1. Crystalline electric field excitations in CeAgSb2
- Author
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Yoshichika Onuki, Naoto Metoki, Arumugam Thamizhavel, and Shingo Araki
- Subjects
Paramagnetism ,Condensed matter physics ,Chemistry ,Heisenberg model ,Spin wave ,Excited state ,Condensed Matter::Strongly Correlated Electrons ,General Materials Science ,Neutron scattering ,Condensed Matter Physics ,Saturation (magnetic) ,Critical field ,Excitation - Abstract
Neutron scattering experiments have been carried out that reveal the magnetic excitation in the ferromagnet CeAgSb2. Crystalline electric field excitations were observed at 5.2 and 12.5 meV in the paramagnetic state, indicative of the localized nature of the Ce 4f electron. Our analysis concluded that |Jz = ±1/2 is the ground state, while the first and second excited levels are mainly due to |±3/2 and |±5/2, respectively. The observed ferromagnetic moment is in good agreement with the ground-state saturation moment, gJμBJz ~ 0.43 μB. The spin wave dispersion is interpreted using the anisotropic Heisenberg model with ferromagnetic exchange interaction up to seventh-nearest neighbours. The spontaneous moment along the c-axis decreases with increasing field perpendicular to the c-axis, and disappears at the critical field Hc, which corresponds to the anomaly which appeared in the magnetization curve.
- Published
- 2003
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