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The hydrodynamics within small boreal lakes have rarely been studied, yet knowing whether turbulence at the air-water interface and in the water column scales with metrics developed elsewhere is essential for computing metabolism and fluxes of climate-forcing trace gases. We instrumented a humic, 4.7 ha, boreal lake with two meteorological stations, three thermistor arrays, an infrared (IR) camera to quantify surface divergence, obtained turbulence as dissipation rate of turbulent kinetic energy (epsilon) using an acoustic Doppler velocimeter and a temperature-gradient microstructure profiler, and conducted chamber measurements for short periods to obtain fluxes and gas transfer velocities (k). Near-surface epsilon varied from 10(-8) to 10(-6) m(2) s(-3) for the 0-4 m s(-1) winds and followed predictions from Monin-Obukhov similarity theory. The coefficient of eddy diffusivity in the mixed layer was up to 10(-3) m(2) s(-1) on the windiest afternoons, an order of magnitude less other afternoons, and near molecular at deeper depths. The upper thermocline upwelled when Lake numbers (L-N) dropped below four facilitating vertical and horizontal exchange. k computed from a surface renewal model using epsilon agreed with values from chambers and surface divergence and increased linearly with wind speed. Diurnal thermoclines formed on sunny days when winds were < 3 m s(-1), a condition that can lead to elevated near-surface epsilon and k. Results extend scaling approaches developed in the laboratory and for larger water bodies, illustrate turbulence and k are greater than expected in small wind-sheltered lakes, and provide new equations to quantify fluxes.

From observations in a High Arctic valley and ice-free fjord in Svalbard during March and April 2013 we show that, while some caution needs to be applied, ordinary slow-response instruments placed over a snow-water-snow surface can be effectively used as a proxy for more sophisticated measuring techniques at complex sites such as leads or a polynyas. The turbulent fluxes of momentum, sensible and latent heat were measured at three locations with a snow-water-snow fetch. At the snow site upwind of the water, the stability was generally stable, the momentum flux small, and the sensible heat flux positive. Over the water however, the internal boundary layer that was formed gave on average an increased vertical gradient in wind speed, temperature, and humidity and turbulent heat fluxes exceeding 400 W m−2. At the snow surface downwind of the water, the conditions were highly variable and all the fluxes were, on average, of very small magnitude. That the behaviour of the internal boundary layers can be highly variable is demonstrated through four case studies. This phenomenon is likely to increase in occurrence with a changing climate.

Eddy-covariance measurements made in the marine atmospheric boundary layer above a high Arctic fjord (Adventfjorden, Svalbard) are analyzed. When conditions are unstable, but close to neutral −0.1 < z/L < 0, where z is the height, and L is the Obukhov length, the exchange coefficient for sensible heat CH is significantly enhanced compared with that expected from classical surface-layer theory. Cospectra of the vertical velocity component (w) and temperature (T) reveal that a high-frequency peak develops at f ≈ 1 Hz for z/L > − 0.15. A quadrant analysis reveals that the contribution from downdrafts to the vertical heat flux increases as conditions become close to neutral. These findings are the signature of the evolving unstable very-close-to-neutral (UVCN) regime previously shown to enhance the magnitude of sensible and latent heat fluxes in the marine surface layer over the Baltic Sea. Our data reveal the significance of the UVCN regime for the vertical flux of the carbon dioxide (CO2) concentration (C). The cospectrum of w and C clearly shows how the high-frequency peak grows in magnitude for z/L > − 0.15, while the high-frequency peak dominates for z/L > − 0.02. As found for the heat flux, the quadrant analysis of the CO2 flux shows a connection between the additional small-scale turbulence and downdrafts from above. In contrast to the vertical fluxes of sensible and latent heat, which are primarily enhanced by the very different properties of the air from aloft (colder and drier) during UVCN conditions, the increase in the air–sea transfer of CO2 is possibly a result of the additional small-scale turbulence causing an increase in the water-side turbulence. The data indicate an increase in the gas-transfer velocity for CO2for z/L > − 0.15 but with a large scatter. During the nearly 2 months of continuous measurements (March–April 2013), as much as 36% of all data are associated with the stability range −0.15 < z/L < 0, suggesting that the

In Arctic fjords and high-latitude seas, strong surface cooling dominates during a large part of the year, generating water-side convection (w*w) and enhanced turbulence in the water. These regions are key areas for the global carbon cycle; thus, a correct description of their air-sea gas exchange is crucial. CO2-data were measured via the eddy covariance technique in marine Arctic conditions and reveal that water-side convection has a major impact on the gas transfer velocity. This is observed even at wind speeds as high as 9 m s-1, where convective motions are generally thought to be suppressed by wind-driven turbulence. The enhanced air-sea transfer of CO2 caused by water-side convection nearly doubled the CO2uptake, after scaled to open sea conditions the contribution from to the CO2 flux remained as high as 34%; this phenomenon is expected to be highly important for the total carbon uptake in marine Arctic areas.

