Search

The structure of Po-208 populated through the EC/beta(+) decay of At-208 is investigated using gamma-ray spectroscopy at the ISOLDE Decay Station. The presented level scheme contains 27 new excited states and 43 new transitions, as well as a further 50 previously observed. rays which have been (re)assigned a position. The level scheme is compared to shell model calculations. Through this analysis approximately half of the beta-decay strength of At-208 is found to proceed via allowed decay and half via first-forbidden decay. The first-forbidden transitions predominantly populate core excited states at high excitation energies, which is qualitatively understood using shell model considerations. This mass region provides an excellent testing ground for the competition between allowed and first-forbidden beta-decay calculations, important for the detailed understanding of the nucleosynthesis of heavy elements.

We report on spectroscopic information and lifetime measurements of even-even neutron-rich Te isotopes. Excited states were populated in fast-neutron induced fission of U238 at the ALTO facility of IJCLab with the LICORNE neutron source and detected using the hybrid ν-ball spectrometer. We provide first results on lifetimes of the 61+ state in Te136 and the (61+), (41+), and (21+) states in Te138 and discuss the results in the context of large-scale shell-model calculations. The level schemes of Te136 and Te138 are revised in terms of lifetimes of their 21+,41+ states and updated information on the (42+) state in Te136 is presented. In addition, previously reported data on spectroscopy and lifetimes in Te134 are reexamined. This work provides new insights into the evolution of collectivity for Te isotopes with N=82,84,86.

Prompt and delayed γ -ray spectroscopy of the neutron-rich 94 Kr was performed, as part of the fission campaign at the ALTO facility of the IPN Orsay, using the fast-neutron-induced fission reaction 238 U ( n , f ) in combination with the ν -Ball array, a novel hybrid γ spectrometer for energy and lifetime measurements. Several new yrast and nonyrast transitions were observed for the first time, extending the previously known level scheme. Additionally, we report on the observation of a new short-lived isomer at 3444 keV with a half-life of 32(3) ns. The analysis of the Nilsson orbitals obtained from Gogny cranked Hartree-Fock-Bogoliubov calculations suggests a ( 9 − ) spin and an oblate deformation for this isomer corresponding to a two-quasineutron state, indicating an isomeric structure very similar to that of the neighboring isotones 96 Sr and 92 Se

The β decay of ^{208}Hg into the one-proton hole, one neutron-particle _{81}^{208}Tl_{127} nucleus was investigated at CERN-ISOLDE. Shell-model calculations describe well the level scheme deduced, validating the proton-neutron interactions used, with implications for the whole of the N>126, Z

The beta-decay of Zn-81 to the neutron magic N = 50 nucleus Ga-81, with only three valence protons with respect to Ni-78, was investigated. The study was performed at the ISOLDE facility at CERN by means of gamma spectroscopy. The 81Zn half-life was determined to be T-1/2 = 290(4) ms while the beta-delayed neutron emission probability was measured as P-n = 23(4)%. The analysis of the beta-gated gamma-ray singles and gamma-gamma coincidences from the decay of Zn-81 provides 47 new levels and 70 new transitions in Ga-81. The beta(-)n decay of Zn-81 was observed and a new decay scheme into the odd-odd Ga-80 nucleus was established. The half-lives of the first and second excited states of Ga-81 were measured via the fast-timing method using LaBr3(Ce) detectors. The level scheme and transition rates are compared to large-scale shell-model calculations. The low-lying structure of (81)Gais interpreted in terms of the coupling of the three valence protons outside the doubly magic Ni-78 core.

Twenty-one two-proton knockout (p; 3p) cross sections from neutron-rich nuclei at ~ 250 MeV/nucleon were measured. For the first time, the angular distribution of the three emitted protons were measured in coincidence with the tracker and hydrogen target MINOS, demonstrating that the (p; 3p) kinematics is consistent with two sequential proton-proton collisions within the projectile nucleus. Ratios of (p; 3p) over (p; 2p) inclusive cross sections follow the trend of other many-proton (neutron) removal reactions, further reinforcing the sequential nature of (p; 3p) in neutron-rich nuclei.

