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The Zirconium (Z = 40) isotopic chain has attracted interest for more than four decades. The abrupt lowering of the energy of the first $2^+$ state and the increase in the transition strength B(E2; $2_1^\rightarrow 0_1^+$ going from $^{98}$Zr to $^{100}$Zr has been the first example of "quantum phase transition" in nuclear shapes, which has few equivalents in the nuclear chart. Although a multitude of experiments have been performed to measure nuclear properties related to nuclear shapes and collectivity in the region, none of the measured lifetimes were obtained using the Recoil Distance Doppler Shift method in the $\gamma\gamma$-coincidence mode where a gate on the direct feeding transition of the state of interest allows a strict control of systematical errors. This work reports the results of lifetime measurements for the first yrast excited states in $^{98-104}$Zr carried out to extract reduced transition probabilities. The new lifetime values in $\gamma\gamma$-coincidence and $\gamma$-single mode are compared with the results of former experiments. Recent predictions of the Interacting Boson Model with Configuration Mixing, the Symmetry Conserving Configuration Mixing model based on the Hartree-Fock-Bogoliubov approach and the Monte Carlo Shell Model are presented and compared with the experimental data.

Dosimetry in BNCT poses significant challenges due to the indirect effect of neutrons interacting with elements within the body and uncertainties associated with the uptake of boron compounds used in clinical practice. Current treatment planning relies on unconventional estimates of boron tumor uptake derived from prior PET scans and thus, an online boron-uptake monitor would be highly convenient. This work presents the first pilot experiments carried out at ILL-Grenoble with the high-efficiency Compton camera i-TED, hereby aiming at demonstrating its applicability for BNCT dosimetry by introducing real-time measurement of the boron concentration and imaging capabilities of spatial dose distribution. In this experiment, we measured the $^{10}$B uptake of different cancer cells of tongue squamous cell carcinoma, malignant melanoma and glioblastoma treated with BPA (80~ppm of $^{10}$B). The samples were irradiated with the thermal neutron spectrum of ILL-Grenoble and the 478keV $\gamma$-rays from the $^{7}$Li de-excitation after the neutron-boron reaction were registered both with the Compton imager and the high-sensitivity FIPPS HPGe array. These series of measurements allowed us to demonstrate the imaging capabilities of the Compton imaging device for this type of application, as well as to assess its sensitivity, which was found to be below 1 $\mu$g of $^{10}$B., Comment: 10 pages, 12 figures, submitted to the Special Issue of Applied Radiation and Isotopes associated to the 20th International Congress on Neutron Capture Therapy (20th ICNCT)

The first systematic experimental study of the neutron-rich Br isotopes with two complementary state-of-the-art techniques is presented. These isotopes have been populated in the fission process at two different facilities, GANIL and ILL. New spectroscopic information has been obtained for odd-even $^{87-93}$Br isotopes and the experimental results have been compared with state-of-the-art Large-Scale Shell-Model and DNO Shell-Model calculations. As a result of such theoretical approaches, a transition from prolate ($^{87,89}$Br) to oblate ($^{91,93}$Br) shapes is obtained from the subtle balance between proton and neutron quadrupole deformations, as a clear signature of pseudo-SU3 quadrupole regime., Comment: 17 pages, 24 figures, 5 tables

The excited states of unstable $^{20}$O were investigated via $\gamma$-ray spectroscopy following the $^{19}$O$(d,p)^{20}$O reaction at 8 $A$MeV. By exploiting the Doppler Shift Attenuation Method, the lifetime of the 2$^+_2$ and 3$^+_1$ states were firmly established. From the $\gamma$-ray branching and E2/M1 mixing ratios for transitions deexciting the 2$^+_2$ and 3$^+_1$ states, the B(E2) and B(M1) were determined. Various chiral effective field theory Hamiltonians, describing the nuclear properties beyond ground states, along with a standard USDB interaction, were compared with the experimentally obtained data. Such a comparison for a large set of $\gamma$-ray transition probabilities with the valence space in medium similarity renormalization group ab-initio calculations was performed for the first time in a nucleus far from stability. It was shown that the ab-initio approaches using chiral EFT forces are challenged by detailed high-precision spectroscopic properties of nuclei. The reduced transition probabilities were found to be a very constraining test of the performance of the ab-initio models., Comment: Supplemental Material available

