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Neutron beams are an essential tool to investigate material structure and perform nondestructive analysis, as they give unique access to element composition, thus ideally complementing density analysis allowed by standard x-rays investigation. Laser-driven neutron sources, though compact and cost-effective, currently have lower average flux than conventional neutron sources, due to the limited repetition rate of the lasers used so far. However, advancements in laser technology allow nowadays to address this challenge. Here, we report results obtained at the Advanced Laser Light Source characterizing stable production of broadband (0.1–2 MeV) neutrons produced at a high repetition rate (0.5 Hz). The interaction of laser pulses of 22 fs duration and 3.2 J on-target energy with 2- μ m-thick tantalum targets produced protons in the Target Normal Sheath Acceleration (TNSA) regime up to 7.3 MeV. These protons were subsequently converted into neutrons by (p,n) reactions in lithium fluoride (LiF). Activation measurements and bubble detectors were used to characterize neutron emissions, with a neutron fluence of up to ∼ 1.4 × 10 5 neutrons/shot/sr and energies mainly between a few hundred of kilo-electron volt and 2 MeV. The total neutron yield was ∼ 5 × 10 5 neutrons/shot. This paves the way for numerous applications, e.g., in homeland security, materials science, or cultural heritage. [ABSTRACT FROM AUTHOR]

Laser-driven proton accelerators are relevant candidates for many applications such as material science or medicine. Today, there are multi-hundred-TW table-top laser systems that can generate relativistic peak intensities >1018 W/cm2 and routinely reach proton energies in the MeV range. However, for most desired applications, there is still a need to optimize the quality and stability of the laser-generated proton beam. In this work, we developed a 0.625 Hz high repetition-rate setup in which a laser with 2.5% RMS energy stability is irradiating a solid target with an intensity of 1019 to 1020 W/cm2 to explore proton energy and yield variations, both with high shot statistics (up to about 400 laser shots) and using different interaction targets. Investigating the above-mentioned parameters is important for applications that rely on specific parts of the proton spectrum or a high ion flux produced over quick multi-shot irradiation. We demonstrate that the use of a stable "multi-shot mode" allows improving applications, e.g., in the detection of trace elements using laser-driven particle-induced x-ray emission., (© 2023 Author(s). Published under an exclusive license by AIP Publishing.)

By extending the concept of thin film compression [Mourou et al., Eur. Phys. J. Spec. Top. 223(6), 1181 (2014)] to a thin plate, nonlinear post-compression from 24 fs to 13 fs of sub-petawatt laser pulses is demonstrated experimentally using a 1 mm-thick silica plate and chirped mirrors with a total anomalous dispersion of −50 fs2. The measurements were implemented with a specially designed dispersionless vacuum frequency-resolved optical gating, which is based on second harmonic generation of tested pulses in a 10 μm β-barium borate crystal glued on a 1 mm fused silica substrate. The used compression scheme is implemented in a geometry compatible with high power on-target experiment realization. [ABSTRACT FROM AUTHOR]

We report on the cross-calibration of Thomson Parabola (TP) and Time-of-Flight (TOF) detectors as particle diagnostics, implemented on the most recent setup of the ALLS 100 TW laser-driven ion acceleration beamline. The Microchannel Plate (MCP) used for particle detection in the TP spectrometer has been calibrated in intensity on the tandem linear accelerator at the Université de Montréal. The experimental data points of the scaling factor were obtained by performing a pixel cluster analysis of single proton impacts on the MCP. A semi-empirical model was extrapolated and fitted to the data to apply the calibration also to higher kinetic energies and to extend it to other ion species. Two TOF lines using diamond detectors, placed at +6° and −9° with respect to the target-normal axis, were benchmarked against the TP spectrometer measurements to determine the field integrals related to its electric and magnetic dispersions. The mean integral proton numbers obtained on the beamline were about 4.1 × 1011 protons/sr with a standard deviation of 15% in the central section of the spectrum around 3 MeV, hence witnessing the high repeatability of the proton bunch generation. The mean maximum energy was of 7.3 ± 0.5 MeV, well in agreement with similar other 100 TW-scale laser facilities, with the best shots reaching 9 MeV and nearly 1012 protons/sr. The used particle diagnostics are compatible with the development of a high-repetition rate targetry due to their fast online readout and are therefore a crucial step in the automation of any beamline. [ABSTRACT FROM AUTHOR]

In this paper, we report on bi-dimensional Particle-In-Cell simulations performed in order to reproduce the laser-driven proton acceleration obtained when a commercial 200 TW Ti:Sa Laser hits a solid target. The laser-to prepulse contrast was enhanced using plasma mirrors yielding to a main-to-prepulse contrast of ~1012. We varied the pulse duration from 30 fs to 500 fs and the target thickness from 30 nm to several tens of μm. The on-target laser energy was up to 1.8J leading to an intensity in excess of 1020W cm-2. A comparison between numerical and existing experimental data [S. Fourmaux et al., Phys. Plasmas 20, 013110 (2013)] is performed, showing a good agreement between experimental results and simulations which confirms that for ultra-thin targets there is an optimum expansion regime. This regime depends on the target thickness and on the laser intensity: if the target is too expanded, the laser travels through the target without being able to deposit its energy within the target. If the target is not sufficiently expanded, the laser energy is reflected by the target. It is important to note that maximum proton energies are reached at longer pulse durations (in the 100 fs regime) than what is currently the best compression pulse length for this type of lasers (typically 20-30 fs). This duration, around 50-100 fs, can be considered a minimum energy transfer time between hot electrons to ions during the considered acceleration process. [ABSTRACT FROM AUTHOR]

