1. Multiexciton recombination dynamics in CsPbBr3 perovskite nanocrystals revealed by femtosecond transient absorption and single dot spectroscopies
- Author
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Toshiharu Teranishi, Ryota Sato, Masaki Saruyama, Hirokazu Tahara, Tokuhisa Kawawaki, Naoki Yarita, Toshiyuki Ihara, and Yoshihiko Kanemitsu
- Subjects
Materials science ,Auger effect ,business.industry ,Exciton ,02 engineering and technology ,021001 nanoscience & nanotechnology ,symbols.namesake ,Semiconductor ,Ultrafast laser spectroscopy ,Femtosecond ,symbols ,Optoelectronics ,Spontaneous emission ,0210 nano-technology ,business ,Biexciton ,Perovskite (structure) - Abstract
Recently, metal-halide perovskite semiconductors have been extensively studied because of their potential use in solar-cell, photodetector, light-emitting-diode, and laser applications. In particular, perovskite nanocrystals (NCs) are gaining more and more attention because their optical spectra can be manipulated by changing the NC size and the halogen composition [1]. In contrast to the conventionally structured NCs such as colloidal CdSe NCs, high-quality perovskite NCs with unique cubic shapes and large sizes can be fabricated. However, their intrinsic photocarrier recombination dynamics have not yet been understood. Especially, the recombination dynamics of exciton complexes including biexcitons and charged excitons (trions) are complicated due to the fast Auger recombination [2]. Thus, a combination of different optical techniques for ensemble and single NC samples should be performed for a deep understanding of multiexciton dynamics in perovskites.
- Published
- 2017
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