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Cyclones are essential components of weather patterns in the densely populated Mediterranean region, providing necessary rainfall for both the environment and human activities. The most intense of them also lead to natural disasters because of their strong winds and heavy precipitation. Identifying sources of errors in the predictability of Mediterranean cyclones is therefore essential to better anticipate and prevent their impact. The aim of this work is to characterise the medium-range cyclone predictability in the Mediterranean. Here, it is investigated in a systematic framework using the European Centre for Medium-Range Weather Forecasts fifth-generation reanalysis (ERA5) and ensemble reforecasts in a homogeneous configuration over the 2001–2021 period. First, a reference dataset of 1960 cyclones is obtained for the period by applying a tracking algorithm to the ERA5 reanalysis. Then the predictability is systematically evaluated in the ensemble reforecasts. It is quantified using a new probabilistic score based on the error distribution of cyclone location and intensity (mean sea level pressure). The score is firstly computed for the complete dataset and then for different categories of cyclones based on their intensity, deepening rate, motion speed, and geographic area and season in which they occur. When crossing the location and intensity errors with the different categories, the conditions leading to poorer or better predictability are discriminated. The motion speed of cyclones appears to be crucial for the predictability of the location: the slower the cyclone, the better the forecast location. In particular, the location of stationary lows located in the Gulf of Genoa is remarkably well predicted. The intensity of deep and rapid-intensification cyclones, occurring mostly during winter, is for its part particularly poorly predicted. This study provides the first systematic evaluation of cyclone predictability in the Mediterranean and opens up possibilities to identify the key processes leading to forecast errors in the region. [ABSTRACT FROM AUTHOR]

Mediterranean cyclones are essential components of the climate in a densely populated area, providing beneficial rainfall for both the environment and human activities. The most intense of them also lead to natural disasters because of their strong winds and heavy precipitation. Identifying error sources in the predictability of Mediterranean cyclones is therefore essential to better anticipate and prevent their impact. The aim of this work is to characterise the cyclone predictability in this region. Here, it is investigated in a systematic framework using European Centre for Medium range Weather Forecasting (ECMWF) fifth generation reanalysis (ERA5) and ensemble reforecasts in a homogeneous configuration over 20 years (2001–2021). First, a reference data set of 2853 cyclones is obtained for the period by applying a tracking algorithm to the ERA5 reanalysis. Then the predictability is systematically evaluated in the ensemble reforecasts. It is quantified using a new probabilistic score based on the error distribution of cyclone location and intensity (mean sea level pressure). The score is firstly computed for the complete data set and then for different categories of cyclones based on their intensity, deepening rate, velocity and on the geographic area and the season in which they occur. When crossing the location and intensity errors with the different categories, the conditions leading to a poorer or better predictability are discriminated. The velocity of cyclones appears to be determinant in the predictability of the location, the slower the cyclone the better the forecast location. Particularly, the position of stationary lows located in the Gulf of Genoa is remarkably well predicted. The intensity of deep and rapid-intensification cyclones, occurring mostly during winter, is for its part particularly poorly predicted. This study provides the first systematic evaluation of the cyclone predictability in the Mediterranean and opens the way to identify the key processes leading to forecast errors in the region. [ABSTRACT FROM AUTHOR]