We show through experiments that a transition from laser wakefield acceleration (LWFA) regime to a plasma wakefield acceleration (PWFA) regime can drive electrons up to energies close to the GeV level. Initially, the acceleration mechanism is dominated by the bubble created by the laser in the nonlinear regime of LWFA, leading to an injection of a large number of electrons. After propagation beyond the depletion length, leading to a depletion of the laser pulse, whose transverse ponderomotive force is not able to sustain the bubble anymore, the high energy dense bunch of electrons propagating inside bubble will drive its own wakefield by a PWFA regime. This wakefield will be able to trap and accelerate a population of electrons up to the GeV level during this second stage. Three dimensional particle-in-cell simulations support this analysis and confirm the scenario. [ABSTRACT FROM AUTHOR]

We have developed a laser wakefield generated X-ray probe to directly measure the temporal evolution of the ionization states in warm dense aluminum by means of absorption spectroscopy. As a promising alternative to the free electron excited X-ray sources, Betatron X-ray radiation, with femtosecond pulse duration, provides a new technique to diagnose femtosecond to picosecond transitions in the atomic structure. The X-ray probe system consists of an adjustable Kirkpatrick-Baez (KB) microscope for focusing the Betatron emission to a small probe spot on the sample being measured, and a flat Potassium Acid Phthalate Bragg crystal spectrometer to measure the transmitted X-ray spectrum in the region of the aluminum K-edge absorption lines. An X-ray focal spot size of around 50 μm was achieved after reflection from the platinum-coated 10-cm-long KB microscope mirrors. Shot to shot positioning stability of the Betatron radiation was measured resulting in an rms shot to shot variation in spatial pointing on the sample of 16 μm. The entire probe setup had a spectral resolution of ∼1.5 eV, a detection bandwidth of ∼24 eV, and an overall photon throughput efficiency of the order of 10-5. Approximately 10 photons were detected by the X-ray CCD per laser shot within the spectrally resolved detection band. Thus, it is expected that hundreds of shots will be required per absorption spectrum to clearly observe the K-shell absorption features expected from the ionization states of the warm dense aluminum. [ABSTRACT FROM AUTHOR]

Quasimonoenergetic electron beams with maximum energy >0.5 GeV and 2 mrad divergence have been generated in pure nitrogen gas via wakefield acceleration with 80 TW, 30 fs laser pulses. Long low energy tail features were typically observed due to continuous ionization injection. The measured peak electron energy decreased with the plasma density, agreeing with the predicted scaling for electrons. The experiments showed a threshold electron density of 3×1018cm-3 for self-trapping. Our experiments suggest that pure Nitrogen is a potential candidate gas to achieve GeV monoenergetic electrons using the ionization induced injection scheme for laser wakefield acceleration. [ABSTRACT FROM AUTHOR]

Using a laser plasma accelerator, experiments with a 80 TW and 30 fs laser pulse demonstrated quasi-monoenergetic electron spectra with maximum energy over 0.4 GeV. This is achieved using a supersonic He gas jet and a sharp density ramp generated by a high intensity laser crossing pre-pulse focused 3 ns before the main laser pulse. By adjusting this crossing pre-pulse position inside the gas jet, among the laser shots with electron injection, more than 40% can produce quasi-monoenergetic spectra. This could become a relatively straight forward technique to control laser wakefield electron beams parameters. [ABSTRACT FROM AUTHOR]

Recent progress in high intensity ultrafast laser systems provides the opportunity to produce laser plasma x-ray sources exhibiting broad spectrum and high average x-ray flux that are well adapted to x-ray absorption measurements. In this paper, the development of a laser based x-ray absorption near edge structure (XANES) beamline exhibiting high repetition rate by using the Advanced Laser Light Source (ALLS) facility 100 Hz laser system (100 mJ, 35 fs at 800 nm) is presented. This system is based on a broadband tantalum solid target soft x-ray source and a grazing incidence grating spectrometer in the 1–5 nm wavelength range. To demonstrate the high potential of this laser based XANES technique in condensed matter physics, material science, or biology, measurements realized with several samples are presented: VO2 vanadium L edge, Si3N4 nitrogen K edge, and BPDA/PPD polyimide carbon K edge. The characteristics of this laser based beamline are discussed in terms of brightness, signal to noise ratio, and compared to conventional synchrotron broadband x-ray sources which allow achieving similar measurements. Apart from the very compact size and the relative low cost, the main advantages of such a laser based soft x-ray source are the picosecond pulse duration and the perfect synchronization between this x-ray probe and a laser pulse excitation which open the way to the realization of time resolved x-ray absorption measurements with picosecond range time resolution to study the dynamics of ultrafast processes and phase transition. [ABSTRACT FROM AUTHOR]

