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Every year, structural flaws or breakdowns cause thousands of people to be harmed and cost billions of dollars owing to the limitations of design methods and materials to withstand extreme earthquakes. Since earthquakes have a significant effect on sustainability factors, there is a contradiction between these constraints and the growing need for more sustainable structures. There has been a significant attempt to circumvent these constraints by developing various techniques and materials. One of these viable possibilities is the application of smart structures and materials such as shape memory and piezoelectric materials. Many scholars have examined the use of these materials and their structural characteristics up to this point, but the relationship between sustainability considerations and the deployment of smart materials has received little attention. Therefore, through a review of previous experimental, numerical, and conceptual studies, this paper attempts to draw a more significant relationship between smart materials and structural sustainability. First, the significant impact of seismic events on structural sustainability and its major aspects are described. It is then followed by an overview of the fundamentals of smart material’s behaviour and properties. Finally, after a comprehensive review of the most recent applications of smart materials in structures, the influence of their deployment on sustainability issues is discussed. The findings of this study are intended to assist researchers in properly addressing sustainability considerations in any research and implementation of smart materials by establishing a more explicit relationship between these two concepts.