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The thin-film post-compression technique has the ability to reduce the pulse duration in PW-class lasers, increasing the peak power. Here, the nonlinear response of an increasingly available optical thermoplastic demonstrates enhanced spectral broadening, with corresponding shorter pulse duration compared to fused silica glass. The thermoplastic can be used close to its damage threshold when refreshed using a roller mechanism, and the total amount of material can be varied by folding the film. As a proof-of-principle demonstration scalable to 10-PW, a roller mechanism capable of up to 6 passes through a sub-millimeter thermoplastic film is used in vacuum to produce two-fold post-compression of the pulse. The compact design makes it an ideal method to further boost ultrahigh laser pulse intensities with benefits to many areas, including driving high energy acceleration.

Ultra-intense laser pulses with helical phases are of interest in laser-driven charged particle acceleration and related experiments with extreme light. However, such optical vortices can be affected by the presence of residual spatial-temporal couplings. Their field distributions after propagating in free-space and in the focal plane of an ideal focusing mirror were assessed through numerical modeling, based on the Gaussian decomposition method for a 25 fs pulse with a Supergaussian spatial profile. The wash-out of the central hole in the doughnut-shaped profile in the focal plane corresponds to the rotation of the phase discontinuity.