologies improved after the understanding of the Chirped Pulse Amplification (CPA) which allows energetic laser beams to be compressed to tens of femtosecond (fs) pulse durations and focused to few $\mu$m. Protons of tens of MeV can be accelerated using for instance the Target Normal Sheath Acceleration (TNSA) method and focused on secondary targets. In such conditions, nuclear reactions can occur and radioisotopes relevant for medical purposes be produced. High repetition lasers can be used to produce enough isotopes for medical applications. This route is competitive to conventional methods mostly based on accelerators. In this paper we study the production of $^{67}$Cu, $^{63}$Zn, $^{18}$F and $^{11}$C currently used in positron emission tomography (PET) and other applications. At the same time, we study the reaction $^{10}$B(p,$\alpha$)$^{7}$Be and $^{70}$Zn(p,4n)$^{67}$Ga to put further constraints to the proton distributions at different angles and to the reaction $^{11}$B(p,$\alpha$)$^{8}$Be relevant for energy production. The experiment was performed at the 1 petawatt (PW) laser facility at Vega III located in Salamanca-Spain. Angular distributions of radioisotopes in the forward (with respect to the laser direction) and backward directions were measured using a High Purity Germanium Detector (HPGE). Our results are reasonably reproduced by the numerical estimates following the approach of Kimura et al. (NIMA637(2011)167)

Ion acceleration from gaseous targets driven by relativistic-intensity lasers was demonstrated as early as the late 90s, yet most of the experiments conducted to date have involved picosecond-duration, Nd:glass lasers operating at low repetition rate. Here, we present measurements on the interaction of ultraintense ($\sim 10^{20}\,\rm W\,cm^{-2}$, 1 PW), ultrashort ($\sim 70\,\rm fs$) Ti:Sa laser pulses with near-critical ($\sim 10^{20}\,\rm cm^{-3}$) helium gas jets, a debris-free targetry compatible with high ($\sim 1\,\rm Hz$) repetition rate operation. We provide evidence of $\alpha$ particles being forward accelerated up to $\sim 2.7\,\rm MeV$ energy with a total flux of $\sim 10^{11}\,\rm sr^{-1}$ as integrated over $>0.1 \,\rm MeV$ energies and detected within a $0.5\,\rm mrad$ solid angle. We also report on on-axis emission of relativistic electrons with an exponentially decaying spectrum characterized by a $\sim 10\,\rm MeV$ slope, i.e., five times larger than the standard ponderomotive scaling. The total charge of these electrons with energy above 2 MeV is estimated to be of $\sim 1 \,\rm nC$, corresponding to $\sim 0.1\,\%$ of the laser drive energy. In addition, we observe the formation of a plasma channel, extending longitudinally across the gas density maximum and expanding radially with time. These results are well captured by large-scale particle-in-cell simulations, which reveal that the detected fast ions most likely originate from reflection off the rapidly expanding channel walls. The latter process is predicted to yield ion energies in the MeV range, which compare well with the measurements. Finally, direct laser acceleration is shown to be the dominant mechanism behind the observed electron energization.

We present a parametric study based on 1-D particle-in-cell (PIC) simulations conducted with the objective of understanding the interaction of intense lasers with near-critical non-uniform density gas targets. Specifically, we aim to find an optimal set of experimental parameters regarding the interaction of a $\lambda_L$ = 0.8 $\mu$m, $I_L =10^{20}$ W/cm$^2$ ($a_0 = 8.8$), $\tau_L = 30$ fs laser pulse with a near-critical non-uniform pure nitrogen gas profile produced by a non commercial gas nozzle. The PIC code Calder developed at CEA was used, and both the maximum electron density and the direct laser contribution to ion acceleration were studied. Shock formation was achieved for a peak electron density $n_e$ ranging between 0.35 $n_c$ and 0.7 $n_c$. In this density interval, the survival of a percentage of the laser pulse until the gas density peak, while being strongly absorbed ($>$90$\%$) and creating a hot electron population in the gas up-ramp, is singled out as a necessary condition for shock formation. Moreover, the laser absorption must give rise to a super ponderomotive heating of the target electrons in order to launch an electrostatic shock inside the plasma. The direct laser effect on ion acceleration consists in a strong initial density perturbation that enhances charge separation while the electron pressure gradients are identified as fundamental for shock formation. The production of a controlled and repetitive gas profile as well as the possibility of performing measurements with statistical meaning are highlighted as fundamental for conducting a thorough experimental study., Comment: 14 pages, 13 figures

Strong electromagnetic pulses (EMP) are generated from intense laser interactions with solid-density targets, and can be guided by the target geometry, specifically through conductive connections to the ground. We present an experimental characterization, by time- and spatial-resolved proton deflectometry, of guided electromagnetic discharge pulses along wires including a coil, driven by 0.5 ps, 50 J, 1e19 W/cm2 laser pulses. Proton-deflectometry data allows to time-resolve first the EMP due to the laser-driven target charging and then the return EMP from the ground through the conductive target stalk. Both EMPs have a typical duration of tens of ps and correspond to currents in the kA-range with electric-field amplitudes of multiple GV/m. The sub-mm coil in the target rod creates lensing effects on probing protons, due to both magnetic- and electric-field contributions. This way, protons of 10 MeV-energy range are focused over cm-scale distances. Experimental results are supported by analytical modelling and high-resolution numerical particle-in-cell simulations, unraveling the likely presence of a surface plasma, which parameters define the discharge pulse dispersion in the non-linear propagation regime.