Numerical atmospheric dispersion models (ADMs) are used for predicting the health and environmental consequences of nuclear accidents in order to anticipate countermeasures necessary to protect the populations. However, these simulations suffer from significant uncertainties, arising in particular from input data: weather conditions and source term. Meteorological ensembles are already used operationally to characterize uncertainties in weather predictions. Combined with dispersion models, these ensembles produce different scenarios of radionuclide dispersion, called "members", representative of the variety of possible forecasts. In this study, the fine-scale operational weather ensemble AROME-EPS (Applications of Research to Operations at Mesoscale-Ensemble Prediction System) from Météo-France is coupled with the Gaussian puff model pX developed by the IRSN (French Institute for Radiation Protection and Nuclear Safety). The source term data are provided at 10 min resolution by the Orano La Hague reprocessing plant (RP) that regularly discharges 85 Kr during the spent nuclear fuel reprocessing process. In addition, a continuous measurement campaign of 85 Kr air concentration was recently conducted by the Laboratory of Radioecology in Cherbourg (LRC) of the IRSN, within 20 km of the RP in the North-Cotentin peninsula, and is used for model evaluation. This paper presents a probabilistic approach to study the meteorological uncertainties in dispersion simulations at local and medium distances (2–20 km). First, the quality of AROME-EPS forecasts is confirmed by comparison with observations from both Météo-France and the IRSN. Then, the probabilistic performance of the atmospheric dispersion simulations was evaluated by comparison to the 85 Kr measurements carried out during a period of 2 months, using two probabilistic scores: relative operating characteristic (ROC) curves and Peirce skill score (PSS). The sensitivity of dispersion results to the method used for the calculation of atmospheric stability and associated Gaussian dispersion standard deviations is also discussed. A desirable feature for a model used in emergency response is the ability to correctly predict exceedance of a given value (for instance, a dose guide level). When using an ensemble of simulations, the "decision threshold" is the number of members predicting an event above which this event should be considered probable. In the case of the 16-member dispersion ensemble used here, the optimal decision threshold was found to be 3 members, above which the ensemble better predicts the observed peaks than the deterministic simulation. These results highlight the added value of ensemble forecasts compared to a single deterministic one and their potential interest in the decision process during crisis situations. [ABSTRACT FROM AUTHOR]

Numerical models of atmospheric dispersion are used for predicting the health and environmental consequences of nuclear accidents, in order to anticipate the countermeasures necessary to protect the populations. However, the simulations of these models suffer from significant uncertainties, arising in particular from input data: weather conditions and source term. To characterize weather uncertainties, it is essential to combine a well-known source term data and meteorological ensembles to generate ensemble dispersion simulations which has the potential to produce different possible scenarios of radionuclides dispersion during emergency situations. In this study, the fine-scale operational weather ensemble AROME-EPS from Météo-France is coupled to the Gaussian puff model pX developed by French Institute for Radiation Protection and Nuclear Safety (IRSN). The source term data is provided by Orano La Hague reprocessing plant (RP) that regularly discharges 85Kr during the spent nuclear fuel reprocessing process. Then, to evaluate the dispersion results, a continuous measurement campaign of 85Kr air concentration was recently conducted by the Laboratory of Radioecology in Cherbourg (LRC) of IRSN, around RP in the North-Cotentin peninsula. This paper presents a probabilistic approach to study the meteorological uncertainties in dispersion simulations at local and medium distances (2–20 km). As first step, the quality of AROME-EPS forecasts is confirmed by comparison with observations from both Météo-France and IRSN. The following step is to assess the probabilistic performance of the dispersion ensemble simulation, as well as the sensitivity of dispersion results to the method used to calculate atmospheric stability fields and their associated dispersion Gaussian standard deviations. Two probabilistic scores are used: Relative Operating Characteristic (ROC) curves and Peirce Skill Score (PSS). The results show that the stability diagnostics of Pasquill provides better dispersion simulations. In addition, the ensemble dispersion performs better than deterministic one, and the optimum decision threshold (PSS maximum) is 3 members. These results highlight the added value of ensemble forecasts compared to a single deterministic one, and their potential interest in the decision process during crisis situations. [ABSTRACT FROM AUTHOR]

Numerical dispersion models are used operationally worldwide to mitigate the effect of volcanic ash on aviation. In order to improve the representation of the horizontal dispersion of ash plumes and of the 3D concentration of ash, a study was conducted using the MOCAGE model during the European Natural Airborne Disaster Information and Coordination System for Aviation (EUNADICS-AV) project. Source term modelling and assimilation of different data were investigated. A sensitivity study of source term formulation showed that a resolved source term, using the FPLUME plume rise model in MOCAGE, instead of a parameterised source term, induces a more realistic representation of the horizontal dispersion of the ash plume. The FPLUME simulation provides more concentrated and focused ash concentrations in the horizontal and the vertical dimensions than the other source term. The assimilation of Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol optical depth has an impact on the horizontal dispersion of the plume, but this effect is rather low and local compared to source term improvement. More promising results are obtained with the continuous assimilation of ground-based lidar profiles, which improves the vertical distribution of ash and helps in reaching realistic values of ash concentrations. Using this configuration, the effect of assimilation may last for several hours and it may propagate several hundred kilometres downstream of the lidar profiles. [ABSTRACT FROM AUTHOR]