The 2D projection phase-contrast imaging performance of the ultrafast laser-based x-ray (ULX) source has been investigated. The potential of such a novel x-ray source has been assessed by imaging a reference object (Contrast Detail Evaluation phantom) in the in-line holography geometry and by applying a simple 1D numerical model to the data analysis. The results indicate that the ULX is a promising technique for 2D projection phase-contrast imaging and for implementation of phase-contrast micro-Computed Tomography (μ-CT). This is because by using high contrast laser pulse ULX simultaneously provides a very small x-ray source size along with a high average x-ray flux. In addition, due to the ultrashort x-ray burst duration, ULX might allow practical implementation of ultrafast phase-contrast stroboscopy and time-of-flight based electronic scatter rejection. This technique is also of interest for time resolved radiography to follow shock waves and radiative fronts propagating in an opaque matter. [ABSTRACT FROM AUTHOR]

We demonstrate the feasibility of phase-contrast imaging with an ultrafast laser-based hard x-ray source. Hard x rays are generated during the interaction of a high-intensity femtosecond laser pulse (10 TW, 60 fs, 10 Hz) focused onto solid target in a very small spot (3 μm diam). Such a novel x-ray source has a number of advantages over other sources previously used for phase-contrast imaging: It is very compact and much cheaper than a synchrotron, it has higher power and better x-ray spectrum control than a microfocal x-ray tube, and it has much higher repetition rate than an x-pinch source. The Kα line at 17 keV produced using a solid Mo target, and the in-line imaging geometry have been utilized in this study. Phase-contrast images of test objects and biological samples have been realized. The characteristics of the images are the significant enhancement of interfaces due to an x-ray phase shift that reveal details that were hardly observable, or even undetectable, in absorption images and suppression of optically dense structures well defined in the absorption images. Our study indicates that the absorption and the phase-contrast images obtained with an ultrafast laser-based x-ray source provide complementary information about the imaged objects, thus enriching our arsenal of research tools for laboratory or clinic-based biomedical imaging. [ABSTRACT FROM AUTHOR]

Interaction of intense Ti:sapphire laser with solid targets has been studied experimentally by measuring hard x-ray and hot electron generation. Hard x-ray (8–100 keV) emission spectrum and Kα x-ray conversion efficiency (ηK) from plasma have been studied as a function of laser intensity (1017–1019 W/cm2), pulse duration (70–400)fs, and laser pulse fluence. For intensity I>1×1017 W/cm2, the Ag ηK increases to reach a maximum value of 2×10-5 at an intensity I=4×1018 W/cm2. Hot electron temperature (KTh) and ηK scaling laws have been studied as a function of the laser parameters. A stronger dependence of KTh and ηK as a function of the laser fluence than on pulse duration or laser intensity has been observed. The contribution of another nonlinear mechanism, besides resonance absorption, to hard x-ray enhancement has been demonstrated via hot electron angular distribution and particle-in-cell simulations. [ABSTRACT FROM AUTHOR]

Terahertz time-domain spectroscopy is used to measure the complex terahertz conductivity of a nanogranular vanadium dioxide (VO2) thin film as a function of temperature through the metal-insulator transition. The Drude-Smith model provides a good fit to the observed terahertz conductivity, revealing a metallic state that forms via switching of individual nanograins and strong carrier confinement within the nanograins due to scattering off grain boundaries. Furthermore, the directly applied Drude-Smith model provides a more accurate description of the measured terahertz conductivity in this material than either Bruggeman or Maxwell-Garnett effective medium theories. [ABSTRACT FROM AUTHOR]

We study the photoinduced insulator-metal transition in VO2, correlating its threshold and dynamics with excitation wavelength. In single crystals, switching can only be induced with photon energies above the 670 meV gap. This contrasts with the case of polycrystalline films, where formation of the metallic state can be initiated also with photon energies as low as 180 meV, which are well below the bandgap. Perfection of this process may become conducive to schemes for optical switches, limiters, and detectors operating at room temperature in the mid-infrared. [ABSTRACT FROM AUTHOR]

Single-phase vanadium dioxide (VO2) thin films have been grown on Si3N4/Si substrates by means of a well-controlled magnetron sputtering process. The deposited VO2 films were found to exhibit a semiconductor-to-metal transition (SMT) at ∼69 °C with a resistivity change as high as 3.2 decades. A direct and clear-cut correlation is established between the SMT characteristics (both amplitude and abruptness of the transition) of the VO2 films and their crystallite size. [ABSTRACT FROM AUTHOR]

In recent studies, it has been shown that under optimal dual pulse irradiation, it is possible to generate anomalous relativistic temperature (> 500 keV) electron emission even with mJ/pulse lasers at 1/100th of the relativistic intensity when micrometer droplets of methanol are used as a high repetition rate target. In this paper, we present the results of doping these droplets with CH3I to bring out a 30-fold enhancement in electron emission. Experiments and simulations presented here find a route to enhance electron emission driven by two plasmon decay instability. Improving compact laser plasma based sources of MeV electrons, x-ray emission schemes that use a high repetition rate, and mJ/pulse laser systems is important not only for basic science but also applications of imaging and radiography. [ABSTRACT FROM AUTHOR]