At the land-based marine measuring site Östergarnsholm in the Baltic Sea, the eddy covariance technique was used to measure air-sea fluxes of carbon dioxide and oxygen. High- frequency measurements of oxygen were taken with a Microx TX3 optode using the luminescence lifetime technique. The system gives reasonable oxygen fluxes after the limited frequency response of the sensor was corrected for. For fluxes of carbon dioxide the LICOR-7500 instrument was used. Using flux data to estimate transfer velocities indicates higher transfer velocity for oxygen compared to carbon dioxide for winds above 5 m/s. There are too few data for any extensive conclusions, but a least-square fit of the data gives a cubic wind speed dependence of oxygen corresponding to k 660 = 0.074U 3 10. The more effective transfer for oxygen compared to carbon dioxide above 5 m/s is most likely due to enhanced efficiency of oxygen exchange across the surface. Oxygen has lower solubility compared with carbon dioxide and might be more influenced by near surface processes such as microscale wave breaking or sea spray.

Air-sea gas transfer velocity for O2 is calculated using directly measured fluxes with the eddy covariance technique. It is a direct method and is frequently used to determine fluxes of heat, humidity, and CO2, but has not previously been used to estimate transfer velocities for O2, using atmospheric eddy covariance data. The measured O2 fluxes are upward directed, in agreement with the measured air-sea gradient of the O-2 concentration, and opposite to the direction of the simultaneously measured CO2 fluxes. The transfer velocities estimated from measurements are compared with prominent wind speed parameterizations of the transfer velocity for CO2 and O2, previously established from various measurement techniques. Our result indicates stronger wind speed dependence for the transfer velocity of O2 compared to CO2 starting at intermediate wind speeds. This stronger wind speed dependence appears to coincide with the onset of whitecap formation in the flux footprint and the strong curvature of a cubic wind -dependent function for the transfer velocity provides the best fit to the data. Additional data using the measured O2 flux and an indirect method (based on the Photosynthetic Quotient) to estimate oxygen concentration in water, support the stronger wind dependence for the transfer velocity of O2 O-2 to CO2.

During the years 2010-13, atmospheric eddy covariance measurement of oxygen was performed at the marine site Ostergarnsholm in the Baltic Sea. The fast response optode Microx TX3 was used with two different types of tapered sensors. In spite of the increased lifetime, the optical isolated sensor is limited by the slower response time and is unsuitable for ground-based eddy covariance measurements. The sensor without optical isolation shows a -2/3 slope within the inertial subrange and attains sufficient response time and precision to be used in air-sea applications during continuous periods of 1-4 days. Spectral and cospectral analysis shows oxygen measured with the nonoptical isolated sensor to follow the same shape as for CO2 and water vapor when normalized. The sampling rate of the Microx TX3 is 2Hz; however, the sensor was found to have a limited response and resolution, yielding a flux loss in the frequency range f > 0.3Hz. This can be corrected for by applying cospectral similarity simultaneously using measurements of latent heat as the reference signal. On average the magnitude of the cospectral correction added 20% to the uncorrected oxygen flux during neutral atmospheric stratification.

Eddy covariance measurements over a high Arctic fjord reveals higher turbulent levels than normally found from classical surface layer theory. When conditions become unstable close to neutral i.e. -0.15-0.15, simultaneously quadrant analysis displays how the contribution from downdrafts to the vertical flux of temperature and CO2 increases. These findings are the signature of the evolving UVCN (Unstable Very Close to Neutral) regime, previously shown to enhance the vertical fluxes of temperature and humidity. In this study we show that the additional small scale turbulence related to these conditions also has the potential to enhance the vertical flux of CO2. Different to the vertical flux of temperature and humidity wq, the enhancement are not solely explained by the different properties of the air from aloft. We suggest that a part of the observed increase in CO2 flux and gas transfer velocity of CO2 when z/L> -0.1, also is generated by the increased levels of , causing higher levels of water-side turbulence. In winter the Arctic marine boundary layer is characterized by unstable stratification and during the nearly two months of measurements presented here as much as 36% of all data where associated to conditions with z/L in the range -0.15