1. Comparative assessment of TROPOMI and OMI formaldehyde observations and validation against MAX-DOAS network column measurements
- Author
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European Space Agency, Belgian Science Policy Office, Royal Belgian Institute for Space Aeronomy, German Centre for Air and Space Travel, University of Bremen, Max Planck Institute for Chemistry, Wageningen University and Research Centre, Environmental Restoration and Conservation Agency (Japan), Smedt, Isabelle de, Pinardi, Gaia, Vigouroux, Corinne, Compernolle, Steven, Bais, Alkis, Benavent, Nuria, Boersma, Folkert, Chan, K.L., Donner, Sebastian, Eichmann, K.U., Hedelt, Pascal, Hendrick, Francois, Irie, Hitoshi, Kumar, Vinod, Lambert, J. C., Langerock, Bavo, Lerot, C., Liu, Cheng, Loyola, Diego, Piters, Ankie, Richter, Andreas, Rivera Cárdenas, Claudia, Romahn, Fabian, Ryan, Robert G., Sinha, V., Theys, Nicolas, Vlietinck, Jonas, Wagner, Thomas, Wang, Teng, Yu, Huan, Van Roozendael, M., European Space Agency, Belgian Science Policy Office, Royal Belgian Institute for Space Aeronomy, German Centre for Air and Space Travel, University of Bremen, Max Planck Institute for Chemistry, Wageningen University and Research Centre, Environmental Restoration and Conservation Agency (Japan), Smedt, Isabelle de, Pinardi, Gaia, Vigouroux, Corinne, Compernolle, Steven, Bais, Alkis, Benavent, Nuria, Boersma, Folkert, Chan, K.L., Donner, Sebastian, Eichmann, K.U., Hedelt, Pascal, Hendrick, Francois, Irie, Hitoshi, Kumar, Vinod, Lambert, J. C., Langerock, Bavo, Lerot, C., Liu, Cheng, Loyola, Diego, Piters, Ankie, Richter, Andreas, Rivera Cárdenas, Claudia, Romahn, Fabian, Ryan, Robert G., Sinha, V., Theys, Nicolas, Vlietinck, Jonas, Wagner, Thomas, Wang, Teng, Yu, Huan, and Van Roozendael, M.
- Abstract
The TROPOspheric Monitoring Instrument(TROPOMI), launched in October 2017 on board the Sentinel-5 Precursor (S5P) satellite, monitors the composition of the Earth's atmosphere at an unprecedented horizontal resolution as fine as 3.5×5.5 km2. This paper assesses the performances of the TROPOMI formaldehyde(HCHO) operational product compared to its predecessor, the OMI (Ozone Monitoring Instrument) HCHO QA4ECV product, at different spatial and temporal scales. The parallel development of the two algorithms favoured the consistency of the products, which facilitates the production of long-term combined time series. The main difference between the two satellite products is related to the use of different cloud algorithms, leading to a positive bias of OMI compared to TROPOMI of up to 30% in tropical regions. We show that after switching off the explicit correction for cloud effects, the two datasets come into an excellent agreement. For medium to large HCHO vertical columns(larger than 5×1015 molec. cm-2) the median bias between OMI and TROPOMI HCHO columns is not larger than 10% (<0.4×1015 molec. cm-2). For lower columns, OMI observations present a remaining positive bias of about 20% (<0.8×1015 molec. cm-2) compared to TROPOMI in midlatitude regions. Here, we also use a global network of 18 MAX-DOAS (multi-axis differential optical absorption spectroscopy) instruments to validate both satellite sensors for a large range of HCHO columns. This work complements the study by Vigouroux et al. (2020), where a global FTIR(Fourier transform infrared) network is used to validate the TROPOMI HCHO operational product. Consistent with the FTIR validation study, we find that for elevated HCHO columns, TROPOMI data are systematically low (-25% for HCHO columns larger than 8 × 1015 molec. cm-2), while no significant bias is found for medium-range column values. We further show that OMI and TROPOMI data present equivalent biases for large HCHO levels. However, TROPOMI significantly i
- Published
- 2021