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We show here that light polarization of a beam propagating through a heliconical cholesteric cell can be controlled by tuning the Bragg resonance of the structure. We demonstrate that this control is achieved by varying either the low-frequency electric field or the intensity of a pump beam impinging on the sample. The study confirms the recently reported phenomenon of optical tuning of the heliconical cholesterics and opens the door for the development of simple and efficient polarization modulators controlled electrically or optically.

We show here that the light-induced tuning of the Bragg reflection recently demonstrated in heliconical cholesterics opens new perspectives to nonlinear optical propagation in liquid crystals. We highlight that, by properly adjusting the static electric field that stabilizes the heliconical structure, a dramatic change of the refractive index of the circularly polarized resonant mode can be achieved. Additionally, a stop band for a definite range of light intensity is obtained that can be tuned in order to get the conditions of self-induced transparency.

Near-infrared light is commonly used to move small objects floating on water by exploiting the Bénard-Marangoni convection. This is because infrared light is absorbed well by water and the induced thermal gradients are responsible for the objects' motion. However, visible light was recently used to move macroscopic objects on the free liquid surfaces. In this work, we show the use of visible light to rotate symmetric millimeter-sized objects. Those objects represent light-driven macro motors that are able to work in a continuous or step-by-step mode. We studied light intensity's effects on our system's angular velocity and estimated the entire process's conversion efficiency.

We report the experimental evidence of nonlinear optical response in DNA lyotropic nematic liquid crystals. Pump-probe experiments indicate that the non-linearity is remarkably large. Quantitative assessment of the non-linear optical coefficient by transient optical grating demonstrates that the response is of the same order of the well-known Giant Optical Nonlinearity (GON) of thermotropic nematics. These results represent a further incentive to the current investigation of potential applications of DNA in biophotonics.

We report the realization and characterization of an optofluidic microlaser based on a Fabry-Perot resonator fabricated by exploiting two direct writing fabrication techniques: the femtosecond laser micromachining and the inkjet printing technology. In this way a standard Fabry-Perot cavity has been integrated into an optofluidic chip. When using rhodamine 6G dissolved in ethanol at concentration of 5∙10 -3 mol/l, laser emission was detected at a threshold energy density of 1.8 μJ/mm 2 at least one order of magnitude lower than state-of-the-art optofluidic lasers. Linewidth below ~0.6 nm was measured under these conditions with a quality factor Q~10 3 . These performances and robustness of the device makes it an excellent candidate for biosensing, security and environment monitoring applications.

We report on the observation of a modulated pattern induced by a single laser beam in a polymeric film. In spite of the simple geometrical configuration, the analysis of the far field diffraction pattern allows a sensitive retrieving of the wavelength of the recording beam and of its incidence angle, pointing out the high information content of the recorded spot. A theoretical model is presented which satisfactorily explains the observed behavior. It takes into account the interaction of structured light with structured matter with the same symmetries and spatial modulation frequencies close to each other. This result shows a feature of the interaction between structured light and structured matter which has not been explored yet.

We report the light-induced control of optical phase shift by a liquid crystal cell made with LiNbO3:Fe crystals as substrates. We show that a phase shift of a few πs can be easily reached for two orthogonal polarizations due to liquid crystal reorientation driven by the photovoltaic electric field originated in the substrates. This effect is exploited to get all-optical switching with a contrast of about 80%, by 2 s pump pulse.

Nonlinear optical response of the cybotactic nematic phase of a bent-core mesogen has been investigated for the first time through self-phase modulation induced by a Gaussian beam. The material exhibits a high nonlinear response achieving a nonlinear index n(2)≈5×10(-5)  cm(2)/W and an unconventional behavior characterized by two different regimes. While the high-intensity regime can be easily explained in terms of a thermal indexing effect, the low-intensity regime is metastable and characterized by an unusual dependence on the irradiation energy. It is suggested that a change of the director configuration, possibly due to a light-induced modification of surface anchoring, is responsible for the observed behavior.

