1. Emergent quasi-two-dimensional ferromagnetic state with perpendicular magnetic anisotropy at La0.7Sr0.3MnO3/SrCuO2 interface.
- Author
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Shi, Wenxiao, Zhang, Jing, Zhan, Xiaozhi, Li, Jialiang, Li, Zhe, Zheng, Jie, Wang, Mengqin, Zhang, Jine, Zhang, Hui, Zhu, Tao, Chen, Yunzhong, Hu, Fengxia, Shen, Baogen, Chen, Yuansha, and Sun, Jirong
- Subjects
PERPENDICULAR magnetic anisotropy ,X-ray absorption spectra ,UNIT cell ,DEGREES of freedom ,CHARGE transfer ,CURIE temperature ,COPPER ,MAGNETIC entropy - Abstract
Due to the strong interlayer coupling between multiple degrees of freedom, oxide heterostructures usually produce distinct interfacial phases with unexpected functionalities. Here, we report on the realization of quasi-two-dimensional ferromagnetic state in ultrathin La
0.7 Sr0.3 MnO3 (LSMO) layer down to two unit cells (u.c.), being sandwiched by the planar infinite-layer structured SrCuO2 layers (P-SCO). We find the LSMO/P-SCO interface coupling has greatly suppressed the magnetic dead layer of LSMO, resulting in an emergent interfacial ferromagnetic phase. Thus, robust ferromagnetic order can be maintained in the 2 u.c.-thick LSMO layer (∼7.7 Å), showing a Curie temperature of ∼260 K and remarkable perpendicular magnetic anisotropy. X-ray absorption spectra reveal notable charge transfer from Mn to Cu at the interface, and thus, resulted preferential d3z 2 −r orbital occupation for interfacial Mn ions plays an important role in the inducing of perpendicular magnetic anisotropy in quasi-two-dimensional LSMO layer. Our work demonstrates a unique approach for tuning the properties of oxides via an interface engineering of oxygen coordination in perovskite/infinite-layer heterostructures. [ABSTRACT FROM AUTHOR]2 - Published
- 2024
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