High-quality volcanic ash forecasts are crucial to minimize the economic impact of volcanic hazards on air traffic. Decision-making is usually based on numerical dispersion modelling with only one model realization. Given the inherent uncertainty of such an approach, a multi-model multi-source term ensemble has been designed and evaluated for the Eyjafjallajökull eruption in May 2010. Its use for flight planning is discussed. Two multi-model ensembles were built: the first is based on the output of four dispersion models and their own implementation of ash ejection. All a priori model source terms were constrained by observational evidence of the volcanic ash cloud top as a function of time. The second ensemble is based on the same four dispersion models, which were run with three additional source terms: (i) a source term obtained from a model background constrained with satellite data (a posteriori source term), (ii) its lower-bound estimate and (iii) its upper-bound estimate. The a priori ensemble gives valuable information about the probability of ash dispersion during the early phase of the eruption, when observational evidence is limited. However, its evaluation with observational data reveals lower quality compared to the second ensemble. While the second ensemble ash column load and ash horizontal location compare well to satellite observations, 3D ash concentrations are negatively biased. This might be caused by the vertical distribution of ash, which is too much diluted in all model runs, probably due to defaults in the a posteriori source term and vertical transport and/or diffusion processes in all models. Relevant products for the air traffic management are horizontal maps of ash concentration quantiles (median, 75 %, 99 %) at a finely resolved flight level grid as well as cross sections. These maps enable cost-optimized consideration of volcanic hazards and could result in much fewer flight cancellations, reroutings and traffic flow congestions. In addition, they could be used for route optimization in the areas where ash does not pose a direct and urgent threat to aviation, including the aspect of aeroplane maintenance. [ABSTRACT FROM AUTHOR]

High quality volcanic ash forecasts are crucial to minimize the economic impact of volcanic hazards on air traffic. Decision-making is usually based on numerical dispersion modeling with only one model realization. Given the inherent uncertainty of such approach, a multi-model multi-source term ensemble has been designed and evaluated for the Eyjafjallajökull eruption in May 2010. Its use for air traffic management is discussed. Two multi-model ensembles were built: the first is based on the output of four dispersion models and their own implementation of ash ejection. All a priori model source terms were constrained by observational evidence of the volcanic ash cloud top as a function of time. The second ensemble is based on the same four dispersion models, which were run with three additional source terms: (i) a source term obtained with background modeling constrained with satellite data (a posteriori source term), (ii) its lower bound estimate, and (iii) its upper bound estimate. The a priori ensemble gives valuable information about the probability of ash dispersion during the early phase of the eruption, when observational evidence is limited. However, its evaluation with observational data reveals lower quality compared to the second ensemble. While the second ensemble ash column load and ash horizontal location compare well to satellite observations, 3D ash concentrations are negatively biased. This might be caused by the vertical distribution of ash, which is too much diluted in all model runs, probably due to defaults in the a posteriori source term and vertical transport and/or diffusion processes in all models. Relevant products for the air traffic management are horizontal maps of ash concentration quantiles (median, 75 %, 99 %) at a fine-resolved flight level grid. These maps can be used for route optimization in the areas where ash does not pose a direct and urgent threat to aviation. Cost-optimized consideration of such hazards will result in much less impact on flight cancellations, reroutings, and traffic flow congestions. [ABSTRACT FROM AUTHOR]

This contribution addresses the characterization of the model-error covariance matrix from the new theoretical perspective provided by the parametric Kalman filter method which approximates the covariance dynamics from the parametric evolution of a covariance model. The classical approach to obtain the modified equation of a dynamics is revisited to formulate a parametric modelling of the model-error covariance matrix which applies when the numerical model is dissipative compared with the true dynamics. As an illustration, the particular case of the advection equation is considered as a simple test bed. After the theoretical derivation of the predictability-error covariance matrices of both the nature and the numerical model, a numerical simulation is proposed which illustrates the properties of the resulting model-error covariance matrix. [ABSTRACT FROM AUTHOR]

