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1. Tandem Oxidation Process Using Ceric Ammonium Nitrate: Three-Component Synthesis of Trisubstituted Imidazoles Under Aerobic Oxidation Conditions

Author

Ali Maleki, Maryam Behnam, and Ahmad Shaabani

Subjects
Solvent, chemistry.chemical_compound, Ethanol, chemistry, Tandem, Organic Chemistry, food and beverages, Organic chemistry, Imidazole, Oxidation process, Condensation reaction, Ceric ammonium nitrate, Ammonium acetate
Abstract

By combining a ceric ammonium nitrate (CAN)–catalyzed aerobic oxidation of α-hydroxy ketones with a subsequent three-component condensation reaction using aldehydes and ammonium acetate, highly substituted imidazole derivatives can be assembled. This reaction is an important approach for the synthesis of highly substituted imidazole derivatives and was carried out in good to excellent yields in ethanol as an environmentally benign solvent.

Published
2008
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