Here we present new information on the shape evolution of the very neutron-rich ^{92,94}Se nuclei from an isomer-decay spectroscopy experiment at the Radioactive Isotope Beam Factory at RIKEN. High-resolution germanium detectors were used to identify delayed γ rays emitted following the decay of their isomers. New transitions are reported extending the previously known level schemes. The isomeric levels are interpreted as originating from high-K quasineutron states with an oblate deformation of β∼0.25, with the high-K state in ^{94}Se being metastable and K hindered. Following this, ^{94}Se is the lowest-mass neutron-rich nucleus known to date with such a substantial K hindrance. Furthermore, it is the first observation of an oblate K isomer in a deformed nucleus. This opens up the possibility for a new region of K isomers at low Z and at oblate deformation, involving the same neutron orbitals as the prolate orbitals within the classic Z∼72 deformed hafnium region. From an interpretation of the level scheme guided by theoretical calculations, an oblate deformation is also suggested for the ^{94}Se_{60} ground-state band.

The β decay of 207Hg into the single-proton-hole nucleus 207Tl has been studied through γ-ray spectroscopy at the ISOLDE Decay Station (IDS) with the aim of identifying states resulting from coupling of the πs−11/2, πd−13/2, and πh−111/2 shell model orbitals to the collective octupole vibration. Twenty-two states were observed lying between 2.6 and 4.0 MeV, eleven of which were observed for the first time, and 78 new transitions were placed. Two octupole states (s1/2-coupled) are identified and three more states (d3/2-coupled) are tentatively assigned using spin-parity inferences, while further h11/2-coupled states may also have been observed for the first time. Comparisons are made with state-of-the-art large-scale shell model calculations and previous observations made in this region, and systematic underestimation of the energy of the octupole vibrational states is noted. We suggest that in order to resolve the difference in predicted energies for collective and noncollective t=1 states (t is the number of nucleons breaking the 208Pb core), the effect of t=2 mixing may be reduced for octupole-coupled states. The inclusion of mixing with t=0,2,3 excitations is necessary to replicate all t=1 state energies accurately.

We report on the measurement of lifetimes of excited states in the near-mid-shell nuclei Dy164,166 using the gamma-ray coincidence fast-timing method. The nuclei of interest were populated using reactions between an O18 beam and a gold-backed isotopically enriched Dy164 target of thickness 6.3mg/cm2 at primary beam energies of 71, 76, and 80 MeV from the IPN-Orsay laboratory, France. Excited states were populated in Dy164, Dy166, and W178,179 following Coulomb excitation, inelastic nuclear scattering, two-neutron transfer, and fusion-evaporation reaction channels respectively. Gamma rays from excited states were measured using the ν-Ball high-purity germanium (HPGe)-LaBr3 hybrid γ-ray spectrometer with the excited state lifetimes extracted using the fast-timing coincidence method using HPGe-gated LaBr3-LaBr3 triple coincident events. The lifetime of the first Iπ=2+ excited state in Dy166 was used to determine the transition quadrupole deformation of this neutron-rich nucleus for the first time. The experimental methodology was validated by showing consistency with previously determined excited state lifetimes in Dy164. The half-lives of the yrast 2+ states in Dy164 and Dy166 were 2.35(6) and 2.3(2) ns, respectively, corresponding to transition quadrupole moment values of Q0=7.58(9) and 7.5(4) eb, respectively. The lifetime of the yrast 2+ state in Dy166 is consistent with a quenching of nuclear quadrupole deformation at β≈0.35 as the N=104 mid-shell is approached.

Using a hybrid Gammasphere array coupled to 25 LaBr3(Ce) detectors, the lifetimes of the first three levels of the yrast band in ¹¹⁴Pd populated via ²⁵²Cf decay, have been measured. The measured lifetimes are τ₂+=103(10)ps, τ₄+=22(13)ps, and τ₆+≤10ps for the 2⁺₁, 4⁺₁, and 6⁺₁ levels, respectively. Palladium-114 was predicted to be the most deformed isotope of its isotopic chain, and spectroscopic studies have suggested it might also be a candidate nucleus for low-spin stable triaxiality. From the lifetimes measured in this work, reduced transition probabilities B(E2;J→J−2) are calculated and compared with interacting boson model, projected shell model, and collective model calculations from the literature. The experimental ratio RB(E₂)=B(E2;4⁺₁→2⁺₁)/B(E2;2⁺₁→0⁺₁)=0.80(42) is measured for the first time in ¹¹⁴Pd and compared with the known values RB(E₂) in the palladium isotopic chain: the systematics suggest that, for N=68, a transition from γ-unstable to a more rigid γ-deformed nuclear shape occurs.

Fifty-five inclusive single nucleon removal cross sections from medium mass neutron-rich nuclei impinging on a hydrogen target at � 250 MeV/nucleon were measured at the RIKEN Radioactive Isotope Beam Factory. Systematically higher cross sections are found for proton removal from nuclei with an even number of protons compared to odd-proton number projectiles for a given neutron separation energy. Neutron removal cross sections display no even-odd splitting contrary to nuclear cascade model predictions. Both effects are understood through simple considerations of neutron separation energies and bound state level densities originating in pairing correlations in the daughter nuclei. These conclusions are supported by comparison with semi-microscopic model predictions,highlighting the enhanced role of low-lying level densities in nucleon removal cross sections from loosely-bound nuclei.