Volcanic eruptions comprise an important airborne hazard for aviation. Although significant events are rare, e.g. compared to the threat of thunderstorms, they have a very high impact. The current state of tools and abilities to mitigate aviation hazards associated with an assumed volcanic cloud was tested within an international demonstration exercise. Experts in the field assembled at the Schwarzenberg barracks in Salzburg, Austria, in order to simulate the sequence of procedures for the volcanic case scenario of an artificial eruption of the Etna volcano in Italy. The scope of the exercise ranged from the detection (based on artificial observations) of the assumed event to the issuance of early warnings. Volcanic-emission-concentration charts were generated applying modern ensemble techniques. The exercise products provided an important basis for decision-making for aviation traffic management during a volcanic-eruption crisis. By integrating the available wealth of data, observations and modelling results directly into widely used flight-planning software, it was demonstrated that route optimization measures could be implemented effectively. With timely and rather precise warnings available, the new tools and processes tested during the exercise demonstrated vividly that a vast majority of flights could be conducted despite a volcanic plume being widely dispersed within a high-traffic airspace over Europe. The resulting number of flight cancellations was minimal. [ABSTRACT FROM AUTHOR]

This contribution adresses the characterization of the model-error covariance matrix from the new theoretical perspective provided by the parametric Kalman filter method which approximates the covariance dynamics from the parametric evolution of a covariance model. The classical approach to obtain the modified equation of a dynamics is revisited to formulate a parametric diagnosis of the model-error covariance matrix. As an illustration, the particular case of the advection equation is considered as a simple test bed. After the theoretical derivation of both the forecast-error and the predictability-error covariance matrices, a numerical simulation is proposed which demonstrates the skill of the parametric methodology in reproducing the model-error covariance matrix information. [ABSTRACT FROM AUTHOR]

Multi-axis differential optical absorption spectroscopy (MAX-DOAS) tropospheric NO2 column retrievals from four European measurement stations are compared to simulations from five regional air quality models which contribute to the European regional ensemble forecasts and reanalyses of the operational Copernicus Atmosphere Monitoring Service (CAMS). Compared to other observational data usually applied for regional model evaluation, MAX-DOAS data are closer to the regional model data in terms of horizontal and vertical resolution, and multiple measurements are available during daylight, so that, for example, diurnal cycles of trace gases can be investigated. In general, there is good agreement between simulated and retrieved NO2 column values for individual MAX-DOAS measurements with correlations between 35 % and 70 % for individual models and 45 % to 75 % for the ensemble median for tropospheric NO2 vertical column densities (VCDs), indicating that emissions, transport and tropospheric chemistry of NOx are on average well simulated. However, large differences are found for individual pollution plumes observed by MAX-DOAS. Most of the models overestimate seasonal cycles for the majority of MAX-DOAS sites investigated. At the urban stations, weekly cycles are reproduced well, but the decrease towards the weekend is underestimated and diurnal cycles are overall not well represented. In particular, simulated morning rush hour peaks are not confirmed by MAX-DOAS retrievals, and models fail to reproduce observed changes in diurnal cycles for weekdays versus weekends. The results of this study show that future model development needs to concentrate on improving representation of diurnal cycles and associated temporal scalings. [ABSTRACT FROM AUTHOR]

Volcanic eruptions comprise one of the most important airborne hazards for aviation. Although significant events are rare, they have a very high impact. The current state of tools and abilities to mitigate aviation hazards associated with an assumed volcanic cloud was tested within an international demonstration exercise. Experts in the field assembled at the Schwarzenberg barracks in Salzburg, Austria, in order to simulate the sequence of procedures for the volcanic case scenario of an artificial eruption of Etna volcano in Italy. The scope of the exercise ranged from the detection of the assumed event to the issuance of early warnings. Volcanic emission concentration charts were generated applying modern ensemble techniques. The exercise products provided an important basis for decision making for aviation traffic management during a volcanic eruption crisis. By integrating the available wealth of data, observations and modelling results directly into a widely used flight planning software, it was demonstrated that route optimization measures could be implemented effectively. With timely and rather precise warnings available, the new tools and processes tested during the exercise demonstrated vividly that a vast majority of flights could be conducted despite a volcanic plume widely dispersed within a high-traffic airspace over Europe. The resulting number of flight cancellations was minimal. [ABSTRACT FROM AUTHOR]

