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In this work, we investigate the use of post-fabrication thermal nanoconversion (TNC), using a heated scanning probe tip, to modify the magnetic properties of Ni80Fe20 elliptical nanoislands with varying aspect ratio. Despite Ni80Fe20 being unoptimized for TNC, by comparing quasistatic and dynamic magneto-optical Kerr effect microscopy measurements, we demonstrate that TNC at a contact temperature of 250 °C increases the saturation magnetization of the treated nanoislands, reaching a value close to 800 kA/m. Micromagnetic simulations of the nanoislands indicate that the TNC technique can be used to alter the remanent state, from a single domain to a vortex. These results demonstrate the opportunities afforded by TNC to modify the properties of selected areas in a thin film or a patterned sample, particularly when designing magnonic crystals and other nanomagnetic devices. [ABSTRACT FROM AUTHOR]

Artificial multiferroics consist of two types of ferroic materials, typically a ferroelectric and a ferromagnet, often coupled interfacially by magnetostriction induced by the lattice elongations in the ferroelectric. In BaTiO3, the magnitude of strain induced by these elongations is heavily temperature dependent, varying greatly between each of the polar crystal phases and exerting a huge influence over the properties of a coupled magnetic film. Here, we demonstrate that temperature and, thus, strain are effective means of controlling the magnetic anisotropy in BaTiO3(111)/CoFeB heterostructures. We investigate the three polar phases of BaTiO3: tetragonal (T) at room temperature, orthorhombic (O) below 280 K, and rhombohedral (R) below 190 K across a total range of 77–420 K. We find two distinct responses: a step-like change in the anisotropy across the low-temperature phase transitions and a sharp high-temperature reduction around the ferroelectric Curie temperature, measured from hard axis hysteresis loops. Using our measurements of this anisotropy strength, we are then able to show by micromagnetic simulation the behavior of all possible magnetic domain wall states and determine their scaling as a function of temperature. The most significant changes occur in the head-to-head domain wall states, with a maximum change of 210 nm predicted across the entire range, effectively doubling the size of the domain wall as compared to room temperature. Notably, similar changes are seen for both high and low temperatures, which suggests different routes for potential control of magnetic anisotropy and elastically pinned magnetic domain walls. [ABSTRACT FROM AUTHOR]

Picosecond magnetization dynamics in the free and pinned layers of a microscale magnetic tunnel valve have been studied using time-resolved scanning Kerr microscopy. A comparison of the observed dynamics with those of individual free and pinned layers allowed the effect of interlayer coupling to be identified. A weak interlayer coupling in the tunnel valve continuous film reference sample was detected in bulk magnetometry measurements, while focused Kerr magnetometry showed that the coupling was well maintained in the patterned structure. In the tunnel valve, the free layer precession was observed to have reduced amplitude and an enhanced relaxation. During magnetization reversal in the pinned layer, its frequency approached that of the low frequency mode associated with the free layer. At the pinned layer switching field, the linewidth of the free layer became similar to that of the pinned layer. The similarity in their frequencies promotes the formation of precessional modes that exhibit strong collective properties such as frequency shifting and enhanced linewidth, while inhomogeneous magnetization of the pinned layer during reversal may also play a role in these observations. The collective character of precessional dynamics associated with mixing of the free and pinned layer magnetization dynamics must be accounted for even in tunnel valves with a small interlayer coupling. [ABSTRACT FROM AUTHOR]

A selective area chemical vapour deposition technique has been used to fabricate continuous and patterned epitaxial CrO2 thin films on (100)-oriented TiO2 substrates. Precessional magnetization dynamics were stimulated both electrically and optically, and probed by means of time-resolved Kerr microscopy and vector network analyser ferromagnetic resonance techniques. The dependence of the precession frequency and the effective damping parameter upon the static applied magnetic field were investigated. All films exhibited a large in-plane uniaxial anisotropy. The effective damping parameter was found to exhibit strong field dependence in the vicinity of the hard axis saturation field. However, continuous and patterned films were found to possess generally similar dynamic properties, confirming the suitability of the deposition technique for fabrication of future spintronic devices. [ABSTRACT FROM AUTHOR]

