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4. ChemInform Abstract: Copper-Catalyzed Insertion into Heteroatom-Hydrogen Bonds with Trifluorodiazoalkanes

Author

Stephen C. Hyde, Janis Veliks, Marc Taillefer, Benoit Liegault, Veronique Gouverneur, and David Grassi

Subjects
Hydrogen bond, Chemistry, Heteroatom, Copper catalyzed, Enantioselective synthesis, General Medicine, Combinatorial chemistry
Abstract

Copper-catalyzed Si-H, B-H, P-H, S-H, and N-H insertion reactions of 2,2,2-trifluoro-1-diazoethane and 1-aryl 2,2,2-trifluorodiazoethanes generated a large number of new fluorine-containing chemical entities for medicinal chemists. With selected Si-H and B-H insertion reactions, we demonstrate successful extension to asymmetric catalysis.

Published
2016

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