AGATA is a modern $\gamma$-ray spectrometer for in-beam nuclear structure studies, based on $\gamma$-ray tracking. Since more than a decade, it has been operated performing experimental physics campaigns in different international laboratories (LNL, GSI, GANIL). This paper reviews the obtained results concerning the performances of $\gamma$-ray tracking in AGATA and associated algorithms. We discuss $\gamma$-ray tracking and algorithms developed for AGATA. Then, we present performance results in terms of efficiency and peak-to-total for AGATA. The importance of the high effective angular resolution of $\gamma$-ray tracking arrays is emphasised, e.g. with respect to Doppler correction. Finally, we briefly touch upon the subject of $\gamma$-ray imaging and its connection to $\gamma$-ray tracking.

Classical novae are thermonuclear explosions in stellar binary systems, and important sources of $^{26}$Al and $^{22}$Na. While gamma rays from the decay of the former radioisotope have been observed throughout the Galaxy, $^{22}$Na remains untraceable. The half-life of $^{22}$Na (2.6 yr) would allow the observation of its 1.275 MeV gamma-ray line from a cosmic source. However, the prediction of such an observation requires good knowledge of the nuclear reactions involved in the production and destruction of this nucleus. The $^{22}$Na($p,\gamma$)$^{23}$Mg reaction remains the only source of large uncertainty about the amount of $^{22}$Na ejected. Its rate is dominated by a single resonance on the short-lived state at 7785.0(7) keV in $^{23}$Mg. In the present work, a combined analysis of particle-particle correlations and velocity-difference profiles is proposed to measure femtosecond nuclear lifetimes. The application of this novel method to the study of the $^{23}$Mg states, combining magnetic and highly-segmented tracking gamma-ray spectrometers, places strong limits on the amount of $^{22}$Na produced in novae, explains its non-observation to date in gamma rays (flux < 2.5x$10^{-4}$ ph/(cm$^2$s)), and constrains its detectability with future space-borne observatories., Comment: 18 pages, 3 figures, 1 table

Simulations of explosive nucleosynthesis in novae predict the production of $^{22}$Na, a key astronomical observable to constrain nova models. Its gamma-ray line at 1.275 MeV has not yet been observed by the gamma-ray space telescopes. The $^{20}$Ne/$^{22}$Ne ratio in presolar grains, a possible tool to identify nova grains, also depends on $^{22}$Na produced. Uncertainties on its yield in classical novae currently originate from the rate of the $^{22}$Na(p, $\gamma$)$^{23}$Mg reaction. At peak novae temperatures, this reaction is dominated by a resonance at E$_{\text{R}}$=0.204 MeV, corresponding to the $E_x$=7.785 MeV excited state in $^{23}$Mg. The resonance strengths measured so far disagree by one order of magnitude. An experiment has been performed at GANIL to measure the lifetime and the proton branching ratio of this key state, with a femtosecond resolution for the former. The reactions populating states in $^{23}$Mg have been studied with a high resolution detection set-up, i.e. the particle VAMOS, SPIDER and gamma tracking AGATA spectrometers, allowing the measurements of lifetimes and proton branchings. We present here a comparison between experimental results and shell-model calculations, that allowed us to assign the spin and parity of the key state. Rather small values obtained for reduced $M1$ matrix elements, $|M(M1)|\lesssim 0.5$ $\mu_N$, and proton spectroscopic factors, $C^{2}S_{\text{p}}$<10$^{-2}$, seem to be beyond the accuracy of the shell model. With the reevaluated $^{22}$Na(p, $\gamma$)$^{23}$Mg rate, the $^{22}$Na detectability limit and its observation frequency from novae are found promising for the future space telescopes., Comment: 6 pages, 4 figures, proceedings of the conference Nuclear Physics in Astrophysics - X (NPA-X, Cern 2022), accepted in EPJ Web of Conferences