Time-resolved scanning Kerr microscopy has been used to perform optically detected, phase-resolved spin–orbit torque ferromagnetic resonance (SOT-FMR) measurements on a microscale CoFeB ellipse at the center of a Pt Hall cross subject to RF and DC current. Time-resolved polar Kerr images revealed localized dynamics with large amplitude at the center and weaker amplitude at the edges. Therefore, field swept SOT-FMR spectra were acquired from the so-called center mode to probe the SOTs active at the center of the ellipse, thus minimizing non-uniform edge contributions. When the magnetic field was applied at 30° from the hard axis of the ellipse and a DC current was applied, a marked asymmetry was observed in the amplitude and linewidth of the FMR peaks as the applied field was reversed. Both absorptive and dispersive parts of the spectra were in good agreement with a macrospin calculation. The damping parameter (α) and the Slonczewski torque parameter were determined to be 0.025 and (6.75 ± 0.75) × 10−7 Oe A−1 cm2, respectively. The hard axis SOT-FMR linewidth was found to be almost independent of the DC current value, suggesting that the SOT has a minimal influence in the hard axis configuration and that thermal effects were insignificant. This study paves the way for spatially resolved measurements of SOT probed using localized modes of microscale devices that go beyond the spatially averaged capability of electrical measurement techniques. [ABSTRACT FROM AUTHOR]

Micromagnetic simulations have been performed to investigate the frequencies and relative amplitudes of resonant magnetic modes within nanomagnetic elements of varying size that have been previously studied by time resolved Kerr magnetometry. The magnetic response of a nanoscale element generally consists of the edge and center localized modes. For 2.5 nm thick elements, a crossover from center to edge mode excitation occurs as the element size is reduced to less than 220 nm. Additional modes appear in the spin wave spectrum as the thickness of the element is increased. The frequency of the edge mode is particularly sensitive to the strength of the exchange interaction, dipolar interactions with nearest neighbor elements, and rounding of the corners of the element. Simulations with in-plane pulsed fields show that the edge mode becomes dominant in elements of somewhat larger size, emphasizing the importance of the edge mode in technological applications. [ABSTRACT FROM AUTHOR]

Time-resolved scanning Kerr microscopy (TRSKM) has been used to image precessional magnetization dynamics excited by a DC current within a nano-contact (NC) spin Hall nano-oscillator (SHNO). Injection of a radio frequency (RF) current was used to phase lock the SHNO to TRSKM. The out of plane magnetization was detected by means of the polar magneto optical Kerr effect (MOKE). However, longitudinal MOKE images were dominated by an artifact arising from the edges of the Au NCs. Time resolved imaging revealed the simultaneous excitation of a non-linear "bullet" mode at the centre of the device, once the DC current exceeded a threshold value, and ferromagnetic resonance (FMR) induced by the RF current. However, the FMR response observed for sub-critical DC current values exhibits an amplitude minimum at the centre, which is attributed to spreading of the RF spin current due to the reactance of the device structure. This FMR response can be subtracted to yield images of the bullet mode. As the DC current is increased above threshold, the bullet mode appears to increase in size, suggesting increased translational motion. The reduced spatial overlap of the bullet and FMR modes, and this putative translational motion, may impede the injection locking and contribute to the reduced locking range observed within NC-SHNO devices. This illustrates a more general need to control the geometry of an injection-locked oscillator so that the autonomous dynamics of the oscillator exhibit strong spatial overlap with those resulting from the injected signal. [ABSTRACT FROM AUTHOR]

Time-resolved scanning Kerr microscopy has been used to directly observe magnetostatically coupled transverse domain walls (TDWs) in a pair of closely spaced, curved nanowires (NWs). Kerr images of the precessional response of the magnetic domain to either side of the TDW revealed the TDW as a minimum in the Kerr signal in the region of closest NW separation. When the TDWs were ejected from the NW pair, the minimum in the Kerr signal was no longer observed. By imaging this transition, the static de-coupling field was estimated to be in the range from 38 to 48Oe in good agreement with a simple micromagnetic model. This work provides a novel technique by which DC and microwave assisted decoupling fields of TDWs may be explored in NW pairs of different width, separation, and curvature. [ABSTRACT FROM AUTHOR]

A partially built hard disk writer structure with a NiFe/CoFe/Ru/NiFe/CoFe synthetic antiferromagnetic (SAF) yoke was studied by time and vector resolved scanning Kerr microscopy. All three time dependent components of the magnetization were recorded simultaneously as a bipolar current pulse with 1MHz repetition rate was delivered to the coil. The component of magnetization parallel to the symmetry axis of the yoke was compared at the pole and above a coil winding in the centre of the yoke. The two responses are in phase as the pulse rises, but the pole piece lags the yoke as the pulse falls. The Kerr signal is smaller within the yoke than within the confluence region during pulse cycling. This suggests funneling of flux into the confluence region. Dynamic images acquired at different time delays showed that the relaxation is faster in the centre of the yoke than in the confluence region, perhaps due to the different magnetic anisotropy in these regions. Although the SAF yoke is designed to support a single domain to aid flux conduction, no obvious flux beaming was observed, suggesting the presence of a more complicated domain structure. The SAF yoke writer hence provides relatively poor flux conduction but good control of rise time compared to single layer and multi-layered yokes studied previously. [ABSTRACT FROM AUTHOR]

