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Phase transitions leading to cloud glaciation occur at temperatures that vary between −38°C and 0°C depending on aerosol types and concentrations, the meteorology, and cloud microphysical and macrophysical parameters, although the relationships remain poorly understood. Here, we statistically retrieve a cloud glaciation temperature from two passive space‐based instruments that are part of the NASA/CNES A‐Train, the POLarization and Directionality of the Earth's Reflectances (POLDER) and the MODerate resolution Imaging Spectroradiometer (MODIS). We compare the glaciation temperature for varying bins of cloud droplet effective radius, latitude, and large‐scale vertical pressure velocity and specific humidity at 700 hPa. Cloud droplet size has the strongest influence on glaciation temperature: For cloud droplets larger than 21 μm, the glaciation temperature is 6°C higher than for cloud droplets smaller than 9 μm. Stronger updrafts are also associated with lower glaciation temperatures. Key Points: The temperature at which liquid clouds glaciate is inferred using passive space‐based instrumentsGlaciation temperature is classified by droplet radius, latitude, updraft speed, and specific humiditySubstantially less supercooling is required for glaciation of liquid clouds composed of large droplets [ABSTRACT FROM AUTHOR]

Abstract: The rate of warming in the Arctic depends upon the response of low‐level microphysical and radiative cloud properties to aerosols advected from distant anthropogenic and biomass‐burning sources. Cloud droplet cross‐section density increases with higher concentrations of cloud condensation nuclei, leading to an increase of cloud droplet absorption and scattering radiative cross sections. The challenge of assessing the magnitude of the effect has been decoupling the aerosol impacts on clouds from how clouds change solely due to natural meteorological variability. Here we address this issue with large, multi‐year satellite, meteorological, and tracer transport model data sets to show that the response of low‐level clouds in the Arctic to anthropogenic aerosols lies close to a theoretical maximum and is between 2 and 8 times higher than has been observed elsewhere. However, a previously described response of arctic clouds to biomass‐burning plumes appears to be overstated because the interactions are rare and modification of cloud radiative properties appears better explained by coincident changes in temperature, humidity, and atmospheric stability. [ABSTRACT FROM AUTHOR]

Reduced precipitation rates allow pollution within air parcels from midlatitudes to reach the Arctic without being scavenged. We use satellite and tracer transport model data sets to evaluate the degree of supercooling required for 50% of a chosen ensemble of low‐level clouds to be in the ice phase for a given meteorological regime. Our results suggest that smaller cloud droplet effective radii are related to higher required amounts of supercooling but that, overall, pollution plumes from fossil fuel combustion lower the degree of supercooling that is required for freezing by approximately 4 °C. The relationship between anthropogenic plumes and the freezing transition temperature from liquid to ice remains to be explained. Plain Language Summary: Anthropogenic pollution plumes from midlatitudes can be transported long distances to the Arctic. In this study, we analyze the impact of these plumes on how easily liquid clouds over the Arctic Ocean freeze by using a novel combination of satellite measurements and a pollution transport model. We find that liquid clouds in polluted air switch phase to become ice clouds at temperatures that are 4 °C higher they would otherwise in pristine air. Because ice clouds in the Arctic precipitate more easily than liquid clouds, the potential is that distant industrial pollution sources are acting to reduce arctic cloud life time. Key Points: MODIS and POLDER‐3 can be used to provide space‐based measurements of phase transitions in liquid arctic cloudsA smaller droplet effective radius is associated with an increase in the amount of supercooling required for freezingAnthropogenic pollution plumes are associated with a decrease in the amount of supercooling required for freezing [ABSTRACT FROM AUTHOR]