1. Low-energy spin excitations in the molecular magnetic cluster V 15
- Author
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Grégory Chaboussant, P. Koegerler, Stefan T. Ochsenbein, Andreas Sieber, R.E. Lechner, H. U. Guedel, Arnaud Desmedt, Mark T. F. Telling, Reto Basler, and A. Mueller
- Subjects
Physics ,Strongly Correlated Electrons (cond-mat.str-el) ,Geometrical frustration ,FOS: Physical sciences ,General Physics and Astronomy ,Spectral line ,Inelastic neutron scattering ,Condensed Matter - Strongly Correlated Electrons ,Coupling (physics) ,Deuterium ,Cluster (physics) ,Condensed Matter::Strongly Correlated Electrons ,Atomic physics ,Ground state ,Spin (physics) - Abstract
We report an Inelastic Neutron Scattering (INS) study of the fully deuterated molecular compound K6[V15As6O42].9(D2O) (V15). Due to geometrical frustration, the essential physics at low temperatures of the V15 cluster containing 15 coupled V4+ (S=1/2) is determined by three weakly coupled spin-1/2 on a triangle. The INS spectra at low-energy allow us to directly determine the effective exchange coupling J0 = 0.211 meV within the triangle and the gap 2 \Delta = 0.035(2)meV between the two spin-1/2 doublets of the ground state. Results are discussed in terms of deviations from trigonal symmetry and Dzyaloshinskii-Moriya (DM) interactions., Comment: 8 pages, 4 figures. to appear in Europhysics Letters
- Published
- 2002
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