The study assesses the possible benefit of assimilating aerosol optical depth (AOD) from the future space-borne sensor FCI (Flexible Combined Imager) for air quality monitoring in Europe. An observing system simulation experiment (OSSE) was designed and applied over a 4-month period, which includes a severe-pollution episode. The study focuses on the FCI channel centred at 444 nm, which is the shortest wavelength of FCI. A nature run (NR) and four different control runs of the MOCAGE chemistry transport model were designed and evaluated to guarantee the robustness of the OSSE results. The synthetic AOD observations from the NR were disturbed by errors that are typical of the FCI. The variance of the FCI AOD at 444 nm was deduced from a global sensitivity analysis that took into account the aerosol type, surface reflectance and different atmospheric optical properties. The experiments show a general benefit to all statistical indicators of the assimilation of the FCI AOD at 444 nm for aerosol concentrations at the surface over Europe, and also a positive impact during the severe-pollution event. The simulations with data assimilation reproduced spatial and temporal patterns of PM 10 concentrations at the surface better than those without assimilation all along the simulations and especially during the pollution event. The advantage of assimilating AODs from a geostationary platform over a low Earth orbit satellite has also been quantified. This work demonstrates the capability of data from the future FCI sensor to bring added value to the MOCAGE aerosol simulations, and in general, to other chemistry transport models. [ABSTRACT FROM AUTHOR]

Stratosphere-to-troposphere transport (STT) is an important natural source of tropospheric ozone, which can occasionally influence ground-level ozone concentrations relevant for air quality. Here, we analyse and evaluate the Copernicus Atmosphere Monitoring Service (CAMS) global and regional forecast systems during a deep STT event over Europe for the time period from 4 to 9 January 2017. The predominant synoptic condition is described by a deep upper level trough over eastern and central Europe, favouring the formation of tropopause folding events along the jet stream axis and therefore the intrusion of stratospheric ozone into the troposphere. Both global and regional CAMS forecast products reproduce the "hook-shaped" streamer of ozonerich and dry air in the middle troposphere depicted from the observed satellite images of water vapour. The CAMS global model successfully reproduces the folding of the tropopause at various European sites, such as Trapani (Italy), where a deep folding down to 550 hPa is seen. The stratospheric ozone intrusions into the troposphere observed by WOUDC ozonesonde and IAGOS aircraft measurements are satisfactorily forecasted up to 3 days in advance by the CAMS global model in terms of both temporal and vertical features of ozone. The fractional gross error (FGE) of CAMS ozone day 1 forecast between 300 and 500 hPa is 0.13 over Prague, while over Frankfurt it is 0.04 and 0.19, highlighting the contribution of data assimilation, which in most cases improves the model performance. Finally, the meteorological and chemical forcing of CAMS global forecast system in the CAMS regional forecast systems is found to be beneficial for predicting the enhanced ozone concentrations in the middle troposphere during a deep STT event. [ABSTRACT FROM AUTHOR]

The study assesses the possible benefit of assimilating Aerosol Optical Depth (AOD) from the future spaceborne sensor FCI (Flexible Combined Imager) for air quality monitoring in Europe. An Observing System Simulation Experiment (OSSE) was designed and applied over a 4-months period that includes a severe pollution episode. The study focuses on the FCI channel centred at 444 nm, which is the shortest wavelength of FCI. A Nature Run (NR) and four different Control Runs of the MOCAGE chemistry-transport model were designed and evaluated to guarantee the robustness of the OSSE results. The AOD synthetic observations from the NR were disturbed by errors that are typical of the FCI. The variance of the FCI AOD at 444 nm was deduced from a global sensitivity analysis that took into account the aerosol type, surface reflectance and different atmospheric optical properties. The experiments show a general benefit on all statistical indicators of the assimilation of the FCI AOD at 444 nm for aerosol concentrations at surface over Europe, and also a positive impact during the severe pollution event. The simulations with data assimilation reproduced spatial and temporal patterns of PM10 concentrations at surface better than without assimilation all along the simulations and especially during the pollution event. This work demonstrates the capability of data from the future FCI sensor to bring an added value to the MOCAGE aerosol simulations, and in general, to other chemistry transport models. [ABSTRACT FROM AUTHOR]