We present experimental results for the controlled mitigation of electromagnetic pulses (EMP) produced in interactions of the 1PW high-power 30fs Ti:Sa laser VEGA-3 with matter. This study aims at the band of very high frequencies (VHF), notably hundreds of MHz, comprising the fundamental cavity modes of the rectangular VEGA-3 vacuum chamber. We demonstrate mode suppression by tailoring of the laser-produced space charge distribution., Comment: submitted to the proceedings of the 48th EPS Conference on Plasma Physics

We experimentally study entangled two-photon absorption in Rhodamine 6G as a function of the spatial properties of a high flux of broadband entangled photon pairs. We first demonstrate a key signature dependence of the entangled two-photon absorption rate on the type of entangled pair flux attenuation: linear, when the laser pump power is attenuated, and quadratic, when the pair flux itself experiences linear loss. We then perform a fluorescence-based Z-scan measurement to study the influence of beam waist size on the entangled two-photon absorption process and compare this to classical single- and two-photon absorption processes. We demonstrate that the entangled two-photon absorption shares a beam waist dependence similar to that of classical two-photon absorption. This result presents an additional argument for the wide range of contrasting values of quoted entangled two-photon absorption cross-sections of dyes in literature.

A novel detector based on a polycrystalline diamond sensor is here employed in an advanced Time-Of-Flight scheme for the characterization of energetic ions accelerated during laser-matter interactions. The optimization of the detector and of the advanced TOF methodology allow to obtain signals characterized by high signal-to-noise ratio and high dynamic range even in the most challenging experimental environments, where the interaction of high-intensity laser pulses with matter leads to effective ion acceleration, but also to the generation of strong Electromagnetic Pulses (EMPs) with intensities up to the MV/m order. These are known to be a serious threat for the fielded diagnostic systems. In this paper we report on the measurement performed with the PW-class laser system Vega 3 at CLPU (30 J energy, 10^21 W/cm2 intensity, 30 fs pulses) irradiating solid targets, where both tens of MeV ions and intense EMP fields were generated. The data were analyzed to retrieve a calibrated proton spectrum and in particular we focus on the analysis of the most energetic portion (E > 5.8 MeV) of the spectrum showing a procedure to deal with the intrinsic lower sensitivity of the detector in the mentioned spectral-range.

We demonstrate laser-driven Helium ion acceleration with cut-off energies above 25 MeV and peaked ion number above $10^8$ /MeV for 22(2) MeV projectiles from near-critical density gas jet targets. We employed shock gas jet nozzles at the high-repetition-rate (HRR) VEGA-2 laser system with 3 J in pulses of 30 fs focused down to intensities in the range between $9\times10^{19}$ W/cm$^2$ and $1.2\times10^{20}$ W/cm$^2$. We demonstrate acceleration spectra with minor shot-to-shot changes for small variations in the target gas density profile. Difference in gas profiles arise due to nozzles being exposed to a experimental environment, partially ablating and melting., Comment: 22 pages, 28 figures

We report on the development of a highly directional, narrow energy band, short time duration proton beam operating at high repetition rate, suitable for measurements of stopping power in high energy density plasmas as well as other applications. The protons are generated with an ultrashort-pulse laser interacting with a solid target and converted to a pencil-like narrow-band beam using a compact magnet-based energy selector. We experimentally demonstrate the production of a proton beam with an energy of 500 keV and energy spread well below 10%, and a pulse duration of 260 ps. The energy loss of this beam is measured in a 2 ${\mu}$m thick solid Mylar target and found to be in within 1% of theoretical predictions. The short time duration of the proton pulse makes it particularly well suited for applications involving the probing of highly transient plasma states produced in laser-matter interaction experiments, in particular measurements of proton stopping power.

We theoretically investigate the generation of two entangled beams of light in the process of single-pass type-I noncollinear frequency degenerate parametric downconversion with an ultrashort pulsed pump. We find the spatio-temporal squeezing eigenmodes and the corresponding squeezing eigenvalues of the generated field both numerically and analytically. The analytical solution is obtained by modeling the joint spectral amplitude of the field by a Gaussian function in curvilinear coordinates. We show that this method is highly efficient and is in a good agreement with the numerical solution. We also reveal that when the total bandwidth of the generated beams is sufficiently high, the modal functions cannot be factored into a spatial and a temporal parts, but exhibit a spatio-temporal coupling, whose strength can be increased by shortening the pump., Comment: accepted version, 19 pages, 10 figures