The precessional dynamics of a 2×2 μm2 CoFe/NiFe (4.6 nm) element stimulated by an in-plane pulsed magnetic field have been investigated using time- and vector-resolved Kerr microscopy measurements and micromagnetic simulations. The time-resolved signals were normalized to in-plane hysteresis loops obtained from the patterned material, and suggest that the magnetization reorients through an angle of 100°±10°. The simulations reveal that only the magnetization of the center region undergoes large angle reorientation, while the canted magnetization at the edges of the element remains pinned. An enhanced Gilbert damping parameter of 0.1 was required to reproduce the experimentally observed Kerr signals. [ABSTRACT FROM AUTHOR]

The design and fabrication of a novel plasmonic cavity, intended to allow far-field recovery of signals arising from near field magneto-optical interactions, is presented. Finite element modeling is used to describe the interaction between a gold film, containing cross-shaped cavities, with a nearby magnetic under-layer. The modeling revealed strong electric field confinement near the center of the cross structure for certain optical wavelengths, which may be tuned by varying the length of the cross through a range that is compatible with available fabrication techniques. Furthermore, the magneto optical Kerr effect (MOKE) response of the composite structure can be enhanced with respect to that of the bare magnetic film. To confirm these findings, cavities were milled within gold films deposited upon a soluble film, allowing relocation to a ferromagnetic film using a float transfer technique. Cross cavity arrays were fabricated and characterized by optical transmission spectroscopy prior to floating, revealing resonances at optical wavelengths in good agreement with the finite element modeling. Following transfer to the magnetic film, circular test apertures within the gold film yielded clear magneto-optical signals even for diameters within the sub-wavelength regime. However, no magneto-optical signal was observed for the cross cavity arrays, since the FIB milling process was found to produce nanotube structures within the soluble under-layer that adhered to the gold. Further optimization of the fabrication process should allow recovery of magneto-optical signal from cross cavity structures. [ABSTRACT FROM AUTHOR]

The angular dependence of the in-plane magnetization reversal in hexagonally ordered Co arrays has been investigated. A sixfold anisotropy has been observed which mirrors the structural symmetry of the array. The arrays consist of polycrystalline, circular elements with constant center-to-center separation and diameters of 360 nm and below. It has been observed that the anisotropy is strongly dependent on element diameter and disappears for densely packed elements. This anisotropic coupling cannot be explained by a simple model of interacting point dipoles situated at regular lattice sites, as this predicts an isotropic interaction field for a hexagonal array. Instead, it is believed that the anisotropy arises from interactions between unsaturated regions of the elements, particularly at adjacent edges. [ABSTRACT FROM AUTHOR]

It is shown that a coplanar stripline structure containing indium tin oxide windows can be used to perform optical ferromagnetic resonance measurements on a sample grown on an opaque substrate, using a pulsed magnetic field of any desired orientation. The technique is demonstrated by applying it to a thin film of permalloy grown on a Si substrate. The measured precession frequency was found to be in good agreement with macrospin simulations. The phase of the oscillatory Kerr response was observed to vary as the probe spot was scanned across the coplanar stripline structure, confirming that the orientation of the pulsed field varied from parallel to perpendicular relative to the plane of the sample. [ABSTRACT FROM AUTHOR]

Four different designs of partially built hard disk write heads with a yoke comprising four repeats of NiFe (1 nm)/CoFe (50 nm) were studied by both x-ray photoemission electron microscopy (XPEEM) and time-resolved scanning Kerr microscopy (TRSKM). These techniques were used to investigate the static equilibrium domain configuration and the magnetodynamic response across the entire structure, respectively. Simulations and previous TRSKM studies have made proposals for the equilibrium domain configuration of similar structures, but no direct observation of the equilibrium state of the writers has yet been made. In this study, static XPEEM images of the equilibrium state of writer structures were acquired using x-ray magnetic circular dichroism as the contrast mechanism. These images suggest that the crystalline anisotropy dominates the equilibrium state domain configuration, but competition with shape anisotropy ultimately determines the stability of the equilibrium state. Dynamic TRSKM images were acquired from nominally identical devices. These images suggest that a longer confluence region may hinder flux conduction from the yoke into the pole tip: the shorter confluence region exhibits clear flux beaming along the symmetry axis, whereas the longer confluence region causes flux to conduct along one edge of the writer. The observed variations in dynamic response agree well with the differences in the equilibrium magnetization configuration visible in the XPEEM images, confirming that minor variations in the geometric design of the writer structure can have significant effects on the process of flux beaming. [ABSTRACT FROM AUTHOR]

Sub-wavelength metallic planar cavities, closed at one end, have been constructed by wrapping aluminium foil around teflon or ferrite slabs. Finite cavity width perturbs the fundamental cavity mode frequency of ferrite-filled cavities due to different permeability inside and outside of the cavity, in contrast to teflon-filled cavities, while the cavity length required to achieve a specific resonance frequency is significantly reduced for a ferrite-filled cavity. Ferrite-filled cavities may be excited by an in-plane alternating magnetic field and may be advantageous for high-frequency (HF) and ultra HF tagging and radio frequency identification of metallic objects within security, manufacturing, and shipping environments. [ABSTRACT FROM AUTHOR]