Tropospheric NO2 is hazardous to human health and can lead to tropospheric ozone formation, eutrophication of ecosystems and acid rain production. It is therefore important to establish accurate data based on models and observations to understand and monitor tropospheric NO2 concentrations on a regional and global scale. In the present study, MAX-DOAS tropospheric NO2 column retrievals from four European measurement stations are compared to regional model ensemble simulations. The latter are based on regional air quality models which contribute to the European regional ensemble forecasts and reanalyses of the operational Copernicus Atmosphere Monitoring Service (CAMS). Compared to other observational data usually applied for regional model validation, MAX-DOAS data is closer to the regional model data in terms of horizontal and vertical resolution and measurements are available during daylight. In general, there is a good agreement between simulated and retrieved NO2 column values for individual MAX-DOAS measurements with correlations between 45 and 75 % for tropospheric NO2 VCDs, indicating that the model ensemble represents the emission and tropospheric chemistry of NOx (NO + NO2) well. Pollution transport towards the stations is on average well represented by the models. However, large differences are found for individual pollution plumes. Seasonal cycles are overestimated, weekly cycles are reproduced well and diurnal cycles poorly represented by the model ensemble. In particular, simulated morning rush hour peaks are not confirmed by MAX-DOAS retrievals. Our results demonstrate that a large number of validation points are available from MAX-DOAS measurements, which should therefore be used more extensively in future regional air quality modelling studies. [ABSTRACT FROM AUTHOR]

A 6-models strong European ensemble of Copernicus Atmospheric Monitoring Service (CAMS) was run through the season of 2014 computing the olive pollen dispersion in Europe. The simulations have been compared with observations in 6 countries, members of the European Aeroallergen Network. Analysis was performed for individual models, the ensemble mean and median, and for a dynamically optimized combination of the ensemble members obtained via fusion of the model predictions with observations. The models, generally reproducing the olive season of 2014, showed noticeable deviations from both observations and each other. In particular, the season start was reported too early, by 8 days but for some models the error mounted to almost two weeks. For the season end, the disagreement between the models and the observations varied from a nearly perfect match up to two weeks too late. A series of sensitivity studies performed to understand the origin of the disagreements revealed crucial role of ambient temperature, especially systematic biases in its representation by meteorological models. A simple correction to the heat sum threshold eliminated the season shift but its validity in other years remains to be checked. The short-term features of the concentration time series were reproduced better suggesting that the precipitation events and cold/warm spells, as well as the large-scale transport were represented rather well. Ensemble averaging led to more robust results. The best skill scores were obtained with data fusion, which used the previous-days observations to identify the optimal weighting coefficients of the individual model forecasts. Such combinations were tested for the forecasting period up to 4 days and shown to remain nearly optimal throughout the whole period. [ABSTRACT FROM AUTHOR]

Atmospheric aerosols are of natural and anthropogenic origin. They are the subject of many researches because of their involvement particularly in the climate system and the air quality standards with significant induced effects on human health. Regional air quality is particularly affected by local anthropogenic aerosols as well as the long-range transport of desert dust, biomass fires or volcanic ash. The MOCAGE model is able to describe the three-dimensional evolution of several types of primary and secondary aerosols involved in the definition of air quality standards. The MOCAGE model is also coupled to an assimilation system capable of assimilating the Aerosol Optical Depth (AOD) or lidar profiles in order to better constrain the three-dimensional distribution of the total aerosol concentration. The objective of this contribution is to evaluate the ability of different aerosol products from multisensor instruments (AOD and lidar profiles) assimilated individually or in synergy to improve the three-dimensional concentration of the aerosol and particularly the air quality at local scale. [ABSTRACT FROM AUTHOR]