Wilfried Blanc, Ali Albalawi, Stefano Varas, Anna Lukowiak, Hrvoje Gebavi, Wedad Albalawi, Alessandro Chiasera, Stefano Taccheo, Maurizio Ferrari, Rolindes Balda, College of Engineering [Swansea], Swansea University, Caratterizzazione e Sviluppo di Materiali per la Fotonica e l'Optoelecttronica (CSMFO), CNR Istituto di Fotonica e Nanotecnologie [Trento] (IFN), Consiglio Nazionale delle Ricerche [Roma] (CNR)-Consiglio Nazionale delle Ricerche [Roma] (CNR), Istituto di Fotonica e Nanotecnologie (IFN), Consiglio Nazionale delle Ricerche [Roma] (CNR), Rudjer Boskovic Institute [Zagreb], Institut de Physique de Nice (INPHYNI), Centre National de la Recherche Scientifique (CNRS)-Université Côte d'Azur (UCA)-Université Nice Sophia Antipolis (... - 2019) (UNS), COMUE Université Côte d'Azur (2015-2019) (COMUE UCA)-COMUE Université Côte d'Azur (2015-2019) (COMUE UCA), Universidad del Pais Vasco / Euskal Herriko Unibertsitatea [Espagne] (UPV/EHU), School 4, Institute of Low Temperature and Structure Research [Polish Academy of Sciences], Polska Akademia Nauk = Polish Academy of Sciences (PAN)-Polska Akademia Nauk = Polish Academy of Sciences (PAN), European Commission, Centre National de la Recherche Scientifique (France), and Institute of Low Temperature and Structure Research
In this paper, we numerically investigate the fluorescence decay of Tm-doped tellurite glasses with different dopant concentrations. The aim is to find a set of data that allows the prediction of material performance over a wide range of doping concentrations. Among the available data, a deep investigation of the reverse cross-relaxation process (F,F,→H,H) was not yet available. The numerical simulation indicates that the reverse cross-relaxation process parameter can be calculated by fitting the slow decaying H fluorescence tails emitted when the pump level is almost depopulated. We also show that the floor of the H decay curve is indeed related to a second exponential constant, half the F lifetime, kicking in once the H level depopulates. By properly fitting the whole set of decay curves for all samples, the proposed value for the reverse cross-relaxation process is 0.03 times the cross-relaxation parameter. We also comment on the measurement accuracy and best set-up. Excellent agreement was found between the simulated and experimental data, indicating the validity of the approach. This paper therefore proposes a set of parameters validated by fitting experimental fluorescence decay curves of both the H and F levels. To the best of our knowledge, this is the first time a numerical simulation has been able to predict the fluorescence behavior of glasses with doping levels ranging from 0.36 mol% to 10 mol%. We also show that appropriate calculations of the reverse cross-relaxation parameter may have a significant effect on the simulation of laser and amplifier devices., This article is based upon work from H2020 COST Action MP1401 on “Fiber Lasers and Their Applications” supported by COST “(European Cooperation in Science and Technology)”. M. Ferrari acknowledges CNRS support, part of this research has been supported during his visit at UMR7010 INPHYNI - Institute de Physique de Nice.