The structure of $^{83}$As, $^{85}$As and $^{87}$As have been studied in fusion-fission reaction $^{238}$U+$^9$Be. Fission fragments were identified in mass and atomic number using the VAMOS++ spectrometer and the coincident $\gamma$-rays were detected in the $\gamma$-ray tracking array AGATA. New transitions in $^{83}$As and $^{85}$As are reported and placed in the level schemes. A level scheme of the excited states in $^{87}$As is proposed for the first time. The data are interpreted in frame of Large-Scale Shell-Model calculations, SU3 symmetries and Beyond Mean-Field frameworks. A spherical regime at magic number $N$=50 is predicted and the location of the proton $g_{9/2}$ orbital is proposed for the first time. Development of collectivity in a prolate deformed, $\gamma$-soft regime in the open shell cases $^{85}$As and $^{87}$As, most neutron-rich isotopes beyond $N$=50, is concluded. Data and theoretical calculations give confidence to a relatively high extrapolated excitation energy about 4 MeV of the $9/2^+$ state in $^{79}$Cu, one proton above $^{78}$Ni.

High-resolution gamma-ray spectroscopy of 18N is performed with the Advanced GAmma Tracking Array AGATA, following deep-inelastic processes induced by an 18O beam on a 181Ta target. Six states are newly identified, which together with the three known excitations exhaust all negative-parity excited states expected in 18N below the neutron threshold. Spin and parities are proposed for all located states on the basis of decay branchings and comparison with large-scale shell-model calculations performed in the p-sd space, with the YSOX interaction. Of particular interest is the location of the 0^-_1 and 1^-_2 excitations, which provide strong constrains for cross-shell p-sd matrix elements based on realistic interactions, and help to simultaneously reproduce the ground and first-excited states in 16N and 18N, for the first time. Understanding the 18N structure may also have significant impact on neutron-capture cross-section calculations in r-process modeling including light neutron-rich nuclei.

The heaviest N=Z doubly-magic nucleus, $^{100}$Sn, and the neighboring nuclei offer unique opportunities to investigate the properties of nuclear interaction in extreme conditions. In particular, the Cd isotopes are expected to present features similar to those found in the Sn isotopic chain, since they have only two proton holes in the Z=50 shell. In this manuscript, the lifetime measurements of low-lying states in the even-mass $^{102-108}$Cd is presented. Thanks to the powerful detection capabilities of AGATA array and VAMOS++ spectrometer, the unusual employment of multi-nucleon transfer reactions permitted to investigate the first 2$^+$ and 4$^+$ states in all these nuclei, together with various deformed bands in $^{106}$Cd. The results were interpreted in the context of new state-of-the-art beyond-mean-field calculations, using the symmetry-conserving configuration-mixing approach. Despite the similarities in the electromagnetic properties of the low-lying states, there is a fundamental structural difference between the ground-state bands in the Z=48 and Z=50 isotopes. The comparison between experimental and theoretical results revealed a rotational character of the Cd nuclei, which have prolate-deformed ground states with $\beta_2 \approx 0.2$. At this deformation Z=48 becomes a closed-shell configuration, which is favored with respect to the spherical one., Comment: V1 : 14 pages, 12 figures. V2 : 16 pages, 11 figures. V3 : 16 pages, 11 figures (figure 11 corrected); triaxiality evaluated with "quadrupole sum rule". submitted to Phys.Rev.C

A novel Monte Carlo technique has been developed to determine lifetimes of excited states in the tens-to-hundreds femtoseconds range. The method is applied to low-energy heavy-ion binary reactions populating nuclei with complex velocity distributions. Its relevance is demonstrated in connection with the $^{18}$O(7.0 MeV/u) + $^{181}$Ta experiment, performed at GANIL with the AGATA+VAMOS+PARIS setup, to study neutron-rich O, C, N, ... nuclei. Excited states in $^{17}$O and $^{19}$O, with known lifetimes, are used to validate the method over the $\sim$20-400 fs lifetime-sensitivity range. Emphasis is given to the unprecedented position resolution provided by $\gamma$-tracking arrays, which turns out to be essential for reaching the required accuracy in Doppler-shift correction, at the basis of the detailed analysis of $\gamma$-ray lineshape and resulting state lifetime determination. The technique is anticipated to be an important tool for lifetime investigations in exotic neutron-rich nuclei, produced with intense ISOL-type beams.

