January 2014 saw the congregation in Abingdon (UK) of scientists from across the world, to discuss the current state and future of spectroscopy using epithermal neutrons. This meeting was the sixth in a series of workshops held in collaboration between the Science and Technology Facilities Council (UK) and the Consiglio Nazionale delle Ricerche (Italy), aimed at bringing together researchers with an interest in the use of electron-volt neutrons in spectroscopic studies [1]. This technique is termed Deep Inelastic Neutron Scattering (DINS), and also Neutron Compton Scattering (NCS) in reference to the analogy with Compton scattering of X-rays from electrons. In particular, this meeting centred jointly around experimentalists and theoreticians, formulating animated discussions as to the current overview of DINS and future horizons facing the field. The use of electron Volt neutrons for spectroscopic measurements dates back to the advent of proton-driven spallation neutron sources in the 1970s and 1980s. Following an initial scientific meeting in Los Alamos (USA) [2], the first two meetings in this series were held in Abingdon (UK) in 1995 and 1998, with subsequent meetings held in Santa Fe (USA) in 2005 [3], Oak Ridge National Laboratory (USA) in 2006 [4], and Rome, Italy; in 2010 [5]. The flagship instrument serving a continual user-programme for DINS measurements, and the main focus of this meeting, has been the VESUVIO spectrometer at ISIS [6, 7]. Subsequent instruments like SEQUOIA in the USA [8, 9] and a newer spectrometer in the Bariloche LINAC in Argentina [10, 11] have also been commissioned and began serving a growing user community. The availability of DINS measurements has extended the range of possible spectroscopic techniques that utilise neutrons into the kinematic region of high energy and momentum transfers, shown schematically in Figure 1. Spectroscopic instrument suites such as that of ISIS are thus able to probe processes on timescales across nine orders of magnitude, from quantum tunnelling and molecular diffusion up to nuclear recoil under the impulse approximation. DINS is one of the most direct techniques for probing nuclear quantum dynamics in condensed matter, with the ability to measure nuclear kinetic energies and momentum distributions of light nuclei. A major theme for current DINS research relates to the study of nuclear quantum effects, particularly regarding the non-classical behaviour of hydrogen or deuterium. This emphasis was reflected by the meeting's opening session dealing with the measurement of momentum distributions in hydrogen-bonded and aqueous systems (see Table 1). Whilst concentrating on experimental studies, data were presented from the outset alongside state-of-the-art path-integral molecular dynamics (PIMD) calculations, affording an animated discussion as to the interpretation of measured neutron Compton profiles in spatially disordered systems. The extension of DINS to heavier nuclei was visited in the second session of the meeting, under the over-arching theme of MAss-selective Neutron SpEctroscopy (MANSE). The ability of DINS to examine atomically distinct species in condensed matter has garnered interest from the chemistry and materials communities, with both binary systems and more complex materials being presented in this session. Nuclei of interest in applied materials research were highlighted, including oxygen, lithium and fluorine, alongside an assessment of current capabilities and future developments in their examination by DINS. The concluding session of the first day of the meeting was concerned with instrumentation. The detection of epithermal neutrons requires technologies unique relative to their lower-energy counterparts, and the first talk of this session outlined how detector capabilities on existing instruments has been revolutionised in recent years. Resonance detectors and techniques involving analyser-foil cycling were detailed, explaining how they have improved not only the count-rate but also the spectral resolution of instruments such as VESUVIO. Beyond NCS, the detection of nuclear resonances were also considered. An overview of VESUVIO (a time-of-flight instrument operating in so-called indirect geometry) was then given, alongside ways it could be improved upon in light of growing demands from the user community. This discussion was complemented by a presentation of the use of direct-geometry instruments such as SEQUOIA for DINS measurements, highlighting the complementarity with parallel studies on VESUVIO. The second day of the meeting was given over to the theoretical aspects of nuclear momentum distributions. Delegates were presented with the manner in which we can computationally incorporate nuclear quantum effects, along with their output in terms of 'measureables', relating to a varied range of systems. Results were presented from hydrogen-bonded liquids, ferroelectric materials, biological systems, and mixed bosonic-fermionic calculations. The ability to now approach experimental measurement with theoretical insight, and vice versa, is a sea-change in research into nuclear quantum effects. This field is a high-profile area in chemical physics and materials research, and a concerted approach by theory and experimentation allows us to explore and explain the dynamical state of matter at the atomic level in a manner previously unobtainable. Concluding each session throughout the meeting were periods of open discussion, wherein all present could comment or expand upon themes arising from the preceding talks. These discussions were then further distilled and clarified during the final section of the meeting, the 'Frontiers and Horizons' discussion, open to all present to delineate the next steps in DINS as a whole. Experimentalists and theoreticians were able to present their views on how each community could move forward to complement each other, not only separately but with specific projects and milestones in mind. These discussions have been included within these proceedings to highlight the future outlook of DINS. It is the hope of these editors that this meeting will allow spectroscopy with epithermal neutrons to further develop, explaining the very quantum nature of dynamics in condensed matter. Bringing together, as it did, international researchers in fields at the frontiers of their respective experimental and theoretical communities, we hope that the next meeting in this series will see the fruition of concepts and projects instigated by this one.