Laser wakefield acceleration of 500 MeV to 1 GeV electron bunches has been demonstrated using ionization injection in mixtures of 4% to 10% of CO2 in He. 80 TW laser pulses were propagated through 5 mm gas jet targets at electron densities of 0.4-1.5×1019cm-3. Ionization injection led to lower density thresholds, a higher total electron charge, and an increased probability of producing electrons above 500 MeV in energy compared to self-injection in He gas alone. Electrons with GeV energies were also observed on a few shots and indicative of an additional energy enhancement mechanism. [ABSTRACT FROM AUTHOR]

We report optimization of laser-driven proton acceleration, for a range of experimental parameters available from a single ultrafast Ti:sapphire laser system. We have characterized laser-generated protons produced at the rear and front target surfaces of thin solid targets (15 nm to 90 μm thicknesses) irradiated with an ultra-intense laser pulse (up to 1020 W·cm-2, pulse duration 30 to 500 fs, and pulse energy 0.1 to 1.8 J). We find an almost symmetric behaviour for protons accelerated from rear and front sides, and a linear scaling of proton energy cut-off with increasing pulse energy. At constant laser intensity, we observe that the proton cut-off energy increases with increasing laser pulse duration, then roughly constant for pulses longer than 300 fs. Finally, we demonstrate that there is an optimum target thickness and pulse duration. [ABSTRACT FROM AUTHOR]

The use of laser–plasma-based x-ray sources is discussed, with a view to carrying out time-resolved x-ray absorption spectroscopy measurements, down to the femtosecond timescale. A review of recent experiments performed by our team is presented. They concern the study of the nonequilibrium transition of metals from solid to the warm dense regime, which imposes specific constraints (the sample being destroyed after each shot). Particular attention is paid to the description of experimental devices and methodologies. Two main types of x-ray sources are compared, respectively, based on the emission of a hot plasma, and on the betatron radiation from relativistic electrons accelerated by laser. [ABSTRACT FROM AUTHOR]

One of the most prominent applications of modern particle accelerators is the generation of radiation. In a synchrotron or an x-ray free electron laser (XFEL), high energy electrons oscillating in periodic magnetic structures emit bright x rays. In spite of their scientific appeal that will remain evident for many decades, one limitation of synchrotrons and XFELs is their typical mile-long size and their cost, which often limits access to the broader scientific community. This tutorial reviews the principles and prospects of using plasmas produced by intense lasers as particle accelerators and x-ray light sources, as well as some of the applications they enable. A plasma is an ionized medium that can sustain electrical fields many orders of magnitude higher than that in conventional radio frequency accelerator structures and can be used to accelerate electrons. When short, intense laser pulses are focused into a gas, it produces electron plasma waves in which electrons can be trapped and accelerated to GeV energies. This process, laser-wakefield acceleration (LWFA), is analogous to a surfer being propelled by an ocean wave. Many radiation sources, from THz to gamma-rays, can be produced by these relativistic electrons. This tutorial reviews several LWFA-driven sources in the keV-MeV photon energy range: betatron radiation, inverse Compton scattering, bremsstrahlung radiation, and undulator/XFEL radiation. X rays from laser plasma accelerators have many emerging applications. They can be used in innovative and flexible x-ray imaging and x-ray absorption spectroscopy configurations, for use in biology, industry, and high-energy density science. [ABSTRACT FROM AUTHOR]

We present a method to calculate the shift of the K edge in warm dense aluminum. We use the average-atom model and show how to build the energy of an electronic configuration with integer subshell populations and by taking into account the interaction of the bound electrons with the free electrons. We successfully compare our calculation of the spectral opacity with the Henke table for aluminum at solid density and 300 K. We found a redshift of the K edge along the principal Hugoniot consistent with experimental data. We also compute the 2s and 2p edges. We obtain L edge redshifts similar to the K edge redshift. [ABSTRACT FROM AUTHOR]

High-power, short-pulse laser-driven fast electrons can rapidly heat and ionize a high-density target before it hydrodynamically expands. The transport of such electrons within a solid target has been studied using two-dimensional (2D) imaging of electron-induced Kα radiation. However, it is currently limited to no or picosecond scale temporal resolutions. Here, we demonstrate femtosecond time-resolved 2D imaging of fast electron transport in a solid copper foil using the SACLA x-ray free electron laser (XFEL). An unfocused collimated x-ray beam produced transmission images with sub-micron and ∼10 fs resolutions. The XFEL beam, tuned to its photon energy slightly above the Cu K-edge, enabled 2D imaging of transmission changes induced by electron isochoric heating. Time-resolved measurements obtained by varying the time delay between the x-ray probe and the optical laser show that the signature of the electron-heated region expands at ∼25% of the speed of light in a picosecond duration. Time-integrated Cu Kα images support the electron energy and propagation distance observed with the transmission imaging. The x-ray near-edge transmission imaging with a tunable XFEL beam could be broadly applicable for imaging isochorically heated targets by laser-driven relativistic electrons, energetic protons, or an intense x-ray beam. [ABSTRACT FROM AUTHOR]

The generation of an electron beam through longitudinal field acceleration from a tightly focused radially polarized (TM01) laser mode is reported. The longitudinal field is generated by focusing a TM01 few-cycle laser pulse (1.8 μm, 550 μJ, 15 fs) with a high numerical aperture parabola. The created longitudinal field in the focal region is intense enough to ionize atoms and accelerate electrons to 23 keV of energy from a low density oxygen gas. The characteristics of the electron beam are presented. [ABSTRACT FROM AUTHOR]