We present recent results on the structure of the one-valence-particle $^{41}$Ca and $^{49}$Ca, and one-valence-hole $^{47}$Ca, nuclei. The isotopes of interest were populated via the cold-neutron capture reactions $^{40}$Ca(n,$\gamma$), $^{48}$Ca(n,$\gamma$) and $^{46}$Ca(n,$\gamma$), respectively. The experiments were performed at the Institut Laue-Langevin, within the EXILL campaign, which employed a large array of HPGe detectors. The $\gamma$ decay and level schemes of these nuclei were investigated by $\gamma$-ray coincidence relationships, leading to the identification of 41, 10, and 6 new transitions in $^{41}$Ca, $^{47}$Ca, and $^{49}$Ca, respectively. Branching ratios and intensities were extracted for the $\gamma$ decay from each state, and $\gamma$-ray angular correlations were performed to establish a number of transition multipolarities and mixing ratios, thus helping in the spin assignment of the states. The experimental findings are discussed along with microscopic, self-consistent beyond-mean-field calculations performed with the Hybrid Configuration Mixing model, based on a Skyrme SkX Hamiltonian. The latter suggests that a fraction of the low-spin states of the $^{41}$Ca, $^{49}$Ca, and $^{47}$Ca nuclei is characterized by the coexistence of either 2p-1h and 1p-2h excitations, or couplings between single-particle/hole degrees of freedom and collective vibrations (phonons) of the doubly-magic "core".

An extended investigation of the low-spin structure of the $^{65}$Ni nucleus was performed at the Institut Laue-Langevin, Grenoble, via the neutron capture reaction $^{64}$Ni(n,$\gamma$)$^{65}$Ni, using the FIPPS HPGe array. The level scheme of $^{65}$Ni was significantly expanded, with 2 new levels and 87 newly found transitions. Angular correlation analyses were also performed, allowing us to assign spins and parities for a number of states, and to determine multipolarity mixing ratios for selected $\gamma$ transitions. The low-energy part of the experimental level scheme (up to about 1.4 MeV) was compared with Monte Carlo Shell Model calculations, which predict spherical shapes for all states, apart from the 9/2$^+$ and the second excited 1/2$^-$ states of oblate deformation.

The performance of the Advanced GAmma Tracking Array (AGATA) at GANIL is discussed, on the basis of the analysis of source and in-beam data taken with up to 30 segmented crystals. Data processing is described in detail. The performance of individual detectors are shown. The efficiency of the individual detectors as well as the efficiency after $\gamma$-ray tracking are discussed. Recent developments of $\gamma$-ray tracking are also presented. The experimentally achieved peak-to-total is compared with simulations showing the impact of back-scattered $\gamma$ rays on the peak-to-total in a $\gamma$-ray tracking array. An estimate of the achieved position resolution using the Doppler broadening of in-beam data is also given. Angular correlations from source measurements are shown together with different methods to take into account the effects of $\gamma$-ray tracking on the normalization of the angular correlations., Comment: published in Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment

The low-spin structure of the semimagic 64Ni nucleus has been considerably expanded: combining four experiments, several 0+ and 2+ excited states were identified below 4.5 MeV, and their properties established. The Monte Carlo shell model accounts for the results and unveils an unexpectedly complex landscape of coexisting shapes: a prolate 0+ excitation is located at a surprisingly high energy (3463 keV), with a collective 2+ state 286 keV above it, the first such observation in Ni isotopes. The evolution in excitation energy of the prolate minimum across the neutron N = 40 subshell gap highlights the impact of the monopole interaction and its variation in strength with N.

