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Numerical models have been developed to investigate and understand responses of biogeochemical cycle to global changes. Steady state, when a system is in dynamic equilibrium, is generally required to initialize these model simulations. However, the spin‐up process that is used to achieve steady state pose a great burden to computational resources, limiting the efficiency of global modeling analysis on biogeochemical cycles. This study introduces a new Semi‐Analytical Spin‐Up (SASU) to tackle this grand challenge. We applied SASU to Community Land Model version 5 and examined its computational efficiency and accuracy. At the Brazil site, SASU is computationally 7 times more efficient than (or saved up to 86% computational cost in comparison with) the traditional native dynamics (ND) spin‐up to reach the same steady state. Globally, SASU is computationally 8 times more efficient than the accelerated decomposition spin‐up and 50 times more efficient than ND. In summary, SASU achieves the highest computational efficiency for spin‐up on site and globally in comparison with other spin‐up methods. It is generalizable to wide biogeochemical models and thus makes computationally costly studies (e.g., parameter perturbation ensemble analysis and data assimilation) possible for a better understanding of biogeochemical cycle under climate change. Plain Language Summary: Land carbon cycle models, a critical component of earth system models, have been developed to investigate and understand ecological responses to global changes. However, the model spin‐up process to achieve steady state are usually time‐consuming and pose great computational burden. The spin‐up problem hinders our ability to study some key issues in land carbon cycle modeling, such as sensitivity analysis. This paper applies a new SASU framework to accelerate spin‐up of Community Land Model matrix version 5. Compared with traditional native dynamic approach, SASU speeds up the spin‐up by approximately 50 times, achieving the fastest spin‐up speed than all the previously recorded methods. Our SASU method is applicable to biogeochemical models and, therefore, liberates the models for computationally costly studies, such as parameter perturbation ensemble analysis and data assimilation. Key Points: A new semi‐analytical spin‐up (SASU) framework combines the default accelerated spin‐up method and matrix analytical algorithmSASU accelerates CLIM5 spin‐up by tens of times, becoming the fastest method to our knowledgeSASU is applicable to most biogeochemical models and enables computationally costly study, for example, sensitivity analysis [ABSTRACT FROM AUTHOR]