Mean lifetimes of yrast states of the isotopes 174,176,178,180Hf have been measured using fast- electronic scintillation timing. Excited states of 74,176,178Hf were populated via β decay, while 180Hf was populated via Coulomb excitation. The lifetimes of the 2+ 1 and 4+ 1 states of all isotopes and the lifetimes of the 6+ 1 states of 174,178Hf were measured, using the slope and the centroid shift methods. The mean lifetime, τ (4+ 1 ) = 85(13) ps, of 178Hf has been determined for the first time. In addition, the mean lifetimes of the 2− 1 and the 3− 1 states of 176Hf have been determined. Systematic uncertainties on the evolution of data as a function of neutron number were reduced by using the same setup for all the isotopes of interest. The data are in agreement with other recent lifetime measurements where available and shows a shift of the maximum of collectivity for the Hf isotopic chain from neutron midshell at N = 104 to N = 100.

The existence of two close-lying nuclear states in ⁷³Ga has recently been experimentally determined: a 1/2⁻ spin-parity for the ground state was measured in a laser spectroscopy experiment, while a J_π = 3/2⁻ level was observed in transfer reactions. This scenario is supported by Coulomb excitation studies, which set a limit for the energy splitting of 0.8 keV. In this work, we report on the study of the excited structure of ⁷³Ga populated in the β decay of ⁷³Zn produced at ISOLDE, CERN. Using β-gated, γ-ray singles, and γ –γ coincidences, we have searched for energy differences to try to delimit the ground-state energy splitting, providing a more stringent energy difference limit. Three new half-lives of excited states in ⁷³Ga have been measured using the fast-timing ;method with LaBr₃(Ce) detectors. From our study, we help clarify the excited structure of ⁷³G and we extend the existing ⁷³Zn decay to ⁷³Ga with 8 new energy levels and 35 γ transitions. We observe a 195-keV transition consistent with a γ ray de-exciting a short-lived state in the β-decay parent ⁷³Zn.

ray transitions between low-spin states of the neutron-rich 84;86;88Ge were measured by means of in-flight -ray spectroscopy at 270 MeV/u. Excited 6+ 1 , 4+ 1;2 and 2+ 1;2 states of 84;86Ge and 4+ 1 and 2+ 1;2 states of 88Ge were observed. Furthermore a candidate for a 3+ 1 state of 86Ge was identified. This state plays a key role in the discussion of ground-state triaxiality of 86Ge, along with other features of its low-energy level scheme. A new region of triaxially deformed nuclei is proposed in the Ge isotopic chain.

We report on the first γ-ray spectroscopy of low-lying states in neutron-rich 98,100Kr isotopes obtained from 99,101Rb(p,2p) reactions at ∼ 220 MeV/nucleon. A reduction of the 2+ 1 state energies beyond N = 60 demonstrates a significant increase of deformation, shifted in neutron number compared to the sharper transition observed in strontium and zirconium isotopes. State-of-theart beyond-mean-field calculations using the Gogny D1S interaction predict level energies in good agreement with experimental results. The identification of a low-lying (0+ 2 , 2+ 2 ) state in 98Kr provides the first experimental evidence of a competing configuration at low energy in neutron-rich krypton isotopes consistent with the oblate-prolate shape coexistence picture suggested by theory

The properties of excited states in the neutron-rich nucleus 194Os have been investigated using the 192Os(18O,16O)194Os reaction with an 80 MeV beam provided by the IFIN-HH Laboratory, Bucharest. Discrete γ -ray decays from excited states have been measured using the hybrid HPGe-LaBr3(Ce) array RoSPHERE. The current work identifies a number of previously unreported low-lying nonyrast states in 194Os as well as the first measurement of the half-life of the yrast 2+ state of 302(50) ps. This is equivalent to a B(E2 : 2+ → 0+) = 45(16) W.u. and intrinsic quadrupole deformation of βeff = 0.14(1). The experimental results are compared with Hartree-Fock-Bogoliubov–interacting-boson-model calculations and are consistent with a reduction in a quadrupole collectivity in Os isotopes with increasing neutron number.