The experiments have revealed a "threshold" target thickness for proton acceleration by a femtosecond petawatt class laser above which the forward accelerated proton energy weakly depends on the target thickness, while for thinner targets, it gradually decreases. For targets thicker than the threshold, the pre-pulse-induced preplasma at the target front can boost ion acceleration by increasing laser absorption, while this is ineffective for thinner targets due to prepulse-induced plasma formation at the target rear. This dual nature of the preplasma is described analytically, and particle-in-cell simulations confirm this concept. A linear dependence of threshold target thickness on the prepulse intensity is predicted. [ABSTRACT FROM AUTHOR]

We investigate the dynamics of hot refluxing electrons in the interaction of an ultra-short relativistic laser pulse with a thin foil target via particle-in-cell (PIC) simulations, which is governed by the multidimensional spatiotemporal evolution of a self-generated sheath field. The comparison of time-integrated energy spectra of refluxing and escaping electrons indicates the refluxing efficiency is higher than 95% in average for each bounce. The characteristics of wide transverse spatial distribution and energy-resolved angular distribution caused by the refluxing electrons show a direct correlation with the angular-dependent photon yield of bremsstrahlung emission, as verified by the hybrid simulations of coupling the PIC results with Monte Carlo particle transport code. We further clarify the energy dissipation mechanisms of refluxing electrons through the recirculation in the thin target under the electron-refluxing dominated regime and conclude that the self-generated sheath field plays a dominant role over the competing processes, such as the radiation loss, collisional stopping, and anomalous inhibition via the resistive field. The lifetime of recirculation is calculated to be a few hundred femtoseconds, that is, one order of magnitude shorter than the timescale of collisional dissipation, while it is one order of magnitude longer than the laser pulse duration. The results could provide useful insights to understand the hot electron transport and stopping, secondary radiation generation, and ion acceleration in the high energy density plasmas. [ABSTRACT FROM AUTHOR]

Measurements of Kα line and bremsstrahlung continuous x-ray emission from high-intensity laser-irradiated thin targets are presented. The experiments were performed at the SG-II UP Petawatt laser. Self-standing Sn foils varying thicknesses and Sn foils backed by the thick substrate were irradiated by the laser pulses up to 300 J of energy with peak intensity higher than 1018 W/cm2. A transmission curved crystal spectrometer and a filter-stack spectrometer were used to measure the Kα line and bremsstrahlung x-ray spectral distribution, respectively. Both Kα and 70–200 keV x-ray yields decrease 3- to 5-fold for target backed by the substrate. 2- to 4-fold reduction of Kα and 70–200 keV x-ray yields for the 8.5 μm targets relative to 50 μm targets was observed. Moreover, a significant background x-ray emission generated from the target holder reduces the ratio of signal to noise. Adopting a low-Z material holder can mitigate the x-ray background noises. This study is instructive to optimize target design for the high-intensity laser-driven Kα or continuous x-ray sources. [ABSTRACT FROM AUTHOR]

A theoretical study complemented with published experimental data of proton acceleration from sub-micron (thickness < 1 µm) foils irradiated by ultra-high contrast (>1010) short pulse lasers is presented. The underlying physics issues pertinent to proton acceleration are addressed using two-dimensional particle-in-cell simulations. For laser energy ε ≤ 4 J (intensity I ≤ 5 x 1020 W/cm²), simulation predictions agree with experimental data, both exhibiting scaling superior to Target Normal Sheath Acceleration's model. Anomalous behavior was observed for ε > 4 J (I > 5 x 1020 W/cm²), for which the measured maximum proton energies were much lower than predicted by scaling and these simulations. This unexpected behavior could not be explained within the frame of the model, and we conjecture that pre-pulses preceding the main pulse by picoseconds may be responsible. If technological issues can be resolved, energetic proton beams could be generated for a wide range of applications such as nuclear physics, radiography, and medical science. [ABSTRACT FROM AUTHOR]

In the context of current efforts to compress PW-level laser pulses to an order of 10 fs, the 3D optimization particle-in-cell (PIC) simulations of proton acceleration have been performed to maximize the proton energy cutoffs using CH2 foils as an example. This was complemented by a simple theoretical model to which PIC simulation results were qualitatively compared. Such a model accounted for a fast increase in a backside surface hot spot, transition of plasma expansion from isothermal regime to the adiabatic one, and effect of target semitransparency that is important for the considered extremely short pulses. It was found that the twofold increase in a shortened laser pulse focal spot size is fraught with a loss in the maximum energy of accelerated protons even when the pulse energy is the same. The PIC simulation optimization study revealed the optimal target thicknesses and the corresponding maximum energies of accelerated protons for shortened PW pulses, and also showed that advantage from their use to increase the proton energy occurs only if the focusability at the target is not worsened. [ABSTRACT FROM AUTHOR]

A scaling study of short-pulse laser-driven proton and electron acceleration was conducted as a function of pulse duration, laser energy, and laser intensity in the multi-picosecond (ps) regime (∼0.8 ps–20 ps). Maximum proton energies significantly greater than established scaling laws were observed, consistent with observations at other multi-ps laser facilities. In addition, maximum proton energies and electron temperatures in this regime were found to be strongly dependent on the laser pulse duration and preplasma conditions. A modified proton scaling model is presented that is able to better represent the accelerated proton characteristics in this multi-ps regime. [ABSTRACT FROM AUTHOR]

