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Basic dyes are highly toxic and have adverse effects on humans such as accelerated heart rate, shock, cyanosis, and tissue necrosis upon ingestion or skin contact. Efficient removal of basic dye pollutants from wastewater is therefore essential for the protection of the environment and human health. Biomolecules exhibit excellent dye removal performance in terms of removal capacity, selectivity, and rate. However, their poor thermal/chemical stability precludes their large-scale industrial applications. Herein, porous aromatic frameworks (PAFs) were utilized for the biomimetic construction of mussel, which included two unique features: (1) multistage pore structures for the rapid transport of dye contaminants and (2) mussel-inspired adhesive surfaces for cationic dye removal. Accordingly, the solid PAFs exhibited a record adsorption capacity of 7300 mg g -1 and ultrahigh adsorption rates for cationic dye (safranine T) (188.78 mg g -1  min -1 in the first 20 min). Notably, the bionic adsorbent system exhibited outstanding dye removal performance under various conditions such as after multiple reuse cycles, acid/alkali environments, presence of multiple anions, and in different water bodies (e.g., seawater, lake water, rainwater, and sanitary wastewater). This demonstrates the broad adaptability of the system and its ability to effectively deal with dye contamination in a variety of environments., Competing Interests: Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper., (Copyright © 2025 Elsevier Inc. All rights reserved.)