1. Orbitally driven spin pairing in the three-dimensional nonmagnetic Mott insulatorBaVS3:Evidence from single-crystal studies
- Author
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F. Zámborszky, L. Forró, Karlo Penc, I. Kézsmárki, G. Mihály, Marko Miljak, Helmuth Berger, and P. Fazekas
- Subjects
Physics ,Phase transition ,Condensed matter physics ,Mott insulator ,02 engineering and technology ,021001 nanoscience & nanotechnology ,01 natural sciences ,Magnetic anisotropy ,Electrical resistivity and conductivity ,Pairing ,0103 physical sciences ,Condensed Matter::Strongly Correlated Electrons ,Strongly correlated material ,Metal–insulator transition ,010306 general physics ,0210 nano-technology ,Single crystal - Abstract
Static electrical and magnetic properties of single crystal ${\mathrm{BaVS}}_{3}$ were measured over the structural ${(T}_{S}=240\mathrm{K}),$ metal insulator ${(T}_{\mathrm{MI}}=69\mathrm{K}),$ and suspected orbital ordering ${(T}_{X}=30\mathrm{K})$ transitions. The resistivity is almost isotropic both in the metallic and insulating states. An anomaly in the magnetic anisotropy at ${T}_{X}$ signals a phase transition to an ordered low-T state. The results are interpreted in terms of orbital ordering and spin pairing within the lowest crystal-field quasidoublet. The disordered insulator at ${T}_{X}lTl{T}_{\mathrm{MI}}$ is described as a classical liquid of nonmagnetic pairs.
- Published
- 2000
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