In the point-projection hard x-ray radiography of dense matter, for example, an inertial confinement fusion implosion capsule at stagnation time, a picosecond laser driven gold microwire is used to produce a short pulse point, bremsstrahlung hard x-ray source. The microwire was held by a low-Z CH thin substrate commonly used to promote experimental performance. We explored the influence of the low-Z thin substrate on the microwire bremsstrahlung hard x-ray source via particle-in-cell and Monte Carlo simulations. It was shown that both of the microwires, with or without the low-Z thin substrate, could emit more intense hard x-ray radiation than the radiator buried in the equal-density substrate, which benefited from efficient electron recirculation. The freestanding microwire exhibited further enhanced electron recirculation compared to that with the low-Z thin substrate, while the increased hot electrons were only present for the energetic electrons of >1 MeV. Thus, the freestanding microwire could produce significantly more intense MeV gamma x-ray emission with respect to that with the substrate, but an ignorable increment was exhibited at the softer x-ray emission of 10–200 keV. These results provided valuable insights into the design of backlighter targets in point-projection x-ray radiography, such as a freestanding microwire being preferred in MeV gamma-ray radiography, while the microwire with the CH thin substrate could be used in the 10–200 keV hard x-ray Compton radiography of an implosion capsule. [ABSTRACT FROM AUTHOR]

The effect of increasing strength of the electric field of separated charge due to the capture of laser-accelerated fast electrons in a thin solid target is theoretically substantiated. The target considered is so thin that a fast electron passes through the target during the time less than at least half of the applied laser pulse with the additional requirement that energy loss of a fast electron in the balk target is negligible compared to the energy transfer to ions accelerated in a sheath field. An analytical model is proposed of sheath field formation when fast electrons oscillate due to their reflections in the double layers at both boundaries of a thin target. It is shown that the increasing density of fast electrons inside the double layer and shortening of this layer are the reasons of sheath field strength amplification in a thin target in comparison with a thick target. The increase in the number and the energy of fast ions due to field amplification in a thin target is discussed. [ABSTRACT FROM AUTHOR]

Ultra-intense laser-produced sub-ps X-ray pulses can detect backscattered signals from objects hidden in aluminium containers. Coincident measurements using primary X-rays enable differentiation among acrylic, copper, and lead blocks inside the container. Backscattering reveals the shapes of the objects, while their material composition can be identified from the modification methods of the energy spectra of backscattered X-ray beams. This achievement is an important step toward more effective homeland security. [ABSTRACT FROM AUTHOR]

This article first gives the authors' perspectives on how the field of plasma-based acceleration (PBA) developed and how the current experiments, theory, and simulations are motivated by long term applications of PBA to a future linear collider and an x-ray free electron laser. We then focus on some early applications that will likely emerge from PBA research such as electron beam radiotherapy, directional but incoherent x-ray beams for science and technology, near single cycle continuously tunable infrared pulses for spectroscopy, and non-perturbative quantum electrodynamics enabled by PBA electron beams. In our opinion, these near term applications could be developed within the next decade with a concerted effort by the community. [ABSTRACT FROM AUTHOR]

Target-normal sheath acceleration (TNSA) of ions by >100-fs relativistic laser pulses irradiating a multichannel target consisting of a row of parallel long wires and a plane back foil is studied. Two-dimensional particle-in-cell simulations show that the laser light pulls out from the wires a large number of dense hot attosecond electron bunches, which are synergetically accelerated forward by the relativistic ponderomotive force of the laser as well as the longitudinal electric field of a transverse magnetic mode that is excited in the vacuum channels between the wires. These electrons are characterized by a distinct two-temperature energy spectrum, with the temperature of the more energetic electrons close to twice the ponderomotive potential energy. After penetrating through the foil, they induce behind its rear surface a sheath electric field that is both stronger and frontally more extended than that without the channels. As a result, the TNSA ions have much higher maximum energy and the laser-to-ion energy conversion efficiency is also much higher. It is found that a laser of intensity 1.37 × 1020 W/cm2, duration 165 fs, and energy 25.6 J can produce 85 MeV protons and 31 MeV/u carbon ions, at 30% laser-to-ion energy conversion efficiency. The effects of the channel size and laser polarization on the TNSA ions are also investigated. [ABSTRACT FROM AUTHOR]

A hohlraum used to create uniform and strongly coupled warm dense matter and its radiation flux study on the SG-III prototype laser facility are described. Time evolution of the radiation temperature from laser entrance hole (LEH) and the incident radiation temperature at the target surface are obtained using flat response X-ray diode detectors. Then, a calculation of the radiation flux evolution for this hohlraum is carried out using a view-factor method, and the calculated results agree well with the experimental data within the error bar. Using the incident radiation at the target surface as a source, the validity to create uniform and strongly coupled warm dense matter by this hohlraum is verified. [ABSTRACT FROM AUTHOR]

