1. Validation of capture reactions cross sections in 252 Cf(s.f.) neutron field.
- Author
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Schulc M, Novák E, Šimon J, Krechlerová A, Košťál M, and Capote R
- Abstract
We have investigated following capture reactions:
197 Au(n,g)198 Au,63 Cu(n,g)64 Cu,45 Sc(n,g)46 Sc,181 Ta(n,g)182 Ta,140 Ce(n,g)141 Ce,139 La(n,g)140 La,176 Yb(n,g)177 Yb,55 Mn(n,g)56 Mn, and141 Pr(n,g)142 Pr in a standard252 Cf(s.f.) neutron field. The experimentally derived reaction rates were compared with calculations using state-of-the-art libraries IRDFF-II, ENDF/B-VIII.0, JENDL-5 and JEFF-3.3 performed in MCNP6.2 transport code. The experiment was focused on capture reactions in high energy neutron range. To suppress scattered low energy neutrons, all activation materials were enclosed by a spherical cadmium surface of 30 cm in diameter. Experimentally derived reaction rates of197 Au(n,g)198 Au,63 Cu(n,g)64 Cu reactions agree with calculations using all state-of-the-art nuclear data libraries. The highest discrepancies were found when evaluating139 La(n,g)140 La and55 Mn(n,g)56 Mn reactions utilizing all libraries. Experimental reaction rates applying data from the JENDL-5 library agree very well with the results of other reactions except for the45 Sc(n,g)46 Sc reaction.181 Ta(n,g)182 Ta reaction rate does not agree within uncertainties using any library. The176 Yb(n,g)177 Yb reaction rate agrees reasonably well only when performing calculation using JENDL-5 and ENDF/B-VIII.0 libraries, unlike JEFF-3.3 library.140 Ce(n,g)141 Ce and141 Pr(n,g)142 Pr reaction rates applying JEFF-3.3 and ENDF/B-VIII.0 libraries do not agree within uncertainties., Competing Interests: Declaration of competing interest The authors declare the following financial interests/personal relationships which may be considered as potential competing interests:Michal Kostal reports financial support was provided by Research Center Rez. If there are other authors, they declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper., (Copyright © 2024 Elsevier Ltd. All rights reserved.)- Published
- 2024
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