A first-order optical Freedericksz transition in a nematic liquid crystal doped by a small quantity of a dichroic dye with negative dichroism is observed. The initial homeotropic state corresponds to maximum absorption for the linearly polarized incident beam, while reorientation reduces absorption increasing the optical torque: this process produces the positive feedback leading to the observed bistable behavior.

We report on the effects of a low-frequency electric field on the optical nonlinear response of thin dye-doped liquid crystal cells. Experimental data show that the external field allows reaching extremely high values of the optical nonlinearity without any critical control of the cell interfaces. A qualitative interpretation of the collected data, based on the light-induced modulation of the bulk voltage through surface modifications, is proposed.

Fast surface reorientation induced by a single 4-ns low-energy laser pulse in dye-doped liquid crystals is reported. The reorientation is due to light-induced modification of the surface anisotropy, which affects the liquid crystal's director through the appearance of a preferred direction on the irradiated surface. The detected signals can be interpreted as being the result of light-induced desorption and adsorption of dye molecules.

We show the possibility of detecting small anisotropies in holographic polymer dispersed liquid-crystal samples, using a simple experimental setup that allows us to determine the behavior of the diffraction efficiency versus incident angle for two reading polarizations. This analysis is extremely sensitive to small changes in the parameters that define the grating anisotropy, giving us a way to determine with great accuracy the components of the modulated part of the dielectric tensor.

We report the results of an investigation carried on Methyl Red-doped nematic liquid crystals with the aim of studying the basic mechanism of the extraordinarily large nonlinear response recently reported. We show that the experimental data can be explained as due to light-induced modifications of the anchoring conditions leading to director reorientation on the irradiated surface, which in turn gives rise to a bulk reorientation through the cell. We have called this phenomenon SINE (Surface Induced Nonlinear Effect) to remind that it occurs "without" (= sine in latin language) a direct optical or electric torque on the director in the bulk.

Light-induced director reorientation in dye-doped nematic liquid crystals was recently reported to be an efficient method of writing permanent holographic gratings with high sensitivity [Phys. Rev. Lett. 82, 1855 (1999)]. We report the achievement of stable director reorientation in the same materials by means of a single 4-ns pulse of the second harmonic of a Nd:YAG laser. Fast recording of high-resolution holographic gratings (more than 500 lines/mm) can be obtained with an energy density as low as 7x10(-3)J /cm(2) .

We report the observation of orientational gratings induced by the photorefractive effect in dye-doped polymer-dispersed liquid crystals. The photorefractive origin of the grating-induction effect is supported by the results of two-beam coupling experiments and by the possibility of erasing the grating by uniform illumination. For all the samples a stable memory effect was observed.

In Ref. 1, the second sentence of the abstract should read as follows: "As compared with other methods that make use of these materials, we have achieved higher sensitivity with good spatial resolution."

We report the observation of light-induced director reorientation under the application of an electric field in a chiral smectic A liquid crystal owing to the temperature dependence of the electroclinic coefficient. We also demonstrate the occurrence of another light-induced phenomenon that leads to optic axis rotation, whose origin is not yet clear. Finally, we show that thermal indexing cannot be neglected when fitting the experimental data.

We report on the observation of strong nonlinear optical behavior of SF59 Schott glass. An unfocused Ar' laser beam undergoing total internal reflection in this glass shows extremely strong selffocusing. This effect is ~ 1 order of magnitude higher than the usual thermal lensing, and, by means of an interferometric technique, we demonstrate that this effect is due to the thermoplastic effect. Focal lengths that are shorter than 10 cm are observed for the beam intensity I asymptotically equal to 30 W/cm(2). The use of this glass as a self-limiter is shown experimentally.

We report what is to our knowledge the first observation of nonlinear light diffraction in polymer-dispersed liquid crystals. The superposition with the self-transparency effect produces a threshold in the observed wave-mixing phenomenon.

We report bistability and self-pulsing effects in the switching from total internal reflection to a transmitting state at a glass-liquid-crystal interface. The role of the phase transition to the isotropic state is underlined, and the generation of 20-msec pulses from a continuous laser beam is observed.