Among the existing elemental characterization techniques, Particle Induced X-ray Emission (PIXE) and Energy Dispersive X-ray (EDX) spectroscopy are two of the most widely used in different scientific and technological fields. Here we present the first quantitative laser-driven PIXE and laser-driven EDX experimental investigation performed at the Centro de L\'aseres Pulsados in Salamanca. Thanks to their potential for compactness and portability, laser-driven particle sources are very appealing for materials science applications, especially for materials analysis techniques. We demonstrate the possibility to exploit the X-ray signal produced by the co-irradiation with both electrons and protons to identify the elements in the sample. We show that, using the proton beam only, we can successfully obtain quantitative information about the sample structure through laser-driven PIXE analysis. These results pave the way towards the development of a compact and multi-functional apparatus for the elemental analysis of materials based on a laser-driven particle source., Comment: This project has received funding from the European Research Council (ERC) under the European Union's Horizon 2020 research and innovation programme (ENSURE grant agreement No. 647554). Submitted to Science Advances on 20th May 20

The double laser pulse approach to relativistic electron beam (REB) collimation has been investigated at the LULI-ELFIE facility. In this scheme, the magnetic field generated by the first laser-driven REB is used to guide a second delayed REB. We show how electron beam collimation can be controlled by properly adjusting laser parameters. By changing the ratio of focus size and the delay time between the two pulses we found a maximum of electron beam collimation clearly dependent on the focal spot size ratio of the two laser pulses and related to the magnetic field dynamics. Cu-K alpha and CTR imaging diagnostics were implemented to evaluate the collimation effects on the respectively low energy (< 100 keV) and high energy (> MeV) components of the REB.

We present a scintillator based detector able to measure both spatial and energy information at High repetition rate (HRR) with a relatively simple design. It has been built at the Center of Pulsed Laser (CLPU) in Salamanca and tested in the proton accelerator at the Centro de Micro-Analisis de Materiales (CMAM) in Madrid. The detector has been demonstrated to work in HRR mode by reproducing the performance of the radiochromic film detector. It represents a new class of on-line detectors for Laser-plasma physics experiments in the new emerging High Power and HRR laser systems., Comment: 6 pages, 10 figures

We study the Bloch-Messiah reduction of parametric downconversion of light in the pulsed regime with a nondegenerate phase matching providing generation of twin beams. We find that in this case every squeezing eigenvalue has multiplicity at least two. We discuss the problem of ambiguity in the definition of the squeezing eigenmodes in this case and develop two approaches to unique determination of the latter. First, we show that the modal functions of the squeezing eigenmodes can be tailored from the Schmidt modes of the signal and idler beams. Alternatively, they can be found as a solution of an eigenvalue problem for an associated Hermitian squeezing matrix. We illustrate the developed theory by an example of frequency non-degenerate collinear twin beams generated in beta barium borate crystal. On this example we demonstrate how the squeezing eigenmodes can be approximated analytically on the basis of the Mehler's formula, extended to complex kernels. We show how the multiplicity of the eigenvalues and the structure of the eigenmodes are changed when the phase matching approaches the degeneracy in frequency., Comment: 18 pages, 9 figures, 1 theorem

A promising prototype of a highly adjustable Kirkpatrick-Baez (KB) microscope has been designed, built and tested in a number of laser driven x-ray experiments using the high power (200TW) VEGA-2 laser system of the Spanish Centre for Pulsed Lasers (CLPU). The presented KB version consists of two, perpendicularly mounted, 500{\mu}m thick Silicon wafers, coated with a few tens of nm layer of Platinum unlike the conventional, coated, millimetre thick glass substrates, affording more bending flexibility and large adjustment range. According to simulations, and based on total external reflection, this KB offers a broad-band multi-keV reflection spectra, allowing more spectral tunablity than conventional Bragg crystals. In addition to be vacuum compatible, the prototype is characterised by a relatively small size (21cm x 31cm x 27cm) and permits remote control and modification of both the radius of curvature (down to 10m) and the grazing incidence angle (up to 60mrad). A few examples of focusing performance tests, limitations and experimental campaign results are discussed.

The Centro de Laseres Pulsados in Salamanca Spain has recently started operation phase and the first User access period on the 6 J 30 fs 200 TW system (VEGA 2) already started at the beginning of 2018. In this paper we report on two commissioning experiments recently performed on the VEGA 2 system in preparation for the user campaign. VEGA 2 system has been tested in different configurations depending on the focusing optics and targets used. One configuration (long focal length f=130 cm) is for under-dense laser-matter interaction where VEGA 2 is focused onto a low density gas-jet generating electron beams (via laser wake field acceleration mechanism) with maximum energy up to 500 MeV and an X-ray betatron source with a 10 keV critical energy. A second configuration (short focal length f=40 cm) is for over-dense laser-matter interaction where VEGA 2 is focused onto an 5 microns thick Al target generating a proton beam with a maximum energy of 10 MeV and average energy of 7-8 MeV and temperature of 2.5 MeV. In this paper we present preliminary experimental results.