1. Soft x-ray induced femtosecond solid-to-solid phase transition
- Author
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Beata Ziaja, Mark J. Prandolini, T. Tanikawa, Franz Tavella, Hauke Höppner, Nikola Stojanovic, Michele Manfredda, Ulrich Teubner, Sven Toleikis, Emanuele Pedersoli, Torsten Golz, Nikita Medvedev, Flavio Capotondi, Yun Kai, and Victor Tkachenko
- Subjects
Nuclear and High Energy Physics ,Phase transition ,Atomic Physics (physics.atom-ph) ,Astrophysics::High Energy Astrophysical Phenomena ,FOS: Physical sciences ,02 engineering and technology ,Soft X-rays ,engineering.material ,01 natural sciences ,Physics - Atomic Physics ,0103 physical sciences ,Irradiation ,010306 general physics ,Physics ,Condensed Matter - Materials Science ,Radiation ,Materials Science (cond-mat.mtrl-sci) ,Diamond ,021001 nanoscience & nanotechnology ,Pulse (physics) ,Femtosecond ,engineering ,Transient (oscillation) ,Atomic physics ,0210 nano-technology ,Ultrashort pulse - Abstract
Soft x-rays were applied to induce graphitization of diamond through a non-thermal solid-to-solid phase transition. This process was observed within poly-crystalline diamond with a time-resolved experiment using ultrashort soft x-ray pulses of duration 52.5 fs and cross correlated by an optical pulse of duration 32.8 fs. This scheme enabled for the first time the measurement of a phase transition on a timescale of ~150 fs. Excellent agreement between experiment and theoretical predictions was found, using a dedicated code that followed the non-equilibrium evolution of the irradiated diamond including all transient electronic and structural changes. These observations confirm that soft x-rays can induce a non-thermal ultrafast solid-to-solid phase transition on a hundred femtosecond timescale., Comment: 27 pages, 17 figures (includes supplementary materials)
- Published
- 2017
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