1. StellarAr36,38(n,γ)Ar37,39Reactions and Their Effect on Light Neutron-Rich Nuclide Synthesis
- Author
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D. Veltum, Bradley S. Meyer, R. C. Pardo, Mario Weigand, Daniel Baggenstos, D. Kijel, N. Hazenshprung, Rashi Talwar, Philippe Collon, R. C. Vondrasek, I. Silverman, R. Scott, Yoav Kashiv, Rene Reifarth, M. Tessler, Asher Shor, Sergio Almaraz-Calderon, Roland Purtschert, Melina Avila, A. Kreisel, Shlomi Halfon, K. E. Rehm, Daniel Santiago-Gonzalez, Michael Paul, and Leonid Weissman
- Subjects
Physics ,010308 nuclear & particles physics ,Analytical chemistry ,General Physics and Astronomy ,7. Clean energy ,01 natural sciences ,Stellar nucleosynthesis ,13. Climate action ,Neutron flux ,0103 physical sciences ,Neutron source ,Neutron ,Nuclide ,010306 general physics ,s-process ,Mass fraction ,Accelerator mass spectrometry - Abstract
The ^{36}Ar(n,γ)^{37}Ar (t_{1/2}=35 d) and ^{38}Ar(n,γ)^{39}Ar (269 yr) reactions were studied for the first time with a quasi-Maxwellian (kT∼47 keV) neutron flux for Maxwellian average cross section (MACS) measurements at stellar energies. Gas samples were irradiated at the high-intensity Soreq applied research accelerator facility-liquid-lithium target neutron source and the ^{37}Ar/^{36}Ar and ^{39}Ar/^{38}Ar ratios in the activated samples were determined by accelerator mass spectrometry at the ATLAS facility (Argonne National Laboratory). The ^{37}Ar activity was also measured by low-level counting at the University of Bern. Experimental MACS of ^{36}Ar and ^{38}Ar, corrected to the standard 30 keV thermal energy, are 1.9(3) and 1.3(2) mb, respectively, differing from the theoretical and evaluated values published to date by up to an order of magnitude. The neutron-capture cross sections of ^{36,38}Ar are relevant to the stellar nucleosynthesis of light neutron-rich nuclides; the two experimental values are shown to affect the calculated mass fraction of nuclides in the region A=36-48 during the weak s process. The new production cross sections have implications also for the use of ^{37}Ar and ^{39}Ar as environmental tracers in the atmosphere and hydrosphere.
- Published
- 2018