Search

Naturally occurring radioactive materials (NORMs: 232 Th, 226 Ra, 40 K) can reach our respiratory system by breathing of road dust which can cause severe health risks. Targeting the pioneering consideration of health risks from the NORMs in road dust, this work reveals the radioactivity abundances of NORMs in road dust from a megacity (Dhaka) of a developing country (Bangladesh). Bulk chemical compositions of U, Th, and K obtained from neutron activation analysis were converted to the equivalent radioactivities. Radioactivity concentrations of 226 Ra, 232 Th, and 40 K in road dust ranged from 60-106, 110-159, and 488-709 Bq kg -1 with an average of 84.4 ± 13.1, 126 ± 11, and 549 ± 48 Bq kg -1 , respectively. Estimated 226 Ra, 232 Th, and 40 K radioactivities were, respectively, 1.7-3.0-, 3.7-5.3-, and 1.2-1.8-folds greater than the affiliated world average values. Mechanistic pathway of NORMs' enrichment and fractionation relative to the major origin (pedosphere) were evaluated concerning the water logging, relative solubility-controlled leaching and translocation, climatic conditions, and aerodynamic fractionations (dry and wet atmospheric depositions). Computation of customary radiological risk indices invokes health risks. Noticing the ingress of NOMR-holding dust into the human respiratory system along with the associated ionizing radiations, the computed radiological indices represent only the least probable health hazards. Nevertheless, in real situations, α-particles from the radioactive decay products of 232 Th and 238 U can create acute radiation damages of respiratory system. Policymakers should emphasize on limiting the dust particle evolution, and public awareness is required to alleviate the health risks., (© 2023. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature.)

The coastal areas of Bangladesh have poor accessibility to fresh drinking water and the groundwater is not suitable for drinking, cooking, and other domestic uses due to high levels of salinity and potentially toxic elements. The current study focuses on understanding of the distribution of some physicochemical parameters (temperature, pH, EC, TDS, and salinity) and chemical elements (Fe, Mn, Zn, Ca, Mg, Na, K, Cu, Co, Pb, As, Cr, Cd, and Ni) with health perspective in drinking water from the southwestern coastal area of Bangladesh. The physicochemical properties of the water samples were examined with a multiparameter meter, while the elemental concentrations were analyzed using atomic absorption spectrometer. Water quality index (WQI) and irrigation indices were utilized to determine the drinking water quality and irrigation feasibility, respectively, whereas hazard quotients (HQs) and hazard index (HI) were used to assess the probable pathways and the associated potential risks to human health. The concentrations of some toxic elements in measured samples were relatively higher compared to drinking water guidelines, indicating that ground and surface water are not apt for drinking and/or domestic uses. The multivariate statistical approaches linked the source of the pollutants in the studied water body mostly to the geogenic origin including saline water intrusion. WQI values ranged from 18 to 430, reflecting excellent to unsuitable categories of water quality. The assessment of human health risks due to exposure to contaminated water demonstrated both carcinogenic and non-carcinogenic health risks in the exposed residents of the study area. Therefore, appropriate long-term coastal area management strategies should be adopted in the study region for environmental sustainability. The findings of this research will be supportive in understanding the actual situation of fresh drinking water in the area for policymakers, planners, and environmentalists to take effective necessary measures to ensure safe drinking water in the study area., (© 2023. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature.)

This study of a downstream segment (Brahmaputra, Bangladesh) of one of the longest transboundary (China-India-Bangladesh) Himalayan rivers reveals elevated radioactivity compared to other freshwater basins across the world. Naturally occurring radioactive nuclides ( 226 Ra, 232 Th, and 40 K) and metal contents (transition metals, Fe, Ti, Sc, and V; rare earth elements, La, Ce, Eu, Sm, Dy, Yb, and Lu; high field strength elements, Ta and Hf; and actinides, Th and U) in thirty sediment samples were measured by HPGe γ-spectrophotometry and research reactor-based neutron activation analysis, respectively. We systematically investigated the mechanism of the deposition of higher radioactivity concentrations and rare earth elements (REEs) associated with heavy minerals (HMs) and photomicrograph-based mineralogical analysis. The results show that total REEs (∑REE) and Ta, Hf, U, and Th are generally 1.5- to 3.0-fold elevated compared to crustal values associated with -δEu and -δCe anomalies, suggesting a felsic source provenance. The enrichment of light REEs (×1.5 upper continental crust (UCC)) and Th (×1.9 UCC), besides Th/U (=7.74 ± 2.35) and 232 Th/ 40 K ratios, along with the micrographic and statistical approaches, revealed the elevated presence of HMs. Fluvial suspended sedimentary transportation (from upstream) followed by mineralogical recycling and sorting enriched the HM depositions in this basin. Bivariate plots, including La/Th-Hf, La/Th-Th/Yb, and La/V-Th/Yb, revealed significant contributions of felsic source rock compared to mafic sources. The assessment of radiological hazards demonstrates ionizing-radiation-associated health risks to the local residents and people inhabiting houses made from Brahmaputra River sediments (as construction material)., (© 2022. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature.)

The original version of this article unfortunately contained an error in eq. 1. The denominator Ɛ of Eq. (1) was missing.

To study the level of radioactivity concentrations from a coal-based power plant (Barapukuria, Bangladesh) and to estimate the associated radiological hazards, coal and associated combustion residuals from the power plant were analyzed by gamma-ray spectrometry with high-purity germanium (HPGe) detector. The results reveal that the mean radioactivity (Bq kg -1 ) concentrations in feed coal samples are 66.5 ± 24.2, 41.7 ± 18.2, 62.5 ± 26.3, and 232.4 ± 227.2 for U-238, Ra-226, Th-232, and K-40, respectively, while in coal combustion residuals (CCRs), they are 206.3 ± 72.4, 140.5 ± 28.4, 201.7 ± 44.7, and 232.5 ± 43.8, respectively. With the exception of K-40, all the determined natural radionuclides are considerably higher in the investigated feed coal and associated combustion residues as compared with the world soil and world coal mean activities. On the average, CCRs contains 3.10-3.37 times more natural radionuclides than the feed coal, except for K-40. The radioactivity of fly ash and bottom ash is fractionated, and ratio ranges from 1.40 to 1.57. The mean values of the radiological hazard indices in the coal and their associated residuals are 153.1 and 446.8 Bq kg -1 for radium equivalent activity, 0.41 and 1.21 for the external hazard index, 70 and 200.1 nGy h -1 for the absorbed gamma dose rate, 0.09 and 0.25 mSv year -1 for the annual effective dose rate, and 3.0 × 10 -4 and 8.6 × 10 -4  Sv -1 for the excess lifetime cancer risk, respectively, most of which exceed the UNSCEAR-recommended respective threshold limits. The outcome of this study suggests a potential radiological threat to the environment as well as to the health of occupational workers and nearby inhabitants from the examined samples.