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In this paper, we investigate the manifolds of three Near-Rectilinear Halo Orbits (NRHOs) and optimal low-thrust transfer trajectories using a high-fidelity dynamical model. Time- and fuel-optimal low-thrust transfers to (and from) these NRHOs are generated leveraging their 'invariant' manifolds, which serve as long terminal coast arcs. Analyses are performed to identify suitable manifold entry/exit conditions based on inclination and minimum distance from the Earth. The relative merits of the stable/unstable manifolds are studied with regard to time- and fuel-optimality criteria, for a set of representative low-thrust family of transfers. [ABSTRACT FROM AUTHOR]