We outline an approach for improving the temporal contrast of a high-intensity laser system by >8 orders of magnitude using noncollinear sum-frequency generation with the signal and idler of an optical parametric amplifier. We demonstrate the effectiveness of this technique by cleaning pulses from a millijoule-level chirped-pulse amplification system to provide >1012 intensity contrast relative to all prepulses and amplified spontaneous emission >5 ps prior to the main pulse. The output maintains percent-level energy stability on the time scales of a typical user experiment at our facility, highlighting the method's reliability and operational efficiency. After temporal cleansing, the pulses are stretched in time before seeding two multipass, Ti:sapphire-based amplifiers. After re-compression, the 1 J, 40 fs (25 terawatt) laser pulses maintain a >1010 intensity contrast >30 ps prior to the main pulse. This technique is both energy-scalable and appropriate for preparing seed pulses for a terawatt- or petawatt-level chirped-pulse amplification laser system. [ABSTRACT FROM AUTHOR]

A cryogenic hydrogen cluster-jet target is described which has been used for laser-plasma interaction studies. Major advantages of the cluster-jet are, on the one hand, the compatibility to pulsed high repetition lasers as the target is operated continuously and, on the other hand, the absence of target debris. The cluster-jet target was characterized using the Mie-scattering technique allowing to determine the cluster size and to compare the measurements with an empirical formula. In addition, an estimation of the cluster beam density was performed. The system was implemented at the high power laser system ARCTURUS, and the measurements show the acceleration of protons after irradiation of the cluster target by high intensity laser pulses with a repetition rate of 5 Hz. [ABSTRACT FROM AUTHOR]

X-ray communication (XCOM) offers important advantages to both civilian and military space projects. Rapid advance in high-intensity laser interaction with plasma has become a driving force for providing a new X-ray carrier generation based on the laser wakefield acceleration scheme. XCOM has the potential to eliminate RF shielding on the ground and communicate with the re-entry supersonic spacecraft during blackout occurrence. In this process, the plasma sheath is formed around the surface due to air compression and ablation, which blocks the traditional communication signals. In this paper, the hazardous substance was proactively exploited and coupled with the modulated laser. Particle-In-Cell simulation results indicate the ultra-bright controllable X-ray emission with a small angular divergence (0.04 rad × 0.03 rad), a tunable X-ray energy range (4.60 keV to 321.48 keV), and high photon yields. Additionally, the data rate of the communication via the X-ray carrier during re-entry was estimated up to ∼20.7 Mbps by considering the transmission model, encoding schemes and photon information efficiency. Combined with an existing or developing X-ray detection technique, this regime can eliminate re-entry blackout and also provide a novel modulated X-ray source to acquire high-rate, low transmit power, and highly secure space-based data links. [ABSTRACT FROM AUTHOR]

We demonstrate the significant enhancement of ion energy from the interaction of intense, chirped pulse amplification based ultrashort laser pulse with thin foil targets by adjusting the laser temporal characteristics with a simple adjustment of grating pair separation inside the pulse compressor. The laser pulse was focused to a maximum intensity of 3.2 × 1019 W/cm2 on to thin metallic foil targets of submicron thickness. The pulse duration was varied from 25 to 500 fs by adjusting the laser pulse compressor grating separation for fixed laser pulse energy (2.1 J). Contrary to the conventional belief, we found that the ion acceleration is not optimum at the shortest laser pulse duration and, thus, at highest intensity as predicted by the previous intensity scaling data. Instead, stretched pulses are better suited for efficient ion acceleration. In addition to this, we found a contrasting effect with respect to the sign of the laser chirp for almost the same laser pulse duration. In particular, we show 70% enhancement in maximum ion energy (from 6 MeV to 10 MeV) with positively chirped 250–350 fs stretched pulses. On the contrary, negatively chirped pulses show gradual monotonic reduction in ion energy and flux. Independent electron energy spectra measurement along the laser forward direction exhibits a strong correlation with proton data. The temporal pulse skewness arising due to displaced grating separation is believed to be responsible for this asymmetric proton acceleration behaviour. Efficient absorption of positively modified skewed pulses (shallow rise time and sharp fall) along with the characteristic ion acceleration time can qualitatively explain the experimental result. The present study can be very much important for efficient ion acceleration based on modern day compact, ultra-short pulse 100 TW to PW class lasers. [ABSTRACT FROM AUTHOR]

During the interaction of intense femtosecond laser pulses with various targets, the natural mechanisms of laser energy transformation inherently lack temporal control and thus commonly do not provide opportunities for a controlled generation of a well-collimated, high-charge beam of ions with a given energy of particular interest. In an effort to alleviate this problem, it was recently proposed that the ions can be dragged by an electron bunch trapped in a controllably moving potential well formed by laser radiation. Such standing-wave acceleration (SWA) can be achieved through reflection of a chirped laser pulse from a mirror, which has been formulated as the concept of chirped-standing-wave acceleration (CSWA). Here, we analyse general feasibility aspects of the SWA approach and demonstrate its reasonable robustness against field structure imperfections, such as those caused by misalignment, ellipticity, and limited contrast. Using this, we also identify prospects and limitations of the CSWA concept. [ABSTRACT FROM AUTHOR]

