Search

Hyperfine structure (HFS) measurements of neutron-rich iridium isotopes $^{196,197,198}\mathrm{Ir}$ ($Z=77,\phantom{\rule{0.16em}{0ex}}N=119$--121) were performed via in-gas-cell laser resonance ionization spectroscopy at the KEK Isotope Separation System. Magnetic dipole moments $\ensuremath{\mu}$ and isotope shifts were determined from the HFS spectra. The variation of mean-square charge radii and quadrupole deformation parameters of these isotopes were evaluated from the isotope shifts. The $\ensuremath{\mu}$ value of $^{197}\mathrm{Ir}$ agreed with a theoretical value based on the strong coupling model, and the Ir nucleus was interpreted as prolately deformed by the theoretical calculations. The $\ensuremath{\mu}$ values of $^{196,198}\mathrm{Ir}$ were also compared with semiempirical values calculated based on the strong coupling model. From the comparison, we can suggest the possible spin values of ${I}^{\ensuremath{\pi}}=1,{2}^{\ensuremath{-}}$ for $^{196}\mathrm{Ir}$ and ${I}^{\ensuremath{\pi}}={1}^{\ensuremath{-}}$ for $^{198}\mathrm{Ir}$.

We performed in-gas-cell laser ionization spectroscopy of $^{194,196}\mathrm{Os}$, which were produced by multinucleon transfer reactions at the KEK Isotope Separation System (KISS). The nuclei of interest were identified through $\ensuremath{\beta}$-decay spectroscopy and a newly applied multireflection time-of-flight mass spectrograph (MRTOF-MS). From the study of laser resonance spectra, isotope shifts (ISs) of the transition ${\ensuremath{\lambda}}_{1}=247.758$ nm for $^{194}\mathrm{Os}$ and $^{196}\mathrm{Os}$ were measured for the first time. The change in the mean-square charge radius $\ensuremath{\delta}{\ensuremath{\langle}{r}^{2}\ensuremath{\rangle}}^{192,A}$ and the quadrupole deformation parameter ${\ensuremath{\langle}{\ensuremath{\beta}}_{2}^{2}\ensuremath{\rangle}}^{1/2}$ were deduced from the IS measurements. The results were compared with the theoretical calculations and the predicted shape transition at $^{194}\mathrm{Os}$ is discussed.

We studied multinucleon transfer reactions in the 197Au+130Te system at Elab=1.07 GeV by employing the PRISMA magnetic spectrometer coupled to a coincident detector. For each light fragment we constructed, in coincidence, the distribution in mass of the heavy partner of the reaction. With a Monte Carlo method, starting from the binary character of the reaction, we simulated the de-excitation process of the produced heavy fragments to be able to understand their final mass distribution. The total cross sections for pure neutron transfer channels have also been extracted and compared with calculations performed with the grazing code.

Magnetic dipole moment and mean-square charge radius of $^{199}$Pt ($I^{\pi}=$ 5/2$^-$) have been evaluated for the first time from the investigation of the hyperfine splitting of the $\lambda_1=$ 248.792 nm transition by in-gas-cell laser ionization spectroscopy. Neutron-rich nucleus $^{199}$Pt was produced by multi-nucleon transfer reaction at the KISS where the nuclear spectroscopy in the vicinity of $N=$ 126 is planed from the aspect of an astrophysical interest as well as the nuclear structure. Measured magnetic dipole moment $+$0.63(13)$\mu_{\rm N}$ is consistent with the systematics of those of nuclei with $I^{\pi}=$ 5/2$^-$. The deformation parameter $| ^{1/2}|$ evaluated from the isotope shift indicates the gradual shape change to spherical shape of platinum isotopes with increasing neutron number toward $N=$ 126.

The $^{8}\mathrm{Li}(\ensuremath{\alpha},n)^{11}\mathrm{B}$ reaction is regarded as the key reaction in the inhomogeneous big bang and in type-II supernova nucleosynthesis. Recently, the importance of this reaction to solving the $^{7}\mathrm{Li}$ problem, i.e., the inconsistency between the predicted and the observed primordial $^{7}\mathrm{Li}$ abundances, has also been noted. The most recent cross-section data published by our collaboration group in 2006 [H. Ishiyama et al., Phys. Lett. B 640, 82 (2006)] cover the 0.7- to 2.6-MeV energy region in the center-of-mass system. Here, we present additional data spanning the 0.45- to 1.8-MeV energy region. Thus, the predominant energy region for the big bang nucleosynthesis, corresponding to ${T}_{9}=1$ (where ${T}_{9}$ is a temperature unit equivalent to ${10}^{9}$ K), is almost completely spanned by the previous [H. Ishiyama et al., Phys. Lett. B 640, 82 (2006)] and present results together.