The fusion and transfer induced fission reaction $^{9}$Be($^{238}$U,~f) with 6.2 MeV/u beam energy, using a unique setup consisting of AGATA, VAMOS++ and EXOGAM detectors, was used to populate through the fission process and study the neutron-rich $^{119,121}$In isotopes. This setup enabled the prompt-delayed $\gamma$-ray spectroscopy of isotopes in the time range of $100~\rm{ns} - 200~\mu\rm{s}$. In the odd-$A$ $^{119,121}$In isotopes, indications of a short half-life $19/2^{-}$ isomeric state, in addition to the previously known $25/2^{+}$ isomeric state, were observed from the present data. Further, new prompt transitions above the $25/2^{+}$ isomer in $^{121}$In were identified along with reevaluation of its half-life. The experimental data were compared with the theoretical results obtained in the framework of large-scale shell-model calculations in a restricted model space. The $\langle \pi g_{9/2} \nu h_{11/2};I \arrowvert \hat{\mathcal{H}}\arrowvert \pi g_{9/2} \nu h_{11/2};I\rangle$ two-body matrix elements of residual interaction were modified to explain the excitation energies and the $B(E2)$ transition probabilities in the neutron-rich In isotopes. The (i) decreasing trend of $E(29/2^{+}) - E(25/2^{+})$ in odd-In (with dominant configuration $\pi g_{9/2}^{-1}\nu h_{11/2}^{-2}$ and maximum aligned spin of $29/2^{+}$) and (ii) increasing trend of $E(27/2^{+}) - E(23/2^{+})$ in odd-Sb (with dominant configuration $\pi g_{7/2}^{+1}\nu h_{11/2}^{-2}$ and maximum aligned spin of $27/2^{+}$) with increasing neutron number could be understood as a consequence of hole-hole and particle-hole interactions, respectively., Comment: Accepted for publication in Phys. Rev. C

To test the predictive power of ab initio nuclear structure theory, the lifetime of the second 2+ state in neutron-rich 20O, tau(2+_2 ) = 150(+80-30) fs, and an estimate for the lifetime of the second 2+ state in 16C have been obtained, for the first time. The results were achieved via a novel Monte Carlo technique that allowed us to measure nuclear state lifetimes in the tens-to-hundreds femtoseconds range, by analyzing the Doppler-shifted gamma-transition line shapes of products of low-energy transfer and deep-inelastic processes in the reaction 18O (7.0 MeV/u) + 181Ta. The requested sensitivity could only be reached owing to the excellent performances of the AGATA gamma-tracking array, coupled to the PARIS scintillator array and to the VAMOS++ magnetic spectrometer. The experimental lifetimes agree with predictions of ab initio calculations using two- and three-nucleon interactions, obtained with the valence-space in-medium similarity renormalization group for 20O, and with the no-core shell model for 16C. The present measurement shows the power of electromagnetic observables, determined with high-precision gamma spectroscopy, to assess the quality of first-principles nuclear structure calculations, complementing common benchmarks based on nuclear energies. The proposed experimental approach will be essential for short lifetimes measurements in unexplored regions of the nuclear chart, including r-process nuclei, when intense ISOL-type beams become available.