Precessional dynamics of a Co50Fe50(0.7)/Ni90Fe10(5)/Dy(1)/Ru(3) (thicknesses in nm) thin film have been explored by low temperature time-resolved magneto-optical Kerr effect and phase-resolved x-ray ferromagnetic resonance measurements. As the temperature was decreased from 300 to 140 K, the magnetic damping was found to increase rapidly while the resonance field was strongly reduced. Static x-ray magnetic circular dichroism measurements revealed increasing ferromagnetic order of the Dy moment antiparallel to that of Co50Fe50/Ni90Fe10. Increased coupling of the Dy orbital moment to the precessing spin magnetization leads to significantly increased damping and gyromagnetic ratio of the film while leaving its magnetic anisotropy effectively unchanged. [ABSTRACT FROM AUTHOR]

Time-resolved scanning Kerr microscopy has been used to make wafer level measurements of magnetization dynamics within the yoke and pole piece of partially built hard disk writer structures. Three Cartesian components of the vector magnetization were recorded simultaneously using a quadrant photodiode polarization bridge detector. The rise time, relaxation time, and amplitude of each component has been related to the magnetic ground state, the initial torque, and flux propagation through the yoke and pole piece. Dynamic images reveal 'flux-beaming' in which the magnetization component parallel to the symmetry axis of the yoke is largest along that axis. [ABSTRACT FROM AUTHOR]

We demonstrate a magnonic architecture that converts global free-space uniform microwaves into spin waves propagating in a stripe magnonic waveguide. The architecture is based upon dispersion mismatch between the narrow magnonic waveguide and a wide 'antenna' patch, both patterned from the same magnetic film. The spin waves injected into the waveguide travel to distances as large as several tens of micrometers. The antennas can be placed at multiple positions on a magnonic chip and used to excite mutually coherent multiple spin waves for magnonic logic operations. This demonstration paves way for 'magnonics' to become a pervasive technology for information processing. [ABSTRACT FROM AUTHOR]

Large amplitude magnetization dynamics of a single square nanomagnet have been studied by time-resolved Kerr microscopy. Experimental spectra revealed that only a single mode was excited for all bias field values. Micromagnetic simulations demonstrate that at larger pulsed field amplitudes the center mode dominates the dynamic response while the edge mode is almost completely suppressed. Controlled suppression of edge modes in a single nanomagnet has potential applications in the operation of nanoscale spin transfer torque oscillators and bistable switching devices for which the amplitude of the magnetization trajectory is often large and a more uniform dynamic response is desirable. [ABSTRACT FROM AUTHOR]

X-ray magnetic circular dichroism (XMCD) is utilized to explore the temperature dependence of the interface moments in Co2MnSi (CMS) thin films capped with aluminum. By increasing the thickness of the capping layer, we demonstrate enhanced interface sensitivity of the measurements. L21-ordered CMS films show no significant temperature dependence of either the Co or Mn interface moments. However, disordered CMS films show a decreased moment at low temperature possibly caused by increased Mn–Mn antiferromagnetic coupling. It is suggested that for ordered L21 CMS films the temperature dependence of the tunneling magnetoresistance is not related to changes in the interface moments. [ABSTRACT FROM AUTHOR]

Phase-resolved x-ray ferromagnetic resonance (XFMR) has been measured in fluorescence yield, extending the application of XFMR to opaque samples on opaque substrates. Magnetization dynamics were excited in a Co50Fe50(0.7)/Ni90Fe10(5) bilayer by means of a continuous wave microwave excitation, while x-ray magnetic circular dichroism (XMCD) spectra were measured stroboscopically at different points in the precession cycle. By tuning the x-ray energy to the L3 edges of Ni and Fe, the dependence of the real and imaginary components of the element specific magnetic susceptibility on the strength of an externally applied static bias field was determined. First results from measurements on a Co50Fe50(0.7)/Ni90Fe10(5)/Dy(1) sample confirm that enhanced damping results from the addition of the Dy cap. [ABSTRACT FROM AUTHOR]

Partially built hard disk writer structures with a multilayered yoke formed from 4 repeats of a NiFe(∼1 nm)/CoFe(50 nm) bilayer were studied by time and vector resolved scanning Kerr microscopy. Dynamic images of the in-plane magnetization suggest an underlying closure domain equilibrium state. This state is found to be modified by application of a bias magnetic field and also during pulse cycling, leading to different magnetization rotation and relaxation behavior within the tip region. [ABSTRACT FROM AUTHOR]