Using a multireflection time-of-flight mass spectrograph located after a gas cell coupled with the gas-filled recoil ion separator GARIS-II, the masses of several $\alpha$-decaying heavy nuclei were directly and precisely measured. The nuclei were produced via fusion-evaporation reactions and separated from projectilelike and targetlike particles using GARIS-II before being stopped in a helium-filled gas cell. Time-of-flight spectra for three isobar chains, $^{204}$Fr-$^{204}$Rn-$^{204}$At-$^{204}$Po, $^{205}$Fr- $^{205}$Rn-$^{205}$At-$^{205}$Po-$^{205}$Bi, and $^{206}$Fr-$^{206}$Rn-$^{206}$At, were observed. Precision atomic mass values were determined for $^{204-206}$Fr, $^{204,205}$Rn, and $^{204,205}$At. Identifications of $^{205}$Bi, $^{204,205}$Po, $^{206}$Rn, and $^{206}$At were made with N$\leq$10 detected ions, representing the next step toward use of mass spectrometry to identify exceedingly low-yield species such as superheavy element ions., 多反射時間飛行質量分析装置を理化学研究所設置の気体充填型反跳分離装置-II型(GARIS-II)と連結したガスセルに配置し、$\alpha$崩壊連鎖を伴う重原子核の質量の直接測定を実施した。融合-蒸発反応で生成された原子核をGARIS-IIを用いて分離し、ヘリウムガスセルで止めて目的の原子核を捕集した。本実験で$^{204}$Fr-$^{204}$Rn-$^{204}$At-$^{204}$Po, $^{205}$Fr-$^{205}$Rn-$^{205}$At-$^{205}$Po-$^{205}$Bi及び$^{206}$Fr-$^{206}$Rn-$^{206}$Atの3つの同重体鎖の時間飛行スペクトルが観測された。その結果、$^{204-206}$Fr, $^{204,205}$Rn、そして$^{204,205}$Atの原子質量値が精密に決定された、今回の解析において、$^{205}$Bi, $^{204,205}$Po, $^{206}$Rn、そして$^{206}$Atの同定は10個以下という少量のイオン数でなされた。この成果は 次のステップとして実施する予定である(生成量が極少量の)超重元素イオンの質量分析につながる成果となる。

We investigate the possibilities of producing neutron-rich nuclides in projectile fission of heavy beams in the energy range of 20 MeV/nucleon expected from low-energy facilities. We report our efforts to theoretically describe the reaction mechanism of projectile fission following a multinucleon transfer collision at this energy range. Our calculations are mainly based on a two-step approach: the dynamical stage of the collision is described with either the phenomenological Deep-Inelastic Transfer model (DIT), or with the microscopic Constrained Molecular Dynamics model (CoMD). The deexcitation/fission of the hot heavy projectile fragments is performed with the Statistical Mul- tifragmentation Model (SMM). We compared our model calculations with our previous experimental projectile-fission data of 238U (20 MeV/nucleon)+208Pb and 197Au (20 MeV/nucleon)+197Au and found an overall reasonable agreement. Our study suggests that projectile fission following periph- eral heavy-ion collisions at this energy range offers an effective route to access very neutron-rich rare isotopes toward and beyond the astrophysical r-process path.

This work aims at investigating the projectile binding energy influence on the reaction dynamics, introducing new results and new data analysis methods in order to overcome some typically encountered problems, such as the identification of reaction products differing by few mass units and the discrimination of direct reaction processes. The $^{17}\mathrm{O}+^{58}\mathrm{Ni}$ collision was studied at five near-barrier energies employing a compact experimental setup consisting of four double-sided silicon strip detectors (DSSSDs). Different reaction processes, namely the elastic and inelastic scattering and the $1n$ stripping, were discriminated by means of a detailed analysis of the experimental energy spectra based on Monte Carlo simulations. The elastic scattering angular distributions were investigated within the framework of the optical model using Woods-Saxon and double-folding potentials. The total reaction cross sections were extracted and the reduced cross sections compared with those obtained for $^{17}\mathrm{F}$ (${S}_{p}=0.600$ MeV), the mirror nucleus of $^{17}\mathrm{O}$ (${S}_{n}=4.143$ MeV), and for the tightly bound $^{16}\mathrm{O}$ projectile. The $^{17}\mathrm{O}+^{58}\mathrm{Ni}$ total reaction cross sections were larger than those for $^{16}\mathrm{O}$ on the same target at the lowest energies studied, becoming identical, within errors, as the incident energy increased above the Coulomb barrier. This behavior was related to a strong contribution from the $1n$-stripping channel at the lowest energies.

