1. The TRIXS end-station for femtosecond time-resolved resonant inelastic X-ray free-electron laser FLASH
- Author
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Dziarzhytski, Siarhei, Biednov, M., Behrens, Christopher, Sinha, M., Schulte, Amelie, Grimm-Lebsanft, B., Chiuzbăian, S. G., Wurth, W., Beye, M., Rübhausen, M., Brenner, Guenter, Dicke, B., Wang, A., Miedema, P. S., Engel, R. Y., Schunck, Jan, Redlin, H., Weigelt, Holger, and Siewert, F.
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ddc:500 - Abstract
We present the experimental end-station TRIXS dedicated to time-resolved soft x-ray resonant inelastic x-ray scattering (RIXS) experiments on solid samples at the free-electron laser FLASH. Using monochromatized ultrashort femtosecond XUV/soft x-ray photon pulses in combination with a synchronized optical laser in a pump-probe scheme, the TRIXS setup allows measuring sub-picosecond time-resolved high-resolution RIXS spectra in the energy range from 35 eV to 210 eV, thus spanning the M-edge (M$_1$ and M$_{2,3}$) absorption resonances of 3d transition metals and N$_{4,5}$-edges of rare earth elements. A Kirkpatrick–Baez refocusing mirror system at the first branch of the plane grating monochromator beamline (PG1) provides a focus of (6 × 6) $μm^2$ (FWHM) at the sample. The RIXS spectrometer reaches an energy resolution of 35–160 meV over the entire spectral range. The optical laser system based on a chirped pulse optical parametric amplifier provides approximately 100 fs (FWHM) long photon pulses at the fundamental wavelength of 800 nm and a fluence of 120 mJ/cm$^2$ at a sample for optical pump-XUV probe measurements. Furthermore, optical frequency conversion enables experiments at 400 nm or 267 nm with a fluence of 80 and 30 mJ/cm$^2$, respectively. Some of the first (pump-probe) RIXS spectra measured with this setup are shown. The measured time resolution for time-resolved RIXS measurements has been characterized as 287 fs (FWHM) for the used energy resolution.
- Published
- 2020
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