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The explosive population growth and economic development in cities have led to continuous but diverse urban regionalization. The resulting urban agglomerations (UAs) exhibit differentiation at both regional and local scales. Few studies have documented the disparities in UAs regarding land use and geography. In this study, we investigated the county-level land use features of 19 China's planned UAs by using a land use intensity (LUI) metric. We employed the spatial autocorrelation, inequality statistics, and imbalance estimation models to estimate the agglomeration, inequalities, and coordination of land use, and we combined those indicators to distinguish the development pattern of all UAs. Our findings revealed that spatial pattern of LUIs and their autocorrelations over time are closely associated with the evolution of urban regionalization. The widening gaps of land use exist more within the UAs than among them. Based on the LUI inequality and its relations to population and economy, UAs were classified into core-driven, differentiated, coordinated, and mismatched ones. Our conclusions highlighted that policy incentives for sustainable urbanization help decouple the synchronism of socioeconomic and LUI inequality. • Spatial patterns of LUIs and their autocorrelation are closely associated with the evolution of urban regionalization. • The widening gaps of land use exist more within each UA than between UAs. • The LUI inequality and the imbalances between LUI and GDP/population jointly determine the development pattern of a UA. • Policy incentives for sustainable urbanization help decouple the synchronism of socioeconomic and LUI inequality. [ABSTRACT FROM AUTHOR]