The first measurement of the low-lying states of the neutron-rich 110 Zr and 112 Mo was performed via in-beam γ -ray spectroscopy after one proton removal on hydrogen at ∼ 200 MeV / nucleon . The 2 + 1 excitation energies were found at 185(11) keV in 110 Zr , and 235(7) keV in 112 Mo , while the R 42 = E ( 4 + 1 ) / E ( 2 + 1 ) ratios are 3.1(2), close to the rigid rotor value, and 2.7(1), respectively. These results are compared to modern energy density functional based configuration mixing models using Gogny and Skyrme effective interactions. We conclude that first levels of 110 Zr exhibit a rotational behavior, in agreement with previous observations of lighter zirconium isotopes as well as with the most advanced Monte Carlo shell model predictions. The data, therefore, do not support a harmonic oscillator shell stabilization scenario at Z = 40 and N = 70 . The present data also invalidate predictions for a tetrahedral ground state symmetry in 110 Zr .

The B(E2) excitation strength of the first excited 2(+) state in even-even nuclei should directly correlate with the size of the valence space and maximize at mid-shell. A previously found saturation of B(E2) strengths in well-deformed rotors at mid-shell is tested through high-precision measurements of the lifetimes of the lowest-lying 2(+) states of the Hf-168 and W-174 rare earth isotopes. Measurements were performed using fast LaBr3 scintillation detectors. Combined with the recently remeasured B(E2; 2(1)(+) -> 0(1)(+)) values for Hf and W isotopes the new data remove discrepancies observed in the differentials of B(E2) values for these isotopes.

Background: The available data for $E2$ transition strengths in the region between neutron-deficient hafnium and platinum isotopes are far from complete. More and precise data are needed to enhance the picture of structure evolution in this region and to test state-of-the-art nuclear models. In a simple model, the maximum collectivity is expected at the middle of the major shell. However, for actual nuclei, particularly in heavy-mass regions, which should be highly complex, this picture may no longer be the case, and one should use a more realistic nuclear-structure model. We address this point by studying the spectroscopy of Hf as a representative case.Purpose: We remeasure the ${2}_{1}^{+}$ half-lives of $^{172,174,176}\mathrm{Hf}$, for which there is some disagreement in the literature. The main goal is to measure, for the first time, the half-lives of higher-lying states of the rotational band. The new results are compared to a theoretical calculation for absolute transition strengths.Method: The half-lives were measured using $\ensuremath{\gamma}\text{\ensuremath{-}}\ensuremath{\gamma}$ and conversion-electron-$\ensuremath{\gamma}$ delayed coincidences with the fast timing method. For the determination of half-lives in the picosecond region, the generalized centroid difference method was applied. For the theoretical calculation of the spectroscopic properties, the interacting boson model is employed, whose Hamiltonian is determined based on microscopic energy-density functional calculations.Results: The measured ${2}_{1}^{+}$ half-lives disagree with results from earlier $\ensuremath{\gamma}\text{\ensuremath{-}}\ensuremath{\gamma}$ fast timing measurements, but are in agreement with data from Coulomb excitation experiments and other methods. Half-lives of the ${4}_{1}^{+}$ and ${6}_{1}^{+}$ states were measured, as well as a lower limit for the ${8}_{1}^{+}$ states.Conclusions: This work shows the importance of a mass-dependent effective boson charge in the interacting boson model for the description of $E2$ transition rates in chains of nuclei. It encourages further studies of the microscopic origin of this mass dependence. New experimental values on transition rates in nuclei from neighboring isotopic chains could support these studies.

A new level scheme of 80Ga has been determined. This nucleus was populated following the β− decay of 80Zn at ISOLDE, CERN. The proposed level scheme is significantly different compared to the previously reported one and contains 26 levels up to 3.4 MeV in excitation energy. The present study establishes that the previously identified 1.9-s β− -decaying 6− isomer is the ground state of 80Ga and the 1.3-s β− -decaying 3− isomer lies at an excitation energy of 22.4 keV. A new isomeric level was identified at 707.8 keV and its half-life was measured to be 18.3(5) ns, allowing the 685.4-keV transition de-exciting this state to be assigned anM2 multipolarity. The newly measured spectroscopic observables are compared with shell-model calculations using the jj44bpn and JUN45 interactions.

Fast-timing measurements were performed in the region of the medium-mass $^{103,105,107}\mathrm{Cd}$ isotopes, produced in fusion evaporation reactions. Results on new and reevaluated half-lives are analyzed within a systematic study of transition rates. The $7/{2}_{1}^{+}$ states in $^{103,105,107}\mathrm{Cd}$ are interpreted as arising from a single-particle excitation. The $9/{2}^{+}$ states configuration assignment is based on the observed decay branches.