The electric and magnetic fields responsible for electron acceleration in a Laser Wakefield Accelerator (LWFA) also cause electrons to radiate x-ray photons. Such x-ray pulses have several desirable properties including short duration and being well collimated with tunable high energy. We measure the scaling of this x-ray source experimentally up to laser powers greater than 100 TW. An increase in laser power allows electron trapping at a lower density as well as with an increased trapped charge. These effects resulted in an x-ray fluence that was measured to increase non-linearly with laser power. The fluence of x-rays was also compared with that produced from K-α emission resulting from a solid target interaction for the same energy laser pulse. The flux was shown to be comparable, but the LWFA x-rays had a significantly smaller source size. This indicates that such a source may be useful as a backlighter for probing high energy density plasmas with ultrafast temporal resolution. [ABSTRACT FROM AUTHOR]

Target normal sheath acceleration (TNSA) is a method employed in laser-matter interaction experiments to accelerate light ions (usually protons). Laser setups with durations of a few 10 fs and relatively low intensity contrasts observe plateau regions in their ion energy spectra when shooting on thin foil targets with thicknesses of the order of 10 μm. In this paper, we identify a mechanism which explains this phenomenon using one-dimensional particle-in-cell simulations. Fast electrons generated from the laser interaction recirculate back and forth through the target, giving rise to time-oscillating charge and current densities at the target backside. Periodic decreases in the electron density lead to transient disruptions of the TNSA sheath field: peaks in the ion spectra form as a result, which are then spread in energy from a modified potential driven by further electron recirculation. The ratio between the laser pulse duration and the recirculation period (dependent on the target thickness, including the portion of the pre-plasma which is denser than the critical density) determines if a plateau forms in the energy spectra. [ABSTRACT FROM AUTHOR]

A new phenomenon of an enhanced relativistic transparency of overdense plasmas by the influence of hot-electron refluxing has been discovered via particle-in-cell simulations. When a p-polarized laser pulse, with intensity below the self-induced-transparency (SIT) threshold, obliquely irradiates a thin overdense plasma, the initially opaque plasma becomes transparent after a time interval that is linearly dependent on the thickness of the plasma. This phenomenon can be interpreted as a consequence of hot-electron refluxing, which reduces the effective electron density by longitudinal heating. When the laser intensity is higher than the SIT threshold, the penetration velocity of the laser in the plasma is enhanced when the refluxing is present. [ABSTRACT FROM AUTHOR]

Ion acceleration resulting from the interaction of ultra-high intensity and ultra-high contrast (~10-10) laser pulses with thin Al foil targets at 30° angle of laser incidence is studied. Proton maximum energies of 30 and 18MeV are measured along the target normal rear and front sides, respectively, showing intensity scaling as Ib. For the target front bfront = 0.5-0.6 and for the target rear brear = 0.7-0.8 is observed in the intensity range 1020-1021 W/cm2. The fast scaling from the target rear ~I0.75 can be attributed enhancement of laser energy absorption as already observed at relatively low intensities. The backward acceleration of the front side protons with intensity scaling as ~I0.5 can be attributed to the to the formation of a positively charged cavity at the target front via ponderomotive displacement of the target electrons at the interaction of relativistic intense laser pulses with a solid target. The experimental results are in a good agreement with theoretical predictions. [ABSTRACT FROM AUTHOR]

Measurement of angularly dependent spectra of betatron gamma-rays radiated by GeV electron beams from laser wakefield accelerators (LWFAs) are presented. The angle-resolved spectrum of betatron radiation was deconvolved from the position dependent data measured for a single laser shot with a broadband gamma-ray spectrometer comprising four-quadrant sectored range filters and an unfolding algorithm, based on the Monte Carlo code GEANT4. The unfolded gamma-ray spectra in the photon energy range of 0.1-10 MeV revealed an approximately isotropic angular dependence of the peak photon energy and photon energy-integrated fluence. As expected by the analysis of betatron radiation from LWFAs, the results indicate that unpolarized gamma-rays are emitted by electrons undergoing betatron motion in isotropically distributed orbit planes. [ABSTRACT FROM AUTHOR]

Betatron radiation in strongly magnetized plasma is investigated by two dimensional (2D) particlein- cell (PIC) simulations. The results show that the betatron radiation in magnetized plasmas is strongly enhanced and is more collimated compared to that in unmagnetized plasma. Single particle model analysis shows that the frequency and the amplitude of the electrons's betatron oscillation are strongly influenced by the axial external magnetic field and the axial self-generated magnetic field. And the 2D PIC simulation shows that the axial magnetic field is actually induced by the external magnetic field and tends to increase the betatron frequency. By disturbing the perturbation of the plasma density in the laser-produced channel, the hosing instability is also suppressed, which results in a better angular distribution and a better symmetry of the betatron radiation. [ABSTRACT FROM AUTHOR]

We report on a study of the spatial profile of proton beams produced through target normal sheath acceleration using flat target foils and changing the laser intensity distribution on the target front surface. This is done by either defocusing a single laser pulse or by using a split-pulse setup and irradiating the target with two identical laser pulses with variable spatial separation. The resulting proton beam profile and the energy spectrum are recorded as functions of the focal spot size of the single laser pulse and of the separation between the two pulses. A shaping of the resulting proton beam profile, related to both an increase in flux of low-energy protons in the target normal direction and a decrease in their divergence, in one or two dimensions, is observed. The results are explained by simple modelling of rear surface sheath field expansion, ionization, and projection of the resulting proton beam. [ABSTRACT FROM AUTHOR]