The neutron-rich $^{122-131}$Sb isotopes were produced as fission fragments in the reaction $^{9}$Be($^{238}$U,~f) with 6.2 MeV/u beam energy. An unique setup, consisting of AGATA, VAMOS++ and EXOGAM detectors, was used which enabled the prompt-delayed gamma-ray ($\gamma$) spectroscopy of fission fragments in the time range of 100 ns - 200 $\mu$s. New isomers, prompt and delayed transitions were established in the even-A $^{122-130}$Sb isotopes. In the odd-A $^{123-131}$Sb isotopes, new prompt and delayed $\gamma$-ray transitions were identified, in addition to the confirmation of the previously known isomers. The half-lives of the isomeric states and the $B(E2)$ transition probabilities of the observed transitions depopulating these isomers were extracted. The experimental data was compared with the theoretical results obtained in the framework of Large-Scale Shell-Model (LSSM) calculations in a restricted model space. Modifications of several components of the shell model interaction were introduced to obtain a consistent agreement with the excitation energies and the $B(E2)$ transition probabilities in neutron-rich Sn and Sb isotopes. The isomeric configurations in Sn and Sb were found to be relatively pure. Further, the calculations revealed that the presence of a single valence proton, mainly in the $g_{7/2}$ orbital in Sb isotopes, leads to significant mixing (due to the $\nu\pi$ interaction) of: (i) the neutron seniorities ($\upsilon_{\nu}$) and (ii) the neutron angular momentum ($I_{\nu}$). The above features have a weak impact on the excitation energies, but have an important impact on the $B(E2)$ transition probabilities. In addition, a constancy of the relative excitation energies irrespective of neutron seniority and neutron number in Sn and Sb was observed., Comment: 23 pages, 18 figures, 10 tables

The lifetimes of the low-lying excited states $2^+$ and $4^+$ have been directly measured in the neutron-deficient $^{106,108}$Sn isotopes. The nuclei were populated via a deep-inelastic reaction and the lifetime measurement was performed employing a differential plunger device. The emitted $\gamma$ rays were detected by the AGATA array, while the reaction products were uniquely identified by the VAMOS++ magnetic spectrometer. Large-Scale Shell-Model calculations with realistic forces indicate that, independently of the pairing content of the interaction, the quadrupole force is dominant in the $B(E2; 2_1^+ \to 0_{g.s.}^+)$ values and it describes well the experimental pattern for $^{104-114}$Sn; the $B(E2; 4_1^+ \to 2_1^+)$ values, measured here for the first time, depend critically on a delicate pairing-quadrupole balance, disclosed by the very precise results in $^{108}$Sn. This result provides insight in the hitherto unexplained $B(E2; 4_1^+ \to 2_1^+)/B(E2; 2_1^+ \to 0_{g.s.}^+) < 1$ anomaly., Comment: V1: 6 pages, 3 figures, 1 table, theoretical interpretation described in detail in the arXiv paper of A.P.Zuker (cross-reference) V2: added reference to A.P. Zuker paper (arXiv:1905.11479)

The lifetimes of first excited 2$^+$, 4$^+$ and 6$^+$ states in $^{98}$Zr were measured with the Recoil-Distance Doppler Shift method in an experiment performed at GANIL. Excited states in $^{98}$Zr were populated using the fission reaction between a 6.2 MeV/u $^{238}$U beam and a $^{9}$Be target. The $\gamma$ rays were detected with the EXOGAM array in correlation with the fission fragments identified in mass and atomic number in the VAMOS++ spectrometer. Our result shows very small B(E2;2$_1^+$ $\rightarrow$ 0$_1^+$) value in $^{98}$Zr thereby confirming the very sudden onset of collectivity at $N=60$. The experimental results are compared to large-scale Monte Carlo Shell model and beyond mean field calculations. The present results indicate coexistence of two additional deformed shapes in this nucleus along with the spherical ground state.

The gamma-ray decay of excited states of the one-valence-proton nucleus 133Sb has been studied using cold-neutron induced fission of 235U and 241Pu targets, during the EXILL campaign at the ILL reactor in Grenoble. By using a highly efficient HPGe array, coincidences between gamma-rays prompt with the fission event and those delayed up to several tens of microseconds were investigated, allowing to observe, for the first time, high-spin excited states above the 16.6 micros isomer. Lifetimes analysis, performed by fast-timing techniques with LaBr3(Ce) scintillators, reveals a difference of almost two orders of magnitude in B(M1) strength for transitions between positive-parity medium-spin yrast states. The data are interpreted by a newly developed microscopic model which takes into account couplings between core excitations (both collective and non-collective) of the doubly magic nucleus 132Sn and the valence proton, using the Skyrme effective interaction in a consistent way. The results point to a fast change in the nature of particle-core excitations with increasing spin.