1. Strain control of a bandwidth-driven spin reorientation in Ca3Ru2O7.
- Author
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Dashwood, C. D., Walker, A. H., Kwasigroch, M. P., Veiga, L. S. I., Faure, Q., Vale, J. G., Porter, D. G., Manuel, P., Khalyavin, D. D., Orlandi, F., Colin, C. V., Fabelo, O., Krüger, F., Perry, R. S., Johnson, R. D., Green, A. G., and McMorrow, D. F.
- Subjects
NUCLEAR spin ,FERMI surfaces ,LATTICE constants ,DEGREES of freedom ,PHASE transitions ,X-ray scattering ,INELASTIC neutron scattering - Abstract
The layered-ruthenate family of materials possess an intricate interplay of structural, electronic and magnetic degrees of freedom that yields a plethora of delicately balanced ground states. This is exemplified by Ca
3 Ru2 O7 , which hosts a coupled transition in which the lattice parameters jump, the Fermi surface partially gaps and the spins undergo a 90∘ in-plane reorientation. Here, we show how the transition is driven by a lattice strain that tunes the electronic bandwidth. We apply uniaxial stress to single crystals of Ca3 Ru2 O7 , using neutron and resonant x-ray scattering to simultaneously probe the structural and magnetic responses. These measurements demonstrate that the transition can be driven by externally induced strain, stimulating the development of a theoretical model in which an internal strain is generated self-consistently to lower the electronic energy. We understand the strain to act by modifying tilts and rotations of the RuO6 octahedra, which directly influences the nearest-neighbour hopping. Our results offer a blueprint for uncovering the driving force behind coupled phase transitions, as well as a route to controlling them. Ca3 Ru2 O7 is a layered ruthenate, which undergoes a spin-reorientation transition where the spins rotate 90 degrees between two anti-ferromagnetic states. Despite extensive study, the driver of this transition has proved elusive. Here, using neutron and resonant x-ray scattering, Dashwood et al. show that this transition is driven by lattice strain. [ABSTRACT FROM AUTHOR]- Published
- 2023
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