Velocity correlations of intermediate mass fragments (IMFs), produced in central collisions of Au+Au at 150 MeV beam energy, are extracted from measurements with the FOPI (phase I) detector system at SIS in GSI Darmstadt. The IMF correlation function for semicentral events is found to be affected by the directed sideward flow. When rotating the events into a unique reaction plane an enhancement of correlations, resulting from event mixing effects, vanishes. Selecting violent collisions with a high degree of azimuthal symmetry the correlation function appears nearly independent of additional event or single particle gate conditions. The comparison of the data with a Coulomb dominated final-state interaction model points to an expanding and multifragmenting soure with radius [ital R][similar to]14 fm.

Charged particles have been observed in collisions of Au on Au at an incident energy of 150{ital A} MeV using a high-granularity detector system covering approximately the forward hemisphere in the center-of-mass system. Highly central collisions have been studied using a double selection criterion which combines large charged-particle multiplicities with small transverse-momentum directivities. In this class of events about one quarter of the total nuclear charge emerges as intermediate-mass fragments with nuclear charges {ital Z}{gt}2. These fragments are centered at midrapidity and are produced with large transverse velocities.

The {sup 20}Ne(p,t)h{sup 18}Ne reaction has been studied in order to investigate the properties of {sup 18}Ne excited states. A missing 3{sup +} state of {sup 18}Ne, which could have a great influence on the {sup 17}F(p,{gamma})h{sup 18}Ne reaction rate, was searched for, but the existence of this state was not clearly verified. The spins and parities of the 5.11- and 5.15-MeV states were assigned tentatively by angular distribution measurements, as 2{sup +} and 3{sup {minus}}, respectively. We were able to resolve the doublets at 4.5, 5.1, and 6.3 MeV clearly for the first time due to our high precision system, which allowed us to determine the widths of some critical states above the proton threshold of {sup 18}Ne more precisely. {copyright} {ital 1999} {ital The American Physical Society}

We measured evaporation residue (ER) cross sections of the fusion reactions $^{86}\mathrm{Kr}+^{134,138}\mathrm{Ba}$ to investigate the effect of the shell structure of the interacting nuclei on the fusion process. The measured ER cross sections for the reaction $^{86}\mathrm{Kr}+^{138}\mathrm{Ba}$ have a sizable component, 37 nb, at the excitation energy (${E}_{\mathrm{ex}}$) of 12.1 MeV. However, there is no evaporation residue for the reaction $^{86}\mathrm{Kr}+^{134}\mathrm{Ba}$ below the energy ${E}_{\mathrm{ex}}=24.7$ MeV. This result suggests that the neutron shell closure ($N=82$) of $^{138}\mathrm{Ba}$ plays a crucial role in the formation of the compound nucleus.

The ground state and low-lying levels of the unbound ${}^{11}\mathrm{N}$ nucleus were investigated with the three-neutron pickup reaction ${}^{14}\mathrm{N}{(}^{3}\mathrm{He}{,}^{6}\mathrm{He}{)}^{11}\mathrm{N}.$ The energies and widths of these, experimentally observed, levels are compared with other measurements and calculations. Angular distributions were measured for the first time for this reaction. The distorted-wave Born approximation analysis confirms the spin assignments for the lowest levels.

Reaction mechanisms and multifragmentation processes have been studied for Zn-64 + Ni-58 collisions at intermediate energies with the help of antisymmetrized molecular dynamics (AMD-V) model calculations. Experimental energy spectra, angular distributions, charge distributions, and isotope distributions, classified by their associated charged particle multiplicities, are compared with the results of the AMD-V calculations. In general the experimental results are reasonably well reproduced by the calculations. The multifragmentation observed experimentally at all incident energies is also reproduced by the AMD-V calculations. A detailed study of AMD-V events reveals that, in nucleon transport, the reaction shows some transparency, whereas in energy transport the reaction is much less transparent at all incident energies studied here. The transparency in the nucleon transport indicates that. even for central collisions, about 75% of the projectile nucleons appear in the forward direction. In energy transport about 80% of the initial kinetic energy of the projectile in the center-of-mass frame is dissipated. The detailed study of AMD-V events also elucidates the: dynamics of the multifragmentation process. The study suggests that, at 35A MeV, the semitransparency and thermal expansion are the dominant mechanisms for the multifragmentation process, whereas at 49A MeV and higher incident energies a nuclear compression occurs at an early stage of the reaction and plays an important role in the multifragmentation process in addition to that of the thermal expansion and the semitransparency.